technical note: supplemental material: ozonesonde climatology between 1995 and 2011: description,...

23
Manuscript prepared for J. Name with version 3.2 of the L A T E X class copernicus.cls. Date: 9 August 2012 Technical Note: Supplemental Material: Ozonesonde climatology between 1995 and 2011: Description, Evaluation and Applications S. Tilmes 1 , J.-F. Lamarque 1 , L. K. Emmons 1 , A. Conley 1 , M. G. Schultz 2 , M. Saunois 1,3 , V. Thouret 4 , A. M. Thompson 5 , S. J. Oltmans 6 , B. Johnson 6 , and D. Tarasick 7 1 National Center for Atmospheric Research, Boulder, Colorado, USA 2 Research Center J ¨ ulich, J ¨ ulich, Germany 3 Now at Laboratoire des Sciences du Climat et de l’Environnement, CEA-CNRS-UVSQ, Gif-Sur-Yvette, France 4 Laboratoire dA´ erologie, UMR 5560, Universit´ e Paul Sabatier, Toulouse, France 5 NASA Goddard Space Flight Center, Greenbelt, Maryland, USA 6 NOAA Climate Monitoring and Diagnostics Laboratory, Boulder, Colorado, USA 7 Experimental Studies (ARQX), Air Quality Research Division, Environment Canada, 4905 Dufferin Street, Downsview, Ontario Canada Correspondence to: Simone Tilmes, National Center for Atmospheric Research, Boulder, Colorado, USA ([email protected]) 1 Ozonesonde observations available for each station Figure 1 shows timelines of the median of seasonally averaged ozone profiles between 1978 and 2011 (colored diamonds). Years that include less than 12 profiles per season are illustrated as colored points and are likely not representative. After 1995, for most stations at least 12 profiles per season and year were available and the sampling frequency stays rather constant. Therefore, we do not 5 apply any annual weighting to calculate the 17 year average, shown in Figure 5. 2 Impact of the correction factor For most ozone stations a correction factor is provided that is derived by scaling the entire ozone column to an independent measurement of ozone column measured by a Brewer-Dobson spectrom- eter. Profiles that have been corrected by a factor outside the range of 0.8 and 1.2 are often ignored 10 in order to not employ profiles that are heavily corrected (WMO, 1995, 1999). Since the correction factor was scaled with regard to the entire column, it is not necessarily valid for the tropospheric part of the profile. A comparison between MOZAIC aircraft data and ozone sondes has shown that tropospheric comparisons are better when omitting such correction factors (Thouret et al., 1998). Removing profiles that have been corrected by a factor outside the range of 0.8 and 1.2 has little 15 1

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Manuscript prepared for J. Namewith version 3.2 of the LATEX class copernicus.cls.Date: 9 August 2012

Technical Note: Supplemental Material: Ozonesondeclimatology between 1995 and 2011: Description,Evaluation and Applications

S. Tilmes1, J.-F. Lamarque1, L. K. Emmons1, A. Conley1, M. G. Schultz2, M.Saunois1,3, V. Thouret4, A. M. Thompson5, S. J. Oltmans6, B. Johnson6, and D.Tarasick7

1National Center for Atmospheric Research, Boulder, Colorado, USA2Research Center Julich, Julich, Germany3Now at Laboratoire des Sciences du Climat et de l’Environnement, CEA-CNRS-UVSQ,Gif-Sur-Yvette, France4Laboratoire dAerologie, UMR 5560, Universite Paul Sabatier, Toulouse, France5NASA Goddard Space Flight Center, Greenbelt, Maryland, USA6NOAA Climate Monitoring and Diagnostics Laboratory, Boulder, Colorado, USA7Experimental Studies (ARQX), Air Quality Research Division, Environment Canada, 4905Dufferin Street, Downsview, Ontario Canada

Correspondence to: Simone Tilmes, National Center for Atmospheric Research, Boulder,Colorado, USA ([email protected])

1 Ozonesonde observations available for each station

Figure 1 shows timelines of the median of seasonally averaged ozone profiles between 1978 and

2011 (colored diamonds). Years that include less than 12 profiles per season are illustrated as colored

points and are likely not representative. After 1995, for most stations at least 12 profiles per season

and year were available and the sampling frequency stays rather constant. Therefore, we do not5

apply any annual weighting to calculate the 17 year average, shown in Figure 5.

2 Impact of the correction factor

For most ozone stations a correction factor is provided that is derived by scaling the entire ozone

column to an independent measurement of ozone column measured by a Brewer-Dobson spectrom-

eter. Profiles that have been corrected by a factor outside the range of 0.8 and 1.2 are often ignored10

in order to not employ profiles that are heavily corrected (WMO, 1995, 1999). Since the correction

factor was scaled with regard to the entire column, it is not necessarily valid for the tropospheric

part of the profile. A comparison between MOZAIC aircraft data and ozone sondes has shown that

tropospheric comparisons are better when omitting such correction factors (Thouret et al., 1998).

Removing profiles that have been corrected by a factor outside the range of 0.8 and 1.2 has little15

1

Alert 82.N, −62.E

0500

1000

1500

2000

25003000

Ozo

ne (

ppbv

)

100hPa100hPa100hPa100hPa

Eureka 80.N, −86.E

0500

1000

1500

2000

25003000

100hPa100hPa100hPa100hPa

Ny_Alesund 78.N, 11.E

0500

1000

1500

2000

25003000

100hPa100hPa100hPa100hPa

20

40

60

80

100

Ozo

ne (

ppbv

) 500hPa500hPa500hPa500hPa

20

40

60

80

100 500hPa500hPa500hPa500hPa

20

40

60

80

100 500hPa500hPa500hPa500hPa

0

20

40

60

80

Ozo

ne (

ppbv

) 800hPa800hPa800hPa800hPa

0

20

40

60

80800hPa800hPa800hPa800hPa

0

20

40

60

80800hPa800hPa800hPa800hPa

1980 1990 2000 20100

10

20

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40

50

Num

ber/

Sea

son

1980 1990 2000 20100

10

20

30

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1980 1990 2000 20100

10

20

30

40

50

Resolute 74.N, −94.E

0500

1000

1500

2000

25003000

Ozo

ne (

ppbv

)

100hPa100hPa100hPa100hPa

Scoresbysund 70.N, −22.E

0500

1000

1500

2000

25003000

100hPa100hPa100hPa100hPa

Lerwick 60.N, −1.E

0500

1000

1500

2000

25003000

100hPa100hPa100hPa100hPa

20

40

60

80

100

Ozo

ne (

ppbv

) 500hPa500hPa500hPa500hPa

20

40

60

80

100 500hPa500hPa500hPa500hPa

20

40

60

80

100 500hPa500hPa500hPa500hPa

0

20

40

60

80

Ozo

ne (

ppbv

) 800hPa800hPa800hPa800hPa

0

20

40

60

80800hPa800hPa800hPa800hPa

0

20

40

60

80800hPa800hPa800hPa800hPa

1980 1990 2000 20100

10

20

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40

50

Num

ber/

Sea

son

1980 1990 2000 20100

10

20

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50

1980 1990 2000 20100

10

20

30

40

50

Churchill 58.N, −94.E

0500

1000

1500

2000

25003000

Ozo

ne (

ppbv

)

100hPa100hPa100hPa100hPa

Edmonton 53.N, −114.E

0500

1000

1500

2000

25003000

100hPa100hPa100hPa100hPa

Goose_bay 53.N, −60.E

0500

1000

1500

2000

25003000

100hPa100hPa100hPa100hPa

20

40

60

80

100

Ozo

ne (

ppbv

) 500hPa500hPa500hPa500hPa

20

40

60

80

100 500hPa500hPa500hPa500hPa

20

40

60

80

100 500hPa500hPa500hPa500hPa

0

20

40

60

80

Ozo

ne (

ppbv

) 800hPa800hPa800hPa800hPa

0

20

40

60

80800hPa800hPa800hPa800hPa

0

20

40

60

80800hPa800hPa800hPa800hPa

1980 1990 2000 2010

Years

010

20

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50

Num

ber/

Sea

son

1980 1990 2000 2010

Years

010

20

30

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50

1980 1990 2000 2010

Years

010

20

30

40

50

Fig. 1: Time evolution of median ozone mixing ratios derived from the ozone soundings at three

different pressure levels and different seasons (DJF: blue, MAM: green, JJA: red, SON: black) for

42 stations. The total number of profiles per season for each year are illustrated in the bottom plot

of each panel. Seasons that include less than 12 profiles per year are shown as dots.

2

Legionowo 52.N, 20.E

0500

1000

1500

2000

25003000

Ozo

ne (

ppbv

)

100hPa100hPa100hPa100hPa

Lindenberg 52.N, 14.E

0500

1000

1500

2000

25003000

100hPa100hPa100hPa100hPa

Debilt 52.N, 5.E

0500

1000

1500

2000

25003000

100hPa100hPa100hPa100hPa

20

40

60

80

100

Ozo

ne (

ppbv

) 500hPa500hPa500hPa500hPa

20

40

60

80

100 500hPa500hPa500hPa500hPa

20

40

60

80

100 500hPa500hPa500hPa500hPa

0

20

40

60

80

Ozo

ne (

ppbv

) 800hPa800hPa800hPa800hPa

0

20

40

60

80800hPa800hPa800hPa800hPa

0

20

40

60

80800hPa800hPa800hPa800hPa

1980 1990 2000 20100

10

20

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Num

ber/

Sea

son

1980 1990 2000 20100

10

20

30

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1980 1990 2000 20100

10

20

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50

Uccle 50.N, 4.E

0500

1000

1500

2000

25003000

Ozo

ne (

ppbv

)

100hPa100hPa100hPa100hPa

Praha 50.N, 14.E

0500

1000

1500

2000

25003000

100hPa100hPa100hPa100hPa

Hohenpeissenberg 47.N, 11.E

0500

1000

1500

2000

25003000

100hPa100hPa100hPa100hPa

20

40

60

80

100

Ozo

ne (

ppbv

) 500hPa500hPa500hPa500hPa

20

40

60

80

100 500hPa500hPa500hPa500hPa

20

40

60

80

100 500hPa500hPa500hPa500hPa

0

20

40

60

80

Ozo

ne (

ppbv

) 800hPa800hPa800hPa800hPa

0

20

40

60

80800hPa800hPa800hPa800hPa

0

20

40

60

80800hPa800hPa800hPa800hPa

1980 1990 2000 20100

10

20

30

40

50

Num

ber/

Sea

son

1980 1990 2000 20100

10

20

30

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50

1980 1990 2000 20100

10

20

30

40

50

Payerne 46.N, 6.E

0500

1000

1500

2000

25003000

Ozo

ne (

ppbv

)

100hPa100hPa100hPa100hPa

Sapporo 43.N, 141.E

0500

1000

1500

2000

25003000

100hPa100hPa100hPa100hPa

Madrid 40.N, −4.E

0500

1000

1500

2000

25003000

100hPa100hPa100hPa100hPa

20

40

60

80

100

Ozo

ne (

ppbv

) 500hPa500hPa500hPa500hPa

20

40

60

80

100 500hPa500hPa500hPa500hPa

20

40

60

80

100 500hPa500hPa500hPa500hPa

0

20

40

60

80

Ozo

ne (

ppbv

) 800hPa800hPa800hPa800hPa

0

20

40

60

80800hPa800hPa800hPa800hPa

0

20

40

60

80800hPa800hPa800hPa800hPa

1980 1990 2000 2010

Years

010

20

30

40

50

Num

ber/

Sea

son

1980 1990 2000 2010

Years

010

20

30

40

50

1980 1990 2000 2010

Years

010

20

30

40

50

Fig. 1: continued

3

Boulder 40.N, −105.E

0500

1000

1500

2000

25003000

Ozo

ne (

ppbv

)

100hPa100hPa100hPa100hPa

Trinidadhead 41.N, −124.E

0500

1000

1500

2000

25003000

100hPa100hPa100hPa100hPa

Wallops_Island 37.N, −75.E

0500

1000

1500

2000

25003000

100hPa100hPa100hPa100hPa

20

40

60

80

100

Ozo

ne (

ppbv

) 500hPa500hPa500hPa500hPa

20

40

60

80

100 500hPa500hPa500hPa500hPa

20

40

60

80

100 500hPa500hPa500hPa500hPa

0

20

40

60

80

Ozo

ne (

ppbv

) 800hPa800hPa800hPa800hPa

0

20

40

60

80800hPa800hPa800hPa800hPa

0

20

40

60

80800hPa800hPa800hPa800hPa

1980 1990 2000 20100

10

20

30

40

50

Num

ber/

Sea

son

1980 1990 2000 20100

10

20

30

40

50

1980 1990 2000 20100

10

20

30

40

50

Tateno 36.N, 140.E

0500

1000

1500

2000

25003000

Ozo

ne (

ppbv

)

100hPa100hPa100hPa100hPa

Huntsville 34.N, −86.E

0500

1000

1500

2000

25003000

100hPa100hPa100hPa100hPa

Kagoshima 31.N, 130.E

0500

1000

1500

2000

25003000

100hPa100hPa100hPa100hPa

20

40

60

80

100

Ozo

ne (

ppbv

) 500hPa500hPa500hPa500hPa

20

40

60

80

100 500hPa500hPa500hPa500hPa

20

40

60

80

100 500hPa500hPa500hPa500hPa

0

20

40

60

80

Ozo

ne (

ppbv

) 800hPa800hPa800hPa800hPa

0

20

40

60

80800hPa800hPa800hPa800hPa

0

20

40

60

80800hPa800hPa800hPa800hPa

1980 1990 2000 2010

Years

010

20

30

40

50

Num

ber/

Sea

son

1980 1990 2000 2010

Years

010

20

30

40

50

1980 1990 2000 2010

Years

010

20

30

40

50

Naha 26.N, 127.E

50

100

150

200

250300

Ozo

ne (

ppbv

)

100hPa100hPa100hPa100hPa

Hongkong 22.N, 114.E

50

100

150

200

250300

100hPa100hPa100hPa100hPa

Hilo 19.N, −155.E

50

100

150

200

250300

100hPa100hPa100hPa100hPa

20

40

60

80

100

Ozo

ne (

ppbv

) 500hPa500hPa500hPa500hPa

20

40

60

80

100 500hPa500hPa500hPa500hPa

20

40

60

80

100 500hPa500hPa500hPa500hPa

0

20

40

60

80

Ozo

ne (

ppbv

) 800hPa800hPa800hPa800hPa

0

20

40

60

80800hPa800hPa800hPa800hPa

0

20

40

60

80800hPa800hPa800hPa800hPa

1980 1990 2000 2010

Years

010

20

30

40

50

Num

ber/

Sea

son

1980 1990 2000 2010

Years

010

20

30

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1980 1990 2000 2010

Years

010

20

30

40

50

Fig. 1: continued

4

Paramaribo 5.N, −55.E

50

100

150

200

250300

Ozo

ne (

ppbv

)

100hPa100hPa100hPa100hPa

Sancristobal −1.N, −89.E

50

100

150

200

250300

100hPa100hPa100hPa100hPa

Nairobi −1.N, 36.E

50

100

150

200

250300

100hPa100hPa100hPa100hPa

20

40

60

80

100

Ozo

ne (

ppbv

) 500hPa500hPa500hPa500hPa

20

40

60

80

100 500hPa500hPa500hPa500hPa

20

40

60

80

100 500hPa500hPa500hPa500hPa

0

20

40

60

80

Ozo

ne (

ppbv

) 800hPa800hPa800hPa800hPa

0

20

40

60

80800hPa800hPa800hPa800hPa

0

20

40

60

80800hPa800hPa800hPa800hPa

1980 1990 2000 20100

10

20

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50

Num

ber/

Sea

son

1980 1990 2000 20100

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1980 1990 2000 20100

10

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Natal −5.N, −35.E

50

100

150

200

250300

Ozo

ne (

ppbv

)

100hPa100hPa100hPa100hPa

Ascension −7.N, −14.E

50

100

150

200

250300

100hPa100hPa100hPa100hPa

Watukosek −7.N, 112.E

50

100

150

200

250300

100hPa100hPa100hPa100hPa

20

40

60

80

100

Ozo

ne (

ppbv

) 500hPa500hPa500hPa500hPa

20

40

60

80

100 500hPa500hPa500hPa500hPa

20

40

60

80

100 500hPa500hPa500hPa500hPa

0

20

40

60

80

Ozo

ne (

ppbv

) 800hPa800hPa800hPa800hPa

0

20

40

60

80800hPa800hPa800hPa800hPa

0

20

40

60

80800hPa800hPa800hPa800hPa

1980 1990 2000 20100

10

20

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40

50

Num

ber/

Sea

son

1980 1990 2000 20100

10

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1980 1990 2000 20100

10

20

30

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Samoa −14.N, −170.E

50

100

150

200

250300

Ozo

ne (

ppbv

)

100hPa100hPa100hPa100hPa

Fiji −18.N, 178.E

50

100

150

200

250300

100hPa100hPa100hPa100hPa

Reunion −21.N, 55.E

50

100

150

200

250300

100hPa100hPa100hPa100hPa

20

40

60

80

100

Ozo

ne (

ppbv

) 500hPa500hPa500hPa500hPa

20

40

60

80

100 500hPa500hPa500hPa500hPa

20

40

60

80

100 500hPa500hPa500hPa500hPa

0

20

40

60

80

Ozo

ne (

ppbv

) 800hPa800hPa800hPa800hPa

0

20

40

60

80800hPa800hPa800hPa800hPa

0

20

40

60

80800hPa800hPa800hPa800hPa

1980 1990 2000 2010

Years

010

20

30

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50

Num

ber/

Sea

son

1980 1990 2000 2010

Years

010

20

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1980 1990 2000 2010

Years

010

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30

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Fig. 1: continued

5

Broadmeadows −37.N, 144.E

0500

1000

1500

2000

25003000

Ozo

ne (

ppbv

)

100hPa100hPa100hPa100hPa

Lauder −45.N, 169.E

0500

1000

1500

2000

25003000

100hPa100hPa100hPa100hPa

Macquarie −54.N, 158.E

0500

1000

1500

2000

25003000

100hPa100hPa100hPa100hPa

20

40

60

80

100

Ozo

ne (

ppbv

) 500hPa500hPa500hPa500hPa

20

40

60

80

100 500hPa500hPa500hPa500hPa

20

40

60

80

100 500hPa500hPa500hPa500hPa

0

20

40

60

80

Ozo

ne (

ppbv

) 800hPa800hPa800hPa800hPa

0

20

40

60

80800hPa800hPa800hPa800hPa

0

20

40

60

80800hPa800hPa800hPa800hPa

1980 1990 2000 20100

10

20

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50

Num

ber/

Sea

son

1980 1990 2000 20100

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1980 1990 2000 20100

10

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50

Marambio −64.N, −56.E

0500

1000

1500

2000

25003000

Ozo

ne (

ppbv

)

100hPa100hPa100hPa100hPa

Syowa −69.N, 39.E

0500

1000

1500

2000

25003000

100hPa100hPa100hPa100hPa

Neumayer −70.N, −8.E

0500

1000

1500

2000

25003000

100hPa100hPa100hPa100hPa

20

40

60

80

100

Ozo

ne (

ppbv

) 500hPa500hPa500hPa500hPa

20

40

60

80

100 500hPa500hPa500hPa500hPa

20

40

60

80

100 500hPa500hPa500hPa500hPa

0

20

40

60

80

Ozo

ne (

ppbv

) 800hPa800hPa800hPa800hPa

0

20

40

60

80800hPa800hPa800hPa800hPa

0

20

40

60

80800hPa800hPa800hPa800hPa

1980 1990 2000 2010

Years

010

20

30

40

50

Num

ber/

Sea

son

1980 1990 2000 2010

Years

010

20

30

40

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1980 1990 2000 2010

Years

010

20

30

40

50

Fig. 1: continued

6

Resolute (1995−2007)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number Profiles (corrected)DJF: 125.

DJF: 125.

Number Profiles (corrected)

MAM: 102.

MAM: 102.

Number Profiles (corrected)

JJA: 90.2

JJA: 90.2

Number Profiles (corrected)

SON: 91.7

SON: 92.7

−10−5 0 5 10

Lindenberg (1995−2009)

0 2 4 6

Number Profiles (corrected)DJF: 184.

DJF: 198.

Number Profiles (corrected)

MAM: 188.

MAM: 188.

Number Profiles (corrected)

JJA: 196.

JJA: 196.

Number Profiles (corrected)

SON: 167.

SON: 169.

−10−5 0 5 10

Payerne (1995−2009)

0 2 4 6

Number Profiles (corrected)DJF: 497.

DJF: 532.

Number Profiles (corrected)

MAM: 530.

MAM: 555.

Number Profiles (corrected)

JJA: 516.

JJA: 545.

Number Profiles (corrected)

SON: 515.

SON: 545.

−10−5 0 5 10

Sapporo (1995−2009)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number Profiles (corrected)DJF: 146.

DJF: 157.

Number Profiles (corrected)

MAM: 153.

MAM: 159.

Number Profiles (corrected)

JJA: 137.

JJA: 142.

Number Profiles (corrected)

SON: 146.

SON: 154.

−10−5 0 5 10

Tateno (1995−2009)

0 2 4 6

Number Profiles (corrected)DJF: 188.

DJF: 221.

Number Profiles (corrected)

MAM: 190.

MAM: 220.

Number Profiles (corrected)

JJA: 144.

JJA: 157.

Number Profiles (corrected)

SON: 151.

SON: 166.

−10−5 0 5 10

Kagoshima (1995−2005)

0 2 4 6

Number Profiles (corrected)DJF: 129.

DJF: 132.

Number Profiles (corrected)

MAM: 108.

MAM: 112.

Number Profiles (corrected)

JJA: 102.

JJA: 109.

Number Profiles (corrected)

SON: 123.

SON: 126.

−10−5 0 5 10

Naha (1995−2008)

0 2 4 6

Ozone (ppmv)

1000

100

10

Alti

tude

(hP

a)

Number Profiles (corrected)DJF: 131.

DJF: 140.

Number Profiles (corrected)

MAM: 134.

MAM: 141.

Number Profiles (corrected)

JJA: 119.

JJA: 132.

Number Profiles (corrected)

SON: 136.

SON: 145.

−10−5 0 5 10

Difference (%)

Macquarie (1995−2009)

0 2 4 6

Ozone (ppmv)

Number Profiles (corrected)DJF: 90.0

DJF: 90.0

Number Profiles (corrected)

MAM: 100.

MAM: 109.

Number Profiles (corrected)

JJA: 87.0

JJA: 110.

Number Profiles (corrected)

SON: 99.1

SON: 102.

−10−5 0 5 10

Difference (%)

Syowa (1995−2009)

0 2 4 6

Ozone (ppmv)

Number Profiles (corrected)DJF: 174.

DJF: 176.

Number Profiles (corrected)

MAM: 148.

MAM: 164.

Number Profiles (corrected)

JJA: 207.

JJA: 227.

Number Profiles (corrected)

SON: 250.

SON: 266.

−10−5 0 5 10

Difference (%)

Fig. 2: Left plot of each panel: seasonally averaged ozone profiles for available years between 1995

and 2009. The average of all profiles, corrected in the way that those profiles are dismissed that are

corrected by a factor of < 0.8 or > 1.2, is shown as solid lines. The average of all available profiles

is shown in dashed lines (if not on top of the solid lines). The total number of profiles entering

the average are given in the plot. Right plot of each panel: percentage difference between all but

corrected profiles and all profiles. Only those stations are shown, where the percentage difference is

larger 0.5%.

impact on the averaged ozone profiles between 1995 and 2009, as shown in Figure 2. Only those

stations are shown, where the percentage difference between all profiles and only minor corrected

profiles is larger than 0.5%. For a few stations, differences can reach up to 5-10%.

3 Comparison to other studies

A comparison of seasonally averaged ozone profiles for all stations for the period between 198020

and 1994 with the climatology from Logan (1999a,b) is illustrated in Figure 3. We construct ozone

profiles on the same pressure grid as done by Logan (1999a) and Logan (1999b), which results in

a good agreement with these earlier results. Some differences occur around the tropopause, very

likely as a result of a different interval chosen to average over pressure levels around the tropopause,

where the ozone gradient is very large. Besides that, differences between 10 and 20% occur when25

slightly different periods are considered or if a very different number of samples was included in the

7

mean, as it is the case for Payerne. The earlier period considered for Payerne in the climatology by

Logan (1999a) covered the years between 1980-1989, whereas our climatology includes the period

between 1980 and 1993. Especially between 1990 and 1993, ozone strongly increased over Payerne

in the troposphere. Further, problems with data over Payerne exist in earlier years, as summarized30

in Logan et al. (2012).

4 Representativeness of ozone averages in comparison to independent observations, Western

Europe

The comparison of ozone timelines between ozone soundings, surface observations and MOZAIC

aircraft observations in Figure 4 shows very good agreement in the lower troposphere. At the surface,35

surface observations of different hourly intervals vary significantly, because of a strong diurnal cycle,

more pronounced in summer. Ozone soundings agree best with surface observations if the time

interval chosen is between 11am and 2pm, in agreement with the time, when most ozone soundings

are launched in this area. In the upper troposphere, MOZAIC data and ozone from soundings agree

rather well, besides some differences in the first 3-4 years. A detailed discussion of differences40

between ozonesonde, MOZAIC and surface observations for Western Europe is given in (Logan

et al., 2012).

5 Altitude distribution of ozone profiles as disucssed in the main text

The altitude distribution on pressure altitudes and tropopause-referenced altitudes is given for each

station considered in this climatology between 1995 and 2011 (see Figure 5. In addition, the me-45

dian of monthly averaged profiles between 1995-2011 is compared to 1980-1994 values if data are

available.

In Figure 6 and 7, the altitude distribution of the median of monthly averaged profiles is presented

using regional aggregates between 1995-2011 for all regions considered. In addition, the half-width

of the distribution (left) and the interannual variability (right) of each averaged profile are illustrated.50

8

Alert (1987−1993)

0 2 4 6 81000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 135.

− − − Logan Climo(01/88−12/93)DJF: 129.

Number Profiles

MAM: 91.6

− − − Logan Climo(01/88−12/93)

MAM: 82.6

Number Profiles

JJA: 71.2

− − − Logan Climo(01/88−12/93)

JJA: 57.8

Number Profiles

SON: 71.0

− − − Logan Climo(01/88−12/93)

SON: 63.8

−20 0 20 0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 135.

− − − Logan ClimoDJF: 129.

Number Profiles

MAM: 91.6

− − − Logan Climo

MAM: 82.6

Number Profiles

JJA: 71.2

− − − Logan Climo

JJA: 57.8

Number Profiles

SON: 71.0

− − − Logan Climo

SON: 63.8

0 200 400 600 80

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Number ProfilesDJF: 136.

− − − Logan Climo

Number Profiles

MAM: 68.7

− − − Logan Climo

Number Profiles

JJA: 68.8

− − − Logan Climo

Number Profiles

SON: 59.7

− − − Logan Climo

Ny_Alesund (1990−1993)

0 2 4 6 81000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 166.

− − − Logan Climo(10/90−12/93)DJF: 72.0

Number Profiles

MAM: 129.

− − − Logan Climo(10/90−12/93)

MAM: 60.5

Number Profiles

JJA: 81.1

− − − Logan Climo(10/90−12/93)

JJA: 39.8

Number Profiles

SON: 99.5

− − − Logan Climo(10/90−12/93)

SON: 45.7

−20 0 20 0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 166.

− − − Logan ClimoDJF: 72.0

Number Profiles

MAM: 129.

− − − Logan Climo

MAM: 60.5

Number Profiles

JJA: 81.1

− − − Logan Climo

JJA: 39.8

Number Profiles

SON: 99.5

− − − Logan Climo

SON: 45.7

0 200 400 600 80

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Number ProfilesDJF: 169.

− − − Logan Climo

Number Profiles

MAM: 87.0

− − − Logan Climo

Number Profiles

JJA: 72.0

− − − Logan Climo

Number Profiles

SON: 136.

− − − Logan Climo

Resolute (1980−1993)

0 2 4 6 81000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 127.

− − − Logan Climo(01/80−12/93)DJF: 122.

Number Profiles

MAM: 148.

− − − Logan Climo(01/80−12/93)

MAM: 136.

Number Profiles

JJA: 141.

− − − Logan Climo(01/80−12/93)

JJA: 124.

Number Profiles

SON: 131.

− − − Logan Climo(01/80−12/93)

SON: 116.

−20 0 20 0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 127.

− − − Logan ClimoDJF: 122.

Number Profiles

MAM: 148.

− − − Logan Climo

MAM: 136.

Number Profiles

JJA: 141.

− − − Logan Climo

JJA: 124.

Number Profiles

SON: 131.

− − − Logan Climo

SON: 116.

0 200 400 600 80

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Number ProfilesDJF: 136.

− − − Logan Climo

Number Profiles

MAM: 144.

− − − Logan Climo

Number Profiles

JJA: 134.

− − − Logan Climo

Number Profiles

SON: 137.

− − − Logan Climo

Churchill (1980−1993)

0 2 4 6 81000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 117.

− − − Logan Climo(01/80−12/93)DJF: 112.

Number Profiles

MAM: 135.

− − − Logan Climo(01/80−12/93)

MAM: 128.

Number Profiles

JJA: 146.

− − − Logan Climo(01/80−12/93)

JJA: 137.

Number Profiles

SON: 135.

− − − Logan Climo(01/80−12/93)

SON: 111.

−20 0 20 0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 117.

− − − Logan ClimoDJF: 112.

Number Profiles

MAM: 135.

− − − Logan Climo

MAM: 128.

Number Profiles

JJA: 146.

− − − Logan Climo

JJA: 137.

Number Profiles

SON: 135.

− − − Logan Climo

SON: 111.

0 200 400 600 80

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Number ProfilesDJF: 122.

− − − Logan Climo

Number Profiles

MAM: 131.

− − − Logan Climo

Number Profiles

JJA: 141.

− − − Logan Climo

Number Profiles

SON: 122.

− − − Logan Climo

Edmonton (1980−1993)

0 2 4 6 8

Ozone (ppmv)

1000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 125.

− − − Logan Climo(01/80−12/93)DJF: 115.

Number Profiles

MAM: 139.

− − − Logan Climo(01/80−12/93)

MAM: 132.

Number Profiles

JJA: 138.

− − − Logan Climo(01/80−12/93)

JJA: 128.

Number Profiles

SON: 123.

− − − Logan Climo(01/80−12/93)

SON: 108.

−20 0 20

Difference (%)

0 20 40 60 80 100 120 140

Ozone (ppbv)

1000

100 Number ProfilesDJF: 125.

− − − Logan ClimoDJF: 115.

Number Profiles

MAM: 139.

− − − Logan Climo

MAM: 132.

Number Profiles

JJA: 138.

− − − Logan Climo

JJA: 128.

Number Profiles

SON: 123.

− − − Logan Climo

SON: 108.

0 200 400 600 80

Ozone (ppbv)

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Number ProfilesDJF: 127.

− − − Logan Climo

Number Profiles

MAM: 143.

− − − Logan Climo

Number Profiles

JJA: 132.

− − − Logan Climo

Number Profiles

SON: 119.

− − − Logan Climo

Fig. 3: Vertical median profiles of seasonally averaged ozone data between 1980-1993. The pro-

files derived for this figure (solid lines) are interpolated to the same pressure levels used in (Logan,

1999a,b) (dashed lines). Differences in % between the two climatologies are shown on the right side

of the left panel. Different seasons are shown in different colors.

9

Hohenpeissenberg (1980−1993)

0 2 4 6 81000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 502.

− − − Logan Climo(01/80−12/93)DJF: 481.

Number Profiles

MAM: 458.

− − − Logan Climo(01/80−12/93)

MAM: 420.

Number Profiles

JJA: 355.

− − − Logan Climo(01/80−12/93)

JJA: 311.

Number Profiles

SON: 395.

− − − Logan Climo(01/80−12/93)

SON: 374.

−20 0 20 0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 502.

− − − Logan ClimoDJF: 481.

Number Profiles

MAM: 458.

− − − Logan Climo

MAM: 420.

Number Profiles

JJA: 355.

− − − Logan Climo

JJA: 311.

Number Profiles

SON: 395.

− − − Logan Climo

SON: 374.

0 200 400 600 80

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Number ProfilesDJF: 502.

− − − Logan Climo

Number Profiles

MAM: 353.

− − − Logan Climo

Number Profiles

JJA: 351.

− − − Logan Climo

Number Profiles

SON: 494.

− − − Logan Climo

Payerne (1980−1993)

0 2 4 6 81000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 388.

− − − Logan Climo(01/80−12/89)DJF: 275.

Number Profiles

MAM: 397.

− − − Logan Climo(01/80−12/89)

MAM: 287.

Number Profiles

JJA: 421.

− − − Logan Climo(01/80−12/89)

JJA: 276.

Number Profiles

SON: 428.

− − − Logan Climo(01/80−12/89)

SON: 280.

−20 0 20 0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 388.

− − − Logan ClimoDJF: 275.

Number Profiles

MAM: 397.

− − − Logan Climo

MAM: 287.

Number Profiles

JJA: 421.

− − − Logan Climo

JJA: 276.

Number Profiles

SON: 428.

− − − Logan Climo

SON: 280.

0 200 400 600 80

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Number ProfilesDJF: 389.Number Profiles

MAM: 426.

Number Profiles

JJA: 405.

Number Profiles

SON: 411.

Sapporo (1980−1993)

0 2 4 6 81000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 46.7

− − − Logan Climo(01/80−12/95)DJF: 64.0

Number Profiles

MAM: 58.8

− − − Logan Climo(01/80−12/95)

MAM: 69.2

Number Profiles

JJA: 61.7

− − − Logan Climo(01/80−12/95)

JJA: 46.3

Number Profiles

SON: 59.6

− − − Logan Climo(01/80−12/95)

SON: 67.1

−20 0 20 0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 46.7

− − − Logan ClimoDJF: 64.0

Number Profiles

MAM: 58.8

− − − Logan Climo

MAM: 69.2

Number Profiles

JJA: 61.7

− − − Logan Climo

JJA: 46.3

Number Profiles

SON: 59.6

− − − Logan Climo

SON: 67.1

0 200 400 600 80

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Number ProfilesDJF: 47.0

− − − Logan Climo

Number Profiles

MAM: 66.0

− − − Logan Climo

Number Profiles

JJA: 66.0

− − − Logan Climo

Number Profiles

SON: 54.0

− − − Logan Climo

Boulder (1993−1993)

0 2 4 6 81000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 9.81

− − − Logan Climo(01/85−12/93)DJF: 77.8

Number Profiles

MAM: 13.0

− − − Logan Climo(01/85−12/93)

MAM: 82.9

Number Profiles

JJA: 9.90

− − − Logan Climo(01/85−12/93)

JJA: 75.3

Number Profiles

SON: 8.00

− − − Logan Climo(01/85−12/93)

SON: 90.5

−20 0 20 0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 9.81

− − − Logan ClimoDJF: 77.8

Number Profiles

MAM: 13.0

− − − Logan Climo

MAM: 82.9

Number Profiles

JJA: 9.90

− − − Logan Climo

JJA: 75.3

Number Profiles

SON: 8.00

− − − Logan Climo

SON: 90.5

0 200 400 600 80

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Number ProfilesDJF: 9.94

− − − Logan Climo

Number Profiles

MAM: 12.0

− − − Logan Climo

Number Profiles

JJA: 9.00

− − − Logan Climo

Number Profiles

SON: 9.00

− − − Logan Climo

Wallops_Island (1980−1993)

0 2 4 6 8

Ozone (ppmv)

1000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 77.4

− − − Logan Climo(01/80−12/93)DJF: 95.7

Number Profiles

MAM: 78.0

− − − Logan Climo(01/80−12/93)

MAM: 108.

Number Profiles

JJA: 77.3

− − − Logan Climo(01/80−12/93)

JJA: 90.4

Number Profiles

SON: 76.9

− − − Logan Climo(01/80−12/93)

SON: 97.2

−20 0 20

Difference (%)

0 20 40 60 80 100 120 140

Ozone (ppbv)

1000

100 Number ProfilesDJF: 77.4

− − − Logan ClimoDJF: 95.7

Number Profiles

MAM: 78.0

− − − Logan Climo

MAM: 108.

Number Profiles

JJA: 77.3

− − − Logan Climo

JJA: 90.4

Number Profiles

SON: 76.9

− − − Logan Climo

SON: 97.2

0 200 400 600 80

Ozone (ppbv)

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Number ProfilesDJF: 77.7

− − − Logan Climo

Number Profiles

MAM: 92.2

− − − Logan Climo

Number Profiles

JJA: 87.0

− − − Logan Climo

Number Profiles

SON: 78.0

− − − Logan Climo

Fig. 3: continued

10

Tateno (1980−1993)

0 2 4 6 81000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 117.

− − − Logan Climo(01/80−12/95)DJF: 141.

Number Profiles

MAM: 100.

− − − Logan Climo(01/80−12/95)

MAM: 116.

Number Profiles

JJA: 94.7

− − − Logan Climo(01/80−12/95)

JJA: 59.4

Number Profiles

SON: 102.

− − − Logan Climo(01/80−12/95)

SON: 121.

−20 0 20 0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 117.

− − − Logan ClimoDJF: 141.

Number Profiles

MAM: 100.

− − − Logan Climo

MAM: 116.

Number Profiles

JJA: 94.7

− − − Logan Climo

JJA: 59.4

Number Profiles

SON: 102.

− − − Logan Climo

SON: 121.

0 200 400 600 80

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Number ProfilesDJF: 118.

− − − Logan Climo

Number Profiles

MAM: 96.0

− − − Logan Climo

Number Profiles

JJA: 87.0

− − − Logan Climo

Number Profiles

SON: 108.

− − − Logan Climo

Kagoshima (1980−1993)

0 2 4 6 81000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 47.9

− − − Logan Climo(01/80−12/95)DJF: 60.4

Number Profiles

MAM: 54.0

− − − Logan Climo(01/80−12/95)

MAM: 57.5

Number Profiles

JJA: 48.9

− − − Logan Climo(01/80−12/95)

JJA: 36.4

Number Profiles

SON: 60.8

− − − Logan Climo(01/80−12/95)

SON: 62.7

−20 0 20 0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 47.9

− − − Logan ClimoDJF: 60.4

Number Profiles

MAM: 54.0

− − − Logan Climo

MAM: 57.5

Number Profiles

JJA: 48.9

− − − Logan Climo

JJA: 36.4

Number Profiles

SON: 60.8

− − − Logan Climo

SON: 62.7

0 200 400 600 80

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Number ProfilesDJF: 47.7

− − − Logan Climo

Number Profiles

MAM: 48.0

− − − Logan Climo

Number Profiles

JJA: 48.0

− − − Logan Climo

Number Profiles

SON: 55.2

− − − Logan Climo

Naha (1989−1993)

0 2 4 6 81000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 38.0

− − − Logan Climo(09/89−12/95)DJF: 46.6

Number Profiles

MAM: 32.0

− − − Logan Climo(09/89−12/95)

MAM: 46.9

Number Profiles

JJA: 32.9

− − − Logan Climo(09/89−12/95)

JJA: 39.6

Number Profiles

SON: 37.9

− − − Logan Climo(09/89−12/95)

SON: 50.7

−20 0 20 0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 38.0

− − − Logan ClimoDJF: 46.6

Number Profiles

MAM: 32.0

− − − Logan Climo

MAM: 46.9

Number Profiles

JJA: 32.9

− − − Logan Climo

JJA: 39.6

Number Profiles

SON: 37.9

− − − Logan Climo

SON: 50.7

0 200 400 600 80

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Number ProfilesDJF: 38.0

− − − Logan Climo

Number Profiles

MAM: 36.0

− − − Logan Climo

Number Profiles

JJA: 36.0

− − − Logan Climo

Number Profiles

SON: 33.0

− − − Logan Climo

Natal (1980−1993)

0 2 4 6 81000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 18.7

− − − Logan Climo(11/78−10/92)DJF: 56.7

Number Profiles

MAM: 29.7

− − − Logan Climo(11/78−10/92)

MAM: 57.6

Number Profiles

JJA: 44.7

− − − Logan Climo(11/78−10/92)

JJA: 71.0

Number Profiles

SON: 39.6

− − − Logan Climo(11/78−10/92)

SON: 87.4

−20 0 20 0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 18.7

− − − Logan ClimoDJF: 56.7

Number Profiles

MAM: 29.7

− − − Logan Climo

MAM: 57.6

Number Profiles

JJA: 44.7

− − − Logan Climo

JJA: 71.0

Number Profiles

SON: 39.6

− − − Logan Climo

SON: 87.4

0 200 400 600 80

−4

−2

0

2

4R

el. A

ltitu

de (

hPa)

Number ProfilesDJF: 19.0

− − − Logan Climo

Number Profiles

MAM: 27.0

− − − Logan Climo

Number Profiles

JJA: 33.0

− − − Logan Climo

Number Profiles

SON: 30.0

− − − Logan Climo

Ascension (1990−1993)

0 2 4 6 81000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 16.0

− − − Logan Climo(07/90−10/92)DJF: 16.7

Number Profiles

MAM: 17.0

− − − Logan Climo(07/90−10/92)

MAM: 15.6

Number Profiles

JJA: 22.9

− − − Logan Climo(07/90−10/92)

JJA: 6.72

Number Profiles

SON: 35.0

− − − Logan Climo(07/90−10/92)

SON: 26.4

−20 0 20 0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 16.0

− − − Logan ClimoDJF: 16.7

Number Profiles

MAM: 17.0

− − − Logan Climo

MAM: 15.6

Number Profiles

JJA: 22.9

− − − Logan Climo

JJA: 6.72

Number Profiles

SON: 35.0

− − − Logan Climo

SON: 26.4

0 200 400 600 80

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Number ProfilesDJF: 16.0Number Profiles

MAM: 12.0

Number Profiles

JJA: 24.0

Number Profiles

SON: 12.0

Syowa (1980−1993)

0 2 4 6 8

Ozone (ppmv)

1000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 63.3

− − − Logan Climo(01/86−12/93)DJF: 38.1

Number Profiles

MAM: 61.2

− − − Logan Climo(01/86−12/93)

MAM: 39.8

Number Profiles

JJA: 65.7

− − − Logan Climo(01/86−12/93)

JJA: 45.5

Number Profiles

SON: 129.

− − − Logan Climo(01/86−12/93)

SON: 85.4

−20 0 20

Difference (%)

0 20 40 60 80 100 120 140

Ozone (ppbv)

1000

100 Number ProfilesDJF: 63.3

− − − Logan ClimoDJF: 38.1

Number Profiles

MAM: 61.2

− − − Logan Climo

MAM: 39.8

Number Profiles

JJA: 65.7

− − − Logan Climo

JJA: 45.5

Number Profiles

SON: 129.

− − − Logan Climo

SON: 85.4

0 200 400 600 80

Ozone (ppbv)

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Number ProfilesDJF: 63.5Number Profiles

MAM: 32.2

Number Profiles

JJA: 80.5

Number Profiles

SON: 113.

Fig. 3: continued

11

Debilt

Hohenpeissenberg

Lindenberg

Payerne

PrahaUccle

Zingst−Arkona

Zugspitze

Frankfurt

Western Europe Winter

1980 1990 2000

40

50

60

70

80

90

Ozo

ne (

ppbv

)

525_475 hPa

Western Europe Spring

1980 1990 2000

40

50

60

70

80

90

525_475 hPa

Western Europe Summer

1980 1990 2000

40

50

60

70

80

90

525_475 hPa

Western Europe Fall

1980 1990 2000

40

50

60

70

80

90

525_475 hPa

1980 1990 200010

20

30

40

50

60

70

Ozo

ne (

ppbv

)

Zugspitze

850_750 hPa

1980 1990 200010

20

30

40

50

60

70

850_750 hPa

1980 1990 200010

20

30

40

50

60

70

850_750 hPa

1980 1990 200010

20

30

40

50

60

70

850_750 hPa

1980 1990 200010

20

30

40

50

60

70

Ozo

ne (

ppbv

)

Hohenpeissenberg

950_850 hPa Soundings Surface (11am−2pm) Surface (4−8am) Surface (4−8pm) MOZAIC

1980 1990 200010

20

30

40

50

60

70

950_850 hPa

1980 1990 200010

20

30

40

50

60

70

950_850 hPa

1980 1990 200010

20

30

40

50

60

70

950_850 hPa

1980 1990 2000

Years

10

20

30

40

50

60

70

Ozo

ne (

ppbv

)

Zingst−Arkona

1050_950 hPa

1980 1990 2000

Years

10

20

30

40

50

60

70

1050_950 hPa

1980 1990 2000

Years

10

20

30

40

50

60

70

1050_950 hPa

1980 1990 2000

Years

10

20

30

40

50

60

70

1050_950 hPa

Fig. 4: Top panel: Map of ozone stations (black asterisks), surface stations (diamonds) and airport

(triangle) considered. Second to fifth row: Comparison of ozone timelines between ozone sound-

ings (black asterisk: top panel, and black lines: bottom panels), surface ozone observations (red

diamonds, and red lines: bottom panels), and MOZAIC aircraft observations (blue triangle: top

panel, and blue lines: bottom panels) over Western Europe for different pressure levels. Altitude

information of surface stations are included (different sizes of diamonds, going from small to large

with increasing altitude). Seasonal averages of hourly surface observations are further separated into

three different time intervals of the day (see legend).

12

Alert (1995−2008)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 163.

1987−1994DJF: 133.

Number Profiles

MAM: 153.

1987−1994

MAM: 90.2

Number Profiles

JJA: 130.

1987−1994

JJA: 70.0

Number Profiles

SON: 138.

1987−1994

SON: 69.7

−50 −20 0 20 50 0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 163.

1987−1994DJF: 133.

Number Profiles

MAM: 153.

1987−1994

MAM: 90.2

Number Profiles

JJA: 130.

1987−1994

JJA: 70.0

Number Profiles

SON: 138.

1987−1994

SON: 69.7

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

1987−1994DJF: 136.

Number ProfilesDJF: 177.

1987−1994

MAM: 68.7

Number Profiles

MAM: 157.

1987−1994

JJA: 68.8

Number Profiles

JJA: 134.

1987−1994

SON: 59.7

Number Profiles

SON: 145.

Eureka (1995−2008)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 354.

1992−1994DJF: 22.4

Number Profiles

MAM: 281.

1992−1994

MAM: 17.5

Number Profiles

JJA: 157.

1992−1994

JJA: 16.3

Number Profiles

SON: 156.

1992−1994

SON: 22.5

−50 −20 0 20 50 0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 354.

1992−1994DJF: 22.4

Number Profiles

MAM: 281.

1992−1994

MAM: 17.5

Number Profiles

JJA: 157.

1992−1994

JJA: 16.3

Number Profiles

SON: 156.

1992−1994

SON: 22.5

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

1992−1994DJF: 22.9

Number ProfilesDJF: 374.Number Profiles

MAM: 166.

Number Profiles

JJA: 164.

1992−1994

SON: 27.0

Number Profiles

SON: 170.

Ny_Alesund (1995−2006)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 378.

1990−1994DJF: 163.

Number Profiles

MAM: 322.

1990−1994

MAM: 128.

Number Profiles

JJA: 180.

1990−1994

JJA: 79.5

Number Profiles

SON: 187.

1990−1994

SON: 97.1

−50 −20 0 20 50 0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 378.

1990−1994DJF: 163.

Number Profiles

MAM: 322.

1990−1994

MAM: 128.

Number Profiles

JJA: 180.

1990−1994

JJA: 79.5

Number Profiles

SON: 187.

1990−1994

SON: 97.1

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

1990−1994DJF: 169.

Number ProfilesDJF: 390.

1990−1994

MAM: 87.0

Number Profiles

MAM: 224.

1990−1994

JJA: 72.0

Number Profiles

JJA: 185.

1990−1994

SON: 136.

Number Profiles

SON: 216.

Resolute (1995−2007)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 125.

1980−1994DJF: 120.

Number Profiles

MAM: 102.

1980−1994

MAM: 145.

Number Profiles

JJA: 90.2

1980−1994

JJA: 139.

Number Profiles

SON: 92.7

1980−1994

SON: 127.

−50 −20 0 20 50 0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 125.

1980−1994DJF: 120.

Number Profiles

MAM: 102.

1980−1994

MAM: 145.

Number Profiles

JJA: 90.2

1980−1994

JJA: 139.

Number Profiles

SON: 92.7

1980−1994

SON: 127.

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

1980−1994DJF: 136.

Number ProfilesDJF: 139.

1980−1994

MAM: 144.

Number Profiles

MAM: 92.5

1980−1994

JJA: 134.

Number Profiles

JJA: 77.1

1980−1994

SON: 137.

Number Profiles

SON: 97.4

Scoresbysund (1995−2003)

0 2 4 6

Ozone (ppmv)

1000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 139.

1989−1994DJF: 42.3

Number Profiles

MAM: 110.

1989−1994

MAM: 50.5

Number Profiles

JJA: 93.1

1989−1994

JJA: 51.4

Number Profiles

SON: 98.7

1989−1994

SON: 51.3

−50 −20 0 20 50

Difference (%)

0 20 40 60 80 100 120 140

Ozone (ppbv)

1000

100 Number ProfilesDJF: 139.

1989−1994DJF: 42.3

Number Profiles

MAM: 110.

1989−1994

MAM: 50.5

Number Profiles

JJA: 93.1

1989−1994

JJA: 51.4

Number Profiles

SON: 98.7

1989−1994

SON: 51.3

0 200 400 600 800

Ozone (ppbv)

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

1989−1994DJF: 44.4

Number ProfilesDJF: 145.

1989−1994

MAM: 50.4

Number Profiles

MAM: 110.

1989−1994

JJA: 50.4

Number Profiles

JJA: 86.7

1989−1994

SON: 50.0

Number Profiles

SON: 91.8

Fig. 5: Vertical profiles of seasonally averaged ozone profiles (median) between 1995 and 2011

(solid lines) and 1980 and 1994 (dashed-dotted lines, if available). The total number of profiles used

for the period 1995-2011 are shown on the left top and for the period between 1980-1994 on the

right bottom (if available) of each panel. In 1980-1994 most of the stations show a much smaller

sampling frequency than 1995-2011. Differences between the two periods considered are shown on

the right of the left panel. Different seasons are shown in different colors.

13

Lerwick (1995−2008)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 263.

1992−1994DJF: 31.5

Number Profiles

MAM: 202.

1992−1994

MAM: 7.65

Number Profiles

JJA: 138.

1992−1994

JJA: 8.65

Number Profiles

SON: 161.

1992−1994

SON: 10.7

−50 −20 0 20 50 0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 263.

1992−1994DJF: 31.5

Number Profiles

MAM: 202.

1992−1994

MAM: 7.65

Number Profiles

JJA: 138.

1992−1994

JJA: 8.65

Number Profiles

SON: 161.

1992−1994

SON: 10.7

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

1992−1994DJF: 32.0

Number ProfilesDJF: 267.Number Profiles

MAM: 118.

Number Profiles

JJA: 119.

Number Profiles

SON: 165.

Churchill (1995−2007)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 150.

1980−1994DJF: 112.

Number Profiles

MAM: 149.

1980−1994

MAM: 133.

Number Profiles

JJA: 109.

1980−1994

JJA: 143.

Number Profiles

SON: 122.

1980−1994

SON: 132.

−50 −20 0 20 50 0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 150.

1980−1994DJF: 112.

Number Profiles

MAM: 149.

1980−1994

MAM: 133.

Number Profiles

JJA: 109.

1980−1994

JJA: 143.

Number Profiles

SON: 122.

1980−1994

SON: 132.

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

1980−1994DJF: 122.

Number ProfilesDJF: 157.

1980−1994

MAM: 131.

Number Profiles

MAM: 149.

1980−1994

JJA: 141.

Number Profiles

JJA: 127.

1980−1994

SON: 122.

Number Profiles

SON: 130.

Edmonton (1995−2008)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 156.

1980−1994DJF: 122.

Number Profiles

MAM: 193.

1980−1994

MAM: 137.

Number Profiles

JJA: 165.

1980−1994

JJA: 137.

Number Profiles

SON: 154.

1980−1994

SON: 121.

−50 −20 0 20 50 0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 156.

1980−1994DJF: 122.

Number Profiles

MAM: 193.

1980−1994

MAM: 137.

Number Profiles

JJA: 165.

1980−1994

JJA: 137.

Number Profiles

SON: 154.

1980−1994

SON: 121.

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

1980−1994DJF: 127.

Number ProfilesDJF: 163.

1980−1994

MAM: 143.

Number Profiles

MAM: 182.

1980−1994

JJA: 132.

Number Profiles

JJA: 153.

1980−1994

SON: 119.

Number Profiles

SON: 158.

Goose_bay (1995−2007)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 151.

1980−1994DJF: 136.

Number Profiles

MAM: 147.

1980−1994

MAM: 151.

Number Profiles

JJA: 148.

1980−1994

JJA: 134.

Number Profiles

SON: 141.

1980−1994

SON: 131.

−50 −20 0 20 50 0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 151.

1980−1994DJF: 136.

Number Profiles

MAM: 147.

1980−1994

MAM: 151.

Number Profiles

JJA: 148.

1980−1994

JJA: 134.

Number Profiles

SON: 141.

1980−1994

SON: 131.

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

1980−1994DJF: 143.

Number ProfilesDJF: 156.

1980−1994

MAM: 148.

Number Profiles

MAM: 143.

1980−1994

JJA: 143.

Number Profiles

JJA: 153.

1980−1994

SON: 140.

Number Profiles

SON: 131.

Legionowo (1995−2009)

0 2 4 6

Ozone (ppmv)

1000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 251.

1993−1994DJF: 3.96

Number Profiles

MAM: 237.

1993−1994

MAM: 3.96

Number Profiles

JJA: 186.

1993−1994

JJA: 10.8

Number Profiles

SON: 178.

1993−1994

SON: 11.7

0 20 40 60 80 100 120 140

Ozone (ppbv)

1000

100 Number ProfilesDJF: 251.

1993−1994DJF: 3.96

Number Profiles

MAM: 237.

1993−1994

MAM: 3.96

Number Profiles

JJA: 186.

1993−1994

JJA: 10.8

Number Profiles

SON: 178.

1993−1994

SON: 11.7

0 200 400 600 800

Ozone (ppbv)

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Number ProfilesDJF: 254.Number Profiles

MAM: 194.

Number Profiles

JJA: 185.

Number Profiles

SON: 167.

Fig. 5: continued

14

Lindenberg (1995−2009)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 198.

1992−1994DJF: 38.6

Number Profiles

MAM: 188.

1992−1994

MAM: 24.8

Number Profiles

JJA: 196.

1992−1994

JJA: 27.8

Number Profiles

SON: 169.

1992−1994

SON: 21.9

−50 −20 0 20 50 0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 198.

1992−1994DJF: 38.6

Number Profiles

MAM: 188.

1992−1994

MAM: 24.8

Number Profiles

JJA: 196.

1992−1994

JJA: 27.8

Number Profiles

SON: 169.

1992−1994

SON: 21.9

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

1992−1994DJF: 38.7

Number ProfilesDJF: 200.Number Profiles

MAM: 188.

1992−1994

JJA: 21.0

Number Profiles

JJA: 207.

Number Profiles

SON: 158.

Debilt (1995−2009)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 110.

1992−1994DJF: 0.00

Number Profiles

MAM: 93.8

1992−1994

MAM: 0.00

Number Profiles

JJA: 101.

1992−1994

JJA: 0.00

Number Profiles

SON: 112.

1992−1994

SON: 0.00

0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 110.

1992−1994DJF: 0.00

Number Profiles

MAM: 93.8

1992−1994

MAM: 0.00

Number Profiles

JJA: 101.

1992−1994

JJA: 0.00

Number Profiles

SON: 112.

1992−1994

SON: 0.00

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Number ProfilesDJF: 113.Number Profiles

MAM: 81.0

Number Profiles

JJA: 105.

Number Profiles

SON: 106.

Uccle (1995−2007)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 414.

1980−1994DJF: 278.

Number Profiles

MAM: 446.

1980−1994

MAM: 356.

Number Profiles

JJA: 496.

1980−1994

JJA: 359.

Number Profiles

SON: 449.

1980−1994

SON: 342.

−50 −20 0 20 50 0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 414.

1980−1994DJF: 278.

Number Profiles

MAM: 446.

1980−1994

MAM: 356.

Number Profiles

JJA: 496.

1980−1994

JJA: 359.

Number Profiles

SON: 449.

1980−1994

SON: 342.

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Number ProfilesDJF: 422.Number Profiles

MAM: 414.

Number Profiles

JJA: 493.

Number Profiles

SON: 411.

Praha (1995−2009)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 320.

1992−1994DJF: 44.3

Number Profiles

MAM: 490.

1992−1994

MAM: 68.7

−20 0 20 0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 320.

1992−1994DJF: 44.3

Number Profiles

MAM: 490.

1992−1994

MAM: 68.7

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

1992−1994DJF: 44.8

Number ProfilesDJF: 320.

1992−1994

MAM: 67.0

Number Profiles

MAM: 475.

Hohenpeissenberg (1995−2009)

0 2 4 6

Ozone (ppmv)

1000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 484.

1980−1994DJF: 499.

Number Profiles

MAM: 461.

1980−1994

MAM: 456.

Number Profiles

JJA: 377.

1980−1994

JJA: 353.

Number Profiles

SON: 411.

1980−1994

SON: 393.

−50 −20 0 20 50

Difference (%)

0 20 40 60 80 100 120 140

Ozone (ppbv)

1000

100 Number ProfilesDJF: 484.

1980−1994DJF: 499.

Number Profiles

MAM: 461.

1980−1994

MAM: 456.

Number Profiles

JJA: 377.

1980−1994

JJA: 353.

Number Profiles

SON: 411.

1980−1994

SON: 393.

0 200 400 600 800

Ozone (ppbv)

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

1980−1994DJF: 502.

Number ProfilesDJF: 488.

1980−1994

MAM: 353.

Number Profiles

MAM: 377.

1980−1994

JJA: 351.

Number Profiles

JJA: 393.

1980−1994

SON: 494.

Number Profiles

SON: 496.

Fig. 5: continued

15

Payerne (1995−2011)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 642.

1980−1994DJF: 380.

Number Profiles

MAM: 669.

1980−1994

MAM: 391.

Number Profiles

JJA: 665.

1980−1994

JJA: 414.

Number Profiles

SON: 659.

1980−1994

SON: 420.

−50 −20 0 20 50 0 20 40 60 80 100 120 1401000

100

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Sapporo (1995−2009)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 160.

1980−1994DJF: 45.8

Number Profiles

MAM: 167.

1980−1994

MAM: 57.9

Number Profiles

JJA: 149.

1980−1994

JJA: 60.5

Number Profiles

SON: 163.

1980−1994

SON: 58.4

−50 −20 0 20 50 0 20 40 60 80 100 120 1401000

100

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Madrid (1995−2011)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 169.

1994−1994DJF: 0.00

Number Profiles

MAM: 169.

1994−1994

MAM: 0.00

Number Profiles

JJA: 168.

1994−1994

JJA: 0.00

Number Profiles

SON: 160.

1994−1994

SON: 0.00

0 20 40 60 80 100 120 1401000

100

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Trinidathead (1997−2011)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 92.8

1980−1994DJF: 0.00

Number Profiles

MAM: 137.

1980−1994

MAM: 0.00

Number Profiles

JJA: 160.

1980−1994

JJA: 0.00

Number Profiles

SON: 134.

1980−1994

SON: 0.00

0 20 40 60 80 100 120 1401000

100

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Boulder (1995−2009)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 155.

1993−1994DJF: 9.62

Number Profiles

MAM: 168.

1993−1994

MAM: 12.8

Number Profiles

JJA: 226.

1993−1994

JJA: 9.75

Number Profiles

SON: 171.

1993−1994

SON: 7.95

0 20 40 60 80 100 120 1401000

100

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Wallops_Island (1995−2011)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 274.

1980−1994DJF: 75.7

Number Profiles

MAM: 271.

1980−1994

MAM: 76.5

Number Profiles

JJA: 301.

1980−1994

JJA: 76.4

Number Profiles

SON: 281.

1980−1994

SON: 76.0

−50 −20 0 20 50 0 20 40 60 80 100 120 1401000

100

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Fig. 5: continued

16

Tateno (1995−2009)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 228.

1980−1994DJF: 116.

Number Profiles

MAM: 233.

1980−1994

MAM: 99.8

Number Profiles

JJA: 166.

1980−1994

JJA: 93.5

Number Profiles

SON: 179.

1980−1994

SON: 102.

−50 −20 0 20 50 0 20 40 60 80 100 120 1401000

100

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Huntsville (1999−2007)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 114.

1980−1994DJF: 0.00

Number Profiles

MAM: 154.

1980−1994

MAM: 0.00

Number Profiles

JJA: 166.

1980−1994

JJA: 0.00

Number Profiles

SON: 131.

1980−1994

SON: 0.00

0 20 40 60 80 100 120 1401000

100

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Kagoshima (1995−2005)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 132.

1980−1994DJF: 48.5

Number Profiles

MAM: 112.

1980−1994

MAM: 55.3

Number Profiles

JJA: 109.

1980−1994

JJA: 50.2

Number Profiles

SON: 126.

1980−1994

SON: 60.0

−50 −20 0 20 50 0 20 40 60 80 100 120 1401000

100

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Naha (1995−2008)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 140.

1989−1994DJF: 37.8

Number Profiles

MAM: 141.

1989−1994

MAM: 31.9

Number Profiles

JJA: 132.

1989−1994

JJA: 32.6

Number Profiles

SON: 145.

1989−1994

SON: 37.7

−50 −20 0 20 50 0 20 40 60 80 100 120 1401000

100

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Hongkong (2000−2011)

0 2 4 6

Ozone (ppmv)

1000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 105.

1980−1994DJF: 0.00

Number Profiles

MAM: 134.

1980−1994

MAM: 0.00

Number Profiles

JJA: 120.

1980−1994

JJA: 0.00

Number Profiles

SON: 127.

1980−1994

SON: 0.00

0 20 40 60 80 100 120 140

Ozone (ppbv)

1000

100

0 200 400 600 800

Ozone (ppbv)

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Fig. 5: continued

17

Hilo (1996−2011)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 151.

1982−1994DJF: 102.

Number Profiles

MAM: 185.

1982−1994

MAM: 105.

Number Profiles

JJA: 187.

1982−1994

JJA: 105.

Number Profiles

SON: 175.

1982−1994

SON: 108.

−50 −20 0 20 50 0 20 40 60 80 100 120 1401000

100

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Paramaribo (2000−2010)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 93.5

1980−1994DJF: 0.00

Number Profiles

MAM: 105.

1980−1994

MAM: 0.00

Number Profiles

JJA: 106.

1980−1994

JJA: 0.00

Number Profiles

SON: 111.

1980−1994

SON: 0.00

0 20 40 60 80 100 120 1401000

100

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Sancristobal (1998−2008)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 67.5

1980−1994DJF: 0.00

Number Profiles

MAM: 85.6

1980−1994

MAM: 0.00

Number Profiles

JJA: 95.1

1980−1994

JJA: 0.00

Number Profiles

SON: 110.

1980−1994

SON: 0.00

0 20 40 60 80 100 120 1401000

100

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Nairobi (1996−2010)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 132.

1980−1994DJF: 0.00

Number Profiles

MAM: 147.

1980−1994

MAM: 0.00

Number Profiles

JJA: 144.

1980−1994

JJA: 0.00

Number Profiles

SON: 146.

1980−1994

SON: 0.00

0 20 40 60 80 100 120 1401000

100

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Natal (1995−2010)

0 2 4 6

Ozone (ppmv)

1000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 113.

1980−1994DJF: 18.3

Number Profiles

MAM: 115.

1980−1994

MAM: 29.3

Number Profiles

JJA: 126.

1980−1994

JJA: 44.3

Number Profiles

SON: 132.

1980−1994

SON: 38.4

−50 −20 0 20 50

Difference (%)

0 20 40 60 80 100 120 140

Ozone (ppbv)

1000

100

0 200 400 600 800

Ozone (ppbv)

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Fig. 5: continued

18

Ascension (1995−2009)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 121.

1990−1994DJF: 15.7

Number Profiles

MAM: 132.

1990−1994

MAM: 16.7

Number Profiles

JJA: 125.

1990−1994

JJA: 22.6

Number Profiles

SON: 156.

1990−1994

SON: 34.5

−50 −20 0 20 50 0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 121.

1990−1994DJF: 15.7

Number Profiles

MAM: 132.

1990−1994

MAM: 16.7

Number Profiles

JJA: 125.

1990−1994

JJA: 22.6

Number Profiles

SON: 156.

1990−1994

SON: 34.5

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Number ProfilesDJF: 121.Number Profiles

MAM: 123.

1990−1994

JJA: 24.0

Number Profiles

JJA: 141.

Number Profiles

SON: 162.

Java (1998−2009)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 48.0

1980−1994DJF: 0.00

Number Profiles

MAM: 53.0

1980−1994

MAM: 0.00

Number Profiles

JJA: 66.0

1980−1994

JJA: 0.00

Number Profiles

SON: 72.0

1980−1994

SON: 0.00

0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 48.0

1980−1994DJF: 0.00

Number Profiles

MAM: 53.0

1980−1994

MAM: 0.00

Number Profiles

JJA: 66.0

1980−1994

JJA: 0.00

Number Profiles

SON: 72.0

1980−1994

SON: 0.00

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Number ProfilesDJF: 48.0Number Profiles

MAM: 60.0

Number Profiles

JJA: 75.0

Number Profiles

SON: 57.0

Samoa (1995−2009)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 115.

1980−1994DJF: 0.00

Number Profiles

MAM: 120.

1980−1994

MAM: 0.00

Number Profiles

JJA: 118.

1980−1994

JJA: 0.00

Number Profiles

SON: 121.

1980−1994

SON: 0.00

0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 115.

1980−1994DJF: 0.00

Number Profiles

MAM: 120.

1980−1994

MAM: 0.00

Number Profiles

JJA: 118.

1980−1994

JJA: 0.00

Number Profiles

SON: 121.

1980−1994

SON: 0.00

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Number ProfilesDJF: 116.Number Profiles

MAM: 114.

Number Profiles

JJA: 144.

Number Profiles

SON: 123.

Fiji (1997−2008)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 64.0

1980−1994DJF: 0.00

Number Profiles

MAM: 88.9

1980−1994

MAM: 0.00

Number Profiles

JJA: 78.8

1980−1994

JJA: 0.00

Number Profiles

SON: 75.0

1980−1994

SON: 0.00

0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 64.0

1980−1994DJF: 0.00

Number Profiles

MAM: 88.9

1980−1994

MAM: 0.00

Number Profiles

JJA: 78.8

1980−1994

JJA: 0.00

Number Profiles

SON: 75.0

1980−1994

SON: 0.00

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Number ProfilesDJF: 64.0Number Profiles

MAM: 63.0

Number Profiles

JJA: 72.0

Number Profiles

SON: 72.0

Reunion (1998−2009)

0 2 4 6

Ozone (ppmv)

1000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 73.0

1980−1994DJF: 0.00

Number Profiles

MAM: 95.0

1980−1994

MAM: 0.00

Number Profiles

JJA: 87.0

1980−1994

JJA: 0.00

Number Profiles

SON: 89.0

1980−1994

SON: 0.00

0 20 40 60 80 100 120 140

Ozone (ppbv)

1000

100 Number ProfilesDJF: 73.0

1980−1994DJF: 0.00

Number Profiles

MAM: 95.0

1980−1994

MAM: 0.00

Number Profiles

JJA: 87.0

1980−1994

JJA: 0.00

Number Profiles

SON: 89.0

1980−1994

SON: 0.00

0 200 400 600 800

Ozone (ppbv)

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Number ProfilesDJF: 73.0Number Profiles

MAM: 90.0

Number Profiles

JJA: 66.0

Number Profiles

SON: 90.0

Fig. 5: continued

19

Broadmeadows (1999−2009)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 56.3

1980−1994DJF: 0.00

Number Profiles

MAM: 75.8

1980−1994

MAM: 0.00

Number Profiles

JJA: 79.8

1980−1994

JJA: 0.00

Number Profiles

SON: 78.9

1980−1994

SON: 0.00

0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 56.3

1980−1994DJF: 0.00

Number Profiles

MAM: 75.8

1980−1994

MAM: 0.00

Number Profiles

JJA: 79.8

1980−1994

JJA: 0.00

Number Profiles

SON: 78.9

1980−1994

SON: 0.00

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Number ProfilesDJF: 56.9Number Profiles

MAM: 71.8

Number Profiles

JJA: 84.0

Number Profiles

SON: 69.0

Lauder (1995−2008)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 139.

1986−1994DJF: 47.6

Number Profiles

MAM: 154.

1986−1994

MAM: 40.1

Number Profiles

JJA: 144.

1986−1994

JJA: 60.1

Number Profiles

SON: 172.

1986−1994

SON: 86.6

−50 −20 0 20 50 0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 139.

1986−1994DJF: 47.6

Number Profiles

MAM: 154.

1986−1994

MAM: 40.1

Number Profiles

JJA: 144.

1986−1994

JJA: 60.1

Number Profiles

SON: 172.

1986−1994

SON: 86.6

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

1986−1994DJF: 48.8

Number ProfilesDJF: 140.

1986−1994

MAM: 42.0

Number Profiles

MAM: 143.

1986−1994

JJA: 94.4

Number Profiles

JJA: 143.

1986−1994

SON: 80.1

Number Profiles

SON: 189.

Macquarie (1995−2009)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 90.0

1994−1994DJF: 0.00

Number Profiles

MAM: 109.

1994−1994

MAM: 0.00

Number Profiles

JJA: 110.

1994−1994

JJA: 0.00

Number Profiles

SON: 102.

1994−1994

SON: 0.00

0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 90.0

1994−1994DJF: 0.00

Number Profiles

MAM: 109.

1994−1994

MAM: 0.00

Number Profiles

JJA: 110.

1994−1994

JJA: 0.00

Number Profiles

SON: 102.

1994−1994

SON: 0.00

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Number ProfilesDJF: 91.3Number Profiles

MAM: 98.5

Number Profiles

JJA: 104.

Number Profiles

SON: 95.4

Marambio (1995−2009)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 49.1

1988−1994DJF: 27.1

Number Profiles

MAM: 35.9

1988−1994

MAM: 31.0

Number Profiles

JJA: 108.

1988−1994

JJA: 44.8

Number Profiles

SON: 124.

1988−1994

SON: 95.8

−50 −20 0 20 50 0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 49.1

1988−1994DJF: 27.1

Number Profiles

MAM: 35.9

1988−1994

MAM: 31.0

Number Profiles

JJA: 108.

1988−1994

JJA: 44.8

Number Profiles

SON: 124.

1988−1994

SON: 95.8

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

1988−1994DJF: 28.6

Number ProfilesDJF: 49.9

1988−1994

MAM: 30.0

Number Profiles

MAM: 37.2

1988−1994

JJA: 65.1

Number Profiles

JJA: 145.

1988−1994

SON: 99.0

Number Profiles

SON: 143.

Syowa (1995−2009)

0 2 4 61000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 176.

1980−1994DJF: 62.2

Number Profiles

MAM: 164.

1980−1994

MAM: 60.1

Number Profiles

JJA: 227.

1980−1994

JJA: 64.1

Number Profiles

SON: 266.

1980−1994

SON: 126.

−50 −20 0 20 50 0 20 40 60 80 100 120 1401000

100 Number ProfilesDJF: 176.

1980−1994DJF: 62.2

Number Profiles

MAM: 164.

1980−1994

MAM: 60.1

Number Profiles

JJA: 227.

1980−1994

JJA: 64.1

Number Profiles

SON: 266.

1980−1994

SON: 126.

0 200 400 600 800

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

1980−1994DJF: 63.5

Number ProfilesDJF: 177.

1980−1994

MAM: 32.2

Number Profiles

MAM: 226.

1980−1994

JJA: 80.5

Number Profiles

JJA: 269.

1980−1994

SON: 113.

Number Profiles

SON: 267.

Neumayer (1995−2009)

0 2 4 6

Ozone (ppmv)

1000

100

10

Alti

tude

(hP

a)

Number ProfilesDJF: 215.

1992−1994DJF: 16.1

Number Profiles

MAM: 182.

1992−1994

MAM: 18.6

Number Profiles

JJA: 242.

1992−1994

JJA: 25.3

Number Profiles

SON: 361.

1992−1994

SON: 42.3

−50 −20 0 20 50

Difference (%)

0 20 40 60 80 100 120 140

Ozone (ppbv)

1000

100 Number ProfilesDJF: 215.

1992−1994DJF: 16.1

Number Profiles

MAM: 182.

1992−1994

MAM: 18.6

Number Profiles

JJA: 242.

1992−1994

JJA: 25.3

Number Profiles

SON: 361.

1992−1994

SON: 42.3

0 200 400 600 800

Ozone (ppbv)

−4

−2

0

2

4

Rel

. Alti

tude

(hP

a)

Number ProfilesDJF: 216.

1992−1994

MAM: 22.8

Number Profiles

MAM: 202.

1992−1994

JJA: 28.7

Number Profiles

JJA: 304.

1992−1994

SON: 43.1

Number Profiles

SON: 298.

Fig. 5: continued

20

NH Polar East

20 40 60 801000

600

400

300

200

Alti

tude

(hP

a)

TotalDJF 871

Total

MAM 498

Total

JJA 438

Total

SON 531

LerwickNy_AlesundScoresbysund

10 50 10 50

NH Polar West

20 40 60 80

TotalDJF 882

Total

MAM 540

Total

JJA 486

Total

SON 525

AlertEurekaResolute

10 50 10 50

Canada

20 40 60 801000

600

400

300

200

Alti

tude

(hP

a)

TotalDJF 604

Total

MAM 594

Total

JJA 564

Total

SON 543

ChurchillEdmontonGoose_bay

10 50 10 50

Western Europe

20 40 60 80

TotalDJF 2880

Total

MAM 2850

Total

JJA 2994

Total

SON 2919

DebiltHohenpeissenbergLegionowoLindenbergPayernePrahaUccle

10 50 10 50

Eastern US

20 40 60 80

Ozone (ppbv)

1000

600

400

300

200

Alti

tude

(hP

a)

TotalDJF 397

Total

MAM 414

Total

JJA 507

Total

SON 405

HuntsvilleWallops_Island

10 50

H−Width (%)

10 50

Interan. (%)

Japan

20 40 60 80

Ozone (ppbv)

TotalDJF 364

Total

MAM 303

Total

JJA 282

Total

SON 315

KagoshimaTateno

10 50

H−Width (%)

10 50

Interan. (%)

Fig. 6: Altitude distributions (median) of ozone soundings averaged for different seasons and re-

gions in the Northern Hemisphere between 1995 and 2011. Different colors indicate different sea-

sons. The total number of profiles used for each season and region is shown on the top left of each

panel. The stations entering the profiles are noted in the lower right of each panel. The half-width

of the distribution (left) and the interannual variability (right) of each averaged profile are illustrated

on two sub-plots on the right of each panel. The half-width of the distribution is defined here as the

range of the 25th and 75th percentile of the regionally-aggregated ozone distribution (calculated as:

(75th percentile - 25th percentile)/2). The interannual variability is defined as the range of the 5th and

95th percentile of the annual median ozone value (calculated as: (95th percentile - 5th percentile)/2)

for all seasons and regions.

21

NH Subtropic

0 20 40 60 801000

600

400

200

100

Alti

tude

(hP

a)

TotalDJF 413

Total

MAM 447

Total

JJA 510

Total

SON 438

HiloHongkongNaha

10 50 10 50

W−Pacific/E−Indian Ocean

0 20 40 60 80

TotalDJF 268

Total

MAM 276

Total

JJA 348

Total

SON 330

FijiWatukosekSamoa

10 50 10 50

equat.Americas

0 20 40 60 80

Ozone (ppbv)

1000

600

400

200

100

Alti

tude

(hP

a)

TotalDJF 164

Total

MAM 165

Total

JJA 207

Total

SON 198

ParamariboSancristobal

10 50

H−Width (%)

10 50

Interan. (%)

Atlantic/Africa

0 20 40 60 80

Ozone (ppbv)

TotalDJF 382

Total

MAM 393

Total

JJA 429

Total

SON 432

AscensionNairobiNatal

10 50

H−Width (%)

10 50

Interan. (%)

SH Midlat

20 40 60 80

Ozone (ppbv)

1000

600

400

300

200

Alti

tude

(hP

a)

TotalDJF 317

Total

MAM 327

Total

JJA 345

Total

SON 378

LauderMacquarie

10 50

H−Width (%)

10 50

Interan. (%)

SH Polar

20 40 60 80

Ozone (ppbv)

TotalDJF 578

Total

MAM 570

Total

JJA 927

Total

SON 930

MarambioNeumayerSyowa

10 50

H−Width (%)

10 50

Interan. (%)

Fig. 7: As Figure 6, but showing regions in the tropics and the Southern Hemisphere.

References

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and development of a gridded climatology for tropospheric ozone, J. Geophys. Res., 104, 16 115–16 150,

1999a.55

Logan, J. A., An analysis of ozonesonde data for the lower stratosphere: Recommendations for testing models,

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Logan, J. A., Staehelin, J., Megretskaia, I. A., Cammas, J.-P., Thouret, V., Claude, H., Backer, H. D., Stein-

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Thouret, V., Marenco, A., Logan, J., Nedelec, P., and Grouhel, C., Comparisons of ozone measurements from

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the MOZAIC airborne program and the ozone sounding network at eight locations, J. Geophys. Res., 1003,

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23