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  • 8/3/2019 Sergey B Leonov and Dmitry A Yarantsev- Plasma-induced ignition and plasma-assisted combustion in high-speed fl

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    INSTITUTE OF PHYSICS PUBLISHING PLASMA SOURCES SCIENCE AND TECHNOLOGY

    Plasma Sources Sci. Technol. 16 (2007) 132138 doi:10.1088/0963-0252/16/1/018

    Plasma-induced ignition and

    plasma-assisted combustion in high-speedflow

    Sergey B Leonov and Dmitry A Yarantsev

    Institute of High Temperatures RAS (IVTAN), Izhorskaya str., 13/19, Moscow, 125412,

    Russia

    E-mail: [email protected] and [email protected]

    Received 17 March 2006, in final form 10 July 2006Published 20 December 2006Online at stacks.iop.org/PSST/16/132

    AbstractThe suitability of the electrical discharge technique for application inplasma-induced ignition and plasma-assisted combustion in high-speed flowis reviewed. Nonequilibrium, unsteady and nonuniform modes are underanalysis to demonstrate the advantage of such a technique over heating. Areduction in the required power deposition is possible due to unsteadyoperation and non-homogeneous spatial distribution. Mixing intensificationin non-premixed flow could be achieved by nonuniform electricaldischarges. The scheme of fuel ignition behind the wallstep and in the cavityis under consideration. Experimental results on multi-electrode dischargemaintenance in the separation zone of supersonic flow are presented. The

    model test on hydrogen and ethylene ignition is demonstrated at direct fuelinjection. An energetic threshold of fuel ignition under separation and in theshear layer is measured under the experimental conditions.

    (Some figures in this article are in colour only in the electronic version)

    1. Introduction. Plasma-assisted combustionapproach

    Analysis of supersonic combustor performance shows that

    several principal problems related to supersonic combustion

    and flame stabilization are to be solved for the practical

    implementation of such a technology, especially in the case ofhydrocarbon fuels. The plasma-based methods of combustion

    management under scramjet conditions are now considered

    as one of the most promising technologies in this field

    [17]. Electrical discharge properties strongly depend on the

    conditions of excitation, flow parameters and characteristics

    of the supplying electromagnetic power. The analysis of

    applicable discharge types can be done from the viewpoint

    of the plasma-assisted combustion concept, which consists

    of three important items: ignition and combustion chemistry

    enhancement due to heating and active particle generation (1),

    airfuel mixing intensification in flow (2) and flow structure

    management for flame front stabilization (3). At least four

    This paper was presented at the Second International Symposiumon Nonequilibrium Processes, Combustion, and Atmospheric Phenomena(Dagomys, Sochi, Russia, 37 October 2005).

    mechanisms of theplasma effect on flow structure, ignition and

    combustion processes might be listed: fast local ohmic heatingof the medium (1), nonequilibrium excitation and dissociationof air and fuel molecules due to electron collisions and UV

    radiation (2), momentum transfer in electric and magneticfields (3) and shocks/instabilities generation (4). The electrical

    discharges, which are generated under the conditions of high-speed flow, possess several specific properties. These featuresmight be important for the discharge applications for flow

    parameter and structure control and combustion enforcementunder unfavourable conditions.

    Local heating of the medium leads to intensification ofthe chemical reactions in these areas. A controlled energydeposition affects the flow structure, including generation of

    zones with artificial separation at a sufficiently high level ofinput power [8, 9]. It is a method of flow structure steering.

    It allows increasing local residence time to provide a zone oflocal combustion. The airfuel mixing is intensified as well.

    Active radical generation is due to molecule dissociation

    and excitation by electrons in the electric field, radiationand more complex processes. The presence of chemical

    radicals (for example, O, OH, H, NOx ) or vibrationally excited

    0963-0252/07/010132+07$30.00 2007 IOP Publishing Ltd Printed in the UK 132

    mailto:%[email protected]:%[email protected]://stacks.iop.org/ps/16/132mailto:%[email protected]:%[email protected]://dx.doi.org/10.1088/0963-0252/16/1/018
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    Plasma-induced ignition and plasma-assisted combustion

    molecules can effectively improve ignition conditions but

    the problem is at the level of the required electric power.

    If the chain chemical reactions are realized, the production

    of even a small amount of active particles can lead to a

    large (synergetic) benefit in total reaction rates, as well as

    in diminishing of the required power input. Gas dischargepotentials for the gas non-equilibrium excitation are widely

    discussed as an advanced technology. Generally speaking, any

    type of excitation (dissociation, ionization, electron excitation

    or vibrational excitation) affects the reaction rates positively.

    Two main processes can result in excitation of an atom or

    molecule: electron impact and photo-excitation. The first one

    is effective at a high magnitude of the reduced electric field,

    E/N. The second one is effective at superheating of the

    dischargechannel (highintensityof thethermal radiation). The

    first effect occurs mostly in high-frequency and short-pulsed

    discharges or at intensive cooling of the discharge area [9].

    The second one could be realized at high values of specific

    energy input (several eV per atom/molecule) [10].Shock wave generation promotes the mixing processes

    in a heterogeneous medium and initiates chemical reactions

    due to heating in the shock front zone. Also there can exist

    various typesof plasmainstabilities, for example, longitudinal-

    transverse instability of plasma filament, which has been

    revealed recently [9]. It leads to intensive small scale mixing

    inflow. It should be noted that in general there are no methods

    to separate the specific mechanisms of the plasma effect

    because of interference between them.

    Typical conditionsfordischargemaintenance in aerospace

    science: pressure P = 0.11 bar, velocity of the flow V =

    1001000 m s1. Characteristic temperatureof gas varies from

    T = 200 K (ambient conditions) to T 2 kK for the com-bustion chamber. As a rule, at such conditions the plasma

    of electric discharges appears in the filamentary form due to

    instabilities mostly associatedwiththe mechanism of electrical

    field enhancement in the vicinity of the heated plasmachannel.

    At present, there are no reliable universal rules for the appear-

    ance of any electric discharges at high temperature. Under

    high pressure and high-speed flow most types of discharge

    are nonuniform and nonequilibrium. The high-pressure glow

    discharge [11, 12] is a rather homogeneous one, and the high-

    current longitudinal arc produces the equilibrium plasma. The

    strong non-uniformity of the plasma inflow renders a chance

    for a significant decrease in the required electrical power for a

    predefined effect. This idea is in local multi-points influencewith sequential expansion of flame fronts.

    The complete management of the combustion process

    under any conditions requires a large level of additional

    energy deposition (in a range of flow enthalpy) that is beyond

    practical interest. The idea is not related to the strong effect

    of energy release but to the gentle control of the chemical

    reaction rate and local multi-ignition. The second direction

    is to give the gear to force the combustor to work under

    off-design conditions. It may be a temporal mode when

    the level of required electric energy is not vitally important.

    Unfortunately, specific information available now is not quite

    sufficient for the proper choice of the discharge type. Our

    understanding is that there is no versatile solution to the designand method of application of plasma for combustion. Each

    specific situation has to be considered separately. But it seems

    (a)

    (b)

    Figure 1. Basic scheme of electrode arrangement.

    clear that thenonequilibrium andnonuniform operationmodes

    are preferable. Our understanding also is that plasma has to

    be generated in situ just in the location of the fueloxidizer

    interaction but not by an external device.

    2. Experimental facility pwt-50

    A deeply renovated experimental facility PWT-50 is used for

    testing of the hydrogen ignition by the electrical discharge

    behind the wallstep and in a cavity of the high-speed duct.

    The following gasdynamic parameters of the test are provided

    by PWT-50: Mach number in duct M = 1.92; initial static

    pressure Pst = 0.120.25 bar; stagnation temperature of theair

    T0 = 300K; test section dimensions 7260 mm; steady-stage

    operation time 0.30.5 s.

    Themeasuring systemincludesthe sensors of pressure and

    temperature of the initial flow, pressure transducers (pressure

    distribution measurements), spectroscopic system, optical

    sensors, Schlieren system, fast video cameras, electrical

    parameter sensors, IR camera and IR spectroscopy. Thedata acquisition system includes PC-based individual devices

    for pressure distribution records, video camera control,

    spectroscopic and operation parameter records.

    The plasma generator was designed and constructed for

    applications in high-speed flow on the basis of experimental

    results obtained during a previous study of quasi-dc, pulse

    periodic and modulated RF discharges [810, 13]. The

    electrode configuration (line near the edge of the wallstep and

    line at the bottom of the separation zone) was proposed and

    described in [16]. Figure 1 presents the scheme of electrode

    arrangement and corresponding photo of the real device.

    It consists of two insertions made of refractory insulating

    material. The first insertion is arranged on the edge of thebackward wall-step, andthe secondone is located at thebottom

    of the separation zone. Both of them are flush mounted as

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    S B Leonov and D A Yarantsev

    well as the electrodes themselves. Each insertion has the

    same construction: nine electrodes in two rows arranged in

    an interlacing manner (4 + 5).

    In thefirstinsertionthe first row isapplied forthe discharge

    primary initiation, whereas the second row contains working

    anodes. The first line of electrodes in the second insertion isreserved for extra control of the discharge and measurements

    of the cathode voltage drop; the second line is operated as

    working cathodes. Such electrode arrangement allows for

    quite flexible operation. The discharge operates with the

    following parameters: type of dischargefilamentary quasi-

    continuous; operation time of dischargetpl = 50500ms;

    current through eachelectrodeIpl1 = 14A; mean electrical

    input powerWpl = 110 kW that is equivalent to mean gas

    temperature elevation less than Tav = 20K.

    The fuel injectors are installed directly on the bottom wall

    of the test section as shown in figure 1. They contain a fuel

    capacitor at 56 bar of pressure and fast pulse valve with EM

    control. Thefuel dose and duration of the injection depends onthe EM pulse duration and the repetition rate. Minimal dose

    at the single pulse is about 1mg. Maximal mass flow rate is

    about 5g s1.

    3. Discharge appearance near the backwardwallstep and cavity (experiment and CFD)

    Numerous experiments were done at different conditions:

    subsonic and supersonic flow; wallstep, long cavity (l/d =

    6.5) and short cavity (l/d = 3.3); different pressure; current

    from 5 to 20 A; both polarities, etc. Here the data for the

    wallstep in supersonic mode are shown for the typical electric

    current.

    3.1. Plasma filament dynamics in high-speed flow

    The discharge dynamics in flow behind the wallstep was

    explored using a high-speed digital CMOS camera with a

    typical frame rate of2000 fpsat 1280250pixelsand exposure

    down to 30 s. As a sample in figure 2 two selected frames

    are presented for operation in supersonic mode in the cavity

    and behind the wallstep correspondingly.

    It is seen that in the first case the discharge cord looks

    unstable. A full frame sequence shows a fast movement of

    them in the separation zone. The S-type of the plasma cord

    shape reflects the flow velocity distribution under separation.

    An intensification of flow circulation due to energy release isproved also by simulation (see below). In contrast with that

    the shape of the discharge cords is very stable in the supersonic

    mode with the backward wallstep. Cord location repeats the

    edge of the separation zone (in this case the zone has a minimal

    size among others).

    3.2. Voltagecurrent measurements

    Measurements of voltagecurrent characteristics were made

    for the 5-cords plasma generator. Figure 3 presents

    oscillograms of the discharge voltage, current and recalculated

    power for two cases: discharge in the cavity and behind the

    backward wallstep.The input power weakly depends on static pressure under

    the explored conditions (M = 1.9). The greatest effect can

    (a)

    (b)

    Figure 2. Discharge appearance in the supersonic mode at thecavity and behind the backward wallstep.

    (a)

    (b)

    Figure 3. Typical oscillograms of the discharge operation insupersonic operation mode, M0 = 1.9, short cavity (a) and wallstep(b). Average power is calculated.

    be obtained by electric current regulation. In the case of

    supersonic flow over the cavity (short cavity and long cavityboth) electric parameter behaviour is very similar to in the

    subsonic mode. It is characterized by a significant level of

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    Plasma-induced ignition and plasma-assisted combustion

    voltage vibrations. This fact reflects the close aerodynamic

    situations when the plasma filaments migrate in the separation

    zone with wide variation of their length that is a result of

    gas movement (see above). In the case of discharge in the

    cavity the characteristic frequency of the voltage oscillations

    was about f = 12 kHz, which corresponds to the internalflow velocity in a range V = 1040ms1.

    In the case of the supersonic mode in the duct with the

    backward wallstep the amplitude of such vibrations was much

    less which is seen in the following graphs. The appropriate

    frequency is higher. The plasma cord position is quite stable

    in theshear layer andthefilaments areshorter themselves. The

    fields magnitude is significantly higher than in the case of the

    subsonic flow. Dueto field elevation (E/ n 51016 V cm2)

    the electron temperature has to be increased from Te = 0.8 ev

    to Te = 1.5 evapproximately. Plasma-chemicalreactions have

    to be activated as well.

    3.3. Measurements of plasma temperature

    Optical spectroscopy is used to measure the plasma

    temperature [17, 18]. Measurements were carried out at three

    different values of ballast resistance (1+0 .2 kOhm, 1+1 kOhm

    and1+2 kOhm)in theseparation zone of theduct. Temperature

    was measured by fitting of the experimental and the calculated

    spectra of the N2 second positive system (00, 337.1 nm) and

    of the violet system of CN (388.9 nm).

    By the analysis of N2 spectra the rotational temperature

    was found to be the same for different conditions; its value

    is Trot = 3.0 0.2 kK. Temperature measurements carried

    out by the CN spectrum give the following results: Tvib =

    7.50.5kK; Trot = 70.5 kK.Suchhigh values areexplained

    by the fact that we measure temperature of the exited state of

    the CN molecules whereas rotational temperature measured

    by the N2 spectrum is equal to the temperature of the N2ground state. It is clear that under conditions of high non-

    uniformity of the discharge structure the measured magnitude

    of temperature is between the maximal and average values. As

    a result the different molecular bands can give different formal

    temperatures. The averaged gas temperature in the cavity is

    evaluated at Tcav = 200 K.

    3.4. Discharge effect on flow structure near the wall step and

    cavity

    Two methods were utilized mainly to study the dischargeeffect on flow structure behind the wallstep and in the

    cavity: pressure measurements and Schlieren visualization.

    A 16-channel pressure recorder was used in the tests. The

    sensor arrangement is shown near an appropriate picture.

    Typical data are presented in figure 4.

    Summarizing the discharge effect on pressure distribution

    in the cavity and behind the wallstep it should be considered

    that, as a rule, the pressure rises noticeably just near the

    discharge zone and its distribution occurs more smoothly in

    the cavity as a whole.

    3.5. Schlieren visualization

    The Schlieren system was adjusted to work in the pulse mode

    of the flash-lamp with frame frequency f = 100 Hz. The

    Figure 4. M= 1.9, discharge is switched on before flow start andswitched off in t= 0.17s.

    (a)

    (b)

    Figure 5. Schlieren photos of the discharge effect on flow structure.Supersonic mode, wallstep.

    images are presented as a pair (discharge off/on) for the

    operation modes when the power deposition is in the range

    Wav = 57kW, staticpressure in thesupersonic M1.9 mode

    Pst = 120180 Torr. The exposure time of the photos in

    figure 5 was t= 1 s.

    As can be easily recognized, the discharge effect on the

    flow structure in the cavity and behind the wallstep lies in

    an intensive turbulization of gas in the interaction area at asimultaneous slight increase in the separation zone volume.

    Numerical modelling of flow in the experimental set-up

    was based on the solution of 3D time-dependent Reynolds

    averaged NavierStoke equations (URANS-method) with the

    utilization of the widely used two-equation SST-model of

    turbulence. Calculation of three-dimensional turbulent flow

    in the frame of the model of perfect gas (5 components) in the

    experimental set-up was executed by modelling a heat supply

    causedby the direct current electric discharge. Constant values

    of velocity V = 317ms1, total pressure P0 = 105 Pa and

    temperature T = 250 K were specified in the initial section of

    the calculation domain being the critical section of supersonic

    nozzle M = 2. Zero gradients of flow parameters in theoutlet section of the calculation domain were fixed. Non-

    slip and adiabatic conditions were specified on the upper,

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    S B Leonov and D A Yarantsev

    Figure 6. Isothermal surfaces Tg = 2000K.

    lower and lateral walls of the duct as well as on the cavity

    walls. Symmetry conditions were used in the median section

    of theduct to decrease thecalculation domain which contained

    600000 mesh points.

    The results of computational analysis were obtained forpower deposition Wpl = 5 kW that is close to the experimental

    value. As far as possible, the results of simulations are

    compatible with experimental data. The isothermal surfaces

    are presented in figure 6 for a sample. The essentially three-

    dimensional character of the considered flow is demonstrated

    by this. The important issue is a rate of gas exchange between

    the main flow and the separation zone. The calculated values

    are equal to G0 = 0.0054kgs1 and GQ = 0.0074kgs

    1,

    respectively, without heat input and with it. The experimental

    value on the velocity of gas circulation in the cavity gave a

    similar result. On thebasisof these data thefirst approximation

    for the required amount of the injected fuel to provide a

    stoichiometric gas composition in the cavity can be calculated:GH2 0.15gs1 and GC2H4 0.4 g s

    1.

    4. Hydrogen ignition under separation in supersonicflow (experiment)

    Preliminary results of hydrocarbon fuel ignition behind a

    backward wallstep were published in [1,1315]. The results

    of the recent tests on hydrogen ignition in the separation

    zone of low-temperature supersonic flow are presented in

    this section. Several diagnostics were applied: natural

    observations, Schlieren photos, spectroscopy, pressure record,

    etc. The most reliable way to recognize combustion was a

    great pressure growth in the separation zone.Figure 7 presents typical experimental data on the

    hydrogen ignition by the discharge in the short cavity. The

    first frame shows the discharge just before the fuel injection,

    the second frame related to the combustion. The third plot

    shows time behaviour of pressure near the zone of interaction:

    total pressure P0 downstream of the cavity and normalized

    static pressure Ps in the separation zone Ps = Pst1 Pst0 +

    Pst0(t = 0), where Pst1 is static pressure in cavity, Pst0 the

    static pressure upstream. The data are synchronized with

    the discharge current. The temperature of the downstream

    (inclined) wall is shown as measured by a thermocouple (it

    reflects the trend only). The heating of this wall by the

    discharge does notexceed 30 K. Thefourthpicture presents theSchlierenphotosof interaction. An estimationand comparison

    with numerical simulations indicate a level of pressure step

    (a)

    (b)

    (c)

    (d)

    Figure 7. Discharge interaction with injected hydrogen. Photos (a),(b), pressure (c), Schlieren photos (d).

    P = 1020 Torr in the cavity in case the oxidizer is provided

    by circulating air.

    Two modes of discharge-fuel-flow interaction were

    observed: fuel ignition and combustion just in a cavity and

    fuel combustion in a shear layer of supersonic freestream. In

    the case of hydrogen injection both the modes were detected.Under experimental conditions, the ethylene combustion was

    detected in the cavity only.

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    Plasma-induced ignition and plasma-assisted combustion

    (a)

    (b)

    Figure 8. Discharge interaction with injected hydrogen behindwallstep. Pressure (a), Schlieren photos (b).

    The hydrogen combustion in the cavity takes place if

    the power deposition in the discharge W > 1 kW. If the

    discharge was turned off, the combustion in the cavity reaches

    the unstable mode. Increase in the hydrogen flow rate over the

    stoichiometric ratio pushes the combustion above the cavity, if

    the power deposition is not less than Wpl = 3 kW. When the

    thermal power of combustion grows more than Wfuel = 20kW

    a thermal choking of the duct occurred.

    It is well known that some widening of the gasdynamic

    duct downstream helps to prevent a thermal chocking. Figure8demonstrates the hydrogen combustion in the shear layer of

    free stream in a configuration with the backward wallstep

    for the hydrogen mass flow rate increased up to GH2 =

    4 g s1. The reactions were very intensive without blockage

    of the supersonic operation mode. It is seen how the flow

    disturbances produced by combustion occupied almost an

    entire duct. The discharge switching off destroys this regime

    immediately.

    It is clear that the flash of radiation does not reflect the

    fact of fuel combustion itself. One important feature of the

    discharge-fuel interaction is the dramatic growth in radiation

    intensity from the volume, especially for hydrocarbon fuel.

    Sometimes it exceeds a factor of magnitude 103

    . This rise takeplace in continuous spectra and molecular bands CN, C2 and

    others. In [14] the effect wasnamed as cyan catastrophe. For

    (a)

    (b)

    Figure 9. Samples of time behaviour of the discharge spectrumunder ethylene (a) and hydrogen (b) injection. Each spectrum has10 ms exposure.

    illustration purposes, some results of spectral measurements

    are shown in figure 9 for the ethylene and hydrogen injection.

    Analysis of the spectral data leads to consideration of the

    important role of atomic oxygen generated by the discharge

    for the combustion chemistry. Figure 9(b) presents a spectral

    sequence when the discharge is operated slightly before the

    hydrogen injection. It is seen that theamplitudeof theresonant

    spectral line of atomic oxygen grows in the discharge area

    and drops at combustion. Generally, this situation should

    be analysed in more detail to find the quantitative relations

    between radiation intensityandconcentration of excited atoms.

    Of interest is thefact that thedischarge switching-off leads

    to immediate extinction of the hydrogen flame in a free stream,

    but the combustion in the cavity can continue. The power

    threshold of hydrogen ignition in the shear layer wasmeasured

    by variation of powerdeposition. It is about Wpl = 3 kW under

    the conditions of the test.

    5. Conclusions

    Control of ignition in aircraft jet engines is of crucial

    importance for their performance over a wide range of

    operation parameters, such as altitude, flight speed and

    thrust. Reduction in ignition delay time, flameholding and

    flame stability improvement, flame blow-off prevention andextension of fuel flammability limits are some of the key

    technicalissues in this field. In this paper theextramechanisms

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    S B Leonov and D A Yarantsev

    (plasma technology) aredescribedas promisingcontenders for

    the mechanical methods.

    A conception of plasma-assisted combustion has been

    formulated. Methods for high-speed combustion control

    were considered: plasma-induced ignition, plasma-intensified

    mixing and flame-holding by plasma generation. The mainphysical mechanisms of the plasma effect are described.

    Previously proposed multi-electrode quasi-dc discharge

    through theseparation zone wasdeveloped forutilization in the

    cavity and wallstep of the supersonic duct. The peculiarities

    of the filamentary discharge maintenance in high-speed flow

    under separation were explored experimentally. 3D CFD

    simulation was performed for getting a deeper insight into

    and prediction of critical parameters for the plasma-ignition

    experiment.

    The results of model experiments on the ignition of non-

    premixed air-fuel (hydrogen and ethylene) streams in high-

    speed low-temperature flow behind a backward wallstep and

    in the cavity are presented. The energetic threshold of thehydrogen ignition in the shear layer was measured at a value

    W = 3 kW for the experimental conditions. It is concluded

    that the detection of the radiation increase is not a reliable

    method of combustion monitoring, if an electric discharge is

    maintained.

    Experimental and theoretical efforts for a broader range

    of parameters are planned for the future.

    Acknowledgments

    The authors express their gratitude to Dr Valentin Bityurin

    for multiple discussions regarding CFD efforts, Mr Konstantin

    Savelkin of IVTAN for valuable assistance in experimentalwork, Dr Valery Sermanov of TsAGI for consultation on the

    high-speedcombustion techniqueandDr Michail Starodubtsev

    for CFD efforts. The results would not be possible without

    the excellent work of IVTANs laboratory personnel who

    participated in the experimental efforts.

    Currently the work is funded by EOARD (ISTC Project

    3057p, Dr Campbell Carter technical supervision). Some parts

    of this work were supported by Program #20 of the Russian

    Academy of Science (co-ordinator Academecian. Gorimir

    Cherny).

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