sergey b leonov and dmitry a yarantsev- plasma-induced ignition and plasma-assisted combustion in...
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INSTITUTE OF PHYSICS PUBLISHING PLASMA SOURCES SCIENCE AND TECHNOLOGY
Plasma Sources Sci. Technol. 16 (2007) 132138 doi:10.1088/0963-0252/16/1/018
Plasma-induced ignition and
plasma-assisted combustion in high-speedflow
Sergey B Leonov and Dmitry A Yarantsev
Institute of High Temperatures RAS (IVTAN), Izhorskaya str., 13/19, Moscow, 125412,
Russia
E-mail: [email protected] and [email protected]
Received 17 March 2006, in final form 10 July 2006Published 20 December 2006Online at stacks.iop.org/PSST/16/132
AbstractThe suitability of the electrical discharge technique for application inplasma-induced ignition and plasma-assisted combustion in high-speed flowis reviewed. Nonequilibrium, unsteady and nonuniform modes are underanalysis to demonstrate the advantage of such a technique over heating. Areduction in the required power deposition is possible due to unsteadyoperation and non-homogeneous spatial distribution. Mixing intensificationin non-premixed flow could be achieved by nonuniform electricaldischarges. The scheme of fuel ignition behind the wallstep and in the cavityis under consideration. Experimental results on multi-electrode dischargemaintenance in the separation zone of supersonic flow are presented. The
model test on hydrogen and ethylene ignition is demonstrated at direct fuelinjection. An energetic threshold of fuel ignition under separation and in theshear layer is measured under the experimental conditions.
(Some figures in this article are in colour only in the electronic version)
1. Introduction. Plasma-assisted combustionapproach
Analysis of supersonic combustor performance shows that
several principal problems related to supersonic combustion
and flame stabilization are to be solved for the practical
implementation of such a technology, especially in the case ofhydrocarbon fuels. The plasma-based methods of combustion
management under scramjet conditions are now considered
as one of the most promising technologies in this field
[17]. Electrical discharge properties strongly depend on the
conditions of excitation, flow parameters and characteristics
of the supplying electromagnetic power. The analysis of
applicable discharge types can be done from the viewpoint
of the plasma-assisted combustion concept, which consists
of three important items: ignition and combustion chemistry
enhancement due to heating and active particle generation (1),
airfuel mixing intensification in flow (2) and flow structure
management for flame front stabilization (3). At least four
This paper was presented at the Second International Symposiumon Nonequilibrium Processes, Combustion, and Atmospheric Phenomena(Dagomys, Sochi, Russia, 37 October 2005).
mechanisms of theplasma effect on flow structure, ignition and
combustion processes might be listed: fast local ohmic heatingof the medium (1), nonequilibrium excitation and dissociationof air and fuel molecules due to electron collisions and UV
radiation (2), momentum transfer in electric and magneticfields (3) and shocks/instabilities generation (4). The electrical
discharges, which are generated under the conditions of high-speed flow, possess several specific properties. These featuresmight be important for the discharge applications for flow
parameter and structure control and combustion enforcementunder unfavourable conditions.
Local heating of the medium leads to intensification ofthe chemical reactions in these areas. A controlled energydeposition affects the flow structure, including generation of
zones with artificial separation at a sufficiently high level ofinput power [8, 9]. It is a method of flow structure steering.
It allows increasing local residence time to provide a zone oflocal combustion. The airfuel mixing is intensified as well.
Active radical generation is due to molecule dissociation
and excitation by electrons in the electric field, radiationand more complex processes. The presence of chemical
radicals (for example, O, OH, H, NOx ) or vibrationally excited
0963-0252/07/010132+07$30.00 2007 IOP Publishing Ltd Printed in the UK 132
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Plasma-induced ignition and plasma-assisted combustion
molecules can effectively improve ignition conditions but
the problem is at the level of the required electric power.
If the chain chemical reactions are realized, the production
of even a small amount of active particles can lead to a
large (synergetic) benefit in total reaction rates, as well as
in diminishing of the required power input. Gas dischargepotentials for the gas non-equilibrium excitation are widely
discussed as an advanced technology. Generally speaking, any
type of excitation (dissociation, ionization, electron excitation
or vibrational excitation) affects the reaction rates positively.
Two main processes can result in excitation of an atom or
molecule: electron impact and photo-excitation. The first one
is effective at a high magnitude of the reduced electric field,
E/N. The second one is effective at superheating of the
dischargechannel (highintensityof thethermal radiation). The
first effect occurs mostly in high-frequency and short-pulsed
discharges or at intensive cooling of the discharge area [9].
The second one could be realized at high values of specific
energy input (several eV per atom/molecule) [10].Shock wave generation promotes the mixing processes
in a heterogeneous medium and initiates chemical reactions
due to heating in the shock front zone. Also there can exist
various typesof plasmainstabilities, for example, longitudinal-
transverse instability of plasma filament, which has been
revealed recently [9]. It leads to intensive small scale mixing
inflow. It should be noted that in general there are no methods
to separate the specific mechanisms of the plasma effect
because of interference between them.
Typical conditionsfordischargemaintenance in aerospace
science: pressure P = 0.11 bar, velocity of the flow V =
1001000 m s1. Characteristic temperatureof gas varies from
T = 200 K (ambient conditions) to T 2 kK for the com-bustion chamber. As a rule, at such conditions the plasma
of electric discharges appears in the filamentary form due to
instabilities mostly associatedwiththe mechanism of electrical
field enhancement in the vicinity of the heated plasmachannel.
At present, there are no reliable universal rules for the appear-
ance of any electric discharges at high temperature. Under
high pressure and high-speed flow most types of discharge
are nonuniform and nonequilibrium. The high-pressure glow
discharge [11, 12] is a rather homogeneous one, and the high-
current longitudinal arc produces the equilibrium plasma. The
strong non-uniformity of the plasma inflow renders a chance
for a significant decrease in the required electrical power for a
predefined effect. This idea is in local multi-points influencewith sequential expansion of flame fronts.
The complete management of the combustion process
under any conditions requires a large level of additional
energy deposition (in a range of flow enthalpy) that is beyond
practical interest. The idea is not related to the strong effect
of energy release but to the gentle control of the chemical
reaction rate and local multi-ignition. The second direction
is to give the gear to force the combustor to work under
off-design conditions. It may be a temporal mode when
the level of required electric energy is not vitally important.
Unfortunately, specific information available now is not quite
sufficient for the proper choice of the discharge type. Our
understanding is that there is no versatile solution to the designand method of application of plasma for combustion. Each
specific situation has to be considered separately. But it seems
(a)
(b)
Figure 1. Basic scheme of electrode arrangement.
clear that thenonequilibrium andnonuniform operationmodes
are preferable. Our understanding also is that plasma has to
be generated in situ just in the location of the fueloxidizer
interaction but not by an external device.
2. Experimental facility pwt-50
A deeply renovated experimental facility PWT-50 is used for
testing of the hydrogen ignition by the electrical discharge
behind the wallstep and in a cavity of the high-speed duct.
The following gasdynamic parameters of the test are provided
by PWT-50: Mach number in duct M = 1.92; initial static
pressure Pst = 0.120.25 bar; stagnation temperature of theair
T0 = 300K; test section dimensions 7260 mm; steady-stage
operation time 0.30.5 s.
Themeasuring systemincludesthe sensors of pressure and
temperature of the initial flow, pressure transducers (pressure
distribution measurements), spectroscopic system, optical
sensors, Schlieren system, fast video cameras, electrical
parameter sensors, IR camera and IR spectroscopy. Thedata acquisition system includes PC-based individual devices
for pressure distribution records, video camera control,
spectroscopic and operation parameter records.
The plasma generator was designed and constructed for
applications in high-speed flow on the basis of experimental
results obtained during a previous study of quasi-dc, pulse
periodic and modulated RF discharges [810, 13]. The
electrode configuration (line near the edge of the wallstep and
line at the bottom of the separation zone) was proposed and
described in [16]. Figure 1 presents the scheme of electrode
arrangement and corresponding photo of the real device.
It consists of two insertions made of refractory insulating
material. The first insertion is arranged on the edge of thebackward wall-step, andthe secondone is located at thebottom
of the separation zone. Both of them are flush mounted as
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well as the electrodes themselves. Each insertion has the
same construction: nine electrodes in two rows arranged in
an interlacing manner (4 + 5).
In thefirstinsertionthe first row isapplied forthe discharge
primary initiation, whereas the second row contains working
anodes. The first line of electrodes in the second insertion isreserved for extra control of the discharge and measurements
of the cathode voltage drop; the second line is operated as
working cathodes. Such electrode arrangement allows for
quite flexible operation. The discharge operates with the
following parameters: type of dischargefilamentary quasi-
continuous; operation time of dischargetpl = 50500ms;
current through eachelectrodeIpl1 = 14A; mean electrical
input powerWpl = 110 kW that is equivalent to mean gas
temperature elevation less than Tav = 20K.
The fuel injectors are installed directly on the bottom wall
of the test section as shown in figure 1. They contain a fuel
capacitor at 56 bar of pressure and fast pulse valve with EM
control. Thefuel dose and duration of the injection depends onthe EM pulse duration and the repetition rate. Minimal dose
at the single pulse is about 1mg. Maximal mass flow rate is
about 5g s1.
3. Discharge appearance near the backwardwallstep and cavity (experiment and CFD)
Numerous experiments were done at different conditions:
subsonic and supersonic flow; wallstep, long cavity (l/d =
6.5) and short cavity (l/d = 3.3); different pressure; current
from 5 to 20 A; both polarities, etc. Here the data for the
wallstep in supersonic mode are shown for the typical electric
current.
3.1. Plasma filament dynamics in high-speed flow
The discharge dynamics in flow behind the wallstep was
explored using a high-speed digital CMOS camera with a
typical frame rate of2000 fpsat 1280250pixelsand exposure
down to 30 s. As a sample in figure 2 two selected frames
are presented for operation in supersonic mode in the cavity
and behind the wallstep correspondingly.
It is seen that in the first case the discharge cord looks
unstable. A full frame sequence shows a fast movement of
them in the separation zone. The S-type of the plasma cord
shape reflects the flow velocity distribution under separation.
An intensification of flow circulation due to energy release isproved also by simulation (see below). In contrast with that
the shape of the discharge cords is very stable in the supersonic
mode with the backward wallstep. Cord location repeats the
edge of the separation zone (in this case the zone has a minimal
size among others).
3.2. Voltagecurrent measurements
Measurements of voltagecurrent characteristics were made
for the 5-cords plasma generator. Figure 3 presents
oscillograms of the discharge voltage, current and recalculated
power for two cases: discharge in the cavity and behind the
backward wallstep.The input power weakly depends on static pressure under
the explored conditions (M = 1.9). The greatest effect can
(a)
(b)
Figure 2. Discharge appearance in the supersonic mode at thecavity and behind the backward wallstep.
(a)
(b)
Figure 3. Typical oscillograms of the discharge operation insupersonic operation mode, M0 = 1.9, short cavity (a) and wallstep(b). Average power is calculated.
be obtained by electric current regulation. In the case of
supersonic flow over the cavity (short cavity and long cavityboth) electric parameter behaviour is very similar to in the
subsonic mode. It is characterized by a significant level of
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Plasma-induced ignition and plasma-assisted combustion
voltage vibrations. This fact reflects the close aerodynamic
situations when the plasma filaments migrate in the separation
zone with wide variation of their length that is a result of
gas movement (see above). In the case of discharge in the
cavity the characteristic frequency of the voltage oscillations
was about f = 12 kHz, which corresponds to the internalflow velocity in a range V = 1040ms1.
In the case of the supersonic mode in the duct with the
backward wallstep the amplitude of such vibrations was much
less which is seen in the following graphs. The appropriate
frequency is higher. The plasma cord position is quite stable
in theshear layer andthefilaments areshorter themselves. The
fields magnitude is significantly higher than in the case of the
subsonic flow. Dueto field elevation (E/ n 51016 V cm2)
the electron temperature has to be increased from Te = 0.8 ev
to Te = 1.5 evapproximately. Plasma-chemicalreactions have
to be activated as well.
3.3. Measurements of plasma temperature
Optical spectroscopy is used to measure the plasma
temperature [17, 18]. Measurements were carried out at three
different values of ballast resistance (1+0 .2 kOhm, 1+1 kOhm
and1+2 kOhm)in theseparation zone of theduct. Temperature
was measured by fitting of the experimental and the calculated
spectra of the N2 second positive system (00, 337.1 nm) and
of the violet system of CN (388.9 nm).
By the analysis of N2 spectra the rotational temperature
was found to be the same for different conditions; its value
is Trot = 3.0 0.2 kK. Temperature measurements carried
out by the CN spectrum give the following results: Tvib =
7.50.5kK; Trot = 70.5 kK.Suchhigh values areexplained
by the fact that we measure temperature of the exited state of
the CN molecules whereas rotational temperature measured
by the N2 spectrum is equal to the temperature of the N2ground state. It is clear that under conditions of high non-
uniformity of the discharge structure the measured magnitude
of temperature is between the maximal and average values. As
a result the different molecular bands can give different formal
temperatures. The averaged gas temperature in the cavity is
evaluated at Tcav = 200 K.
3.4. Discharge effect on flow structure near the wall step and
cavity
Two methods were utilized mainly to study the dischargeeffect on flow structure behind the wallstep and in the
cavity: pressure measurements and Schlieren visualization.
A 16-channel pressure recorder was used in the tests. The
sensor arrangement is shown near an appropriate picture.
Typical data are presented in figure 4.
Summarizing the discharge effect on pressure distribution
in the cavity and behind the wallstep it should be considered
that, as a rule, the pressure rises noticeably just near the
discharge zone and its distribution occurs more smoothly in
the cavity as a whole.
3.5. Schlieren visualization
The Schlieren system was adjusted to work in the pulse mode
of the flash-lamp with frame frequency f = 100 Hz. The
Figure 4. M= 1.9, discharge is switched on before flow start andswitched off in t= 0.17s.
(a)
(b)
Figure 5. Schlieren photos of the discharge effect on flow structure.Supersonic mode, wallstep.
images are presented as a pair (discharge off/on) for the
operation modes when the power deposition is in the range
Wav = 57kW, staticpressure in thesupersonic M1.9 mode
Pst = 120180 Torr. The exposure time of the photos in
figure 5 was t= 1 s.
As can be easily recognized, the discharge effect on the
flow structure in the cavity and behind the wallstep lies in
an intensive turbulization of gas in the interaction area at asimultaneous slight increase in the separation zone volume.
Numerical modelling of flow in the experimental set-up
was based on the solution of 3D time-dependent Reynolds
averaged NavierStoke equations (URANS-method) with the
utilization of the widely used two-equation SST-model of
turbulence. Calculation of three-dimensional turbulent flow
in the frame of the model of perfect gas (5 components) in the
experimental set-up was executed by modelling a heat supply
causedby the direct current electric discharge. Constant values
of velocity V = 317ms1, total pressure P0 = 105 Pa and
temperature T = 250 K were specified in the initial section of
the calculation domain being the critical section of supersonic
nozzle M = 2. Zero gradients of flow parameters in theoutlet section of the calculation domain were fixed. Non-
slip and adiabatic conditions were specified on the upper,
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S B Leonov and D A Yarantsev
Figure 6. Isothermal surfaces Tg = 2000K.
lower and lateral walls of the duct as well as on the cavity
walls. Symmetry conditions were used in the median section
of theduct to decrease thecalculation domain which contained
600000 mesh points.
The results of computational analysis were obtained forpower deposition Wpl = 5 kW that is close to the experimental
value. As far as possible, the results of simulations are
compatible with experimental data. The isothermal surfaces
are presented in figure 6 for a sample. The essentially three-
dimensional character of the considered flow is demonstrated
by this. The important issue is a rate of gas exchange between
the main flow and the separation zone. The calculated values
are equal to G0 = 0.0054kgs1 and GQ = 0.0074kgs
1,
respectively, without heat input and with it. The experimental
value on the velocity of gas circulation in the cavity gave a
similar result. On thebasisof these data thefirst approximation
for the required amount of the injected fuel to provide a
stoichiometric gas composition in the cavity can be calculated:GH2 0.15gs1 and GC2H4 0.4 g s
1.
4. Hydrogen ignition under separation in supersonicflow (experiment)
Preliminary results of hydrocarbon fuel ignition behind a
backward wallstep were published in [1,1315]. The results
of the recent tests on hydrogen ignition in the separation
zone of low-temperature supersonic flow are presented in
this section. Several diagnostics were applied: natural
observations, Schlieren photos, spectroscopy, pressure record,
etc. The most reliable way to recognize combustion was a
great pressure growth in the separation zone.Figure 7 presents typical experimental data on the
hydrogen ignition by the discharge in the short cavity. The
first frame shows the discharge just before the fuel injection,
the second frame related to the combustion. The third plot
shows time behaviour of pressure near the zone of interaction:
total pressure P0 downstream of the cavity and normalized
static pressure Ps in the separation zone Ps = Pst1 Pst0 +
Pst0(t = 0), where Pst1 is static pressure in cavity, Pst0 the
static pressure upstream. The data are synchronized with
the discharge current. The temperature of the downstream
(inclined) wall is shown as measured by a thermocouple (it
reflects the trend only). The heating of this wall by the
discharge does notexceed 30 K. Thefourthpicture presents theSchlierenphotosof interaction. An estimationand comparison
with numerical simulations indicate a level of pressure step
(a)
(b)
(c)
(d)
Figure 7. Discharge interaction with injected hydrogen. Photos (a),(b), pressure (c), Schlieren photos (d).
P = 1020 Torr in the cavity in case the oxidizer is provided
by circulating air.
Two modes of discharge-fuel-flow interaction were
observed: fuel ignition and combustion just in a cavity and
fuel combustion in a shear layer of supersonic freestream. In
the case of hydrogen injection both the modes were detected.Under experimental conditions, the ethylene combustion was
detected in the cavity only.
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Plasma-induced ignition and plasma-assisted combustion
(a)
(b)
Figure 8. Discharge interaction with injected hydrogen behindwallstep. Pressure (a), Schlieren photos (b).
The hydrogen combustion in the cavity takes place if
the power deposition in the discharge W > 1 kW. If the
discharge was turned off, the combustion in the cavity reaches
the unstable mode. Increase in the hydrogen flow rate over the
stoichiometric ratio pushes the combustion above the cavity, if
the power deposition is not less than Wpl = 3 kW. When the
thermal power of combustion grows more than Wfuel = 20kW
a thermal choking of the duct occurred.
It is well known that some widening of the gasdynamic
duct downstream helps to prevent a thermal chocking. Figure8demonstrates the hydrogen combustion in the shear layer of
free stream in a configuration with the backward wallstep
for the hydrogen mass flow rate increased up to GH2 =
4 g s1. The reactions were very intensive without blockage
of the supersonic operation mode. It is seen how the flow
disturbances produced by combustion occupied almost an
entire duct. The discharge switching off destroys this regime
immediately.
It is clear that the flash of radiation does not reflect the
fact of fuel combustion itself. One important feature of the
discharge-fuel interaction is the dramatic growth in radiation
intensity from the volume, especially for hydrocarbon fuel.
Sometimes it exceeds a factor of magnitude 103
. This rise takeplace in continuous spectra and molecular bands CN, C2 and
others. In [14] the effect wasnamed as cyan catastrophe. For
(a)
(b)
Figure 9. Samples of time behaviour of the discharge spectrumunder ethylene (a) and hydrogen (b) injection. Each spectrum has10 ms exposure.
illustration purposes, some results of spectral measurements
are shown in figure 9 for the ethylene and hydrogen injection.
Analysis of the spectral data leads to consideration of the
important role of atomic oxygen generated by the discharge
for the combustion chemistry. Figure 9(b) presents a spectral
sequence when the discharge is operated slightly before the
hydrogen injection. It is seen that theamplitudeof theresonant
spectral line of atomic oxygen grows in the discharge area
and drops at combustion. Generally, this situation should
be analysed in more detail to find the quantitative relations
between radiation intensityandconcentration of excited atoms.
Of interest is thefact that thedischarge switching-off leads
to immediate extinction of the hydrogen flame in a free stream,
but the combustion in the cavity can continue. The power
threshold of hydrogen ignition in the shear layer wasmeasured
by variation of powerdeposition. It is about Wpl = 3 kW under
the conditions of the test.
5. Conclusions
Control of ignition in aircraft jet engines is of crucial
importance for their performance over a wide range of
operation parameters, such as altitude, flight speed and
thrust. Reduction in ignition delay time, flameholding and
flame stability improvement, flame blow-off prevention andextension of fuel flammability limits are some of the key
technicalissues in this field. In this paper theextramechanisms
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S B Leonov and D A Yarantsev
(plasma technology) aredescribedas promisingcontenders for
the mechanical methods.
A conception of plasma-assisted combustion has been
formulated. Methods for high-speed combustion control
were considered: plasma-induced ignition, plasma-intensified
mixing and flame-holding by plasma generation. The mainphysical mechanisms of the plasma effect are described.
Previously proposed multi-electrode quasi-dc discharge
through theseparation zone wasdeveloped forutilization in the
cavity and wallstep of the supersonic duct. The peculiarities
of the filamentary discharge maintenance in high-speed flow
under separation were explored experimentally. 3D CFD
simulation was performed for getting a deeper insight into
and prediction of critical parameters for the plasma-ignition
experiment.
The results of model experiments on the ignition of non-
premixed air-fuel (hydrogen and ethylene) streams in high-
speed low-temperature flow behind a backward wallstep and
in the cavity are presented. The energetic threshold of thehydrogen ignition in the shear layer was measured at a value
W = 3 kW for the experimental conditions. It is concluded
that the detection of the radiation increase is not a reliable
method of combustion monitoring, if an electric discharge is
maintained.
Experimental and theoretical efforts for a broader range
of parameters are planned for the future.
Acknowledgments
The authors express their gratitude to Dr Valentin Bityurin
for multiple discussions regarding CFD efforts, Mr Konstantin
Savelkin of IVTAN for valuable assistance in experimentalwork, Dr Valery Sermanov of TsAGI for consultation on the
high-speedcombustion techniqueandDr Michail Starodubtsev
for CFD efforts. The results would not be possible without
the excellent work of IVTANs laboratory personnel who
participated in the experimental efforts.
Currently the work is funded by EOARD (ISTC Project
3057p, Dr Campbell Carter technical supervision). Some parts
of this work were supported by Program #20 of the Russian
Academy of Science (co-ordinator Academecian. Gorimir
Cherny).
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