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Real and futuristicspin qubits –from GaAs to graphene
Yukawa International SeminarKyoto, November 2007
Lieven Vandersypen
Spin qubits in quantum dots – key elements
Initialization 1 electron, low T, high B0
Read-out spin-to-charge conversion
ESR pulsed microwave magnetic field
SWAP exchange interaction
Coherence T1, T2
↑
↓EZ = gµµµµBB
↑
↓EZ = gµµµµBB
↑ ↓J(t)↑ ↓J(t)
SL SR
↑ ↓
Loss & DiVincenzo, PRA 1998LMKV et al., Proc. MQC02 (quant-ph/0207059)
Delft Nature 2004
Harvard Science 2005
Single-electron spin resonanceF. Koppens et al., Nature 2006
↑
↓EZ = gµµµµBB
↑
↓EZ = gµµµµBB
VAC
ICPS
1 mmBext
BAC
0 50 100 150-50-100-150
100
200
300
400
500
600
700
0Magnetic field (mT)
200
300
400
I dot(fA
0
100R
F fr
eque
ncy
(MH
z)
|g|-factor ~ 0.35
S(0,2)
T(0,2)
0
0.5
RF offDot
cur
rent
(pA
)
Magnetic field (mT)-150 150
RF at 460 MHz
Driven rotations of a single electron spin
Dot current (fA)
Koppens, Buizert, Tielrooij, Vink, Nowack, Meunier, Kouwenhoven, LMKV, Nature 2006
1000
110
0
12
70 3.5
fRabi
(MHz)
Stripline current (mA)
π/2 pulse in 25ns
max B1 ~ 1.9 mT, compare BN,z ~ 1.3 mT
BN,z
B1
Beff
Electrical single-spin control
Vac (a.u.)0 5 10 150
1
2
3
4
Rab
i fre
q (M
Hz) 14 GHz
Nowack, Koppens, Nazarov, LMKV, Science Express 2007
DC
AC
0 0.5 1 1.5 2 2.5 30
5
10
15
RF
freq
uenc
y (G
Hz)
external magnetic field (T)0 1 2 3Bext (T)
RF
freq
. (G
Hz)
0
5
10
15 g ~ 0.39
0 200 400 600 80020
40
60
80
100
120
140
160
180
200
Burst time (ns)
Dot
cur
rent
(fA
)
15.2 GHz
0 400 800
RF burst length (ns)
0.2
0.1
0
dot c
urre
nt (
pA)
Easier local addressingAll-electrical control possible
Mechanism: spin-orbit interaction
Theory: Golovach, Borhani, Loss, PRB 2006
Efl
fB acSO
Rabi
r1~,1
)()( yyxxxyyxR ppppH σσβσσα −+−=Rashba Dresselhaus
)( αβ ±=
mlSO
h
fac (GHz)
lSO ~ 30 µµµµm
Bext // E(t) // [110] or [110]
Ramsey fringes and dephasing
Free evolution
xy
z
xy
z
xy
z3π/2
xy
zπ/2
Free evolution time (ns)
T2*~35ns
average over nuclear fields
T2* ~ 35 ns
60
80
100
120
140
160
Relative phase 2nd pulse0 π 2π−2π −π
curr
ent (
pA)
Spin echo – unwind dephasingnuclear spins evolve only slowly Koppens, Nowack, LMKV,
arXiv:0711.0479
π/2 π/2τ τ
π
2τ (ns)
Bext = 48 mT
T2,echo~ 0.26 µsBext = 70 mT
T2,echo~ 0.47 µs
2τ (ns)
Y
X
Nuclear spin dynamics
Theory:de Sousa, das Sarma, PRB 2003Coish, Loss PRB 2004Witzel, de Sousa, das Sarma, PRB 2005
• nuclear-nuclear flip-flops through direct dipole-dipole coupling (> 100 µs)
• electron-nuclear flip-flops (strongly suppressed for B ≠≠≠≠ 0)
• nuclear-nuclear flip-flops through two virtual electron-nuclear flip-flops
T2,echo depends on timescale (tnuc) and magnitude (1/T2*)of nuclear field fluctuations
Klauder & Anderson, PR 1962
E.g. can have tnuc = 10 sec, T2* = 10 ns, giving T2,echo = 10 µs
Yao, Liu, Sham, PRB 2006Deng & Hu, PRB 2006…
C = 1.5µF
Faster charge detection (cryogenic amplifier)
1K
4K
RT
40mK
0 200
I QP
C[a
.u.]
Time [ µµµµs]
Signal bandwidth: ~1 kHz – 1 MHz
Single-charge detection in smaller bandwidth
Vink, Nooitgedagt, Schouten, LMKV, APL 2007
Other decoherence mechanismsvirtual tunneling processes to the reservoirs
• was limitation for max. power in ESR • can be suppressed by raising tunnel barriers
B = 0.02T
0 4 8 20
//1
0.5
0
waiting time (ms)
frac
tion
of ‘T
’
1/T1
T
S
//
Hanson et al., PRL 2005 Elzerman et al.,Nature 2004Amasha et al., cond-mat/0607110
T1 up to 1 sec !
spin-orbit interactionT2 = 2 T1 Golovach, Khaetskii, Loss, PRL 04
Spin-orbit with phonons dominates T1
Meunier, Vink, Willems v Beveren, Tielrooij, Hanson,Koppens, Tranitz, Wegscheider, Kouwenhoven, LMKV, PRL 2007
Theory: Golovach, Khaetskii, Loss, PRL 2004
0.0 0.2 0.4 0.6 0.8 1.0 1.2 1.40
1
2
3
T1
[ms]
S-T splitting [meV]
|`↑↑↑↑´⟩⟩⟩⟩ = |↑↑↑↑g⟩⟩⟩⟩ + α|↓↓↓↓e⟩⟩⟩⟩
|`↓↓↓↓´⟩ = |↓g⟩⟩⟩⟩ - α|↑↑↑↑e⟩⟩⟩⟩
phonon wavelengthmatches dot size
|g⟩⟩⟩⟩
|e⟩⟩⟩⟩
Spin qubits in quantum dots – status
Initialization 1-electron, low T, high B0
1-qubit gate electron spin resonancegate duration ~ 25 ns; observed 8 periods
2-qubit gate exchange interactiongate duration ~ 0.2 ns; observed 3 periods
SL SR
Read-out via spin-charge conversion
See also Hanson et al, Rev. Mod. Phys. 2007
duration ~ 100 µs; 82-97% fidelity
duration ~ 5 T1; 99% fidelity ?
Decoherence T1 ~ 1 ms – 1 secT2* ~ 20 ns; T2 > 1 µs
spin-orbit + phononsnuclear spins
Main themes in the coming years
Controlling thenuclear spin bath
Bell’s inequalities
Novel materialssystems
Quantum control and entanglement
RF1
RF2
J
Hyperfine in graphene is tiny
1) Only 1% of carbon atoms have a nuclear spin (13C)Furthermore, 99.9% pure 12C is easily available,and synthetic graphene exists
| ( ) |H E kψ ψ>= >r
2pz2s
2) The conduction and valence band are made from p-orbitals,which don’t overlap with the nuclei (no contact hyperfine)
Spin coherence time ?dipole dipole coupling?anisotropic hyperfine?
Spin-orbit in graphene is weak as well
Carbon is a light element
HSO = λSO σz sz τz
HR = λR (σx sy τz - σy sx)
λSO ~ 0.5 µeV
λR ~ 0.1 µeV / VG
Min et al, cond-mat/0606504Yao et al, cond-mat/0606350Huertas-Hernando et al, cond-mat/0606580
sublatticespin
valley
HD = β ( -σx px + σypy)
HR = α ( σx py - σypx)
β pF ~ 150 µeV (n=1011cm-2)
comparable
Compare GaAs:
Spin relaxation time ?electron phonon coupling?
other heat baths?
Trombos et al., Nature 2007But: spin flip time in 2D graphene ~ few 100 ps
Graphene quantum dots ?Etching
Top gating
“Bad” contacts
by far preferred(control and tunability)
© Geim© McEuen
© Dekker © Eriksson
Electrostatic barriers and Klein tunneling
No electrostatic confinement!Need to create a semiconducting gap
Katsnelson, Novoselov, Geim, Nature Phys. 2006
Bandgap from confinement (ribbons)
Armchair edges: insulating, except for N=3n-1
Zigzag edges: always metallic (edge states at zero energy)
Tight binding Nakada et al., PRB 54, 17954, 1996
Gap from spin-ordering at edges ? Son, Cohen, Louie PRL 2006
Always gap from lattice deformation at edges ? Son et al., PRL 2006
Bandgap in ribbons (1)
-40 0 40-3
-2
-1
0
1
2
3
10V 20V 0V
I sd(n
A)
VSD
(mV)
r60_iv5,6,8
Wehenkel, Heersche et al, See also Han et al, PRL 2007
0 5 10 15 20 25 30 35 40 45 50
5
10
15
20
25
30 C
G (
µS)
Vg (V)
r70_li1
VG (V)
G (
µS)
70 nm
60 nm
Bandgap in ribbons (2)
Delft (Wehenkel, Heersche et al) Columbia , PRL 2007
Always gapped even though edges were not controlled
In addition: charging contributionVG (V)
10 200
0
100
-100
VS
D(m
V)
60 nm
0 20 40 60 80 100 1200.0
0.2
0.4
0.6
0.8
1.0
gap-1
(m
eV-1)
width (nm)
Extracted gap size versus ribbon width
0 20 40 60 80 100 1201
10
100
gap
(meV
)
width (nm)
Kim Delft
Bandgap in asymmetrically doped bilayers
Expt.: Ohta et al, Science 2006Also: Castro et al, cond-mat/0611342
Chemical doping of top layer (SiC substrate)
Theory: McCann & Falko, PRL 2006McCann, PRB 2006Min et al, PRB 2006
Vbg > 0 > Vtg
McCann, PRB 2006Min et al, PRB 2006
SiO2
backgate
Bare gap (meV)
Sel
fcon
sist
ent g
ap (
meV
)
1000 50
40
20
0
EF
Vbg > 0
Electric control of bandgap and Fermi level
bilayer
topgate
300 nm
15 nm
-50 V
2.5 V
50 mV bare gap
< 10 meV actual gap0.3 nm
Single layer
Bilayer
Low temperature measurements of bilayer graphene
Oostinga, Heersche, Liu, Morpurgo, LMKV, arXiv:0707.2487
T = 55, 270, 600, 1200 mK
Electrically induced insulating state
Temperature dependence peak resistance
55 mK – 5 K range: variable-range hopping (for highest fields)
Points at gap with localized states inside the gap (disorder)
Oostinga, Heersche, Liu, Morpurgo, LMKV, arXiv:0707.2487
Magnetoresistance in graphene rings
Russo, Oostinga, Wehenkel, Heersche, Sobhani, LMKV, Morpurgo, arXiv:0711.0479
150 mK
Observations:• Weak localization (probably)• Aperiodic conductance fluctuations• Aharonov-Bohm conductance oscillations
Procedure:lock-intwo-terminalcurrent-biased
Temperature dependence AB amplitude
Expect ∆Grms ~ exp[-πR/Lφ(T)] (ETh / kT)-1/2
Observe thermal averaging (note Eth ~ 10 µeV < 150mK ~ kB T)
Indicates Lφ > few µm
See also WL data of Tikhonenko et al, arXiv:0707.0140
Gate voltage dependence AB amplitude
AB amplitude linear in conductance
Russo, et al, arXiv:0711.0479
Magnetic field dependence AB amplitude
Not due to magnetic impuritiesPossibly orbital origin
800 mK
150 mK
Message for graphene spin qubits
It may be possible to define dots using electrostatic gates
Role of disorder to be explored further
Spin coherence time could be very long
Jeroen Elzerman (ETH)Ronald Hanson (UCSB)
Laurens Willems v Beveren (UNSW)Josh Folk (UBC)Frank Koppens
Ivo VinkChristo Buizert (U Tokyo)
Klaas-Jan Tielrooij (AMOLF)Tristan MeunierKatja Nowack
Tjitte NooitgedachtHan Keijzers
Leo KouwenhovenLieven Vandersypen
External collaborationsLoss group (Basel)Nazarov (Delft)Rudner & Levitov (MIT)Wegscheider (Regensburg)Tarucha group (Tokyo)
GaAs spin qubits
People and collaborations
GrapheneHubert Heersche
Pablo Jarillo-Herrero (Columbia) Jeroen Oostinga
Xinglan LiuAlberto Morpurgo
Lieven Vandersypen