presente e futuro/ present status and future...
TRANSCRIPT
Presente e Futuro/
Present Status and Future Developments
Conference Proceedings Vol. 96
“The Nuclear Physics from the f7/2 to the Quark - Gluon Plasma”
F. Gramegna, M. Cinausero, D. Fabris (Eds.)
SIF, Bologna 2008
THE 1f7/2 SAGA
R.A. Ricci
I.N.F.N.- Laboratori Nazionali di Legnaro and University of Padova
INTRODUCTION
This is just a personal “historical” review
concerning the evolution of nuclear spectroscopy
of the “magic” shell-model region (the 1f7/2 one)
and the corresponding experimental and
theoretical investigations to which a large part of
my scientific career and even of my human
journey was devoted.
Fig. 1: The γ-ray and γ−γ summing coincidence
spectrum and level scheme of 50Ti (left) compared with 42Ca (right).
Another important reason is that the foundation of
nuclear spectroscopy in Italy did occur at the
beginning of the 60’s when I came to Naples
back from Amsterdam where I spent one of the
most pleasant and fruitful periods of my
scientific life. It was characterized by the
experimental investigation of an impressive
number of new decay schemes due to the
possibility of producing radioactive nuclear
species with dedicated charged particle
accelerators or neutron generators and of
measuring the associated γ-rays via the only just
invented scintillation detection technique. These
researches were performed at the Philips
Cyclotron of IKO (“Instituut voor Kernphysics
Onderzoeck”) in Amsterdam and at the 14 MeV
neutron generator in Napoli in the years 1950-
1960.
The starting point of the “1f7/2 saga” was
the investigation of the 50
Ti γ-spectrum
following the β-decay of 50
Sc produced by the 50
Ti(n,p)50
Sc reaction with the 14 MeV neutrons
arising from the 400 keV Van der Graaff
accelerator [1] (see Fig. 1).
Fig.2: Cover of the experimental nuclear
spectroscopy “Bible” in the ‘60th.
151
The main experimental tool which was of
paramount importance in such investigations was
the γ-scintillation spectrometry as described in the
chapter devoted to the “Procedures for the
investigation of the disintegration schemes-
Scintillation spectra analysis” of the famous
book edited by K. Siegbahn in 1965 on “Alpha,
Beta and Gamma-Ray Spectroscopy” [2] (see
Fig. 2).
The power of such a methodology is well
illustrated in Fig. 1 by the γ-scintillation spectrum
of 50
Ti analyzed by means of the “peeling”
technique; the γ-spectrum under study was
decomposed into its single γ contributing parts by
comparison with the pulse-height distributions of
standard calibration sources (with well known
γ−ray energies) measured under the same
experimental and geometrical conditions.
The case of 50
Ti is also a typical example
of the application of the “summing technique” for
detecting γ−γ coincidences. It consists in
exploiting in a proper way the “summing effect”,
which is present in the crystal when random and
true coincidence occur between the absorbed
γ−rays and the coincident radiations are detected
within the resolving time of the detector (normally
1 μsec for a NaI(Tl) crystal coupled to a standard
pulse-height analyzer). The corresponding photo-
peaks will overlap giving rise to a summing
photo-peak whose energy is the sum of the single
γ-ray energies. The effect is emphasized by
varying the distance (i.e. the solid angle) between
the source and the detector and, in particular, by
using a geometry close to 4π, i.e. a “well-type”
crystal with the source in the well.
The 50
Ti γ-spectrum reported in Fig. 1 as
measured with the source outside and inside the
well-type crystal clearly shows the double and
triple coincidences corresponding to the cascade
γ-rays in the level scheme also reported in Fig. 1,
in comparison with that of 47
Ca (two neutrons in
the f7/2 shell).
1. THE (1f7/2)2 TWO PARTICLE SPECTRA
The 50
Ti result showed for the first time
the coincidence of the effective two-particle
interaction both for protons (1f7/2)2p and
neutrons (1f7/2)2n in the T= 1 states (0
+, 2
+, 4
+,
6+). The other states in
42Ca are of different
configuration (collective states).
Another important feature revealed was
the fact that the two-particle spectra are simpler
and easier to be recognized near 48
Ca as, for
example, 50
Ti and 48
Sc than near 40
Ca as 42
Ca
and 42
Sc [3]. In fact the information about the
effective two-body force in the f7/2 region is
really powerful since there are, in principle,
eight nuclei which can provide different types of
particle-particle, particle-hole and hole-hole
spectra. It can be seen, as I will report later that,
at a first approximation, the behavior of the T=0
and T=1 two-body spectra are in fair agreement
with the charge and symmetry independence of
the effective interaction.
It is interesting to quote here the important
observations of two pioneers in the field, who
represented for me and for the Italian groups
involved in the development of nuclear structure
studies in Italy not only very nice personal
friends but also invaluable advisors. I am
referring to Igal Talmi and Haru Morinaga1.
In his remarks on “the shell model
approach to the f7/2 shell” in the occasion of the
“famous” (let me use this expression)
International “Topical Conference on the
Structure of 1f7/2 nuclei” (Legnaro, 1971) [4],
I. Talmi argued about the persistent problem
“….why does the shell model apply at all”,
asking the question of understanding even the
title of that Conference.
In fact: “ ...If 40
Ca is very far from being
a closed shell, what sense does it make to speak
on the f7/2 shell. Still, I am happy to see that our
1 The presence of Igal Talmi today is really very
gratifying. Haru Morinaga, who has not been able to
come, still remains for us a reference person so as Bob
Van Lieshout, Aaldert Wapstra, Maurice Jean and Allan
Bromley.
152
experimental friends were not brainwashed and
still think that there is such an object. Certainly
nuclei in this region show many features which
go beyond simple f7/2 configurations, like the
existence of excited deformed states, p3/2
admixtures etc. Nevertheless, I believe that we
should still try to see the general features of the
forest in spite of the very many interesting trees in
it…………already in 42
Ca we encounter some of
these extra features. Above the first excited 2+
state there are 0+ and 2
+ states which are most
probably due to deformed core excited states. The
existence of these two states, which were even
given many years ago 4+ and 6
+ assignments,
prevented the emergence of the f7/2 picture”.
As he mentioned, that the (f7/2)n
description could work well for proton
configuration was shown by Lawson and Uretsky
[5] and this opened the way to apply this approach
also to the Calcium isotopes for neutron
configuration.
It should not be surprising that the 42
Ca
spectrum was considered a “puzzling” problem
(another one was the 42
Sc, T=0, spectrum for the
complete knowledge of the two-particle
interaction).
In the 1f7/2 shell there are simple
configurations with maximum isospin which
contain only neutrons or protons outside the
closed shells and where the shell-model
calculations are successful. A more complete
description, taking into account both protons and
neutrons were performed for the first time in the
pioneering work of McCullen, Bayman and
Zamick [6] (the so called MBZ approach).
On the other hand, in his concluding
remarks, H. Morinaga [7] mentioned that the main
problem was to compare the 1f7/2 proton and
neutron spectra on sound experimental basis. This
was of course very important for the extraction of
the “effective two-body interaction” as assumed
by I. Talmi for the calculation of energy levels
and effective operators in a single jn
configuration.
Morinaga did remind that the concept of a
single 1f7/2 shell was born already in 1948 when
Meyer and Jensen proposed the shell model but
that the first quantitative efforts started in 1955
when Ford and Levinson [8] tried to calculate
the 43
Ca spectrum taking the single-particle
energies from 41
Ca and the two-body residual
interaction from the 42
Ca spectrum, known at
that time.
After a first positive finding however:
“……there arose doubt about experimental
results on 43
Ca. Then soon after, there came
doubt on the spin assignments in 42
Ca. The β-
decay of 50
Sc was then studied but the spectrum
of 50
Ti was quite different from that of 42
Ca.
We have then studied the β-decay of 42
K and
found that the 1.836 MeV state in 42
Ca was 0+
instead of 4+ and moreover the 2.422 MeV state
was 2+. The 4+ state had to be pushed up to
2.76 MeV. But there was still uncertainty in the
β-decay of 50
Sc. That time we could not
distinguish the 6+-4
+ 0.52 MeV transition from
annihilation radiation”.
“Waiting for Godot” one could say.
And then (quoting Morinaga again):
“The final touch for the 50
Sc level scheme was
made by the Napoli group (i.e. G. Chilosi, P.
Cuzzocrea, R. A. Ricci, G. B. Vingiani) with
their 400 keV accelerator. This was one of the
most pleasant experiments I was ever involved
with. Of course the part of the spectra, the 0-2-
4-6, was very satisfactory. The same time the
problem of the foreign 0+
, 2+ in
42Ca came up.
We suspected the fact that it could only be
explained as the core-excited state, although as
experimentalists we never tried to say that this
is a seriously deformed state. This 0+ state have
been since then many times rediscovered by
clever theoretical physicists in the nuclear data
sheets”.
It is of course rewarding to notice that,
already at that time and, more precisely,
afterwards [9], the comparison of the two-
neutron spectrum of 42
Ca with the two-proton
one has been extended to the mirror 42
Ti where
not only the same 0+, 2
+, 4
+, 6
+ two particle
sequence has been observed but also 0+, 2
+ extra
(deformed ?) states as expected by the influence
153
of the 40
Ca core (less rigid than 48
Ca) [2, 9].
Perhaps the proper way to resume the interest of
the 1f7/2 nuclear region is to quote the pertinent
part of my introductory talk to the Legnaro
Conference in 1971 “Why 1f7/2 nuclei”.
.. One should also keep in mind the following
points :
a) this is a region where most of the
meaningful tests of nuclear wave functions
by means of lifetime measurements,
electromagnetic transition rates and
spectroscopic strengths are being
collected.
b) In spite of the overcoming old superstition
about the possibility of describing the
whole 1f7/2 region by the simplest pure-
configuration model, such class of nuclei,
which is confined in a “compact” area
characterized by the three “doubly-closed
shell cores”, i.e. 40
Ca, 48
Ca and 56
Ni, still
needs to be “privileged”.
As a consequence, designating them as
“the 1f7/2 nuclei” preserves some
meaning.
c) There are, in this “1f7/2” region, 49
nuclides, so far known, with 18 stable
nuclear species, so that the different types
of available reactions can, in principle, be
used to provide information on almost all
the nuclear spectra of interest”.
The “so far” known nuclei were indicated by a
“triangle” in a Z-N representation as shown in
Fig. 3, with the 3 vertices on 40
Ca, 48
Ca and 56
Ni
(see ref. [3]).
Quoting my introduction again:
“One can already draw, in this representation,
some borderlines to distinguish the “gross
features” of these nuclei. Near the 48
Ca-56
Ni line,
one has the “spherical shell-model region”; in
fac, it is known that 48
Ca (and perhaps 56
Ni) is a
better closed-shell core than 40
Ca and that the
N=28 isotones are quite well described by the
simple shell model without too many theoretical
sophistications. Following the 40
Ca-48
Ca line, we
find the Calcium isotopes, which start to display
core-excited effects, especially near 40
Ca and
open the way to deformations and rotational
like bands displayed by the nuclei following the
diagonal lines from 43
Sc to 49
Cr and from 45
Sc to 45
V”.
Fig. 3: The “1f7/2 “ nuclear region in a Z-N
representation; the borderline from 56
Ni to 46
Ca
indicates at the right-hand side the “good” shell
model nuclei. Nuclei represented with horizontal
bars display core-excitation effects; nuclei with
diagonal bars display some deformation effects; the
doubly diagonal bars indicate the presence of
rotational-like spectra.
A particular case which was emphasized in that
context was 42
Sc which was of great importance
in providing both T=0 and T=1 two-body
spectra for the 1f7/2 nuclei. The story of such a
nucleus is really interesting since one had to
wait the evolution of the experimental data
which was seriously modified as compared with
the old data (see ref. [2]).
The 42
Sc level sequence reported in Fig.
4 together with those of other well established
(1f7/2)2 nuclei refer to the data taken by W.
Kutschera et al. in 1977 [10] where the
evolution of the (1f7/2)+2
T=0,1 normalized to the
6+ levels (the less perturbed by Coulomb shift
corrections) is reported.
154
These data were summarized at the second
topical Conference on the “Physics of Medium-
Weight Nuclei” held in Florence in 1977 [11],
where also the high-spin configuration, the
electromagnetic properties, the Yrast bands and
the rotational bands in the region were reviewed.
Fig. 4: The (1f7/2)±2
T=0, T=1 spectra normalized to 6+
levels.
2. THE ENERGY SPECTRA AND THE
PRODUCTION OF NUCLEAR STATES IN
THE 1f7/2 REGION
The 1f7/2 problem in Nuclear Spectroscopy was
reviewed in 1969 in the so called “Bible” (the
definition is of Gerry Brown) of the properties of
such nuclei by P. Maurenzig and myself [12] (see
Fig. 5).
That review came from a set of
experimental data and theoretical calculations
arising from radioactive decays, stripping and
pick-up reactions, in-beam γ−ray spectroscopy,
lifetime and transition probabilities as well as
from some descriptions based on semi-
phenomenological models and few microscopic
approaches performed at that time.
The evolution of the various (1f7/2)n
spectra has been a more and more cogent test of
the model descriptions of the nuclear structure in
the region. An important piece of information was
the sequence of unperturbed single-particle and
single-hole states. Fig. 6 reports the centroids
(energies averaged over the isospin and
spectroscopic strengths) of such states as arising
from various single-particle transfer reaction
experiments [13] (see also ref. [12]).
Fig. 5: The “f7/2 Bible” in 1969
Fig. 6: Centroids of the unperturbed single-particle
and single-hole states referred to 40Ca and 48Ca
cores. The 1f5/2 - 1f7/2 splitting is often taken as ~6.3
MeV.
155
I like to mention here the important
information concerning the 1f7/2-1d3/2 energy
separations obtained by (p, 2p) knock-out
reactions at the 155 MeV synchrocyclotron in
Orsay by measuring the scattered protons at equal
angles with the help of magnetic analyzers. The
results obtained are shown in Fig. 7 where the f7/2-
d3/2 binding energies are reported together with the
excitation energies of s and d hole states in some
1f7/2 nuclei.
Fig. 7: a) Binding energies Bp of 2s1/2 nuclei, from
(p,2p) reactions; the full line connects the data
corresponding to even-even residual nuclei. The target
nuclei are indicated in the upper part of the figure.
The points indicated as 1d3/2 and 1f7/2 correspond to
the proton binding energies in the ground state of the
target nucleus; b) excitation energies E* of 2s1/2 and
1d5/2 proton-hole states in the odd nuclei reported in
a); c) excitation energies E* of 2s1/2 proton-hole
states in the even-even nuclei reported in a). The main
difference between b) and c) is due to pairing effects.
The problem of the evolution of single-
particle energies in this region is also reviewed by
B. Fornal [9] at this Conference, on the basis of
our detailed discussion (see ref. [13]) on the
variation of the 1f and 2p states with their spin-
orbit splitting in filling the 1f7/2 shell either by
neutrons or by protons. Those results already
indicated a strong residual interaction in the T=0
than in T=1 two-nucleon state, which gives rise
to a tighter binding for the protons when the
1f7/2 shell is full of neutrons.
Moreover, not only the 1f7/2 but also the
1d3/2 proton states are pushed down by the
neutron excess in the 1f7/2 shell, and this is in
agreement with the decrease of the mean charge
radius from A=40 to A=48 as observed
experimentally [14].
Since this is a very interesting topic that
I know will be quoted by Fornal in this report, I
like to recall few remarks I did in my report at
the Varenna School in 1967 [12].
“…… Once the 1f7/2 neutron shell has
been filled no important effects are observed in
filling the 1f7/2 proton shell; this could be
associated with a blocking effect of the neutron
excess.
However, all these effects are also
related to the more or less important
modification in the spin-orbit splitting. …….
This splitting……. is not seriously modified both
for neutrons (….. ~ 2 MeV for 41
Ca and 49
Ca)
and for protons (…~ 1.8 MeV for 41Sc and 55
Co,
and ~ 2.5 MeV for 49
Sc)…… The same is not
true for the spin orbit splitting concerning the 1f
state: it changes from 5.5 MeV in 41
Ca to 6.2
MeV in 47
Ca and 7.7 (or 8.7) in 49
Ca; from 5.9
MeV for 41
Sc and 49
Sc to 4.6 MeV for 55
Co. The
fact that it remains constant from 41
Sc to 49
Sc is
due to the self-binding effect in both 1f7/2 and
1f5/2 proton levels when the 1f7/2 neutron shell is
filling”. I leave any other comments to Fornal.
Concerning the more extended problem
of the (1f7/2)n configuration with n>2, an
interesting case was that of (1f7/2)+ 3
nuclei. Just
as an example I like to remind our findings for 51
V and 53
Mn [15] and their comparison with
other similar nuclei [16] . Fig. 8 shows that
comparison as reported by Talmi.
156
Fig. 8: Levels of (1f7/2)n configurations in odd nuclei.
The low-lying levels 7/2-, 5/2
- ,3/2
- are quite
well described by using the two-nucleon matrix
elements arising from the pure (1f7/2)2 interaction;
there were questions concerning the regularity of
the excitation energies with the 5/2- state lying to
low and the 3/2- state too high in
45Ca and also the
possibility of the presence of core-excitations
especially near the 40
Ca core. On the other hand
more crucial tests could be found in the
electromagnetic transitions. A case in point was
the measurement of mean lives (using the Doppler
shift attenuation method) and of branching and
multipole mixing ratios in the γ-transitions of 53
Mn [15].
The results showed that M1 transitions
between states assumed to belong to the basic
(πf7/2)-3
multiplet are retarded by factors of the order
of 10 to 100 and the E2’s enhanced by a factor of
10 in agreement with the behavior of 51
V (with
πf7/23
configuration) supporting the basic shell
model features of nuclei with a 48
Ca core.
A fundamental problem in this context is
that related with the 207
Bii207Pb decay for the
characterization of the ratio of the single particle
f7/2ip3/2 transition to the f7/2if5/2 one (E2/M1).
Fig. 9a) shows the level scheme of 207
Pb
which clearly displays the sequence of the single-
hole states in the unfilled 126 neutron shell, while
in Fig. 9b) the coincidence γ-spectrum taken via
the summing scintillation technique revealing the
γ-decay of the f7/2 level at 2341 keV to the p3/2 one
(E2 transition of 1445 keV) and to the f5/2 level
(pure spin-flip M1 transition) [17] is shown.
Fig. 9: a) Decay scheme of 207Pb following the
decay of 207
Bi. b) Sum coincidences with 2340 keV
sum energy. The inset shows the central part
enlarged.
The measured M1/E2 ratio (0.023+0.002)
showed that the M1 transition is hindered by a
factor of ~ 4. It is a clear case reported by Bohr
and Mottelson [18] in the chapter concerning the
electromagnetic moments particularly with
respect to magnetic dipole effects in single-
particle configurations.
3. DEFORMATIONS IN THE 1f7/2 SHELL
The fact that a quite general
enhancement of E2 transitions [12] was
observed in the 1f7/2 shell could indicate some
kind of deformation in the shell model states
which was also correlated to the fragmentation
of such states and to the presence of positive-
parity states. Questions arose about some
splitting of the shell-model states as arising from
157
the Nilsson diagram, due to an axially symmetric
non spherical field.
Moreover the presence of low 1/2+ and
3/2+ states interpreted as hole s1/2
- and d3/2
- hole
states in odd Scandium isotopes were interpreted
as a particular case of core excitations due to the
deformed 40
Ca core.
I will not enter into details here about the
problem of the “superconducting” behavior
(pairing force, diffuse Fermi surface) of nuclei
like 40
Ca where, as shown by stripping and pick
up reactions, the shell closure N or Z=20 does not
correspond to a sharp Fermi surface. A detailed
discussion can be found in ref. [12].
In any case the possible core excitations
could be taken into account by allowing collective
vibrations (quadrupole and octupole states) and
treating the odd-particle levels as due to the
coupling between single-particle states and the
even core excitations [19].
We were of course aware of the fact that
one should consider such an approach in the
frame of a “weak coupling” model and that, as
shown in more recent and advanced theoretical
descriptions, more configurations are needed [20]
or different coupling scheme like the Interacting
Boson Model [21] could apply.
On the other hand the phenomenology of
the nuclear properties in this region has been
extensively enlarged also by the characterization
of “collective” states as produced in inelastic
scattering experiments. I will report as an
example, the result of (p,p’) inelastic scattering in
that region, performed at Orsay with the 155 MeV
synchrocyclotron [22] .
The collective behavior is normally related
to the first 2+ levels in even-even nuclei, apart
from the shell effects. Fig. 10 shows the situation
summarized in 1969 [12] concerning the energies
and the corresponding transition enhancement
factors as a function of N of the even-even nuclei
filling the 1f7/2 shell.
The strong correlation between the
lowering of the deformation collectiveness with
the increasing of the excitation energy near the
closed shells is clear.
More interesting, and in some sense more
puzzling, was the case of 3- octupole states.
Such states cannot be interpreted in terms of
single particle excitations in the (f7/2)n
configuration since no negative parity states
may be formed by coupling two nucleons in the
1f orbit.
Fig. 10: Excitation energy E(2+) and acceleration
factor G=B(E2Ļ)/B(E2Ĺ)sp of the first level 2+ as a
function of Z and N, in the couple of nuclei f7/2. The
continuous line in the upper panel connect the
values of the parameter β2R0. Their scale is on the
right.
The more realistic assumption was to
consider them as particle-hole states (based on
the promotion of 1d-2s states of the core to the
1f-2p orbits). On the other hand they could be
referred to collective octupole vibrations
lowered in energy by the spin-orbit coupling.
The experimental results as summarized in Fig.
11 for 1f7/2 nuclei show a certain fragmentation
of such levels (in the figure the two main 3-
states are reported) which is not in good
agreement with the particle-hole model. Also
their strength decreases with the addition of
“valence” nucleons.
This does not mean that the “collective”
description is better because this strength does
not increase when the states become nearer to
158
the ground state (contrary to the 2+ states). This
behavior should be referred to the variation of
ground-state correlations approaching 48
Ca.
In conclusion, this review that I have
presented here as a kind of recollection of the
“1f7/2 saga” is only a part of a long history dealing
with very interesting aspects of the nuclear
structure investigations. And it is very rewarding
to notice today how this subject is enjoying a real
revival.
Fig. 11: Excitation energy E(3-) and acceleration
factor G=B(E3Ļ)/B(E3Ĺ)sp of the 3-
level observed in
the couple of nuclei f7/2. The vertical bars represent
the position of the levels deriving from the
configurations (f7/2)(d1/2)-1
.
4. THE REVIVAL OF (1f7/2) NUCLEI
I think that such a revival is strongly
connected with the advent of the “heavy-ion era”,
which provided the possibility of producing high-
energy, high-spin states, new nuclear species and,
at the same time, the extension and improvement
of detection techniques (γ-arrays in the on-line “in
beam” γ-spectroscopy).
The research field opened in this way also
here in Legnaro with the installation of the first
Italian heavy-ion accelerator (the XTU Tandem of
16 MV) [23] .
Moreover, the advent of the ALPI
(Acceleratore Lineare per Ioni), the new
superconducting LINAC and the new ERC
injector have provided the LNL with more
energetic beams. With heavy ions new
possibilities were open.
Fig. 12: 48
Cr level scheme; experiment vs theory
(shell model with interaction).
A special case was the production of
new isotopes in the region near the proton drip
lines (neutron-deficient nuclei). Exotic 1f7/2
nuclei are of great interest, of course, and will
contribute to new insight into nuclear structure
understanding. Among them are 48
Cr24, 45
Fe19, 46
Mn21, 48
Ni20, 49
Ni21, 50
Cr23.
Another important issue is the finding of
super-and hyper-deformed rotational bands
displaying back-bending (i.e. the inversion of
the moment of inertia).
159
Let me consider some cases in point. I
start first with the 48
Ca24 and 50
Cr26 nuclei, since
they are related to results already found in the
70’s, especially when our group was involved in a
systematic research program as the Tandem
accelerator in Munich [24] .
Figure 12 shows the γ-decay scheme of 48
Cr, which is a typical (N=Z,T=0)nucleus in the
middle of 1f7/2 shell, already far from the stability
line. It is found to be a good rotor ((Q) gives
β=0.3, where β is the deformation parameter) and
its quadrupole properties are well accounted for
by the interacting shell-model (full f-p space
reducing the valence nucleons to 1f7/2-2p3/2),
together with the excellent reproduction of the
energy levels (24)
.
Figure 13 shows the plot of the yrast band
of 48
Cr showing the back bending at J>10h, as
compared with shell-model and mean-field
calculations. The good agreement with the first is
really interesting.
Fig. 13: Back-bending plot of the yrast band of 48
Cr.
Shell-model (SM), means field (CHFB) and experiment
(Exp). (J vs Eγ).
Even more interesting is the case of 50
Cr.
Recent investigations (25)
did confirm the double
back-bending as predicted, due to the addition of
two neutrons. Also in this case the collective
behavior is accounted for by the shell-model (see
Fig. 14).
Fig. 14: Back-bending plot (J vs Eγ) of the yrast
band of 50
Cr.
The progress made with respect to the
previous experiments by the Munich-Padova-
Florence group in the 70’s is evident, in spite of
the fact that the ground-state yrast band was
already found with its collective behavior (see
ref. [24]).
Other recent results are shown in Fig. 15
a), where the T=1 isobaric triplet at A=50 is
reported [26]. It consists of the 50
Cr26, 50
Mn25
and 50
Fe24. Furthermore the f7/2 spin alignment
in the mirror (N3Z) nuclei 50
Cr and 50
Fe is
shown in Fig. 15 b), indicating the possibility of
determining the Coulomb-energy difference as
displayed by the corresponding rotational bands
[27].
160
Fig. 15: a) A=50 , T=1 isobaric triplet; b) The 1f7/2
spin alignment of A=50 mirror nuclei
So far for the 1f7/2 review I could have
mentioned other enterprises in the nuclear physics
field along my personal scientific journey
especially those concerning heavy-ion reaction
mechanisms, dissipative (deep inelastic, fusion-
fission) phenomena, clustering and ternary
processes and intermediate resonance states
induced by heavy ion at low energy and in
medium-mass nuclear region; the experiments
performed at the antiproton LEAR facility at
CERN (the OBELIX collaboration) until the
LNL-CERN collaboration in the field of ultra-
relativistic heavy-ions and the search of phase-
transition in nuclear matter, with particular
emphasis on the identification of the Quark-
Gluon-Plasma, with experiments performed at the
SPS and now in preparation at the LHC (Alice
collaboration). For this I will refer to the talks of
other colleagues and friends at this conference
to whom I want to express my deep appreciation
for this gratifying presence and participation.
In fact my scientific contribution to the
conference could be not dedicated to the
research field which has always been in my
hearth and has accompanied me for many years.
So I will leave to my young colleagues (for me
all of you, with few exceptions- the “old
friends” which means “friends for ever”- are
very young) a message that I take from the
already quoted remarks of H. Morinaga.
In ending his talk in 1971 he reported a
Confucius sentence mentioned by Akito Arima
(I will also use the original types as he did):
which means: “Preserving the old and
knowing the new”.
I don’t know if Bogdan Fornal knew that
sentence or if he read the 1f7/2 book of
1971. In any case it was a good idea and a
very appreciated gift to entitle his talk
“Admiring the old and searching for the
new” (in the fp shell)” which could be
considered as a modern version of the
Morinaga quotation of Confucius.
So I will use some Morinaga’s words as
a conclusion of my message referring to a
journey as long as 40 years:
“The way we came to the present status of
1f7/2 shell is an old story (which is familiar to
those old friends of 1f7/2 shell). Actually for
me it is a real pleasure that I could meet
those old friends. But the story is somewhat
a personal version and all the new friends of
1f7/2 shell should understand that all of us,
the old friends of f7/2 shell, have some
parallel story as mine”.
a)
b)
161
On behalf of them and as a pioneer in the field,
welcome to the “new” new friends of 1f7/2 shell
(or, if you want to be more modern, the f-p shell).
Thank you.
[1] G. Chilosi, P. Cuzzocrea, G.B. Vingiani, R.A.
Ricci and H. Morinaga; Il Nuovo Cimento vol.
XXVII, n. 1, 407, 1963
[2] A.C.G. Mitchell, R. Van Lieshout, A.H. Wapstra,
R.A. Ricci and R.K. Girgis in “α,β,γ-ray
spectroscopy” edited by K. Siegbahn, North
Holland, Amsterdam 1965
[3] R.A. Ricci “Why 1f7/2 nuclei” in Proceedings of
the Int. Conf. on the Structure of 1f7/2 nuclei,
Legnaro 1971, Editrice Compositori Bologna
1971, p. 1
[4] I. Talmi, see ref. [3], p. 511
[5] R.D. Lawson and J.L. Uretsky: Phys. Rev. 106,
1369 (1957); see also R.D. Lawson, ref. 3, p. 520
[6] J.D. McCullen, B.F. Bayman and L. Zamick: Phys.
Rev. 134, B515 (1964); see also L. Zamick, ref.
[3], p. 9 ; see also J.N. Ginocchio and J.B. French;
Phys. Lett. 7, 137 (1963)
[7] H. Morinaga: see ref. [3], p. 529
[8] K. Ford and C. Levinson: Phys. Rev. 99, 792
(1955); 100, 1, 13 (1955)
[9] Cfr. B. Fornal, contribution to this conference:
“That problem was dealing with the incoming
extensive investigation on the coexistence of
single-particle and collective states in this nuclear
region which, from the experimental point of view,
has been and still is at the origin of an impressive
set of measurements and data, especially after the
advent of the nuclear structure studies with heavy-
ion reactions. I am spending some time in
reminding you these details but they are a sort of
“milestones” of the 1f7/2 story and it is what I want
to tell you also as an appropriate acknowledgement
of those pioneering works”.
[10] See W. Kutschera in Proc. of the EPS Int. Conf.
on the “Physics of Medium-Weight Nuclei”,
edited by P. Blasi and R.A. Ricci, Florence 1978,
Editrice Compositori, Bologna 1978, p. 120 [11] See R.A. Ricci “Introductory talk” in Proc.
quoted in ref. [10].
[12] R.A. Ricci and P. Maurenzig: Rivista del Nuovo
Cimento 1, 1, 1969, p. 291; see also R.A. Ricci:
Proc. Int. School of Physics, Course XL,
Varenna 1967, Ac. Press. Rend. SIF, 1969
[13] R.A. Ricci: Proc. Int. School of Physics “E.
Fermi”, Course CLIII, edited by A. Molinari, L.
Riccati, W.M. Alberico, M. Morando, 2003,
IOS Press Amsterdam, p. 627
[14] See e.g.: B.F. Baymann: Proc. Int. School of
Physics “E. Fermi”, Course XL,Varenna 1967,
Ac. Press New York 1969, p. 404
[15] See F. Brandolini, A. Brusegan, C. Signorini
and R.A. Ricci, Il Nuovo Cimento 7.1, 1972, p.
xxx; see also ref. [12] and P. Maurenzig
[16] I. Talmi, Proc. Of the Int. School “E. Fermi”,
Varenna 1976, Course LXIX, edited by A. Bohr
and R.A. Broglia, North Holland 1977, p. 352
[17] G. Chilosi, R.A. Ricci, J. Touchard and A.W.
Wapstra, Nucl. Phys. 53, 1964, 23
[18] A. Bohr and B. Mottelson, Nuclear Structure,
Vol. 1 (New York, Amsterdam) 1969, p. 343,
Table 3-3
[19] See A. De Shalit, Phys. Rev. 122, 1961, p.
1530; see also the discussion of the “center of
gravity theorem in nuclear spectroscopy”
reported in ref. [13]
[20] See A. Covello Proc. Int. School of Physics “E.
Fermi”, Course CLIII, Varenna 2002 , edited
by A. Molinari and L. Riccati (IOS Press)
2003, p. 79
[21] See F.Iachello, as ref.. [20], p. 1
[22] R.A.Ricci, J.C. Jacmart, M. Liu, M. Riou and
C. Ruhla: Nucl. Phys. A91, 1967, 609
[23] See: R.A.Ricci, Nuovo Cimento A, 81, 1994, 1;
C. Signorini, G.P. Bezzon, F. Cervellera, P.
Spolaore and R.A. Ricci, Nucl. Instr. And
Methods, 220, 1984, 30; see also R.A. Ricci,
Nucl. Instrum. Methods A, 328, 1993, 355
[24] See C. Signorini: in Proc. of the Int. School of
Physics “E. Fermi”, Course LXII, edited by H.
Faraggi and R.A. Ricci (North Holland) 1876, p.
499; and H. Morinaga ibidem, p. 351
[25] See S.M. Lenzi et al., Phys. Rev. C60, 1989,
1303; see also S.M. Lenzi, Proc. Int. School “E.
Fermi”, Varenna 2007, to be published; see also
B. Fornal, in ref. [9]
[26] S.M. Lenzi et al., Z. Phys. A354, 1996, 117;
C.E. Asvensson et al, Phys. Rev. C, 58, 1998,
R2621
[27] S.M. Lenzi et al. Phys. Rev. C60, 1999, 1303
162
ADMIRING OLD AND SEARCHING FOR NEW
IN THE fp SHELL
Bogdan Fornal
Institute of Nuclear Physics, Polish Academy of Sciences, Krakow, Poland
INTRODUCTION
The f7/2 nuclei have always been a greatscientific passion of Professor Ricci and itwas just this passion that, already in the six-ties, lead him to very extensive studies of nu-clei with 20≤Z, N≤28. The results collectedin the course of those investigations werepublished by R. A. Ricci and P. R. Mau-renzig in the paper entitled ”The f7/2 Prob-lem in Nuclear Spectroscopy” [1], sometimescalled: ”The Bible on f7/2 Nuclei”. Fora nuclear spectroscopist this review articleis invaluable - it offers a fantastic guidancethrough the labyrinths of nuclear structurenot only restricted to the f7/2 shell. Alsoin my presentation, I will use it as a basefor elaborating on one of the central issuesof modern nuclear spectroscopy - the issueconcerning evolution of the single particlestates in energy when mowing toward exoticnuclei.
One of the most striking characteristicsof nuclear structure are magic nucleon num-bers: 2, 8, 20, 28, 50, 82, and 126. Magicnumbers arise from non-uniformities of thequantum states distribution in energy, be-cause those non-uniformities form the shellsseparated by the energy gaps − completefilling of the shells occurs at magic num-bers of nucleons. The existence of the shellsreflects the fact that nucleons occupy welldefined orbitals and this, in turn, tells usthat they move in a well defined average po-tential. Theoretical picture of a nucleus inwhich the single particle states are calcu-
lated in an average potential well with ad-dition of a spin-orbit term, was developedby Maria Goeppert-Maier and Hans Jensenin 1949 (they were awarded for it the NobelPrize in 1963).
It has been widely discussed of what hap-pens to the arrangement of the single par-ticle levels established for nuclei along thestability valley, when going toward exoticregions of the nuclidic chart. In particu-lar, it is not obvious whether the classicalmagic numbers are valid away from the sta-bility line. It is remarkable that the prob-lem of the single particle states evolutionalong isotopic or isotonic chains of nucleiwas addressed and deeply discussed alreadyin ”The Bible on f7/2 Nuclei”, i.e., fourdecades ago. Let us now focus our attentionon the region of nuclei in which the f7/2,p3/2, f5/2, and p1/2 orbitals are being filledand let’s try to see what one can say aboutthe locations of these single particle states.Figure 1 displays a portion of the historicalpicture from Prof. Ricci’s talk in Varenna in1969 [2], in which he illustrates the results ofan extraordinary analysis of the single par-ticle state behavior in energy in nuclei from40Ca to 48Ca and then from 48Ca to 56Ni.
An extended representation of that pic-ture, supplemented by additional informa-tion from Ref. [2] and from the studies ofneutron orbitals along the N = 28 istones,is shown in Figure 2. It is clear that thechanges of relative positions of the orbitalsare huge even though only very limited re-gion of nuclei is examined. For example,
Conference Proceedings Vol. 96“The Nuclear Physics from the f7/2 to the Quark - Gluon Plasma”F. Gramegna, M. Cinausero, D. Fabris (Eds.)SIF, Bologna 2008
163
FIG. 1: Portion of Fig. 11 from Ref. [2] show-ing the changes in energy of proton single par-ticle states in the fp shell from 41Sc to 49Sc.
near the doubly magic 56Ni the three neu-tron single particle states p3/2, p1/2 and f5/2
are very close to each other, whereas near48Ca they are well separated in energy andtheir spacing is of similar size as that be-tween f7/2 and p3/2, the latter being respon-sible for the shell closure in 48Ca.
Such an observation could have pointed tothe presence of subshell closures associatedwith the filling of the p3/2 orbital, i.e., atN = 32 and, possibly, with the filling of thep1/2 state, i.e., at N = 34 in neutron-richnuclei. However, the issue did not receivemuch attention at the time, as the structureof neutron-excessive nuclei with Z ∼ 20 ap-peared to be out of reach.
SUBSHELL CLOSURE AT N = 32
First information on the possible exis-tence of an N = 32 subshell closure forneutron-rich nuclei just above 48Ca came
FIG. 2: Evolution of proton and neutron single-particle energies (relative to the 2p3/2 state),
when moving from 41Sc to 49Sc, and from 49Cato 57Ni.
in the eighties. The phenomenon was sug-gested by A. Huck et al. [3] who tentativelyidentified a candidate for the 2+
1 state in52Ca with an excitation energy of 2563 keVthat is significantly higher than the corre-sponding 2+ energy in 50Ca. However, theconsiderable uncertainty associated with thespin and parity assignments to this state (in52Ca) did not give much credence to the is-sue. Further indication of development of anenergy gap at N = 32 in neutron-rich nucleiarose from the systematic variation of theE(2+
1 ) energy for the chromium (Z = 24)isotopes, which was found to reach a max-imum in 56Cr32 [4]. At that point, it wasobvious that crucial information on the oc-currence of the N = 32 subshell gap shouldbe provided by data on the yrast structuresof the Z = 20−22 species with N ∼ 32, butthese nuclei are again very neutron rich and,until very recently, their structure was com-pletely unknown. This situation, however,was going to change.
In a series of past experiments, we haveshown that the yrast spectroscopy of hard-
164
to-reach neutron-rich nuclei, populated inheavy-ion multi-nucleon transfer reactions(at energies 15-25% above Coulomb bar-rier), can be studied successfully in γγ co-incidence measurements with a thick target[5–7]. Production of neutron-rich species inthese processes is possible due to a tendencytowards N/Z equilibration of the di-nuclearsystem formed during collision. Usually,in the studied reactions the projectile hadlower N/Z ratio than the target nucleusand, as a result, production of species moreneutron-rich than the light colliding part-ner was favored. Taking into account theseconsiderations, the bombardment of thick208Pb and 238U targets with a 48Ca beamseemed to offer good prospects in reachingnuclei with larger neutron excess than 48Ca,i.e., neutron-rich titanium, scandium andcalcium isotopes.
Two experiments were performed at Ar-gonne National Laboratory employing a48Ca beam from the Argonne Tandem Lin-ear Accelerator System (ATLAS) and thegermanium multidetector array GAMMAS-PHERE, which consisted of 101 Compton-suppressed Ge detectors. During the firstrun, a 305 MeV beam was focused on a50 mg/cm2 208Pb target. In the second,the projectile energy was 330 MeV and a50 mg/cm2 238U target was used. Gamma-ray coincidence data were collected with atrigger requiring three or more Compton-suppressed γ rays to be in prompt coinci-dence. Energy and timing information forall Ge detectors that fired within 800 ns ofthe triggering signal was stored. The beam,coming in bursts with ∼0.3 ns time width,was pulsed with ∼400 ns repetition time,providing clean separation between promptand isomeric events. A total of 8.1×108 and2.3×109 three- and higher-fold events wererecorded in the first and second measure-ments, respectively. Conditions set on the
γγ time parameter were used to obtain var-ious versions of prompt and delayed γγ andγγγ coincidence matrices and cubes cover-ing γ-ray energy ranges up to ∼4 MeV.
In γ-ray spectroscopic studies of the deep-inelastic reaction products, identification ofan unknown sequence of γ rays to a spe-cific product may be possible by using thecross-coincidences with transitions in reac-tion partners. In the case of the 48Ca+208Pbsystem, complementary products in binaryreactions leading to Ti isotopes are Hg nu-clei, but a given Ti product is in coincidencewith several Hg partners because of neu-tron evaporation from the fragments afterthe collision. The situation is illustrated inFigure 3, where the spectrum arising from asum of double gates on known transitions in196Hg is presented. This spectrum, accord-ing to expectations, displays known linesfrom 50Ti, 51Ti and 52Ti, which are part-ners to 196Hg associated with 10, 9 and 8evaporated neutrons, respectively. Furtherinspection of the spectrum revealed also thepresence of unknown gamma rays at ener-gies 1002, 1237, 1495 and 1576 keV. Thesegamma rays were observed also in the spec-tra gated on transitions from the Hg iso-topes with A=197-200 which indicated thatthey originate from the titanium products.It seemed very likely that the new transi-tions occur in the Ti isotopes with massesA>52.
Pursuing this hypothesis we applied theidentification method based on the γ-ray cross-coincidence intensities. For the50,51,52Ti reaction products, the mean massAav(Hg) of the complementary mercuryfragments was determined from the Hg γ-ray intensities measured in coincidence withthe γ rays of that particular Ti isotope. Thesame procedure of calculating the Hg meanmass was applied also to newly found 1237,1495 and 1576 keV Ti lines. The results are
165
FIG. 3: Part of a coincidence γ-ray spectrumfrom the 48Ca+208Pb reaction gated on pairs ofyrast transitions in 196Hg showing gamma raysbelonging to Ti partners.
illustrated in Figure 4, where the Aav(Hg)as a function of A(Ti) is shown. The datapoints corresponding to the known gammarays from 50,51,52Ti nuclei exhibit a smoothcorrelation. The Aav(Hg) for the new tran-sitions fit nicely into this pattern, if one as-signs the 1237 and 1576 keV gamma rays to53Ti and the 1495 keV gamma ray to 54Ti.
FIG. 4: Plot of average mass Aav(Hg) ofcomplementary Hg fragments against Ti prod-uct mass A(Ti) deduced from γ-ray cross-coincidence intensities. See text for details.
The suggestion that the 1495 keV line isa transition in 54Ti, was fully supported by
the data from an experiment performed atMichigan State University (National Super-conducting Cyclotron Laboratory), in whicha beta-decay measurement of the 54Sc par-ent produced in fragmentation of a Kr beam,was studied. The MSU measurement iden-tified the first two gamma-ray transitions in54Ti: 2+→0+ with energy of 1495 keV and4+→2+ with energy of 1002 keV [8].
Using the 1495 keV transition as a ”start-ing point” in the analysis of γγ coincidencedata, we could establish the yrast structurein the 54Ti nucleus up to an energy of ∼6.5MeV. The details of the procedure are re-ported in Ref. 8 and the experimental levelscheme of 54Ti is shown in Figure 5a. Thelow lying yrast sequence is dominated by the2+, 4+ and 6+ states, members of the πf2
7/2
multiplet. The higher yrast excitations arisefrom the configurations involving streachedcoupling of the two f7/2 protons and promo-tion of a neutron to the p1/2 and f5/2 singleparticle states.
As we have just seen, valuable results onnew yrast excitations in the 54Ti isotopewere obtained following deep inelastic reac-tions between a thick 208Pb target and a305 MeV 48Ca beam. However, no infor-mation on 56Ti could be derived from thisdata set. It was then decided to investigatethe 48Ca+238U system instead, in order totake advantage of the larger neutron reser-voir provided by the 238U target. The largerN/Z ratio of 1.59 for the latter target com-pared to the corresponding value of 1.54 for208Pb, was viewed as hope for a productdistribution extending significantly towardsmore neutron-rich nuclei, including the 56Tiisotope of interest here.
At first, it should be recognized that inthe case of the 238U target, the target-likeproducts of deep-inelastic processes mostlyundergo fission. Thus, an identificationbased on cross-coincidence relationships be-
166
FIG. 5: Level schemes constructed for 54Ti and56Ti.
tween gamma rays from reaction partners,such as that performed for the 48Ca + 208Pbsystem reported earlier, is not possible. In-stead, another method for identifying thestarting transitions has to be applied. In thecase of 56Ti, a starting point for the analy-sis was provided by a β-decay study of the56Ti parent, 56Sc [9, 10], which identified a2+→0+ γ ray with an energy Eγ=1127 keV.
A search aimed at finding transitions feed-ing this 2+ excitation, i.e., being in coinci-dence with the 1127 keV line in the 48Ca+ 238U coincidence data set, displayed onlytwo, mutually coincident γ rays with en-ergies of 1161.0 and 690 keV. Taking intoaccount that deep-inelastic reactions pref-erentially populate yrast states, an assign-ment of the 1161 and 690 keV γ rays tothe 4+→2+ and 6+→4+ transitions is thenstraightforward. These two transitions lo-cate the 4+ and 6+ levels at excitation en-
ergies of 2290 and 2980 keV, respectively, asindicated in the level scheme of Figure 5b.
Let us take a look at the new findingsin 54,56Ti from the perspective of system-atics of the lowest yrast excitations in theeven Ti nuclei that is shown in Fig. 6.The observed features of yrast structure of54Ti, such as the relatively high energy ofthe 2+
1 state and the energy spacings be-tween the Jπ = 0+, 2+, 4+, 6+ excitationssimilar to those in the N = 20 42Ti andN = 28 50Ti magic isotopes, are charac-teristic for a magic nucleus and fully sup-port the existence of the N=32 subshell clo-sure in neutron-rich species close to Z = 20.This new subshell closure can be attributedto the existence of a sizeable energy gapbetween the νp3/2 and higher lying νp1/2,νf5/2 orbitals for neutron-rich nuclides hav-ing Z<24. Such a scenario is in line with thesingle particle state arrangement reportedby Prof. Ricci in Ref. [2] (Fig. 2.).
FIG. 6: Systematics of the πf27/2 2+, 4+, and
6+ states in even-even Ti isotopes.
Our spectroscopic finding regarding thethree lowest yrast states 2+, 4+ and 6+ in54Ti, which mirror the 2+, 4+ and 6+ ar-rangement in 50Ti, was associated with alot of excitement. Similar excitement musthave experienced also the researchers who
167
located the first three yrast states in 50Tiand found that their energies are almostidentical to those in 42Ti. Among the pi-oneers who explored for the first time thestructure of 50Ti was Professor Ricci. Infact, the first data on the lowest excitationsin 50Ti were obtained by the group of theItalian physicists G. Chilosi, P. Cuzzocrea,G. B. Vingiani, R. A. Ricci and H. Morinagain Napoli in 1962 (they used beta decay ofthe 50Sc parent produced by irradiation of atitanium matallic foil with 14 MeV neutronsfrom the AN 400 accelerator) [11]. As onecan see, it took more than forty years to ex-tend the knowledge on yrast excitations inthe Ti isotopes by 4 neutrons. On this oc-casion, it is also worth to note that in addi-tion to the 50Ti and 54Ti isotopes, membersof the pure f2
7/2configuration are known in
other two magic nuclei: 42Ca and 42Ti. Thepresence of a pure configuration of two iden-tical nucleons on the same high-spin orbitalin four different nuclei is a unique featurein the nuclidic chart. Figure 7 shows theselowest excitations in 42Ca, 42Ti, 50Ti and54Ti − all they are remarkably similar interms of the energy spacings. Apparently,to a good approximation the interaction ofthe two f7/2 nucleons does not depend nei-ther on the isospin nor on the doubly closedcore.
LARGE-SCALE SHELL-MODEL
CALCULATIONS
Recently, it became possible to performshell model calculations in the full fp shelland our new data on the structure ofneutron-rich nuclei may serve as a test-ing ground for various interactions. Letus recall two Hamiltonians developed forthe fp shell: a new interaction, labeledGXPF1A, that was worked out by Honma et
al. [12], and another empirical Hamiltonian
FIG. 7: The πf27/2 2+, 4+, and 6+ states in
two-valence-nucleon nuclei.
constructed for nuclei in the fp-shell, namedKB3G [13]. As shown in Figure 8, thefull fp-shell model calculations employingthe GXPF1A and KB3G Hamiltonians aresuccessful in describing the yrast structurein 54Ti - particularly good agreement pro-vides the GXPF1A interaction and the re-sults from this Hamiltonian often were usedas guidance for the spin-parity assignmentsproposed in the measured level scheme.
Figure 9 compares the results of the fullfp shell-model calculations with the twoHamiltonians to the available data on the2+
1 energies for the Cr, Ti and Ca isotopicchains. Both interactions give a good de-scription of the variations in the experimen-tal 2+
1 energies near N = 28 and N = 32.However, there is a striking discrepancy be-tween the two types of calculations in 54Ca,for which no measured value is available: theGXPF1A Hamiltonian predicts the 2+ en-ergy at very high value, ∼3 MeV, whereasthe KB3G interaction gives for it a valueslightly above 1 MeV.
Differences in the predictions of the twoHamiltonians regarding the 2+
1 location inthe 54Ca nucleus can be associated with dif-ference in the effective single particle ener-
168
FIG. 8: Comparisons between shell-model cal-culations with the GXPF1A and KB3G Hamil-tonians and data for 54Ti.
gies of the νp3/2 and νp1/2 orbitals withrespect to the νf5/2 state in neutron-richnuclei. According to the the GXPF1AHamiltonian the magnitude of this separa-tion in heavy Ca isotopes is large, whereasthe KB3G interaction produces rather smallspacing. As mentioned earlier [2] and shownin Fig. 2, studies of the location of single-particle states in 49Ca pointed to a size-able (∼2 MeV) energy gap between thetwo higher lying neutron orbitals p1/2 andf5/2 - this observation gives support to theGXPF1A predictions. From a broader per-spective, the issue is of special importancebecause the presence of the νp1/2−νf5/2 en-ergy gap could possibly produce a subshellclosure associated with the filling of the p1/2
state, i.e., at N = 34 in neutron-rich nu-
FIG. 9: Systematics of the 2+
1 energies inthe even Cr, Ti and Ca isopes compared tothe results of shell-model calculations with theGXPF1A and KB3G interactions.
clei. To verify this hypothesis, the magni-tude of the energy separation between thef5/2 and p1/2 orbitals in neutron-rich Ca iso-topes needed to be derived from experimen-tal data, although one should be aware thatthis task represents a significant challengeas the states involving the f5/2 neutron inisotopes such as 51,53Ca are rather difficultto reach.
169
IS THERE AN ENERGY GAP
BETWEEN νp1/2 AND νf5/2?
Using again the thick target γγ coinci-dence data from GAMMASPHERE for thesystems 48Ca+208Pb and 48Ca+238U, andanalyzing the observed production yields forthe 48−56Ti isotopes, it became clear that,particularly in reactions on the 238U tar-get, Ca isotopes with masses up to 51 orhigher had to be present in the data set withcross sections sufficient to examine in detailthe coincidence relationships required to es-tablish significant level schemes. This con-clusion was supported further by the factthat coincidence events were observed be-tween known gamma rays emitted in thebeta decay of 51Ca. Firm identification ofgamma rays in the 51Ca case was, how-ever, very difficult because of a rather lowproduction rate and the limited informa-tion on the location of the yrast states pro-vided by the 51,52K beta-decay measure-ments. The help came from a new, inde-pendent experiment in which the same re-action, 48Ca+238U, was studied, but witha thin target and gamma rays were de-tected in coincidence with reaction prod-ucts identified in a magnetic spectrome-ter. In this second measurement, the sameprojectile-target combination, 48Ca+238U,was investigated at the Laboratori Nazion-ali di Legnaro using the ALPI acceleratorand the CLARA+PRISMA detection setup[14–16]. In this case, the 330-MeV 48Cabeam was impinging on a 238U target of 600µg/cm2 thickness, placed in the center of theCLARA germanium detector array consist-ing of 24 Compton-suppressed clover detec-tors. The PRISMA magnetic spectrometer,used to identify product nuclei, was posi-tioned at 53 degrees with respect to beamdirection, i.e., in the vicinity of the grazingangle. The spectrometer was set up for the
detection of nuclei close in mass to the pro-jectile and the event trigger required the de-tection in coincidence of a single gamma rayin CLARA and an ejectile at the PRISMAfocal plane.
Prior to the present investigations, theonly information available on the 51Ca nu-cleus originated from the beta decay studyof neutron-rich 51K and 52K by Perrot etal. [17]. Excited states at 1718, 2377, 2934,3460, 3500 and 4493 keV were proposed, butonly the 3460-keV level was tentatively as-signed 7/2− spin and parity quantum num-bers. The analysis reported here startedfrom the gamma-ray spectrum measured bythe CLARA array in coincidence with 51Caproducts; the latter is presented in Figure10. Among the gamma lines found in thespectrum appear three transitions with re-spective energies of 2378, 2934 and 3462 keVwhich had been observed earlier in beta de-cay. Other weak lines in the spectrum ofFig. 10 must also belong to 51Ca, but theirordering and mutual coincidence relation-ships could not be established due to the lowstatistics of the gamma-gamma-ejectile co-incidence data. In this situation, the set ofgamma-ray coincidence data obtained withthe thick target at GAMMASPHERE pro-vided crucial complementary information.
In thick target experiments only gammarays emitted from stopped products appearin the spectra as sharp lines (with the widthpractically equal to the intrinsic energy res-olution of the germanium crystal). As aresult, one can display only those gammatransitions, for which the cumulative emis-sion time is comparable or longer than theproduct stopping time (typically of the or-der of 1 ps). This feature poses a limitationon this experimental technique. However,since deep-inelastic processes populate pref-erentially yrast states, the associated halflives involved are often long enough to ex-
170
FIG. 10: Gamma-ray spectrum measured in thethin-target experiment with a gate on 51Ca re-action products identified at the focal plane ofthe PRISMA spectrometer.
plore level sequences up to moderate spin.Using the GAMMASPHERE data set, we
examined the gamma-ray spectrum gated onthe 2378 keV transition, which is the mostprominent gamma line observed in coinci-dence with the 51Ca products. The inspec-tion of the spectrum revealed a series ofweak peaks, potential candidates for gammarays in 51Ca. However, only two out of thosecandidates satisfied the condition of beingpresent also in the 51Ca product gated spec-trum: these were 1466 and 1942 keV lines.Subsequently, a double gate set on the 1466and 2378 pair of gamma rays in the promptγγγ cube displayed the 476 and 311 keVlines both also seen in coincidence with the51Ca product. On the basis of those findingsand other coincidence relationships we wereable to construct an extended level schemefor 51Ca that is shown in Figure 11.
The level scheme established in thepresent work for 51Ca is compared in Fig. 11with the results of shell-model calculationswith the GXPF1A interaction. Based onthe fact that deep-inelastic processes, usedhere to produce the nuclei of interest, pop-ulate preferentially the yrast and near-yraststates, taking into consideration the decay
FIG. 11: Comparison between shell-model cal-culations with the GXPF1A Hamiltonian anddata for 51Ca.
pattern, and guided by the results of theshell model calculations we made tentativespin-parity assignments. Of special interestis a state identified at 4320 keV with a spin-parity assignment of 9/2− which is expectedto involve the promotion of a neutron intothe νf5/2 orbital - the relative location inenergy of that orbital near Z ∼ 20 playsa decisive role in the presence or absenceof a significant N = 34 shell gap in 54Ca.With the character of the 9/2− excitation in51Ca established, the opportunity arises toinspect in detail the behavior of the exper-imental and calculated states with configu-rations involving the νf5/2 orbital along anextended isotonic N = 31 chain, as detailedspectroscopic information is also availablefrom Refs. [18, 19] for 53Ti and 52Sc. Figure12 displays the partial level schemes of thethree nuclei and compares the states of in-terest with the results of shell model calcula-tions with the GXPF1A and KB3G interac-tions. The yrast states containing the νf5/2
171
orbital in their main configuration are: the4320-keV, 9/2− level in 51Ca, the 3603-keV,8+ state in 52Sc, and the 21/2− level at 6056keV in 53Ti. For the GXPF1A Hamilto-nian, the agreement between the experimen-tal and the calculated values is very good inthe heaviest isotone. However, the devia-tion between the data and the results of thecalculation, increases slightly in 52Sc, andbecomes even larger for 51Ca. In turn, theKB3G calculations underestimate the 9/2-energy in all three cases by several hundredsof keV. Thus, the observed behavior of thestates with predominant f5/2 configurationsuggests that the f5/2 in Ca nuclei is locatedat higher energy than the value given by theKB3G Hamiltonian, but, on the other hand,this energy might be somewhat smaller thanthat predicted by the GXPF1A interaction.The results, however, do not rule out thepresence of a sizeable gap at N = 34, leav-ing the experimental determination of thisfeature as an interesting challenge.
OUTLOOK
By identifying yrast states in the heavyTi isotopes, we have established the pres-ence of a new subshell closure at N = 32 inneutron excessive nuclei. We have also ob-tained information on the energy separationbetween the νp1/2 and νf5/2 neutron or-bitals in the neutron-rich Ca isotopes, whichdoes not exclude the existence of a sizeableenergy gap at N = 34. Even though theseare only the first steps in exploration of theneutron-rich territory, we already see thatin the new regions of nuclear chart the sin-gle particle structure may be different withrespect to that known in the vicinity of thestability valley. The studies along this lineare particularly important for nuclear astro-physics, because it is the structure of ex-otic nuclei that strongly determines the r-
FIG. 12: Comparisons between experiment andshell-model calculations with the GXPF1A andKB3G Hamiltonians for states involving excita-tions of a νf5/2 neutron in the N = 31 isotones51Ca, 52Sc and 53Ti.
process path. Obviously, to advance theinvestigations one needs radioactive beamfacilities, one also will have to use newexperimental techniques. It is very likelythat one of the most effective methods forstudying the structure of neutron-rich exoticspecies will be the gamma-ray spectroscopyof deep-inelastic reactions products. Lab-oratori Nazionali di Legnaro with the al-ready available instruments like PRISMAand with the ongoing SPES project aimedat development of radioactive beams, may
172
become one of the world centers for such in-vestigations.
The present excellence of LNL owes verymuch to Professor Ricci. On the occa-sion of today’s celebration, I would like towish You, Professor, that always continuesYour passion for nuclear spectroscopy andother fields of nuclear physics, Your pas-sion for science which, as You said to theyoung people during the lecture in Varennain 2003, ”is a great intellectual adventure ofhumankind on one hand and a school of crit-icism, freedom and tolerance on the other”.The outstanding role of science in bringingthose ideas closer to life was proven manytimes in the history. One of the best ex-amples is the work of Nicolaus Copernicus.In the Book 1 of his opus ”De revolution-ibus orbium coelestium” (the manuscript ofwhich is located in the Jagiellonian Libraryin Krakow) one finds a sentence that soundsvery familiarly in the context of our discus-sion: ”All the good arts serve to draw man’smind away from vices and lead it towardbetter things”. The concepts of those ”bet-ter things”, which include ”criticism, free-dom and tolerance” were rooted very deeplyat LNL by Professor Ricci, other Professors,and their Followers and have served as abase for developing many fruitful collabo-rations. The collaboration between the In-stitute of Nuclear Physics PAN in Krakowand LNL is a very good example of it.
ACKNOWLEDGMENTS
The results presented in this lecture havebeen obtained in the frame of collaborationsthat gathered researchers from many insti-tutions. The list of the names includes:R. Broda, W. Krolas, T. Pawlat, and J.Wrzesinski from IFJ PAN Krakow, Poland;R.V.F. Janssens, S. Zhu, M.P. Carpenter,D. Seweryniak et al. from ANL Argonne,
USA; P. Mantica, B.A. Brown et al. fromMSU East Lensing, USA; M. Honma fromthe University of Aizu, Japan; T. Otsukafrom the University of Tokyo, Japan; P.J.Daly, Z.W. Grabowski from Purdue Univer-sity, USA; S. Beghini, M. Cinausero, L. Cor-radi, G. De Angelis, F. Della Vedova, E.Farnea, E. Fioretto, A. Gadea, B. Guiot,S. Lunardi, N. Marginean, P. Mason, G.Montagnoli, D.R. Napoli, F. Scarlassara, A.M. Stefanini, D. Seweryniak, S. Szilner, C.A. Ur, J. J. Valiente-Dobon, G. Viesti etal. from INFN di Legnaro, INFN Sez. DiPadova, and from Padova University.
[1] R. A. Ricci, and P. R. Maurenzig, Riv.Nuovo Cim. 1, 291 (1969).
[2] R. A. Ricci, Proceedings of the Interna-tional School of Physics ”Enrico Fermi”,Course XL, edited by M. Jean and R. A.Ricci (Academic Press) 1969, p. 80.
[3] A. Huck et al., Phys. Rev. C 31, 2226(1985).
[4] J. I. Prisciandaro et al., Phys. Lett. B510,17 (2001).
[5] R. Broda, J. Phys. G 32, R151 (2006).[6] B. Fornal et al., Acta Phys. Pol. B 26, 357
(1995).[7] W. Krolas et al., Nucl. Phys. A724, 289
(2003).[8] R. V. F. Janssens et al., Phys. Lett. B546,
55 (2002).[9] S. N. Liddick et al., Phys. Rev. Lett. 92,
072502 (2004).[10] S. N. Liddick et al., Phys. Rev. C 70,
064303 (2004).[11] G. Chilosi, P. Cuzzocrea, G. B. Vingiani,
R. A. Ricci and H. Morinaga, Nuovo Cim.27, 86 (1963).
[12] M. Honma, T. Otsuka, B. A. Brown, andT. Mizusaki, Eur. Phys. J. A 25 suppl. 1,499 (2005); M. Honma, T. Otsuka, B. A.Brown, and T. Mizusaki, Phys. Rev. C 65,061301(R) (2002).
[13] A. Poves, J. Sanchez-Solano, E. Caurier,F. Nowacki, Nucl. Phys. A694 (2001), 157
173
(2001).[14] A. M. Stefanini et al., Nucl. Phys. A701,
217c (2002).[15] A. Gadea et al., Eur. Phys. J. A 20, 193
(2004).[16] S. Szilner et al., Phys. Rev. C 76, 024604
(2007).
[17] F. Perrot et al., Phys. Rev. C 74, 014313(2006).
[18] B. Fornal et al., Phys. Rev. C 72, 044315(2005).
[19] B. Fornal et al., Phys. Rev. C 77, 014304(2008).
174
REACTION MODELS FOR EXOTIC NUCLEI
Angela Bonaccorso ∗
Istituto Nazionale di Fisica Nucleare, Sez. di Pisa,
Largo Pontecorvo 3, 56127 Pisa, Italy.
I. INTRODUCTION
Nuclear reaction theory has experienceda great revival in the last twenty years fol-lowing the large increase in quantity as wellas quality of experiments with exotic beams.Exotic nuclei are located away from the sta-bility valley and have large differences inthe number of neutrons and protons. Theirvalence particle separation energies Sn aresmaller than the average 8 MeV expectedin nuclear matter. In the extreme case ofhalo nuclei such as several beryllium andlithium isotopes (11Be,12Be,14Be,11Li), Sn
can be even less than 1 MeV. As a conse-quence as much as 10% of the total reactioncross section is due to just one channel: 1nor 2n breakup. Therefore, out of necessity
(N. Orr), breakup has been the most stud-ied reaction for very weak beams and theone for which several new models have beendeveloped.
In this short review I will first present themechanisms which lead to breakup and therelative observables that are measured. Foreach of them a description will follow of themost recent advances in the models used fortheoretical calculations.
∗In collaboration with C.A. Bertulani, G.Blanchon, D.M. Brink, F. Carstoiu, A. Garcıa-Camacho, A.A. Ibraheem, J. Margueron,N.Vinh Mau.
II. CROSS SECTION
Most theoretical methods used so far todescribe breakup rely on a basic approxi-mation to describe the collision with onlythe three-body variables of nucleon coordi-nate, projectile coordinate, and target coor-dinate. Thus the dynamics is controlled bythe three potentials describing nucleon-core,nucleon-target, and core-target interactions.Often the projectile-target relative motion istreated semiclassically by using a trajectoryof the center of the projectile relative to thecenter of the target R (t) = bc + vtz withconstant velocity v in the z direction and im-pact parameter bc in the xy plane. This ap-proximation makes the formalism applica-ble for incident energies above the Coulombbarrier. Along the semiclassical trajectorythe amplitude for a transition from a nu-cleon state ψi bound in the projectile, to afinal continuum state ψf , is given by [1,2]
Afi =1
ih
∫ ∞
−∞
dt〈ψf (r, t)|V (r,R(t))|ψi(r, t)〉,
(1)
where V is the interaction responsible forthe transition which will be specified in thefollowing. The probabilities for differentprocesses can be represented in terms of theamplitude as dP/dξ =
∑
|Afi|2δ(ξ − ξf )
where ξ can be momentum, energy or anyother variable for which a differential crosssection is measured.
Direct one-particle re-arrangment reac-tions of the peripheral type in presence ofstrong core-target absorption can be de-scribed by an equation like [2–5]
Conference Proceedings Vol. 96“The Nuclear Physics from the f7/2 to the Quark - Gluon Plasma”F. Gramegna, M. Cinausero, D. Fabris (Eds.)SIF, Bologna 2008
175
dσ−n
dξf= C2S
∫
dbc
dPbup(bc)
dξfPct(bc), (2)
(see Eq. (2.3) of [3]) and C2S is the spec-troscopic factor for the initial single par-ticle state. The core survival probabilityis defined in terms of a S-matrix functionof the core-target distance of closest ap-proach bc. A simple parameterisation isPct(bc) = |Sct|
2 = e(− ln 2exp[(Rs−bc)/a]). Ittakes into account the peripheral nature ofthe reaction and naturally excludes the pos-sibility of large overlaps between projectileand target. The strong absorption radius
Rs ≈ 1.4(A1/3p + A
1/3t ) fm is defined as the
distance of closest approach for a trajectorythat is 50% absorbed from the elastic chan-nel and a=0.6 fm is a diffuseness parameter.The values of Rs thus obtained agree withina few percent with those of the Kox param-eterization [6].
III. BREAKUP MECHANISMS
Based on the time dependent amplitudeEq.(1) and the classical projectile-targettrajectory of relative motion given above,in Ref. [4] we considered the breakup of ahalo nucleus like 11Be consisting of a neu-tron bound to a 10Be core in a collisionwith a target nucleus. The system of thehalo nucleus and the target was describedby Jacobi coordinates (R, r) where R is theposition of the center of mass of the halonucleus relative to the target nucleus andr is the position of the neutron relative tothe halo core, and the coordinate R is as-sumed to move on a classical path. TheHamiltonian of such a system is H = TR +Tr+Vnc (r)+Vnt (β2r + R)+Vct (R − β
1r) ,
with β1 and β2 the mass ratios of neutronand core, respectively, to that of the projec-tile. TR and Tr are the kinetic energy oper-ators associated with the coordinates R andr and Vcn is a real potential describing theneutron-core final state interaction. Vcn was
neglected under the hypothesis that the ob-servables measured and calculated did notdepend significantly on it. In Sec.V we willdiscuss cases in which such an interactiondominates instead the measured data. Thepotential V2 = Vnt + Vct describes the inter-action between the projectile and the tar-get. It is a sum of two parts depending onthe relative coordinates of the neutron andthe target and of the core and the target.Both Vnt and Vct are represented by com-plex optical potentials. The imaginary partof Vnt describes absorption of the neutronby the target to form a compound nucleus.It gives rise to the stripping part of the halobreakup we will describe in Sec. IV. Theimaginary part of Vct describes reactions ofthe halo core with the target. The poten-tial Vct also includes the Coulomb interac-tion between the halo core and the target.This part of the interaction is responsiblefor Coulomb breakup. In fact the Coulombforce does not act directly on the neutronbut it affects it only indirectly by causingthe recoil of the charged core.
Since the mass ratio β1 is small for ahalo nucleus with a heavy core (β1 ≈0.1 for 11Be) the Coulomb potential wasapproximated by the dipole term in Ref.[4]. Then, making an eikonal approxima-tion for the neutron final state ψf (t) =exp (ik · r − iεkt/h) exp
(
− 1ih
∫ ∞
t V2 (r, t) dt)
,the amplitude became
Alm (k,bc ) =1
ih
∫
d3rdte−ik·r+iωt
×e( 1
ih
∫
∞
tV2 (r,R(t) )dt )
×V2 (r,R(t) )φlm (r) (3)
where ω = (εk − εi) /h and φlm is the ra-dial part of the neutron initial wave func-tion. k is the neutron-core relative momen-tum vector in the final state. The corre-sponding energy is εk, while εi is the initialstate binding energy. Eq. (3) is appropri-ate to calculate the coincidence cross sectionAp → (Ap − 1) + n.
176
The components Vnt and Vct of V2 aretreated differently because of the long rangeof the Coulomb interaction. The neutron-target interaction is strong and has a shortrange. We assumed that the interactiontime τ for this part of the interaction is veryshort in the sense that ωτ is small comparedwith unity. On the other hand the longrange Coulomb interaction between the halocore and the target is weaker and changesmore slowly. The way to treat it is discussedin the next subsection.
A. Coulomb breakup
Introducing the notation Vc = ZcZte2,
Vv = ZvZte2 and VC = (Zv + Zc)Zte
2, withZv = 0, 1 for a neutron and for a protonrespectively, the Coulomb potential can bewritten as
V (r,R) =Vc
|R − β1r|+
Vv
|R + β2r|−
VC
R.
(4)
Here β1 can be also the mass ratio ofthe proton to that of the projectile. InRef. [7] we have shown that the Coulombphase χeff (bc, r, k) =
∫
dteiωtVC(r, t)/h.which is solvable in the dipole approxima-tion, can similarly be calculated with thewhole multipole expansion if a screeningterm is added and subtracted to the poten-tial, suct that it can be written as V (r,R) =
Vsh(r,R) + Vlo(r,R) = VC [( e−γ|R−β1r|
|R−β1r|−
e−γR
R )+(− 1−e−γ|R−β1r|
|R−β1r|+ 1−e−γR
R )]. The term
Vsh contains the singularity at R=0 but de-cays quickly with the impact parameter. Onthe other hand, Vlo, well-behaved at the ori-gin, accounts for the long-range characterof the Coulomb potential. When inserted inthe integral for χeff , these two terms can betreated in different ways if the parameter γis big enough. In this case, as done in [4]
with the nuclear potential, Vsh can be con-sidered in the sudden approximation, yield-ing a phase χsudd(bc, r) =
∫
dtVsh(r, t)/h,whereas Vlo needs to keep the whole timeevolution description, but, being weak,it can be approximated to first orderχpert(bc, r, k) =
∫
dteiωtVlo(r, t)/h. There-fore the Coulomb phase becomes a sum oftwo terms χeff (bc, r, k) = χsudd(bc, r) +χpert(bc, r, k), both of them depending uponthe screening parameter γ. In order forthis approximation to be valid, the screen-ing term γ needs to be sufficiently largeas to ensure that the range of Vsh re-mains short enough, and that Vlo doesnot become too large. This is nextachieved by taking just γ = ∞, in whichcase χsudd = 0, and χeff = χpert =2VC
hv
(
eiβ1ωz/vK0(ωbc/v) − K0(ωR⊥/v))
.
0 5 10 15
ε (MeV)
1
10
100
1000
σ (
mb)
FIG. 1. Integrated breakup cross-section for ahypothetical 34Si beam against Pb at 70 A.MeVas a function of the neutron separation energy.Different initial parameters: circles (squares)are for Coulomb (nuclear) breakup from an ini-tial s-wave; diamonds (triangles) for Coulomb(nuclear) breakup from a d-wave; pluses (stars)for Coulomb (nuclear) breakup from an initialf-wave. Nuclear breakup is the sum of diffrac-tive and stripping contributions.
B. Sudden limit and all-order treatment
Aiming for an all-order formalism, in [4]it was shown that a possible way to achieve
177
this is to use the sudden approximation,subtract the first order term, which divergesfor large impact parameter, and then toadd a first order term calculated in time-dependent perturbation theory. The sud-den limit (ω → 0) must be therefore takenin the above expression for χeff , yielding
χsuddeff = 2VC
hv log bc
R⊥. Following a procedure
analogous to that of [7], the Coulomb phasefor the proton is shown to be [8]
χp =2
hv(Vce
iβ1ωz/vK0(ωbc/v)
− VCK0(ωR⊥/v)
+ Vve−iβ2ωz/vK0(ωbv/v)). (5)
Since VC = Vc + Vv, Eq. (5) can be writ-ten as χp = χ(β1, Vc) + χ(−β2, Vv) whereχ is the χeff of the previous section andbv = bc + r⊥ is the proton impact pa-rameter with respect to the target. TheCoulomb phase is therefore the sum of twoterms: one of them describes the recoil ofthe core whereas the other accounts for thedirect proton-target Coulomb interaction.Of course, in the case of the neutron thelatter vanishes and the phase reduces to theone derived in [7]. It is easy to see that theexpansion of χeff to first order in r yieldsthe well known dipole approximation to thephase: which only differs from the neutronbreakup case in the different constant fac-tor, which is now (Vcβ1 − Vvβ2) instead ofVcβ1 of Ref. [7].
The probability amplitude can be writtenas the sum of three contributions. The recoilterm,
Arec =∫
dre−ik·rφi(r)(
ei 2Vc
hvlog bc
R⊥ − 1
− i2Vc
hvlog
bc
R⊥+ iχ(β1, Vc)) , (6)
where, according to the discussions in [4,7],the sudden limit has been used in order toinclude all orders in the interaction. The di-rect proton Coulomb interaction term Adir
which has the same form as Eq.(6) but withthe substitution Vc →Vv, β1 → −β2 andbc →bv. The nuclear part is given by
Anuc =
∫
dre−ik·r(
eiχnt(bv) − 1)
φi(r),
(7)
which is the eikonal form of the diffrac-tive nuclear breakup with the neutron-target phase χnt(bv) =
∫
dzVnt(bv, z)/(vh).Finally the expression for the differentialcross-section is
dσ−n
dk=
1
8π3
mk
h2
∫
dbc |Anuc + Adir + Arec|2
× |Sct(bc)|2. (8)
-150 -100 -50 0 50 100 150
p|| (MeV/c)
2
4
6dσ
/dp || (
mb/
(MeV
/c))Exptot, nuc-Cou, exc, dipoletot, nuc-Cou, gs, dipoletot, nuc-Cou, excited statetot, nuc-Cou, gs
FIG. 2. Calculated momentum distributionof 7Be fragments after proton-removal from 8Bagainst Pb at 936 MeV/A. Both dipole and fullmultipole results are shown for the ground stateand first excited state. Calculations accordingto Sec. III and Ref.[8] where more details canbe found. Data are from Ref.[17].
In a number of papers higher order ef-fects [9] and proton breakup have been dis-cussed, among which we recall Refs. [10–12].Some works have also addressed the prob-lem of asymmetry in the core parallel mo-mentum distribution after proton knockout[13,14]. The fact that this asymmetry comesfrom high order terms can be directly ex-tracted from our formalism. If the Coulombpart of the amplitude is simply expanded tofirst order in χ, it can be written, in terms
178
of the one-dimensional Fourier transform inz−direction of the initial wave function φi,as
ACou ≃2
hv
∫
dr⊥e−ik⊥·r⊥
× (VcK0(ωbc/v)φi(r⊥, kz − β1ω/v)
− VCK0(ωR⊥/v)φi(r⊥, kz)
+ VvK0(ωbv/v)φi(r⊥, kz + β2ω/v)).
(9)
Thus the Coulomb breakup probabilityamplitude can be regarded as a coherentsum of three terms, each of which contains ashifted z−Fourier transform. The shifts arein opposite directions, β1ω/v and −β2ω/v,but they are not visible directly in the calcu-lated momentum distributions as ω dependson k itself. Moreover, the 1/v factor indi-cates that the asymmetry decreases as thebeam energy increases. In the dipole ap-proximation, however, the amplitude doesnot contain any asymmetry for the mo-mentum distribution as it involves squaremodulii of φi(r⊥, kz) separately. Hence wehave confirmed analytically that the asym-metry in Coulomb breakup parallel momen-tum distributions is due to the presence ofhigher multipole terms, in agreement withearlier works [9,13,14]. However, the pres-ence of the nuclear interaction introduces aninterference that does depend on the signof kz and thus an additional asymmetry tothat due to higher multipole terms in theCoulomb interaction.
We then present two applications of theformalism just discussed. Fig. 1 showscalculations of absolute cross sections forCoulomb and nuclear breakup, according tothe formalism of Secs. II and III, for a heavyexotic projectile 34Si. It intends to demon-strate the feasibility of nuclear breakup ex-periments on heavy targets when the initialneutron separation energy and angular mo-mentum become large. In this way it shouldbe possible to avoid the asymmetries and
deviations from the eikonal model found insome experiments [15,16]. Fig. 2 comparesdata [17] for proton breakup to calculationsfrom our new model [8] shortly describedabove.
IV. TRANSFER TO THE
CONTINUUM
In Ref. [2] the transfer to the contin-uum method (TC) to calculate the nuclearbreakup was introduced in a way that madenumerical calculations relatively easy. Fur-thermore it was shown that breakup givesrise to a stripping cross section σstr and adiffractive breakup cross section σdiff whichare distinguishable experimentally depend-ing on whether the removed neutron is de-tected in the final state or not. The eikonalapproximation to Eq.(1) has been alreadygiven for the diffraction term by Eq.(7). Ex-tending it to the stripping term of the nu-clear breakup [18,19], one derives [20] thetotal one nucleon removal probability
dP−n(bc)
dkz∼
1
2π
∫ ∞
0
dbv|φi(bv − bc, kz)|2
× [|(1 − e−iχ(bv))|2 + 1 − |e−iχ(bv)|2 ], (10)
where e−iχ(bv) is the eikonal form of the neu-tron (proton) target S-matrix already dis-cussed in Sec.III. Notice that in this expres-sion the exact initial state wave function ap-pears, therefore Eq.(10) is valid for a neu-
tron as well as for a proton. |φi(bv−bc, kz)|2
is the longitudinal Fourier transform ofthe initial state wave function. The totalbreakup probability is obtained from the in-tegral of Eq.(10) involving I(kmin
z , kmaxz ) =
∫ kmaxz
kminz
dkz |φi(bv − bc, kz)|2. If the integral
could be extended to ±∞, it would just bethe longitudinal density, and the formulaefor the TC and eikonal model would becomeidentical. In fact in this limit the removalcross section reduces to
179
σ−n = C2S
∫
d2bc
∫
d3r|φi(bv − bc, z)|2
×[
|(1 − S)|2 + 1 − |S|2]
|Sct(bc)|2 (11)
which is consistent with the breakup crosssection originally obtained by Yabana andcollaborators [21]. Notice that Eqs.(10) and(11) are consistent with Eq.(7).
To see how accurate the sudden approx-imation is, the integral I(kmin
z , kmaxz ) was
calculated in Ref. [19] under various condi-tions of angular momentum, neutron bind-ing energy in the projectile, and projectilevelocity. For values of the parameters of in-terest there can be a rather large reductionfor small values of the neutron transverseradius in the projectile, |bv −bc|. However,the approximation becomes increasingly ac-curate as the transverse radius is madelarger. Another sudden model for Coulomband nuclear breakup was presented in Ref.[22] and compared to the present approach.
V. PROJECTILE FRAGMENTATION
We call projectile fragmentation the elas-tic breakup (diffraction dissociation) dis-cussed above, when the observable stud-ied is the neutron-core relative energy spec-trum. This kind of observable has beenwidely measured in relation to the Coulombbreakup on heavy target. Results on lighttargets have also been presented [23]. Thesedata enlighten the effect of the neutron fi-nal state interaction with the core of origin,neglected in the previous sections, while ob-servables like the core energy or momentumdistributions enlighten the effect of the neu-tron final state interaction with the target.
Projectile fragmentation has also beenused experimentally with two neutron haloprojectiles [24]- [41]. In this case it has beensuggested that the reaction might proceedby the simultaneous emission of the two neu-trons or by successive emissions [24]. The
successive emission can be due to a mecha-nism in which one neutron is stripped by theinteraction with the target, as in the one-neutron fragmentation case, while the otheris left behind, for example in a resonancestate, which then decays. This mechanismhas been described by the sudden approx-imation in Ref. [25] under the hypothesisthat while the first neutron is stripped, thesecond neutron is emitted at large impactparameters with no final state interactionwith the target. The emission can be ex-pected sequential if the two neutrons are notstrongly correlated.
If the two neutrons are strongly correlatedthey will preferentially be emitted simulta-neously. If the neutron which is not detectedis stripped while the other suffers an elas-tic scattering on the target, then in bothcases to first order in the interaction theneutron ends-up in a plane wave final state[2]. It can then re-interact with the corewhich, for example, is going to be 10Be inthe case of the one-neutron halo projectile11Be, while it will be 12Be in the case of theprojectile fragmentation of 14Be, since 13Beis not bound or 9Li in the case of the pro-jectile fragmentation of 11Li, since in thiscase 10Li is not bound. Experiments with a14B projectile [26] have also been performed,in which the n-12Be relative energy spec-tra have been reconstructed by coincidencemeasurements. In such a nucleus the valenceneutron is weakly bound, while the valenceproton is strongly bound. Thus the neutronwill probably be emitted in the first step andthen re-scattered by the core minus one pro-ton nucleus. The projectile-target distancesat which this kind of mechanism would berelevant are probably not so large to neglectthe effect of the neutron-target interaction.
A. Inelastic excitation to the continuum.
To first order the inelastic-like excitationscan be described again by the time depen-
180
dent perturbation amplitude Eq.(1) [1,2]. Inthis section also, the potential V (r,R(t)),which is the interaction responsible for theneutron transition, moves past on a constantvelocity path as described in the previoussections. The radial part φi(r) of the singleparticle initial state wave function ψi(r, t)is calculated in a potential VWS(r) which isfixed in space. The coordinate system andother details of the calculations can be foundin Ref. [27]. In the special case of exoticnuclei the traditional approach to inelasticexcitations needs to be modified. For ex-ample the final state can be eigenstate of apotential V1 modified with respect to VWS
because some other particle is emitted dur-ing the reaction process as discussed in theintroduction.
0 1 2 3ε
f (MeV)
0
10
20
30
40
50
dσ/d
εf
(m
b/M
eV)
Sums1/2 to s1/2s1/2 to p3/2s1/2 to p1/2s1/2 to d5/2s1/2 to d3/2CoulombConvolutionExp.
FIG. 3. n-10Be relative energy spectrum, in-cluding Coulomb and nuclear breakup for the re-action 11Be+12C → n+10Be+X at 69 A.MeV.Only the contributions from an s initial statewith spectroscopic factor C2S= 0.84 are calcu-lated. The triangles are the total calculated re-sult after convolution with the experimental res-olution function. The dots are the experimentalpoints from Ref.[23].
The final state interaction might also havean imaginary part which would take intoaccount the coupling between a continuumstate and an excited core. The first or-der time dependent perturbation amplitudethen reads
Afi =1
ihv
∫ ∞
−∞
dxdydz φ∗f (x, y, z)φi(x, y, z)
eiqzV (x − bc, y, q), (12)
where V (x − bc, y, q) =∫ ∞
−∞dzV (x −
bc, y, z)eiqz, and we changed variables andput z′ = z − vt or t = (z − z′)/v, q =εk − εi/hv. In this section εk is the neutron-core relative energy in the final state.
0 1 2 3ε
f (MeV)
0
20
40
60
80
dσ/d
εf
(m
b/M
eV)
FIG. 4. Sum of all transitions from the s ini-tial state with εi=-1.85 MeV (solid line) for thereaction 14Be+12C → n+12Be+X . Experimen-tal points from H. Simon et al. [31] for the samereaction at 250 A.MeV. Dashed line is the fold-ing of the calculated spectrum with the experi-mental resolution curve.
The target represented by V perturbs theinitial bound state wave function and allowsthe transition to the continuum by transfer-ring some momentum to the neutron. Thenit is enough to choose a simplified form ofthe interaction, such as a delta-function po-tential V (r) = v2δ(x)δ(y)δ(z). The value ofthe strength v2 ≡ [MeV fm3] used in the cal-culation is taken equal to the volume inte-gral of the appropriate neutron-target inter-action. It is clear that while in the suddenapproach the initial and final state overlapis taken in the whole coordinate space, irre-spective of the target and of the beam veloc-ity, here the overlap of the initial and finalwave functions depends on the core-targetimpact parameter. The neutron is emittedpreferentially on the reaction plane and the
181
z-component, being along the relative veloc-ity axis is boosted by a momentum q.
0 0.5 1 1.5 2 2.5 3ε
f (MeV)
0
50
100
150
200
dσ/d
εf
(m
b/M
eV)
Exp. data from [2]31% s 45% p 31% s 45% p with exp. conv31% s 45% p without d
5/2
31% s 45% p without d5/2
with exp. conv.
FIG. 5. n-9Li relative energy spectrum, forthe reaction 11Li+12C → n+9Li+X at 264A.MeV. Only the contributions from an s and pinitial state with experimental spectroscopic fac-tors [46] C2S= 0.31 and 0.45 respectively andseparation energy 0.3 MeV are included. Thethin solid curve is the total calculated result.The thick solid curve curve is after convolutionwith the experimental resolution function. Thethin dashed curve is the calculation without thed-resonance while the thick dashed curve is thesame calculation after convolution. The sym-bols with error bars are the experimental pointsfrom Ref.[31]. Calculations are normalised tothe data
Due of the strong core absorption dis-cussed in Secs. 2 and 3 these calculations arealso performed using the asymptotic formof the initial and final state wave functions.Introducing the quantization condition ac-cording to Ref. [2] the probability spectrumreads
dPin
dεk
=2
π
v22C2
i
h2v2
m
h2k
1
2li + 1
× Σmi,mf|1 − Smi,mf
|2|Imi,mf|2. (13)
The generalization including spin is given inAppendix B of Ref. [27] and |Imi,mf
|2 is
|I|2 =∣
∣
∣γk
i
2ili
∫ ∞
−∞
dzeiqzh(1)li
(iγr)h(−)lf
(kr)
×Yli,mi(θ, 0)Ylf ,mf
(θ, 0)∣
∣
∣
2
. (14)
The quantity S = e2i(δ+ν) is an off-the-energy-shell S-matrix representing the finalstate interaction of the neutron with theprojectile core. It depends on a phase whichis the sum of δ, the free particle n-core phaseshift, plus ν the phase of the matrix elementI, Eq.(14). Some examples of our calcula-tions [27] are shown in Figs. 3, 4 and 5and compared to recent data. See also Ref.[28]. Finally we refer to two books [42,43]and recent reviews [44,45] in which furtherdiscussion and bibliography can be found.
VI. CONCLUSIONS AND OUTLOOK
The field of Rare Isotopes Studies is veryactive, growing steadily and rapidly. Somerecent achievements in reaction models forneutron and proton breakup from exoticbeams have been presented. From the struc-ture point of view, in the search for thedripline position, a very important role isplayed by the study of nuclei unstable byneutron emission. On the other hand in-creasing the mass of the projectiles pro-duced we are going to face the problem ofenvisaging new experiments to study them.These two are among the most importantsubjects which need to be adressed andfurther developed in the near future andfor which some suggestions have been pre-sented.
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[16] A. Gade et al., Phys. Rev. C 71 (2005)051301.
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C 61 (2000) 034605.[19] A. Bonaccorso and G.F. Bertsch, Phys.
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C 57 (1998) R22; Phys. Rev. C 58 (1998)2864.
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183
Conference Proceedings Vol. 96
“The Nuclear Physics from the f7/2 to the Quark - Gluon Plasma”
F. Gramegna, M. Cinausero, D. Fabris (Eds.)
SIF, Bologna 2008
NUCLEAR STRUCTURE AT EXTREME CONDITIONS THROUGH γ SPECTROSCOPY
MEASUREMENTS
S. Leoni, A. Bracco, F. Camera
University of Milano and I.N.F.N. sez. Milano
INTRODUCTION
The study of the nucleus at the limits of angular momentum, temperature and neutron/proton number is one of the central topics currently addressed with selective Ȗ-spectroscopy measurements. In these extreme regimes nuclear structure studies are probing nuclear shapes and their evolution, the influence of thermal environments on low-lying modes, collective rotation and giant resonances.
In this contribution we present selected studies of the collective response of the atomic nucleus at extreme conditions, making use of nuclear reactions with stable/radioactive ions. In particular, the nuclear rotation at high spin values and moderate excitation energy is used to study the transition between order and chaos, while the temperature and isospin degrees of freedom are investigated in connection with giant dipole resonances and pygmy states in exotic nuclei.
THE ORDER-TO-CHAOS TRANSITION
IN THE WARM ROTATING NUCLEUS
It has been shown, both experimentally and theoretically, that the atomic nucleus displays properties typical of an ordered system at temperature T = 0 [1], and of a chaotic systems at the compound nucleus level [2]. The transition between order and chaos can be studied through the analysis of the γ-decay of warm rotating nuclei produced at high spins and moderate excitation energy by fusion reactions between heavy ions, with typical beam energies of 5 MeV/A. In fact, after rapid evaporation of light particles, warm rotating nuclei de-excite emitting long sequences of γ transitions, ending up in discrete regular rotational bands when the nuclear temperature of the system is almost zero. Therefore, by detecting the largest number of γ-rays emitted by the excited nucleus, nuclear
structure properties can be investigated as a function of angular momentum and excitation energy. This can be achieved by the use of high-efficiency HpGe-array spectrometers (such as EUROBALL [3] or AGATA [4] in the near future), consisting of more than 100 Ge crystals in 4π geometry around the reaction center, usually combined with other types of detectors.
By constructing γ−γ spectra from the measured Eγ energies of high-fold γ cascades (see figure 1), one can distinguish between the contribution from the COLD region of regular decay at T=0 (“ridges”) and from the WARM region above ≈ 1 MeV internal excitation energy (“valley”). This is where the nuclear rotation becomes damped and the rotational decay is fragmented over a large number of states with an energy spread Γrot ≈ 200 keV, as a consequence of the rapidly increasing level density and of the presence of a residual two-body interaction mixing the nuclear states [5].
Fig. 1: Example of a region of a γ−γ spectrum of a warm rotating nucleus (168Yb), showing the different contributions from the COLD regular decay at zero temperature (ridges) and from the WARM region of rotational damping (valley), where the transition between order and chaos is expected to take place.
168YbRIDGES(COLD-Order)
VALLEY (WARM-Onset of Chaos)168Yb
RIDGES(COLD-Order)
VALLEY (WARM-Onset of Chaos)168Yb
RIDGES(COLD-Order)
VALLEY (WARM-Onset of Chaos)
185
The study of such ridge-valley landscape can
be used to investigate the transition between order and chaos in terms of a gradual vanishing (at T≠0) of the selection rules associated with the quantum numbers at T = 0, such as K (the projection of the angular momentum on the symmetry axis). In this respect, the deformed nucleus
163Er is an ideal case, being characterized
by a number of rotational bands having low-K (K=5/2) and high-K (K=19/2) values [6]. The nucleus
163Er has been populated by the reaction
18O +
150Nd, at Ebeam = 87, 93 MeV, and its
subsequent γ-decay has been detected using the EUROBALL array at the IReS Laboratory (France). The
150Nd target was made of a stack of
two thin foils for a total thickness of 740 μg/cm2
and the corresponding maximum angular momentum reached in the reaction has been calculated to be 40 and 45 h, for the two different bombarding energies. Figure 2 shows examples of 60 keV wide projections, perpendicular to the Eγ1 = Eγ2 diagonal of experimental matrices of 163
Er, gated by transitions among states with low-K (K=5/2) and high-K (K=19/2) quantum numbers [7,8]. The spectra, showing the typical ridge-valley structure resulting from the γ-decay of a deformed rotating nucleus, have been first analyzed by statistical analysis methods [9].
Fig. 2: 60 keV wide projections on the Eγ1-Eγ2 axis of experimental matrices of 163Er, at the average transition energies Eγ = 900 and 960 keV. Panels a) and b) (c) and d)) show spectra obtained from γ−γ matrices gated by low-K (high-K) configurations of 163Er. The smooth curves represent the interpolation of the data by a two-component spectral function [8].
The analysis of the fluctuations of the events collected in the γ−γ spectra allows to estimate the number of bands (named paths, Npath) both in the ridge and valley region, through the relation
being Neve, μ1 and μ2 the number of events
and the first and second moment of the distribution of counts in a given sector [9]. In the previous expression P
(2) is a correction factor
taking into account the finite energy resolution of the detection system. The analysis is typically performed in a two-dimensional energy region where a rotational band contributes in average with one transition, namely ΔEγ×ΔEγ = 4h2
/ℑ(2)×4h2/ℑ(2)
, being ℑ(2) the
effective
dynamic
moment of inertia of the rotational bands. As
shown in the top panel of figure 3, a total number of ~40 discrete excited bands is found to populate the ridge structures of
163Er, half of
which of high-K nature. On the contrary, many more bands, of the order of 10
3-10
5, are found to
populate the valley region, with large differences between low-K and high-K states, being the latter ~10 times fewer, as shown in the bottom panel of figure 3. This suggests that the K-quantum number is at least partially conserved up to moderate excitation energies, of the order of ~1.5 MeV above yrast (corresponding, in the bottom panel of figure 3, to transition energies Eγ ~1.1 MeV), where the rotational motion is damped. At higher excitation energies (namely for Eγ > 1.1 MeV) more similar number of bands are obtained for low-K and high-K gated spectra, pointing to a vanishing of selection rules on K and to the onset of a chaotic regime, in which quantum numbers and selection rules loose their meaning.
The previous results are supported by the analysis of the correlations between spectra gated by different K-states, which can be evaluated in terms of covariance of the spectrum fluctuations [7]. As reported in ref. [7], the covariance analysis of the valley region shows strong similarities/correlation between the high-K and low-K gated distributions at the highest transition energy values, indicating a gradual transition to a chaotic regime around 1.5 MeV of internal energy.
The experimental results shown in figure 3 are well reproduced by the shell model of ref. [10]
d)c)
-1 00 0 10 0
2 0
3 0
4 0
Eγ 1- Eγ2 [keV]
High K
960 keV
15 0
20 0
25 0
Low K
960 keV
a) b)
2 0 0
2 5 0
3 0 0
3 5 0
103
Co
un
ts
L ow K
900 keV
-1 0 0 0 10 0
3 0
4 0
5 0
6 0
Eγ1 - Eγ 2 [keV]
103 C
ou
nts
Hig h K
900 keV
)2(
1
2 1
PN
N evepath ×
−=
μμ
186
which combines a cranked mean-field and a residual two-body interaction, together with a terms taking into account the angular momentum carried by the K-quantum number. According to the model, K-mixing is induced by the interplay of the Coriolis and residual interaction, and it is found to gradually increase until a complete violation of the K-quantum number is reached above 2-2.5 MeV of internal energy, in good agreement with the experimental findings.
Fig. 3: Results of the statistical analysis of the ridge and valley regions of the experimental γ−γ matrices of 163Er. The top panel shows the number of discrete excited bands at T=0, obtained from the fluctuation analysis of the ridge structures of the total spectrum (triangles) and from spectra gated by Low-K and High-K structures (open symbols). The bottom panel gives instead the results of the statistical analysis of the corresponding valley regions, providing information on the regime of strongly interacting bands at ~1.5-2 MeV internal excitation energy [7]. In both panels the lines give the prediction from the cranked-shell model calculation of ref. [10].
The spectral shape of the ridge-valley structure of the γ−γ spectra (see figure 2) can also been used to extract the rotational damping with Γrot [8], which is related to the evolution of the nuclear system towards complexity. Figure 3 shows the values obtained for the rotational damping width, by interpolating the ridge-valley event distribution of the total γ−γ spectrum of 163
Er, by a two component function (smooth curves in figure 2). The damping width is also found to depend on the K value, being ∼ 200 keV for low-K and ∼ 150 keV for high-K states, in agreement with the calculation of the model [10], giving further support to the conservation of K up to moderate excitation energies [11].
Fig. 4: Experimental values of the rotational damping width Γrot, as extracted from the spectral shape analysis of the total γ−γ spectrum of 163Er [11]. Predictions from cranked shell model calculations are shown by the full line [10].
DAMPING MECHANISM OF THE GIANT
DIPOLE RESONANCE IN HOT NUCLEI
The Giant Dipole Resonance (GDR) is a collective excitation of the nucleus in which proton and neutron oscillate with opposite phase. By studying the γ-decay of the GDR it is possible to investigate highly excited nuclei and to explore the basic nuclear structure properties at finite temperature and angular momentum, such as nuclear shapes and thermal effects [12]. In particular, the dependence of the GDR width on temperature and angular momentum provides information on the evolution of the nuclear shapes and on the damping mechanism of this collective state.
There are still open problems concerning the
temperature dependence of the width of the GDR
30 40
100
200
300
Spin [h]
Γ rot [
keV
]
163Er
30 40
100
200
300
Spin [h]
Γ rot [
keV
]
163Er
Eγ [keV]Eγ [keV]
Warmrotation
Low K
High K
10K
Warmrotation
Low K
High K
10
Warmrotation
Low K
High K
10KK
Valley
187
at T > 2.5 MeV. In fact, while, in general, the measured GDR width is well described within the thermal fluctuation model (TFM) [13] for T < 2 MeV, at higher temperature the situation is more complex, also due to the presence of sizable pre-equilibrium emissions which significantly cool down the nuclear system before its thermalization [14]. This implies a correction to the initial compound excitation energy at which the giant dipole resonance is emitted. To properly understand the behaviour of the GDR width with temperature it is therefore important to fix unambiguously the compound excitation energy, namely, experimental data are required which do not contain pre-equilibrium contributions, whose subtraction is model dependent.
An experimental campaign focused to the
measurement of the width of the GDR built on excited nuclei with mass A~130 and with temperature in the range 2-4 MeV has been performed at Legnaro National Laboratory of INFN, making use of the GARFIELD array [15] combined with large volume BaF2 detectors of the HECTOR set up [16] and with two Position Sensitive Parallel Plate Avalanche Counter telescopes (PSPPAC). In this way, high energy γ-rays from the decay of the GDR were measured in coincidence with light charged particles (to identify the possible presence of pre-equilibrium emission and to properly define the compound nucleus temperature) and with evaporation residues (to select the fusion-evaporation channel). Two different reactions were employed, producing the same
132Ce compound
nucleus at excitation energy 100, 150 and 200 MeV: a symmetric one, using a
64Ni beam at
300, 400 and 500 MeV on a 68
Zn target, and an asymmetric one with an
16O beam at 130 and 250
MeV on a 116
Sn target [17]. In this way the pre-equilibrium contribution predicted, in the oxygen case, by Kelly et al. [14] has been measured.
In figure 5 the α particle spectra measured at Θ
= 74° in both the symmetric 64
Ni and asymmetric 16
O reactions are displayed, in the case of beam energy 500 and 250 MeV, respectively. For the two reactions the excitation energy deduced from kinematics is the same, being equal to 200 MeV. While the α particle spectra corresponding to the 64
Ni-induced reaction show a spectral shape in agreement with a statistical emission from a fully thermalized compound system (red curve), in the case of the
16O beam a sizable pre-equilibrium
contribution is observed, as deduced from the
excess yield which is particularly intense at forward angles. As a consequence, the study of the GDR width at different temperature has been restricted to the symmetric
64Ni-induced reaction,
which does not require any correction related to pre-equilibrium effects.
Fig. 5: Measured α-particle spectra at the detection angle Θ = 74° for the 16O-induced reaction (Elab=250 MeV) (right panel) and for the
64Ni-induced reaction
(Elab=500 MeV) (left panel). The solid line corresponds to statistical model calculations assuming emission from a fully thermalized compound system at the kinematical value of the excitation energy common to the two reactions (E*=200 MeV)[17].
Figure 6 shows the high energy γ-ray spectra
measured in coincidence with the recoiling residual nuclei from the symmetric reaction induced by the
64Ni beam at the 3 different
excitation energies. The full lines give the best fitting statistical model calculations performed using the computational code DCASCADE of ref. [18,19] and folded with the response function of the BaF2 array, calculated using the GEANT libraries [20]. The calculations assume a single Lorentzian strength function centered at EGDR = 14 MeV (as in ref. [21]) and a value of the energy-weighted sum rule (EWSR) corresponding to 100% of the Thomas-Reiche-Kuhn formula. The insets of the figure show the GDR spectra linearized according to the procedure described in ref. [17], together with the corresponding best fitting calculated spectrum (full lines) obtained by treating the Lorentzian width and centroid as free parameters.
The nuclear temperature of the compound
nucleus associated with the GDR decay has been calculated with the expression
0 50 100 150
Eα [MeV]
106
105
104
103
102
counts
[arb
. un.]
0 50 100 150
Eα [MeV]0 50 100 150
Eα [MeV]0 50 100 150
Eα [MeV]0 50 100 150
Eα [MeV]
106
105
104
103
102
counts
[arb
. un.]
0 50 100 150
Eα [MeV]0 50 100 150
Eα [MeV]
188
dE
EdT
))((ln(
1
ρ=
as discussed in ref. [22,23], being ρ(E) the
density of levels, which in this case has been described according to the Reisdorf formalism [24]. The value used for the level density parameter a (MeV
-1) linearly increases between
A/9 and A/10 for E* < 100 MeV, between A/10 and A/11 for 100 < E* < 170 MeV, while it is equal to A/12.5 for E* > 170 MeV.
Fig. 6: The measured (filled points) and calculated
statistical model (full drawn lines) high energy γ-ray
spectra for 132Ce at excitation energy of 200, 150
and 100 MeV [17].
Figure 6 shows the measured values of the
GDR width in comparison with results of different theoretical predictions based on the thermal fluctuation model of the nuclear shape [13]. The error bar on the width is the statistical error connected to the fitting procedure. The horizontal bar represents instead the average temperature range associated to 75% (lower value) and 25% (upper value) of the γ-ray yield. The neglected yield in the average corresponds to the decay at the end of the compound nucleus (CN) cascade which is not sensitive to the GDR width because of its spectral shape.
Within the thermal shape fluctuation model the GDR strength function is calculated by averaging the line shape corresponding to the different possible deformations. The averaging over the distribution of shapes is weighted with a Boltzmann factor
where F is the free energy and T the nuclear temperature [13]. At each deformation point the intrinsic width Γ0 of the resonance was chosen equal to the zero temperature value, namely 4.5 MeV, as it was generally done to reproduce the existing majority of data at T < 2.5 MeV. This calculation is shown in figure 6 by the thin continuous line. It is found that the predicted increase does not reproduce the present experimental data. Moreover, the expected increase seems to follow rather well the deformation increase of the compound nucleus induced by temperature. This is also shown in the figure with a dashed line, representing the average deformation of the nucleus obtained by the thermal fluctuation model (scale on the right vertical axis). A possible explanation for the discrepancy between the data and the TFM model at T > 2.5 MeV could be related to the fact that the effect of the lifetime of the compound nucleus plays a role at these temperatures, as originally suggested by Ph.Chomaz et al. [26]. In fact, taking also into account the compound nucleus lifetime much better agreement between data and theory is obtained, as shown in figure 7 by the thick full drawn line. In the present calculation, the CN total lifetimes were calculated with the statistical model, and the obtained lifetime values have been added to the GDR intrinsic width Γ0, before performing the averaging over nuclear shapes [26].
Fig. 7: Comparison between measured (black points) and calculated GDR width [17]. The thick continuous line shows the predictions of the thermal shape fluctuation model with the inclusion of the compound nucleus (CN) lifetime. The thin continuous line indicates the results of shape fluctuations alone. The dashed line shows the average deformation < β > calculated by the thermal fluctuation model [13].
132Ce132Ce
)/),(exp(),( TFP γβγβ −∝
5 10 15 2010
-1
100
101
102
103
104
5 10 15 20 5 10 15 20 25
5 10 15 20
0,04
0,08
5 10 15 20
0,04
0,08
5 10 15 20
0,08
0,16
E*=200MeV
Yie
ld [
arb
.un
.]
Eγ [MeV]
E*=150MeV
Eγ [MeV]
E*=100MeV
Eγ [MeV]
[arb
.un
.]
Eγ [MeV]
[arb
.un
.]
Eγ [MeV] [a
rb
.un
.]
Eγ [MeV]
189
From the results presented in figure 6 one can conclude that, in agreement with the expectation of the theory [12], for T > 2 MeV there is no room for a significant increase of the intrinsic width Γ0 with temperature [27], unless one unrealistically neglects the CN lifetime contribution to the total width.
PYGMY DIPOLE RESONANCE
IN NEUTRON RICH SYSTEMS
Most of our current understanding of nuclear structure results from the study of reactions between stable nuclei, which until now have allowed to produce ~3000 radioactive nuclides, at quite low values of excitation energy and angular momentum . The availability of beams of unstable ions [27] has recently opened up the possibility to explore the properties of the atomic nucleus far away from the stability line, gaining access to a much wider region of exotic, loosely bound nuclear systems, at the limit of the proton and neutron binding energy. The study of nuclei far away from stability is important not only for a full comprehension of the nuclear many-body system, but also for their astrophysical implications, not least the nucleosynthesis of the heavy elements in the stellar environment. In this respect, one of the topic mostly discussed at present is the evolution of the Giant Dipole Resonance strength from stable to exotic, weakly bound, nuclei with extreme neutron to proton ratio, in connection with the existence of the so called Pygmy Resonance (PR) or soft mode [28-30]. This mode of excitation arises from the vibration of the less tightly bound valence neutrons against the residual core and according to different type of calculations, it is expected to appear as a redistribution of the strength towards lower excitation energies, well below the giant resonance region. It is also found that the details of this redistribution depend significantly on the effective forces used in the calculations. Moreover, according to G. Goriely [31], the pygmy resonance strength can have a striking impact on the calculated r-abundance of the elements since it can significantly change the neutron capture process in the r-process nucleosythesis.
In the case of stable nuclei extensive work was made with photon scattering experiments in different regions of mass [32,33] and in general it was seen that the low energy E1 strength increases with increasing N/Z ratio, as expected
from a neutron-skin vibration. For nuclei far from stability the pygmy dipole resonance was investigated with Coulomb break up reactions for the
20-22O and
132-134Sn nuclei [34,35]. Coulomb
excitation followed by gamma decay was instead measured so far only in the case of
20O [36]. In
contrast with the break up technique the measurement of γ-decay following Coulomb excitation allows to search for strength at energies also below the particle separation energy.
Among the unstable neutron-rich nuclei
68Ni
represents a good case to search for pygmy structures being among the experimentally accessible exotic nuclei with the present radioactive beam facilities. Recently, Vretenar et al. [30] have applied the relativistic random phase approximation to predict the evolution of the isovector dipole response in nuclei with a large neutron excess, and their results for the case of the medium-heavy Ni isotopes are shown in figure 8. It is found that the low-energy dipole strength distribution increases with the neutron excess, in agreement with non relativistic Random Phase Approximation calculation by Colò et al. [29].
Fig. 8: The isovector dipole strength distribution for 4 different isotopes of Ni nuclei as predicted by D. Vretnar et al. using the Relativistic Random Phase Approximation approach [30]. The dashed lines separate the region of the giant resonances from the low-energy region around 10 MeV (pygmy region).
The study we report here concern the
measurement of the γ-decay following Coulomb excitation of a
68Ni beam at 600 MeV/A, energy
at which the dipole excitation dominates over the other excitation modes. This is shown in figure 9,
190
where the cross sections for electromagnetic excitation of different collective states as a function of beam energy is given, in the case of a medium mass nucleus on a Au target [37].
Fig. 9: The cross section for electromagnetic excitation for different collective states as a function of beam energy, for medium mass nuclei on a Au target [37].
As one can see in the figure, the dipole cross section increases as the beam energy increases, opposite to the behaviour of the quadrupole cross section. One can than conclude that it is important in a Coulomb excitation process to have the highest possible beam energy in order to ensure to excite mainly dipole states.
The experiment has been performed at the GSI Laboratory (Darmstadt), where
68Ni has been
produced from the fragmentation of 86
Kr at 900 MeV/A from the UNILAC-SIS with an intensity of ∼ 10
10 particle per spill. The spill length was
approximately 6 seconds long with a period of 10 seconds. The primary beam was focused on a Be target 4 g thick and the
68Ni ions were selected
using the Fragment Separator (FRS) facility. The beam cocktail arriving on the
197Au target (3
g/cm2 thick) had an intensity of ∼4 10
4 events
per spill, out of which approximately 30% were 68
Ni isotopes, as can be seen in figure 10. A total of ∼3 10
7 events of
68Ni have been finally
collected after 6 days of beam time [38]. The γ-ray emission from Coulomb excited
68Ni
has been measured using the RISING array [39] located after the FRS spectrometer. The particle identification setup after the target is performed by the CATE calorimeter [40] placed approximately 1.5 m after the target and at 0°.
Fig. 10: The beam cocktail arriving on the secondary target as measured after the FRS. In the x-axis is plotted the Z of the incident isotopes while in the y axis the A/Q ratio is indicated. The strongest spot in the center is relative to
68Ni.
In the present experiment, the calorimeter
consisted of nine position sensitive Si detectors coupled to four 6 cm thick CsI arranged to equally share the intensity of the incident beam. High and low energy γ-rays have been measured using 15 HPGe clusters of the EUROBALL array [3], 7 HPG segmented clusters from the MINIBALL array [41] and 8 BaF2 from the HECTOR array [16] located at different angles.
The upper panel of figure 11 shows the spectrum obtained by the CATE calorimeter requiring incoming
68Ni ions. The achieved
energy resolution (4.4% for Si and 1.2% for CsI detectors) is found to be sufficient to discriminate between different masses and charges. In the bottom panel of figure 11, the Time of Flight spectrum of the BaF2 detectors are shown, with and without the condition of a 68
Ni event detected in CATE. As one can see, such condition eliminates completely almost all background except for the γ flash coming from CATE, arriving ∼12 ns after the prompt peak.
The measured high energy γ-rays spectra in the HpGe cluster detectors and in the BaF2 of the RISING setup are shown in figure 12, top and middle panel. Only the
68Ni events before and
after the target have been selected with the additional condition on the prompt time of flight peak and on the overall RISING γ- multiplicity equal to one. A peak structure is observed in both the Doppler corrected spectra, at ≈10-11 MeV, where theoretical calculations predict the low energy peak associated to the pygmy resonance component, as displayed in the bottom panel of figure 12.
191
Fig. 11: The E-ΔE spectrum acquired with the CATE calorimeter, in coincidence with incoming 68Ni isotopes, is shown in the top part. The bottom panel shows instead the Time of Flight spectrum of BaF2 detectors, before and after the requirement of a 68Ni event in the CATE calorimeter [40].
In the figure, the lines superposed to the
experimental spectra correspond to accurate GEANT [20] simulations of a 10.8 MeV incident γ-ray in the corresponding detector. In the inset of the figure the peak structure observed in the HpGe clusters and BaF2 detectors is shown, after subtracting a background with an exponential-like shape. A similar peak structure at 10-11 MeV, although not well defined as in the case of the HpGe Clusters and BaF2 detectors, is also observed in the γ-ray spectrum from the MINIBALL array which, being placed closer to the target, suffers of a higher background [40].
One can than conclude that, even though the statistic is low and the background is high, a coherent scenario is observed in the different type of detectors of the RISING setup, namely a peak structure between 10-11 MeV, at the place where different theoretical calculations predict an excess of E1 strength associated to a pygmy dipole response. This results represent the first evidence of the pygmy resonance in a measurement using the virtual photon scattering technique, therefore opening possibilities for more systematic studies in the future.
Fig. 12: The high-energy γ-ray spectra measured in the BaF2 detectors and in the EUROBALL cluster detectors are shown in the top and middle panel. The theoretical calculated 68Ni dipole strength is displayed in the lower-right panel [41]. The continuous line superimposed to the experimental spectra are the results of GEANT simulation of the peak line shape of a 10.8 MeV γ-ray.
CONCLUSION
In this contribution we have presented three selected examples of nuclear structure studies at extreme conditions of angular momentum, temperature and N/Z ratio, making use of γ-spectroscopy measurements.
The first is the study of the transition between
order and chaos in the warm rotating nucleus. By comparing γ coincidence spectra gated by low-K
8 10 12 140
10
20
30
40
50
60
5.0 7.5 10.0 12.50
5
10
15
20
25
8 10 12 140
10
20
30
40
50
60
5.0 7.5 10.0 12.50
5
10
15
20
25
8 10 120
2
4
6
Co
un
ts
HPGe-Cluster
Energy [MeV]
Energy [MeV]
Energy [MeV]
Cou
nts
Energy [MeV]
Baf2 Hector
arb
.units
Theory
G. Colò et al.
192
and high-K structures in the nucleus 163
Er, a gradual vanishing of selection rules on the K quantum number is observed with increasing temperature, suggesting a smooth transition between order and chaos at internal excitation energy ∼1.5 MeV. The experimental results are in good agreement with theoretical predictions based on cranked shell model calculations at finite temperature, taking also into account the angular momentum carried by the K quantum number.
The second topic concerns the study of the dependence of the width of the Giant Dipole Resonance with temperature, in the high temperature regime above 2.5 MeV. This is were sizable pre-equilibrium emission may be present, making it more difficult to unambiguously define the excitation energy of the compound nucleus. For this purpose, the GDR decay of the hot
132Ce
nucleus produced in symmetric 64
Ni-induced reactions, free from pre-equilibrium effects, has been studied in the temperature region 2.5-4.1 MeV. The measured Giant Dipole Resonance width shows an almost linear increase with temperature, in good agreement with predictions from the fluctuation model including also the lifetime of the compound nucleus.
As a last topic, the search for the pygmy resonance in the exotic neutron rich nucleus
68Ni,
using the relativistic Coulomb excitation technique, is discussed. The measured γ-ray spectrum shows a peak centered around 10-11 MeV, corresponding to an enhanced strength as compared to the tail of the standard GDR Lorentzian function. Such an excess is also predicted by different type of calculations and it is interpreted as due to the oscillation of the neutron skin against the inert proton-neutron core. This represents the first observation of a pygmy resonance with virtual photon scattering technique, therefore opening the possibility for more systematic studies in the future.
ACKNOWLEDGMENTS
The authors wish to thank the EUROBALL, GARFIELD and RISING collaborations which made possible the technical developments of the various setups and the realization of the experiments here discussed. Fruitful discussions with the nuclear structure theory group of the University of Milano, of the Niels Bohr Institute of Copenhagen and of the Japanese University of Niigata are also acknowledged.
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194
Conference Proceedings Vol. 96
“The Nuclear Physics from the f7/2 to the Quark - Gluon Plasma”
F. Gramegna, M. Cinausero, D. Fabris (Eds.)
SIF, Bologna 2008
THE SPES PROJECT:
AN ISOL FACILITY FOR NEUTRON-RICH BEAMS
G.Prete, on behalf of the SPES Collaboration
INFN Laboratori Nazionali di Legnaro
INTRODUCTION
SPES is an INFN project to develop a
Radioactive Beam facility as an intermediate step
toward EURISOL. The Laboratori Nazionali di
Legnaro (LNL) was chosen as the site for the
facility construction.
The LNL capability to play a role in this
research field is related to the presence of the
superconducting linac ALPI, able to re-accelerate
exotic ions at up to 10÷11 MeV/u, the well
consolidated know-how in linac construction, the
existing detectors and the related know-how.
Moreover, the necessary real estate is available
thanks to the extension of the Laboratory site
(more than a factor two in area with respect to
the actual size). Primary services and new
infrastructures, like a 40 MW power station, are
currently under implementation.
OVERVIEW OF THE SPES PROJECT
The main goal of the proposed facility is to
provide an accelerator system to perform
forefront research in nuclear physics by studying
nuclei far from stability. The SPES project is
concentrating on the production of neutron-rich
radioactive nuclei with mass in the range 80-160.
The emphasis to neutron-rich isotopes is justified
by the fact that this vast territory has been little
explored, at exceptions of some decay and in-
beam spectroscopy following fission. Therefore,
reactions in inverse kinematics will allow a new
class of data to be obtained.
The Rear Ion Beam (RIB) will be produced by
ISOL technique using the proton induced fission
on a Direct Target of UCx. The proton driver is a
Cyclotron with variable energy (15-70 MeV) and
a maximum current of 0.750 mA upgradeable to
1.5 mA and splitted on two exit ports.
The second goal of the facility is achieved by the
use of the second high energy proton beam and
developing an accelerator based Neutron Facility
by the high proton current produced with the
TRASCO injector, that is in an advanced
construction phase and it is able to deliver a
proton beam of 30 mA 5 MeV. The Neutron
Facility has two main applications: the
development of a Boron Neutron Capture
Therapy (BNCT) installation to perform research
in the treatment of cancer and an irradiation-
facility (LENOS) for material research and cross
section measurements. The expected neutron
beam has a fluence of thermal neutrons of 109 n
cm-2
s-1
and a rate of fast neutrons of 1014
n s-1
.
The radioactive beams, in selected forms, are
also valuable tools for biological and medical
research in the field of cancer therapy.
The most critical element of the SPES project
is the Direct Target. Up to day the proposed
target represent an innovation in term of
capability to sustain the primary beam power.
The design is carefully oriented to optimise the
radiative cooling taking advantage of the high
operating temperature of 2000 oC.
An extensive simulation of the target behaviour
has been performed to characterize the thermal
properties and the release process. Experimental
work to bench mark the simulations was carried
out at HRIBF, the Oak Ridge National
Laboratory ISOL facility (USA).
The production target will be designed following
the ISOLDE and EXCYT projects and special
care will be devoted to the safety and
195
radioprotection of the system. According to the
estimated level of activation in the production
target area of 1013
Bq a special infrastructure will
be designed. The use of up-to-date techniques of
nuclear engineering will result in a high security
level of the installation. The radiation
management and the control system will be
integrated and redundancies will be adopted in
the design.
The isotopes will be extracted and ionized at +1
with a source directly connected with the
production target. Several kinds of sources will
be used according to the beam of interest. A laser
source will be implemented in collaboration with
INFN-Pavia with the aim to produce a beam as
pure as possible.
The selection and the transport of the exotic
beam at low energy and low intensity is a
challenging task. Techniques applied for the
EXCYT beam will be of reference for the beam
diagnostic and an online identification station
will be part of the diagnostic system.
To optimize the reacceleration, a Charge Breeder
will be developed to increase the charge state to
+N before to inject the exotic beam in the
Bunching RFQ and PIAVE Superconductive
RFQ which represents the first re-acceleration
stage before the injection in ALPI.
Fig. 1: The SPES layout with the new facility connectd to the existing Tandem-Alpi-Piave complex.
The expected beam on experimental target will
have a rate on the order of 108-10
9 pps for
132Sn,
90Kr,
94Kr and 10
7-10
8 pps for
134Sn,
95Kr with
energies up to 9-11 MeV/u.
The SPES lay-out is shown in Fig. 1. The area
on the left side has to be constructed to house the
cyclotron proton driver, the two RIB targets, the
high intensity proton linac with neutron facility
and the target development laboratory. An
extension building for the second proton beam
from the cyclotron is planned but out of the
scope of the present project.
RARE BEAM PRODUCTION
The evaluation of the in target yield for physics
experiment at SPES has been determined starting
from the production yield (fission fragment
distribution), which was calculated mainly
through a Monte Carlo simulation based on
transportation model MCNPX [1]. This
simulation allows a detailed 3D definition of the
system to be analysed and a full transport
calculation starting from the proton distribution
[2]. The proton fission cross-section, is obtained
from the experimental data and from the
MCNPX calculations using the Bertini model
[3], and benchmarked with others models
(CEM2k, ISALBEL). The target is designed with
the aim to reach a fission rate of about 1013
fission/s, considering this number a challenge.
As far as the final beam current is considered, a
very crucial point is linked to short-life time of
radioactive isotopes which are produced in the
target: the target plus ion source system have to
be built considering with a great care the
properties related to the release and the
efficiency of the system.
The important step for a radioactive beam is the
overall efficiency of the target-source system
plus the efficiency linked to the post-accelerator
configuration: the evaluation of the intensity of
some radioactive beam species, interesting for
the nuclear physics community, has been
performed and validated through the existing
experimental data.
The final radioactive beam current depends on
the efficiencies of several chemical-physical
processes and beam transport elements For ISOL
facilities, the total efficiency is extremely case
dependent and lies between 10-2
to 10-6
. To give
an evaluation of the final beam the exotic species
must be followed all along their path.
196
The exotic species are produced inside the target
as neutral atoms and are extracted in a gas fase
due to the high operating temperature of the
target (2000oC). This process is governed by the
release efficiency: that is the diffusion process in
the uranium carbide grains, the effusion in the
container and the injection in the ion source. As
soon as the atoms are in the ion source they
should be ionized +1 to be extracted and injected
in the transport system; this process is controlled
by the source ionization efficiency. For an
efficient reacceleration it is necessary to increase
the charge state of the ions. This is done by the
Charge Breeder which increases the charge state
from +1 to +N with a breeding efficiency.
Finally, the overall efficiency of the transport
and post-accelerator system (the efficiency of the
separator and finally the transport efficiency
through the post accelerator up to the
experimental set up) must be considered.
All these parameters strongly affect the final
current, but the target efficiency itself is a very
complicated stuff.
The diffusion in the material is a complicated
phenomenon, which is not completely known
especially when the material is at high
temperature: it strictly depends on the material
structure and on the temperature at which the
material is maintained. [4]
A statistical approach is used to describe the
effusion of atoms inside the target powder. After
the diffusion the atoms follow a random walk up
to exit the container following the effusion
process. Experimental data available from
ISOLDE at CERN [5], HRIBF at ORNL [6] and
PNPI at Gatchina (RU) [7] have been used.
Table 1: Target release parameters for some species
The final results of our calculation indicate a
release time of 1 s for Sn isotopes and 10 s for Kr
for the chosen target configuration, mainly due to
the diffusion time, as reported in Table1.
The production rates of exotic beam on the
experimental target were evaluated taking into
account the following efficiencies as well as the
total release fraction of each isotope.
The assumed +1 and +1/+N ionization
efficiencies are 90% (+1) and 12% (+1/+N)
respectively for Kr and Xe, but only 30% (1+)
and 4% (1+/n+) respectively for Zn, Sr, Sn, I and
Cd. These values are obtained by the SPIRAL2
project and are expected for an optimized
extraction in which the source is specifically
designed for each beam. In some case the use of
an ECR source is required.
The Linac ALPI transmission efficiency is
considered 50%.
Using these quantities an evaluation of the beam
current on target, which can be obtained with the
new SPES facility, are then shown in Fig. 2 for
some isotopes.
Fig. 2: Beam on target: Intensities calculates considering emission, ionization and acceleration efficiencies (see text) for different isotopes
In Table 2 we report, for sake of comparison,
some world-wide facilities looking to the fission
rate and to the power deposited in the production
target.
SPES is located to a high production rate of
fission fragments similar to Spiral2. Nevertheless
a comparison with Spiral2, from the point of
view of driver, layout and cost, is doubtful as the
driver of the Spiral2 facility is oriented to the
production of high intensity stable beams and in
this sense the two facilities cannot be compared
at all.
element Diff.
time
(s)
Nr
of
Coll.
Eff.
Time
(s)
Release
Time
(s)
T1/2
(s)
TRF
(%)
132Sn 1 10
5 0.2 1.2 40 98
133Sn 1 10
5 0.2 1.2 1 40
Kr 10 105 0.1 10 1 15
Beam on Target
1.00E+00
1.00E+01
1.00E+02
1.00E+03
1.00E+04
1.00E+05
1.00E+06
1.00E+07
1.00E+08
1.00E+09
1.00E+10
70 80 90 100 110 120 130 140 150
mass
inte
ns
ity
(s
ec
-1)
Series1
132Sn
Ga
KrSr
AgIn
Sn Cs
197
Table 2: Comparison between several ISOL facilities.
PROTON DRIVERS
The driver for the primary proton beam impinging on the UCx fission target is the commercially available cyclotron Cyclone C70 from IBA.
The C70 cyclotron (see Fig. 3) is currently under commissioning in Nantes (ARRONAX project) with the purpose of radioisotopes production for radiochemistry and oncology [8].
As reported in Table 3, the accelerator is equipped with two external ion sources (a multicusp and an ECR) so as to produce 4 types of particles, in particular high intensity, variable energy H
- (30 ÷ 70 MeV, 750 μA).
The 5 MeV, 35 mA proton beam necessary for the operation of the 150 kW beryllium target of the BNCT neutron source and the LENOS neutron facility will be provided by an off resonance ECR source (TRIPS) followed by a RFQ. The TRIPS source was transferred from LNS to LNL at the end of 2005 [9].
Table 3: Cyclotron C70 beam characteristics
Fig. 3: The C70 cyclotron
Installation was completed in late July 2006
and beam extraction was succesfully tested in September 2006 [10].
The RFQ, initially developed for the TRASCO project, has two working regimes, pulsed and cw.
The operating frequency is 352.2 MHz, with the design choice of using a single 1.3 MW klystron already used at LEP. The RF power will be fed by means of eight high power loops.
The RFQ structure consists of six modules 1.18 m long each made of OFHC copper. The vacuum ports are on the first and fourth segments and the couplers on the other four. Particularly challenging are the very tight mechanical tolerances (20 μm) necessary for the purity of the accelerating mode (as required by beam dynamics) that have to be kept in presence of a
Primary
beam
Power
on
target
target Fissions per
sec
ISOLDE p 1GeV
2 microA
0.4
KW
Direct
Convert.
4· 1012
spallation
HRIBF p 40MeV
10 microA
Up-grade:
20 microA
0.4
KW
Direct
4·1011
TRIUMF p 450MeV
(250 MeV
in target)
40 μA
Up-grade:
70 μA
10
KW
17
KW
Direct
spallation
EXCYT
13C
45AMeV
0.5
KW
Direct
Light ions by
direct
reactions
4 108 8Li
(9·106
extracted)
SPIRAL2 d 40 MeV
5 mA
200
KW
Convert. 1013- 1014
SPES-
Direct
Target
p 40 MeV
200 μA
8 KW Direct
1013
Accelerated
beam
Extracted
Energy
(MeV)
Beam
Intensity
(μA)
Exit Ports
H-
D-
4He
2+
HH+
30 ÷ 70
15 ÷ 35
70
35
750
50
70
50
Dual
Dual
Single
Single
198
large power density. To date, the first two modules (RFQ1 (see Fig.
4) and RFQ2) underwent the complete construction cycle and the remaining four modules (RFQ3, RFQ4, RFQ5 and RFQ6) were pre-braze assembled and RF characterized and are ready for brazing at CERN [11].
Fig. 4: RFQ1 after completing construction
REACCELERATION
The linear accelerator ALPI, with a β range between about 0.04 and 0.2 and CW operation, represents an ideal re-accelerator for the radioactive beams. Radioactive ions can be accelerated above the Coulomb Barrier with high efficiency, and with a quasi-continuous time structure well suited for experiments. A time structure suitable for TOF measurements can be implemented by a low energy bunching system.
ALPI underwent a number of significant upgrades, in recent years, which made it a world-class facility in heavy ion stable beam accelerators and which will represent an important added value for its use as a RIB accelerator as well. Alpi has an equivalent acceleration voltage of 40 MV and may accelerates heavy ions in the region of Tin at energies between 6 and 13 AMeV according to their charge state (19+ or 40+ respectively).
To allow the reacceleration with ALPI a new bunching RFQ will be developed and the PIAVE Superconductive RFQ, which represent the actual injector from the ECR heavy ion source, will be moved to accept the low energy exotic beam.
CONCLUSION
The SPES facility is expected tu run the first exotic beam in 2013. Before starting the construction the R&D program will continue for key development subsystems to receive adequate answers; such items like control system final
target design and proton driver analysis, will be completely mature in about one year.
At the same time the detailed design and the procedure needed for the construction authorization will be implemented.
Design and construction of the complete facility will require 4 years, with the installation and commissioning of parts of the machine beginning immediately after the completion of the buildings and related infrastructures. Critical parts as RIB target and high current RFQ are in advanced construction stage and will be ready for laboratory test before the building construction. The implementation of the ALPI re-accelerator is already scheduled starting from the current year.
The evaluated budget is in the order of 43-48 Meuro, compatible with the INFN Road Map for the Nuclear Physics development.
[1] J.S. Hendricks et al., MCNPX vers. 2.5.e, LA-UR-04-0569 (2004) [2] A. Andrighetto, S. Cevolani and C. Petrovich Proceedings of 5
th Italy- Japan Symposium,
Napoli, November 3-7, 2004, p. 409 [3] A. Andrighetto, S. Cevolani, C. Petrovich Europ. Journal of Physics A25 (2005) 41 [4] J. Crank, The Mathematics of Diffusion, Clarendon Press (1956). [5] See web site: www94.web.cern.ch/ISOLDE and private communication [6] K. Carter, presentation at the 1
st Workshop on
Actinide Target Development, April 27-29, 2006, Vancouver Canada [7] M. Barbui et al., LNL Annual Report 2006, p.182 [8] J. Martino et al., and L. Medeiros Romao et al., Proceedings of the 18
th International
Conference on Cyclotrons and their Applications (CYCLOTRONS 2007) September 30, October 3, Giardini Naxos, Italy (www.lns.infn.it/Cyclotrons2007) [9] E. Fagotti et al., LNL Annual Report 2005, p. 150 [10] E. Fagotti et al., LNL Annual Report 2006, p. 189 [11] A. Palmieri et al., LNL Annual Report 2006, p. 193
199
Conference Proceedings Vol. 96
“The Nuclear Physics from the f7/2 to the Quark - Gluon Plasma”
F. Gramegna, M. Cinausero, D. Fabris (Eds.)
SIF, Bologna 2008
NUCLEAR COLLISIONS AND THE LOW DENSITY NUCLEAR
EQUATION OF STATE
J. B. Natowitz1
and
L. Qin1, K. Hagel
1, R. Wada
1, Z. Chen
1, P. Sahu
1, S. Kowalski
2,
S. Shlomo1, M. Barbui
3, D. Fabris
3, M. Lunardon
3, S. Moretto
3, G. Nebbia
3, S. Pesente
3, V. Rizzi
3,
G. Viesti3, M. Cinausero
4, G. Prete
4, T. Keutgen
5, Y. El Masri
5 and Z. Majka
6
1 Cyclotron Institute, Texas A&M University, 2 Silesia University, 3 Dipartimento di Fisica and
INFN Padova, 4 INFN Laboratori Nazionali di Legnaro, 5 Universit´e Catholique de Louvain , 6
Jagellonian University
INTRODUCTION
The opportunity to present a lecture on nuclear
reaction dynamics at the Workshop in Honor of
the 80th Birthday of Professor Renato Angelo
Ricci is itself an honor and a pleasure. Thanks to
a nearly 20 year collaboration with scientists
from Legnaro National Laboratory and the
University of Padova I have had a first hand
opportunity to observe the major impact that this
Laboratory has had on nuclear science and, in
particular, the legacy of Professor Ricci in
setting the course for this very successfiul
program. I congratulate Professor Ricci on his
Birthday and on his scientific acheivements,
many of which are covered in greater detail in
other contributions to this symposium. In
reviewing the progress in nuclear reaction
dynamics over the course of the time that the
Legnaro Lab has been active, I can not help but
recall that our early picture of heavy ion (HI)
collisions, as summarized in Fig. 1 which was
shown at many reactions meetings in the 1960’s,
was indeed a quite limited one.
Much of this simplified view could, of course,
be attributed to the relative youth of the HI field
and to the relatively low energies of the available
heavy ion accelerators at that time. Even so, a
concentrated program of experimental and
theoretical efforts soon resulted in significant
extensions of the simple models and a much
greater understanding of the richness of the HI
collisions and their ability to produce and explore
nuclei at the extremes of angular momentum and
excitation energy and to uncover a rich array of
new structural features. It is not possible in this
limited format to address the many different
works in these areas, so, by way of example,
Fig. 2 presents some results from just one area of
early reaction studies, that of HI fusion reactions
This is an area where the Padova and Legnaro
scientists have made many important
contributions.
Fig. 1: Simple HI Reaction Classification - 1960’s
With the advent of more powerful
accelerators and detector arrays, a much better
appreciation of the reaction landscape was soon
201
developed from a large body of HI reaction
experiments and theoretical models. A more
recent summary of reaction mechanism types is
contained in Fig. 3. Notably, as the beam
energies pass through the Fermi Energy domain,
near 38 MeV/u, a significant change occurs in the
dominant reaction mechanisms, from the
relatively gentle low energy collisions to more
violent collisions which can produce large
thermal and compressional shocks and large
fluctuations in the interacting nucleonic matter.
Fig. 2: Fusion limits and Nuclei at Extremes of Angular Momentum
Fig. 3: A more modern classification of heavy ion
induced nuclear reactions presented as a function of
both impact parameter b and laboratory beam
energy per nucleon of the projectile.
In recent years our own group has actively
pursued several avenues of investigation of
heavy ion reactions focused on understanding the
dynamical evolution [1-3], the degree of
equilibration [1-4], the possibility of critical
disassembly in near Fermi energy collisions [5-
7], the derivation of information on the equation
of state from nuclear caloric curve measurements
[8-10] and determination of symmetry energies
of low density nuclear gases [11].
Understanding the nuclear matter equation of
state over a wide range of temperature and
density is important in both the nuclear and
astrophysical context. In the latter, knowledge of
specific heats and the density dependence of the
symmetry energy are crucial to understanding
Fusion Limits and Nuclei at Extremes of Angular Momentum
R. Grover et al, 1965
202
collapse of supernovae and the properties of
neutron stars resulting from supernova collapse
[12.13]. The initial compression and the thermal
shock in Fermi-Energy heavy ion collisions lead
naturally to the production of nucleonic matter at
varying temperatures and densities which are
interesting in this context. To illustrate the large
fluctuations in density which may be produced,
we present, in Fig. 4, results of AMD
calculations [14] for the system 64
Zn + 124
Sn.
Fig. 4: Density profiles from Antisymmetrized
Molecular Dynamics calculations for collisions of
47A MeV 64Zn with 124 Sn targets. Results are shown
for times ranging from collision to 300 fm/c for
impact parameters ranging from 0.3 to 3.3 Fermis
Conceptually our studies may be understood
by reference to Fig. 5, where the schematic
trajectory of a near-Fermi energy collision
between normal density nuclei is depicted in
temperature-density space. For comparison, the
theoretical phase diagram for infinite nuclear
matter is also depicted on this diagram. It is that
equation of state which one hopes to probe in
collisions which lead to different trajectories in
the Rho-T plane.
Fig. 5: Nuclear collisions of normal density nuclei
create short lived, initially compressed and excited
systems, which expand and cool. During this process,
the properties of the expanding system may be
manifested in the matter flow, in caloric curves and
in the energy spectra, yield patterns and nature of
produced species which emerge from the collision
zone.
Most of our studies are made using the
TAMU NIMROD detector, a 4π charged particle
telescope array inside a 4π neutron calorimeter
[15] in collaboration with colleagues from
Legnaro National Laboratory, the University of
Padova and the Jagiellonian University in
Krakow. (See Fig. 6). Recently, the detection
characteristics of NIMROD have been
considerably enhanced with additional Si wafer
detectors and improved ionization detectors.
The features of NIMROD place us in an
excellent position to take advantage of the
TAMU Accelerator upgrade [16], presently
underway.
In addition to a picture of the NIMROD
Detector, Fig. 6 includes a typical two-
dimensional array depicting the observed
relationship between charged particle
multiplicity and neutron multiplicity in
NIMROD for the reaction 47AMeV 64
Zn + 197
Au. The plot evidences a distinct correlation in
which increasing charged particle multiplicity is
associated with increasing neutron multiplicity.
Exploring The Nuclear Matter Phase
Diagram With Collisional Heating
• .
•
203
Fig. 6: Left- The NIMROD Detector. Right-Plot of
charged particle multiplicity vs neutron multiplicity
for the reaction 47A MeV 64Zn + 197Au.
Although there are significant fluctuations
reflecting both the competition between decay
modes and the detection efficiencies, these
correlations and transverse energy measurements
provide a means for selecting the most violent
collisions.
2. EQUATION OF STATE STUDIES
Since the light particle emission which occurs
during the collisions carries essential information
on the early dynamics and on the degree of
equilibration at each stage of the reaction, we
have emphasized investigations of nucleon and
light cluster emission to obtain a more detailed
experimental picture of the pre-equilibrium,
thermalization and disassembly phases of such
reactions. The kinematic features and yields of
emitted light particles and clusters can been
exploited to probe the nature of the intermediate
system and information on the EOS can be
extracted. Much of our work utilizes coalescence
model based techniques to follow the time
evolution of the reaction [17-18] and references
therein]. Using NIMROD we have made
comprehensive studies of the reaction dynamics
for a number of heavy ion induced reactions in
the Fermi energy domain.
MCP
MN
One theme of our recent work has been the
extensive comparisons of our experimental
results with predictions of an anti-symmetrized
molecular dynamics model code (AMD) [14].
Direct observables, such as multiplicity
distributions, charge distributions, energy spectra
and velocity distributions, are reproduced
reasonably well by the AMD calculations [1] and
such comparisons have proved to be particularly
useful in elucidating the underlying reaction
dynamics and in differentiating between
dynamically driven and thermodynamically
driven processes. With these techniques, we have
explored the dynamic and thermal evolution and
degree of equilibration achieved and extracted
heat capacities of nuclei at temperatures
comparable to those encountered in supernovae,
key sites of nucleo-synthesis of elements heavier
than Fe [1-10]. We have also determined nuclear
symmetry energies at low densities comparable to
those of the neutrino-sphere in supernova
explosions [11,19,20]. In the following we
discuss these last results and proposed extensions
of this work in more detail.
204
LIGHT PARTICLE CLUSTERIZATION IN
NUCLEAR MATTER AT VERY LOW
DENSITY
Reliable understanding of the nuclear EOS over a
range of densities remains a very important
requirement in nuclear astrophysics. Several
extensive calculations and existing tabulations,
based on varying nucleon-nucleon interactions
serve as standards for a wide variety of
astrophysical simulations [21,22]. At low
densities and high temperatures strong alpha
clustering of the matter is predicted. Such
clusterization can be expected in low density
nuclear matter, whether it be gas or the surface of
an expanded high temperature nucleus.
In a recent theoretical paper, Horowitz and
Schwenk have reported the development of a
Virial Equation of State (VEOS) for low density
nuclear matter [19]. This equation of state,
derived from experimental observables should be
“model-independent, and therefore to set a
benchmark for all nuclear equations of state at
low densities.” Its importance in both nuclear
physics and in the physics of the neutrino sphere
in supernovae is emphasized in the VEOS paper
[19].
Fig. 7: Virial equation of state results ( solid lines) at
T = 2, 4 and 8 MeV are compared to those of two
other theoretical models. The present Virial model
does not include heavier nuclei is not expected to be
adequate above the point where the Shen Calculation
peaks.
An important feature of the VEOS is the natural
inclusion of clustering which leads to large
symmetry energies at low baryon density. These
results are compared to those of other
calculations in Fig. 7.
We recently adapted our investigations of the
nucleon and light cluster emission that occurs in
near Fermi energy heavy ion collisions [1-10] to
probe the properties of the low density
participant matter produced in such collisions
[11]. The reactions of 35 MeV/nucleon 64
Zn
projectiles with 92
Mo and 197
Au target nuclei
were studied. The analysis employed the
isoscaling technique which assumes that for two
systems with similar temperatures but different
N/Z ratios, the ratio of yields of a particular
isotope in the two systems may be expressed as
Y2(Z,N)/Y1(Z,N) = Ce – (ĮN + βZ) /T
where C is a constant. For systems of
temperature T, a comparison of such ratios for a
number of isotopes allows extraction of the
parameters Į and β which can be related to the
symmetry energy [23-26]. The data provide
experimental evidence for a large degree of
alpha clustering resulting from nucleon
coalescence in this low density matter, in
agreement with theoretical predictions [11, 19,
21, 22, 27-29]. For nuclear gases with average
proton fraction, Yp ~0.44, and densities at and
below 0.05 times normal nuclear density and
varying temperatures experimental symmetry
energy coefficients of 9 – 14 MeV have been
derived using the isoscaling method.
The resultant symmetry energy
coefficients are plotted against density in Fig. 8
where they are compared to those which are
predicted by the Gogny effective interaction and
to the 31.6 x (Δ/Δ0)1.05
dependence suggested by
a recent analysis of isospin diffusion data [30].
These symmetry energies reported in Fig. 8 are
far above those obtained in common effective
interaction calculations and reflect cluster
formation, primarily of alpha particles, not
included in such calculations. They are in good
205
agreement with those calculated in the VEOS
treatment of reference 19. A detailed description
of this work may be found in reference 11.
Stimulated by these data, Schwenk and his
collaborators have since improved the VEOS
model with the addition of 3H and
3He cluster
coefficients [20].
Fig.8: Derived symmetry energy coefficients as a
function of baryon density. Solid diamonds indicate
results using densities of column 4 in Table 1 of ref
[30]. Solid line indicates the variation predicted by
the Gogny interaction. The dotted line represents the
function 31.6 x (Δ/Δ0)1.05 .
To the best of our knowledge our analysis is the
only one which employs experimentally
determined numbers for all quantities occurring
in the isoscaling relationship and does so as a
function of ejected particle velocity. This
analysis at low density is made possible because
at such low density the chemical equilibrium
model of Albergo et al. should be applicable
[31]. Extracting information at higher densities is
clearly desirable but requires a more
sophisticated analysis. This is made clear from a
number of theoretical results [ 27-29] .
For example, in Fig. 9 and Fig. 10 we present
results of Beyer et al. and of Roepke et al. who
have calculated the in-medium binding energies
of clusters as a function of temperature and
density. As seen in Fig. 9 for a temperature of 10
MeV, the free binding energies of the clusters (at
0 on the density axis) decrease with increasing
density and reach 0 at a point known as the Mott
density. This point is temperature dependent as
seen in Fig. 8 where Mott lines for, d, t nd alpha
particles are represented. This disappearance of
the cluster binding energy in medium is closely
related to the peaks in the calculated alpha mass
fractions seen in Fig. 7.
Fig. 9: In medium binding energies of light
clusters
Using this model, G. Roepke has made
calculations of the low density symmetry energy
for comparison to our experimental results [29].
The agreement between the two is fair, however
we are continuing to discuss these results and G.
Roepke is presently making more complete
calculations which may allow us to push the
experimental analyses to higher densities where
the simple extreme low density chemical
equilibrium model is not appropriate.
0
10
20
30
40
0,001 0,01 0,1 1Rho
Es
ym
M
eV
Esym ShenDens Corr
Gogny
^1.05
206
Fig. 10: Symmetry energies at low density. Points-
Theoretical results of G. Roepke are compared to
experimental results of Kowalski et al. Line-
homogeneous matter calculation by Roepke et al.
In order to pursue this effort of taking the
in medium modifications into account and
broaden the density range over which the
symmetry energies are experimentally
determined we have carried out a series of
experiments in which the reactions of 112
Sn and 124
Sn with a wide range of projectiles, ranging
from p to 64
Zn, all at the same energy per
nucleon, 47Mev/u, could be studied. The
systems chosen for this study, the PhD thesis of
LiJun Qin, were :
1
H + 112
Sn,124
Sn
2
H + 112
Sn,124
Sn 4
He + 112
Sn,124
Sn
1 0
B + 112
Sn,124
Sn
20
Ne + 112
Sn,124
Sn 40
Ar + 112
Sn,124
Sn
64
Zn + 112
Sn,124
Sn
In this series of experiments different collision
systems should lead to different average
densities, The analysis is nearing completion. By
careful comparisons of the yields, spectra and
angular distributions observed for particle
emission from these different systems we are
attempting to cleanly separate early emission
resulting from nucleon-nucleon collisions from
that resulting from evaporation from the
thermalized system and obtain a much cleaner
picture of the dynamic evolution of the hotter
systems. Information on the symmetry potential
included in mean field can then be extracted
from comparison of the data with results of the
dynamic transport model calculations (and
statistical afterburners) using QMD and AMD
models [14, 32] or, guided by such QMD and
AMD calculations, using empirical techniques
such as isoscaling for systems with different
N/Z ratios (see above). Below we present some
preliminary results from this work.
REACTION TOMOGRAPHY
Fig. 11 contains invariant velocity plots of the
yields of p and 4He emitted in the reaction
64Zn+
124Sn as a function of their parallel and
transverse velocities in the laboratory frame.
Fig. 11: Invariant velocity plots for protons (top) and
alpha particles (bottom) emitted in the most violent
collisions of 47A MeV 64Zn + 124Sn.
207
To construct these plots, the data from the
discrete detector rings were smoothed by
assignment of the position for a particle detected
in a given discrete detector according to the
angular distribution function generated with the
source fitting parameters. The plots reveal some
strong similarities for the two different systems,
related to the similar dynamic particle emission
in the two systems.
Within the framework of such velocity
representations it is possible to explore various
quantities, derivable from the particle yields.
||V
||V
Vpar cm/ns
Vp
erp
cm/n
s
Significant Temperature Evolution
with Particle Velocity
Relatively Small Changes
with Projectile Size
10B + 124Sn
20Ne + 124Sn
40Ar + 124Sn
64Zn + 124Sn
Fig. 12: Chemical equilibrium temperatures.
Thus, in Fig. 12 the THHe double isotope ratio
temperatures for reactions of four different 47
MeV/u heavy ion projectiles with 124
Sn are
compared.
For the 64
Zn projectile, Fig. 13 presents a very
preliminary representation of the symmetry free
energies, derived from isoscaling analyses for
the 112
Sn and 124
Sn targets.
Fig. 13: Symmetry free energy in velocity space. See
text.
ACKNOLEDGEMENTS
This work was supported by the United States
Department of Energy under Grant # DE-FG03-
93ER40773 and by The Robert A. Welch
Foundation under Grant # A0330.
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[2] J. Wang et al., Phys.Rev. C 75 (2007)
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[15] TAMU Cyclotron Institute Report,
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[16] http://cyclotron.tamu.edu/
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Ion Collisions at Interm.Energies",
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034607-1
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to appear in Phys. Rev. C (2007).
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209
SUPERHEAVY AND GIANT NUCLEAR SYSTEMS
Walter Greiner1, Valery Zagrebaev2
1Frankfurt Institute for Advanced Studies,
J.W. Goethe-Universitat 60438 Frankfurt am Main, Germany,2Flerov Laboratory of Nuclear Reaction, JINR,
Dubna, 141980, Moscow region, Russia
DEDICATION
I dedicate this talk to my friend Profes-sor Renato Ricci on occasion of his 80thbirthday. I know him for nearly 40 years.Our first encounter was here at Varenna atthe International School on Nuclear Physics,which Renato organized and which wasguided by Victor Weisskopf. I had just com-pleted my PhD and was a student at thattime. For very many years we met at theisland Hvar in Croatia. Nicola Cindro wasthe third important member of the triplet(Cindro, Ricci and myself). Very impor-tant and joyfull were our meetings with D.Allan Bromley at Yale. We spend pleas-ant evenings and dinners together with Mrs.Ricci, Mrs. Bromley and also with my wifeBarbara. With the subject of my talk Iwould like to remind Renato that extremelyimportant physics on time-delay can also bedone (for lighter systems) at Legnaro. I urgeRenato to stimulate and pave the way forthis work there. Dear Renato, stay healthyand be happy for another 20 years. Godbless you!
INTRODUCTION
Superheavy (SH) nuclei obtained in“cold” fusion reactions with Pb or Bi target[1] are along the proton drip line and veryneutron-deficient with a short half-life. Infusion of actinides with 48Ca more neutron-
rich SH nuclei are produced [2] with muchlonger half-life. But they are still far fromthe center of the predicted “island of sta-bility” formed by the neutron shell aroundN=184 (see the nuclear map in Fig. 1).Unfortunately a small gap between the su-perheavy nuclei produced in 48Ca-inducedfusion reactions and those which were ob-tained in the ‘cold” fusion reactions is stillremain which should be filled to get a uni-fied nuclear map.
In the “cold” fusion, the cross sections ofSH nuclei formation decrease very fast withincreasing charge of the projectile and be-come less than 1 pb for Z>112 (see Fig. 1).Heaviest transactinide, Cf, which can beused as a target in the second method, leadsto the SH nucleus with Z=118 being fusedwith 48Ca. Using the next nearest elementsinstead of 48Ca (e.g., 50Ti, 54Cr, etc.) in fu-sion reactions with actinides is expected lessencouraging, though experiments of suchkind are planned to be performed. In thisconnection other ways to the production ofSH elements in the region of the “island ofstability” should be searched for.
In principle, superheavy nuclei may beproduced in explosion of supernova [4]. Ifthe half-life of these nuclei is comparablewith the age of the Earth they could besearched for in nature. However, it is theheightened stability of these nuclei (rare de-cay) which may hinder from their discovery.To identify these more or less stable super-heavy elements supersensitive mass separa-tors should be used. Chemical methods of
Conference Proceedings Vol. 96“The Nuclear Physics from the f7/2 to the Quark - Gluon Plasma”F. Gramegna, M. Cinausero, D. Fabris (Eds.)SIF, Bologna 2008
211
FIG. 1: Superheavy nuclei produced in “cold” and “hot” fusion reactions. Predicted island ofstability are shown around Z=114, 120 and N=184 (right panel). Experimental and predictedevaporation residue cross sections for production of superheavy elements produced in “cold” (1n)and “hot” (3n) fusion reactions [3] (left panel).
E
mc-
2
+mc 2
Dirac see
po
sitro
nyie
ld1s2p
200
10
20
30
40
400 600 800 1000 1200
t
delay
e+E(e+ ), KeVe-
Z1
U + Cm
Z Z1+ 2Z2
FIG. 2: Schematic figure of spontaneous decay of the vacuum and spectrum of the positrons formedin supercritical electric field (Z1 + Z2 > 173).
separation also could be useful here.
About twenty years ago transfer reactionsof heavy ions with 248Cm target have beenevaluated for their usefulness in producingunknown neutron-rich actinide nuclides [5–7]. The cross sections were found to decreasevery rapidly with increasing atomic numberof surviving target-like fragments. However,Fm and Md neutron-rich isotopes have beenproduced at the level of 0.1 µb. Theoret-ical estimations for production of primarysuperheavy fragments in the damped U+Ucollision have been also performed at thistime within the semiphenomenological dif-fusion model [8]. In spite of obtained high
probabilities for the yields of superheavyprimary fragments (more than 10−2 mb forZ=120), the cross sections for productionof heavy nuclei with low excitation energieswere estimated to be rather small: σCN (Z =114, E∗ = 30 MeV) ∼ 10−6 mb for U+Cmcollision at 7.5 Mev/nucleon beam energy.The authors concluded, however, that “fluc-tuations and shell effects not taken into ac-count may conciderably increase the forma-tion probabilities”. Such is indeed the case(see below).
Recently a new model has been proposed[9] for simultaneous description of all thesestrongly coupled processes: deep inelastic
212
(DI) scattering, quasi-fission (QF), fusion,and regular fission. In this paper we ap-ply this model for analysis of low-energydynamics of heavy nuclear systems formedin nucleus-nucleus collisions at the energiesaround the Coulomb barrier. Among oth-ers there is the purpose to find an influ-ence of the shell structure of the driving po-tential (in particular, deep valley caused bythe double shell closure Z=82 and N=126)on formation of compound nucleus (CN) inmass asymmetric collisions and on nucleonrearrangement between primary fragmentsin more symmetric collisions of actinide nu-clei. In the first case, discharge of the sys-tem into the lead valley (normal or sym-metrizing quasi-fission) is the main reactionchannel, which decreases significantly theprobability of CN formation. In collisions ofheavy transactinide nuclei (U+Cm, etc.), weexpect that the existence of this valley maynoticeably increase the yield of survivingneutron-rich superheavy nuclei complemen-tary to the projectile-like fragments (PLF)around lead (“inverse” or anti-symmetrizingquasi-fission reaction mechanism).
Direct time analysis of the collision pro-cess allows us to estimate also the life-time of the composite system consisting oftwo touching heavy nuclei with total chargeZ>180. Such “long-living” configurations(if they exist) may lead to spontaneouspositron emission from super-strong electricfields of giant quasi-atoms by a static QEDprocess (transition from neutral to chargedQED vacuum) [10, 11], see schematic Fig. 2.
NUCLEAR SHELLS
Quantum effects leading to the shellstructure of heavy nuclei play a crucial roleboth in stability of these nuclei and in pro-duction of them in fusion reactions. The fis-
sion barriers of superheavy nuclei (protect-ing them from spontaneous fission and, thus,providing their existence) are determinedcompletely by the shell structure. Studiesof the shell structure of superheavy nucleiin the framework of the meson field the-ory and the Skyrme-Hartree-Fock approachshow that the magic shells in the superheavyregion are very isotopic dependent [12] (seeFig. 3). According to these investigationsZ=120 being a magic proton number seemsto be as probable as Z=114. Estimatedfission barriers for nuclei with Z=120 arerather high though depend strongly on achosen set of the forces [13].
Interaction dynamics of two heavy nu-clei at low (near-barrier) energies is definedmainly by the adiabatic potential energy,which can be calculated, for example, withinthe two-center shell model [14]. An exam-ple of such calculation is shown in Fig. 4 forthe nuclear system consisting of 108 protonsand 156 neutrons. Formation of such heavynuclear systems in fusion reactions as well asfission and quasi-fission of these systems areregulated by the deep valleys on the poten-tial energy surface (see Fig. 4) also causedby the shell effects.
ADIABATIC DYNAMICS OF HEAVY
NUCLEAR SYSTEM
At incident energies around the Coulombbarrier in the entrance channel the fusionprobability is about 10−3 for mass asym-metric reactions induced by 48Ca and muchless for more symmetric combinations usedin the “cold synthesis”. DI scattering andQF are the main reaction channels here,whereas the fusion probability [formationCN] is extremely small. To estimate such asmall quantity for CN formation probability,first of all, one needs to be able to describe
213
FIG. 3: Proton (left column) and neutron (right column) gaps in the N − Z plane calculatedwithin the self-consistent Hartree-Fock approach with the forces as indicated [12]. The forces withparameter set SkI4 predict both Z=114 and Z=120 as a magic numbers while the other sets predictonly Z=120.
well the main reaction channels, namely DIand QF. Moreover, the quasi-fission pro-cesses are very often indistinguishable fromthe deep-inelastic scattering and from regu-lar fission, which is the main decay channelof excited heavy compound nucleus.
To describe properly and simultaneouslythe strongly coupled DI, QF and fusion-fission processes of low-energy heavy-ion col-lisions we have to choose, first, the unifiedset of degrees of freedom playing the prin-cipal role both at approaching stage andat the stage of separation of reaction frag-ments. Second, we have to determine theunified potential energy surface (dependingon all the degrees of freedom) which reg-
ulates all the processes. Finally, the cor-responding equations of motion should beformulated to perform numerical analysis ofthe studied reactions. In contrast with othermodels, we take into consideration all thedegrees of freedom necessary for descriptionof all the reaction stages. Thus, we need notto split artificially the whole reaction intoseveral stages. Moreover, in that case unam-biguously defined initial conditions are eas-ily formulated at large distance, where onlythe Coulomb interaction and zero-vibrationsof the nuclei determine the motion. The dis-tance between the nuclear centers R (cor-responding to the elongation of a mono-nucleus), dynamic spheroidal-type surface
214
FIG. 4: Adiabatic energy levels and potential energy surface for the nuclear system 264108.
FIG. 5: Driving potential for the nuclear system formed in 136Xe+209Bi collision at fixed defor-mations (left) and at contact configuration (right). The solid lines with arrows show schematically(without fluctuations) most probable trajectories.
deformations β1 and β2, mutual in-plane ori-entations of deformed nuclei ϕ1 and ϕ2, andmass asymmetry η = A1−A2
A1+A2
are probablythe relevant degrees of freedom in fusion-fission dynamics.
The two-center shell model [14] seems tobe most appropriate for calculation of theadiabatic potential energy surface. A choiceof dynamic equations for the considered de-grees of freedom is not so evident. Themain problem here is a proper description
of nucleon transfer and change of the massasymmetry which is a discrete variable by itsnature. The corresponding inertia parame-ter µη, being calculated within the Werner-Wheeler approach, becomes infinite at con-tact (scission) point and for separated nu-clei. In Ref. [9] the inertialess Langevintype equation for the mass asymmetry hasbeen derived from the corresponding mas-ter equation for the distribution function.Finally we use a set of 13 coupled Langevin
215
FIG. 6: Angular (a), energy-loss (b) and charge (c) distributions of the Xe-like fragments obtainedin the 136Xe+209Bi reaction at Ec.m.
= 568 MeV. Experimental data are taken from Ref. [16]. Forother notations see the text.
type equations for 7 degrees of freedom (rel-ative distance, rotation and dynamic defor-mations of the nuclei and mass asymmetry)which are solved numerically.
The cross sections for all the processesare calculated in a simple and natural way.A large number of events (trajectories) aretested for a given impact parameter. Thoseevents, in which the nuclear system over-came the fission barrier from the outsideand entered the region of small deforma-tions and elongations, are treated as fusion(CN formation). The other events corre-spond to quasi-elastic, DI and QF processes.Subsequent decay of the excited CN (C →
B + xn + Nγ) is described then within thestatistical model using an explicit expres-sion for survival probability, which directlytakes into account the Maxwell-Boltzmannenergy distribution of evaporated neutrons[15]. The double differential cross-sectionsare calculated as follows
d2ση
dΩdE(E, θ) =
∫∞
0
bdb∆Nη(b, E, θ)
Ntot(b)
1
sin(θ)∆θ∆E.
(1)Here ∆Nη(b, E, θ) is the number of eventsat a given impact parameter b in which thesystem enters into the channel η (definitemass asymmetry value) with kinetic energyin the region (E, E + ∆E) and center-of-
mass outgoing angle in the region (θ, θ+∆θ),Ntot(b) is the total number of simulatedevents for a given value of impact parameter.In collisions of deformed nuclei an averagingover initial orientations is performed. Ex-pression (1) describes the mass, energy andangular distributions of the primary frag-ments formed in the binary reaction (bothin DI and in QF processes). Subsequentde-excitation cascades of these fragmentsvia emission of light particles and gamma-rays in competition with fission were takeninto account explicitly for each event withinthe statistical model leading to the final
mass and energy distributions of the reac-tion fragments. The model allows us to per-form also a time analysis of the studied reac-tions. Each tested event is characterized bythe reaction time τint, which is calculated asa difference between re-separation (scission)and contact times.
DEEP INELASTIC SCATTERING OF
HEAVY NUCLEI
At first we applied the model to de-scribe available experimental data on low-energy damped collision of very heavy nu-clei, 136Xe+209Bi [16], where the DI pro-cess should dominate due to expected preva-
216
lence of the Coulomb repulsion over nuclearattraction. The adiabatic potential energysurface of this nuclear system is shown onthe left panel of Fig. 5 in the space of elon-gation and mass asymmetry at zero dynamicdeformations. The colliding nuclei are verycompact with almost closed shells and thepotential energy has only one deep valley(just in the entrance channel, η ∼ 0.21) giv-ing rather simple mass distribution of the re-action fragments. In that case the reactionmechanism depend mainly on the nucleus-nucleus potential at contact distance, on thefriction forces at this region (which deter-mine the energy loss) and on nucleon trans-fer rate at contact. Note, that there is awell pronounced plateau at contact configu-ration in the region of zero mass asymmetry(see Fig. 5, right panel). It becomes evenlower with increasing the deformations andcorresponds to formation of the nuclear sys-tem consisting of strongly deformed touch-ing fragments 172Er+173Tm (see Fig. 5),which means that a significant mass rear-rangement may occur here leading to addi-tional time delay of the reaction.
On the right panel of Fig. 5 the landscapeof the potential energy is shown at contactconfiguration depending on mass asymme-try and deformation of the fragments. Ascan be seen, after contact and before re-separation the nuclei aim to become moredeformed. Moreover, beside a regular diffu-sion (caused by the fluctuations), the finalmass distribution is determined also by thetwo well marked driving paths leading thesystem to more and to less symmetric con-figurations. They are not identical and thisleads to the asymmetric mass distributionof the primary fragments, see Fig. 6(c).
In Fig. 6 the angular, energy and chargedistributions of the Xe-like fragments areshown comparing with our calculations (his-tograms). In accordance with experimen-
FIG. 7: Time distribution of all the sim-ulated events for 86Kr+166Er collisions atEc.m.
= 464 MeV, in which the energy loss wasfound higher than 35 MeV (totally 105 events).Conditionally fast (< 2 · 10−21 s), intermediateand slow (> 2 ·10−20 s) collisions are marked bythe different colors (white, light gray and darkgray, respectively). The black area correspondsto CN formation (estimated cross section is 120mb), and the arrow shows the interaction time,after which the neutron evaporation may occur.
tal conditions only the events with the to-tal kinetic energy in the region of 260 ≤
E ≤ 546 MeV and with the scattering an-gles in the region of 40o ≤ θc.m. ≤ 100o
were accumulated. The total cross sec-tion corresponding to all these events isabout 2200 mb (experimental estimation is2100 mb [16]). Due to the rather high ex-citation energy sequential fission of the pri-mary heavy fragments may occur in this re-action (mainly those heavier than Bi). Inthe experiment the yield of the heavy frag-ments was found to be about 30% less com-paring with Xe-like fragments. Our calcu-lation gives 354 mb for the cross section ofsequential-fission, which is quite comparablewith experimental data. Mass distributionof the fission fragments is shown in Fig. 6(c)by the dotted histogram. Note that it is acontamination with sequential fission prod-ucts of heavy primary fragments leading to
217
FIG. 8: (a) TKE-charge distribution of the 86Kr+166Er reaction products at Ec.m.
= 464 MeV[17]. (b) Calculated TKE-mass distribution of the primary fragments. Open, gray and black circlescorrespond to the fast (< 2 ·10−21 s), intermediate and long (> 2 ·10−20 s) events (overlapping eachother on the plot).
FIG. 9: Angular (a), energy (b) and charge (c) distributions of the 86Kr+166Er reaction productsat Ec.m.
= 464 MeV. Experimental data (points) are from [17]. Overlapping white, light and darkgray areas in (b) show the contributions of the fast, intermediate and slow events, respectively [seeFig. 7 and Fig. 8(b)].
the bump around Z=40 in the experimentalcharge distribution.
At the second step we analyzed the re-action 86Kr+166Er at Ec.m. = 464 MeV[17], in which the nuclear attractive forcesmay lead, in principle, to the formation ofa mono-nucleus and of CN. The adiabaticpotential energy surface, QF and fusion-fission (FF) processes should in this caseplay a more important role. For the anal-ysis of this reaction we used the same valueof the nucleon transfer rate and the samefriction forces as in the previous case. Forthe nuclear viscosity we choose the value
µ0 = 2 · 10−22 Mev s fm−3 because of inter-mediate values of excitation energies avail-able here as compared with the two previousreactions.
The interaction time is one of the mostimportant characteristics of nuclear reac-tions, though it cannot be measured di-rectly. It depends strongly on the reactionchannel. The time distribution of all the86Kr+166Er collisions at Ec.m. = 464 MeV,in which the kinetic energy loss is higherthan 35 MeV, is shown in Fig. 7. The in-teraction time was calculated starting fromt = 0 at R = Rmax = 40 fm up to
218
FIG. 10: Potential energy at contact “nose-to-nose” configuration and mass distribution of pri-mary fragments for the two nuclear systems formed in 48Ca+248Cm (left) and 232Th+250Cf (right)collisions.
the moment of scission into two fragments(R > Rscission, pR > 0) or up to CN for-mation. The approaching time (path fromRmax to Rcontact) in the entrance channel isvery short (4÷ 5 · 10−22 s depending on theimpact parameter) and may be ignored here.All the events are divided relatively onto thethree groups: fast (τint < 20 · 10−22 s), in-termediate, and slow (τint > 200 · 10−22 s).
A two-dimensional plot of the energy-mass distribution of the primary frag-ments formed in the 86Kr+166Er reaction atEc.m. = 464 MeV is shown in Fig. 8. In-clusive angular, charge and energy distribu-tions of these fragments (with energy lossesmore than 35 MeV) are shown in Fig. 9.Rather good agreement with experimentaldata of all the calculated DI reaction prop-erties can be seen, which was never obtainedbefore in dynamic calculations. Underes-timation of the yield of low-Z fragments[Fig. 9(c)] could again be due to the contri-bution of sequential fission of highly excitedreaction participants not accounted in themodel at the moment.
In most of the damped collisions(Eloss > 35 MeV) the interaction timeis rather short (several units of 10−21 s).These fast events correspond to grazingcollisions with intermediate impact param-eters. They are shown by the white areas in
Figs. 7 and 9(b) and by the open circles intwo-dimensional TKE-mass plot [Fig. 8(b)].Note that a large amount of kinetic energyis dissipated here very fast at relatively lowmass transfer (more than 200 MeV duringseveral units of 10−21 s).
The other events correspond to muchslower collisions with large overlap of nu-clear surfaces and significant mass rear-rangement. In the TKE-mass plot theseevents spread over a wide region of massfragments (including symmetric splitting)with kinetic energies very close to kineticenergy of fission fragments. The solid linein Fig. 8(b) correspond to potential energyat scission point V (r = Rscission, β, α) +Qgg(α) minimized over β. Scission pointis calculated here as Rscission(α, β) =(1.4/r0)[R1(A1, β1) + R2(A2, β2)] + 1 fm,Qgg(α) = B(A1) + B(A2) − B(86Kr) −
B(166Er) and B(A) is the binding energyof a nucleus A. Some gap between the twogroups in the time and energy distributionscan also be seen in Fig. 7 and Fig. 9(b). Allthese make the second group of slow eventsquite distinguished from the first one. Theseevents are more similar to fission than todeep-inelastic processes. Formally, they alsocan be marked as quasi-fission.
219
LOW-ENERGY COLLISIONS OF
TRANSACTINIDE NUCLEI
Reasonable agreement of our calculationswith experimental data on low-energy DIand QF reactions induced by heavy ionsstimulated us to study the reaction dynam-ics of very heavy transactinide nuclei. Thepurpose was to find an influence of the shellstructure of the driving potential (in par-ticular, deep valley caused by the doubleshell closure Z=82 and N=126) on nucleonrearrangement between primary fragments.In Fig. 10 the potential energies are showndepending on mass rearrangement at con-tact configuration of the nuclear systemsformed in 48Ca+248Cm and 232Th+250Cfcollisions. The lead valley evidently revealsitself in both cases (for 48Ca+248Cm sys-tem there is also a tin valley). In the firstcase (48Ca+248Cm), discharge of the sys-tem into the lead valley (normal or sym-metrizing quasi-fission) is the main reac-tion channel, which decreases significantlythe probability of CN formation. In col-lisions of heavy nuclei (Th+Cf, U+Cmand so on) we expect that the existenceof this valley may noticeably increase theyield of surviving neutron-rich superheavynuclei complementary to the projectile-likefragments around 208Pb (“inverse” or anti-symmetrizing quasi-fission process).
Direct time analysis of the reaction dy-namics allows us to estimate also the life-time of the composite system consisting oftwo touching heavy nuclei with total chargeZ>180. Such “long-living” configurationsmay lead to spontaneous positron emis-sion from super-strong electric field of giantquasi-atoms by a static QED process (tran-sition from neutral to charged QED vac-uum) [10]. About twenty years ago an ex-tended search for this fundamental processwas carried out and narrow line structures
in the positron spectra were first reportedat GSI. Unfortunately these results werenot confirmed later, neither at ANL, norin the last experiments performed at GSI.These negative finding, however, were con-tradicted by Jack Greenberg (private com-munication and supervised thesis at WrightNuclear Structure Laboratory, Yale univer-sity). Thus the situation remains unclear,while the experimental efforts in this fieldhave ended. We hope that new experimentsand new analysis, performed according tothe results of our dynamical model, mayshed additional light on this problem andalso answer the principal question: are theresome reaction features (triggers) testifyinga long reaction delays? If they are, new ex-periments should be planned to detect thespontaneous positrons in the specific reac-tion channels.
Using the same parameters of nuclear vis-cosity and nucleon transfer rate as for thesystem Xe+Bi we calculated the yield of pri-mary and surviving fragments formed in the232Th+250Cf collision at 800 MeV center-of mass energy. Low fission barriers of thecolliding nuclei and of most of the reactionproducts jointly with rather high excitationenergies of them in the exit channel willlead to very low yield of surviving heavyfragments. Indeed, sequential fission ofthe projectile-like and target-like fragmentsdominate in these collisions, see Fig. 11. Atfirst sight, there is no chances to get sur-viving superheavy nuclei in such reactions.However, as mentioned above, the yield ofthe primary fragments will increase due tothe QF effect (lead valley) as compared tothe gradual monotonic decrease typical fordamped mass transfer reactions. Secondly,with increasing neutron number the fissionbarriers increase on average (also there is theclosed sub-shell at N=162). Thus we mayexpect a non-negligible yield (at the level of
220
FIG. 11: Mass distributions of primary (solid histogram), surviving and sequential fission fragments(hatched areas) in the 232Th+250Cf collision at 800 MeV center-of-mass energy. On the right theresult of longer calculation is shown.
FIG. 12: (Left panel) Experimental and calculated yields of the elements 98÷101 in the reactions238U+238U (crosses) [5] and 238U+248Cm (circles and squares) [6]. (Right panel) Predicted yieldsof superheavy nuclei in collisions of 238U+238U (dashed), 238U+248Cm (dotted) and 232Th+250Cf(solid lines) at 800 MeV center-of-mass energy. Solid curves in upper part show isotopic distributionsof primary fragments in the Th+Cf reaction.
1 pb) of surviving superheavy neutron richnuclei produced in these reactions [18].
Result of much longer calculations isshown on the right panel of Fig. 11. Thepronounced shoulder can be seen in the massdistribution of the primary fragments nearthe mass number A=208 (274). It is ex-plained by the existence of a valley in the
potential energy surface [see Fig. 10(b)],which corresponds to the formation of dou-bly magic nucleus 208Pb (η = 0.137). Theemerging of the nuclear system into this val-ley resembles the well-known quasi-fissionprocess and may be called “inverse (or anti-symmetrizing) quasi-fission” (the final massasymmetry is larger than the initial one).
221
For η > 0.137 (one fragment becomes lighterthan lead) the potential energy sharply in-creases and the mass distribution of the pri-mary fragments decreases rapidly at A<208(A>274).
In Fig. 12 the available experimental dataon the yield of SH nuclei in collisions of238U+238U [5] and 238U+248Cm [6] are com-pared with our calculations. The estimatedisotopic yields of survived SH nuclei in the232Th+250Cf, 238U+238U and 238U+248Cmcollisions at 800 MeV center-of-mass energyare shown on the right panel of Fig. 12.Thus, as we can see, there is a real chance forproduction of the long-lived neutron-rich SHnuclei in such reactions. As the first step,chemical identification and study of the nu-clei up to 274
107Bh produced in the reaction232Th+250Cf may be performed.
The time analysis of the reactions studiedshows that in spite of absence of an attrac-tive potential pocket the system consistingof two very heavy nuclei may hold in con-tact rather long in some cases. During thistime the giant nuclear system moves overthe multidimensional potential energy sur-face with almost zero kinetic energy (resultof large nuclear viscosity). The total reac-
tion time distribution, dσdlog(τ)
(τ denotes
the time after the contact of two nuclei),is shown in Fig. 13 for the 238U+248Cmcollision. The dynamic deformations aremainly responsible here for the time delay ofthe nucleus-nucleus collision. Ignoring thedynamic deformations in the equations ofmotion significantly decreases the reactiontime, see Fig. 13(a). With increase of theenergy loss and mass transfer the reactiontime becomes longer and its distribution be-comes more narrow.
As mentioned earlier, the lifetime of a gi-ant composite system more than 10−20 sis quite enough to expect positron linestructure emerging on top of the dynami-
cal positron spectrum due to spontaneouse+e− production from the supercritical elec-tric fields as a fundamental QED process(“decay of the vacuum”) [10]. The abso-lute cross section for long events is foundto be maximal just at the beam energy en-suring the two nuclei to be in contact, seeFig. 13(c). The same energy is also optimalfor the production of the most neutron-richSH nuclei. Of course, there are some uncer-tainties in the used parameters, mostly inthe value of nuclear viscosity. However wefound only a linear dependence of the reac-tion time on the strength of nuclear viscos-ity, which means that the obtained reactiontime distribution is rather reliable, see log-arithmic scale on both axes in Fig. 13(a).
Formation of the background positrons inthese reactions forces one to find some ad-ditional trigger for the longest events. Suchlong events correspond to the most dampedcollisions with formation of mostly excitedprimary fragments decaying by fission, seeFigs. 14(a). However there is also a chancefor production of the primary fragments inthe region of doubly magic nucleus 208Pb,which could survive against fission due tonucleon evaporation. The number of thelongest events depends weakly on impactparameter up to some critical value. On theother hand, in the angular distribution ofall the excited primary fragments (stronglypeaked at the center-of-mass angle slightlylarger than 900) there is the rapidly decreas-ing tail at small angles, see Fig. 14(b). Timedistribution for the most damped events(Eloss > 150 MeV), in which a large masstransfer occurs and primary fragments scat-ter in forward angles (θc.m. < 70o), is rathernarrow and really shifted to longer time de-lay, see hatched areas in Fig. 13. For theconsidered case of 238U+248Cm collision at800 MeV center-of-mass energy, the detec-tion of the surviving nuclei in the lead re-
222
FIG. 13: Reaction time distributions for the 238U+248Cm collision at 800 MeV center-of-massenergy. Thick solid histograms correspond to all events with energy loss more than 30 MeV. (a)Thin solid histogram shows the effect of switching-off dynamic deformations. (b) Thin solid, dashedand dotted histograms show reaction time distributions in the channels with formation of primaryfragments with Eloss > 200 MeV, Eloss > 200 MeV and θc.m.
< 70o and A ≤ 210, correspondingly.Hatched areas show time distributions of events with formation of the primary fragments withA ≤ 220 (light gray), A ≤ 210 (gray), A ≤ 204 (dark) having Eloss > 200 MeV and θc.m.
< 70o. (c)Cross section for events with interaction time longer than 10−20 s.
FIG. 14: Energy-time (a) and angular-time (b) distributions of primary fragments in the238U+248Cm collision at 800 MeV (Eloss > 15 MeV).
gion at the laboratory angles of about 25o
and at the low-energy border of their spec-trum (around 1000 MeV for Pb) could be areal trigger for longest reaction time.
CONCLUSION
For near-barrier collisions of heavy ionsit is very important to perform a combined(unified) analysis of all strongly coupled
channels: deep-inelastic scattering, quasi-fission, fusion and regular fission. This am-bitious goal has now become possible. Aunified set of dynamic Langevin type equa-tions is proposed for the simultaneous de-scription of DI and fusion-fission processes.For the first time, the whole evolution of theheavy nuclear system can be traced start-ing from the approaching stage and end-ing in DI, QF, and/or fusion-fission chan-nels. Good agreement of our calculations
223
with experimental data gives us hope toobtain rather accurate predictions of theprobabilities for superheavy element forma-tion and clarify much better than beforethe mechanisms of quasi-fission and fusion-fission processes. The determination of suchfundamental characteristics of nuclear dy-namics as the nuclear viscosity and the nu-cleon transfer rate is now possible. The pro-duction of long-lived neutron-rich SH nu-clei in the region of the “island of sta-bility” in collisions of transuranium ionsseems to be quite possible due to a largemass rearrangement in the inverse (anti-symmetrized) quasi-fission process causedby the Z=82 and N=126 nuclear shells. Asearch for spontaneous positron emissionfrom a supercritical electric field of long-living giant quasi-atoms formed in these re-actions is also quite promising.
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224
Conference Proceedings Vol. 96
“The Nuclear Physics from the f7/2 to the Quark - Gluon Plasma”
F. Gramegna, M. Cinausero, D. Fabris (Eds.)
SIF, Bologna 2008
PROBING THE NUCLEAR EOS WITH REACTION MECHANISMS AT
FERMI ENERGIES
M. Colonna1,2
, V.Baran3, M. Di Toro
1,2
1 LNS-INFN, I-95123, Catania, Italy,
2 Physics and Astronomy Dept. University of Catania, Italy,
3 NIPNE-HH and Bucharest University, Romania
INTRODUCTION
In the last few years the increased accuracy of the experimental techniques has renewed interest in nuclear reactions at Fermi energies. In particular, recent experimental and theoretical analyses were devoted to the study of the properties and effects of the symmetry term of the EOS (iso-EOS) away from saturation conditions [1,2]. In particular, heavy ion reactions with exotic nuclei at Fermi energies can be used to study the properties of the symmetry term at densities below and around the normal value. In central collisions at 30-50 MeV/A, where the full disassembly of the system into many fragments is observed, one can study specifically properties of liquid-gas phase transitions occurring in asymmetric matter [2,3,4,5]. For instance, in neutron-rich matter, phase co-existence leads to a different asymmetry in the liquid and gaseous phase: fragments (liquid) appear more symmetric with respect to the initial matter, while light particles (gas) are more neutron-rich [2-5]. Hence the analysis of the isotopic content of all reaction products, from pre-equilibrium emission to fragments, allows to get information on low-density properties of the isovector part of the nuclear interaction.
In recent years, the properties of fragments and light clusters emitted in systems with different initial asymmetries have been widely investigated [6,7,8,9,10,11] looking in particular at the production yields of various isotopes, as obtained in reactions between proton-rich and neutron-rich systems.
More recently, the study of the isotopic content of pre-equilibrium emission has revealed a good sensitivity to the iso-EOS, considering the emitted neutron to proton ratio as a function of the kinetic energy [12].
Here we extend this type of investigation to fragments. Correlations between fragment
charges and velocities have been recently observed, providing information on the interplay between thermal and entrance channel (collective) effects in the fragmentation mechanism [13,14]. Following this line, one can also investigate correlations between fragment isotopic content and kinematical properties, trying to get a deeper insight into the reaction path and to improve the understanding of the underlying mechanisms. In this way one can also study more in detail the effects of different EOS’s and, in particular, of the symmetry energy on fragment properties. Information on the low densiy behaviour of the symmetry energy can be obtained also from lower energy reactions, where one can study the competition between reaction mechanisms, such as incomplete fusion, deep-inelastic or fragmentation. In particular, in mid-peripheral collisions a large variety of phenomena is observed, ranging from highly dissipative binary evens to neck break-up and non-statistical light fragment emission. As we will discuss in the following, the study of neutron-rich systems reveals new interesting features, opening the possibility to access independent information on the symmetry energy.
THE MODEL
Theoretically, the evolution of complex systems under the influence of fluctuations can be described by a transport equation with a stochastic fluctuating term, the so-called Boltzmann-Langevin equation (BLE):
[ ] [ ]fIfIHft
f
dt
dfcoll δ+=+
∂∂
= , (1)
225
where ( )tprf ,,rr
is the one-body distribution function, ( )tprH ,,
rris the one-body Halmitonian
and ][ fIδ represents the stochastic part of the two-body collision integral [15,16].
Here we will follow the approximate treatment to the BLE presented in Ref.[17], the so-called Stochastic Mean Field (SMF) model, that consists in the implementation of spatial density fluctuations [17]. Calculations have been performed using a BNV code (TWINGO), where the test particle method is used to solve Eq.(1) [18] . We use a soft EOS, with compressibility modulus K=200 MeV and, for the density (ȡ) dependence of the symmetry energy, we consider two representative parameterizations,
( ) AZNIICAIE symsym /)(,)(/, 2 −≡≡ ρρ one showing a rapidly increasing behaviour with density, roughly proportional to ȡ2
(asystiff) and one with a kind of saturation above normal density (asysoft, SKM
*) (see Ref.[2,19] for more
detail). The two parameterizations obviously cross at normal density. The symmetry energy at densities below the normal value is larger in the asysoft case, while above normal density it is higher in the asystiff case. Hence in the low-density regime, that is the region of interest for the analysis of central dissipactive reactions, isospin effects are expected to be more important in the asysoft case.
FRAGMENT ISOTOPIC PROPERTIES
AND CORRELATIONS
We will first focus on central collisions, b= 2 fm, considering symmetric reactions between systems having three different (N/Z)in initial asymmetry:
112Sn +
112Sn,
124Sn +
124Sn,
132Sn +
132Sn, with (N/Z)in = 1.24, 1.48, 1.64,
respectively. The considered beam energy is 50 MeV/A. 1200 events have been run for each reaction and for each of the two symmetry energies adopted. The first two reactions
112Sn +
112Sn and
124Sn +
124Sn, have been widely
investigated both from the experimental and theoretical point of view [6,7,20]. In central collisions, after the initial collisional shock, the system expands and breaks up into many pieces, due to the development of volume (spinodal) and surface instabilities. The formation of a bubble-like configuration is observed, where the initial fragments are located. The average fragment multiplicity is approximately equal to 6 for the reactions considered here [19]. Along the reaction path, several nucleons are emitted at the early stage (pre-equilibrium emission) and/or are
evaporated while fragments are formed. Primary fragments are identified by applying a coalescence procedure to the matter with density larger than ȡcut = 1/5 ȡ0 (liquid phase). The remaining particles are considered as belonging to the gas phase. First, let us briefly recall some general features concerning the isotopic content of fragments and emitted nucleons, as obtained with the two iso-EOS considered. In the following we will restrict our analysis to fragments with charge in the range between 3 and 10 (that we call intermediate mass fragments (IMF's) ). The average N/Z of emitted nucleons (gas phase) and IMF's is presented in Fig.1 as a function of the initial (N/Z)in of the three colliding systems.
Fig. 1: The N/Z of the liquid (squares,left) and of the gas (circles,right) phase is displayed as a function of the system initial N/Z. Full lines and symbols refer to the asystiff parameterization. Dashed lines and open symbols are for asysoft.
One observes that, generally, the gas phase is more neutron-rich in the asysoft case, while IMF's are more symmetric. This is due to the larger value of the symmetry energy at low density for the asysoft parameterization [19]. It is interesting to note that, in the asystiff case, due to the low value of the symmetry energy, Coulomb effects dominate and the N/Z of the gas phase becomes lower than that for IMF's, because protons are preferentially emitted.
Now we move to investigate in more detail correlations between fragment isotopic content and kinematical properties. The idea in this investigation is that fragmentation originates from the break-up of a composite source that expands with a given velocity field. Since neutrons and protons experience different forces, one may expect a different radial flow for the two species. In this case, the N/Z composition of
226
the source would not be uniform, but would depend on the radial distance from the center or mass or, equivalently, on the local velocity. This trend should then be reflected in the fragment asymmetries. As a measure of the isotopic composition of the IMF's, we will consider the sum of neutrons, N = Ȉi Ni, and protons, Z = Ȉi Zi, of all IMF's in a given kinetic energy range, in each event. Then we take the ratio N/Z and we consider the average over the ensemble of events. This observable is plotted in Fig.2 for the three reactions.
Fig. 2: The fragment N/Z (see text) as a function of the kinetic energy. Left panel:asystiff; Rigth panel: asysoft.
The behaviour observed is rather sensitive to the iso-EOS. For the proton-rich system, the N/Z decreases with the fragment kinetic energy, expecially in the asystiff case, where the symmetry energy is relatively low at low density [19]. In this case, the Coulomb repulsion pushes the protons towards the surface of the system. Hence, more symmetric fragments acquire larger velocity. The same effects are responsible for the proton-rich pre-equilibrium emission observed in this case (see Fig.1). The decreasing trend is less pronounced in the asysoft case (right panel) because Coulomb effects are counterbalanced by the larger value of the symmetry energy. In systems with larger initial asymmetry, the decreasing trend is inversed, due to the larger neutron repulsion in neutron-rich systems. Larger slopes are always observed in the asysoft case.
In conclusion, this analysis reveals the existence of significant, EOS-dependent correlations between the N/Z and the kinetic energy of IMF's. This correlation is linked to the different forces experienced by neutrons and protons along the fragmentation path, that in turn
depend on the detail of the isovector part of the nuclear interaction. This study can be considered as complementary to the pre-equilibrium emission studies [12]. A parallel investigation of pre-equilibrium and fragment emissions would be very important for a cross-check of model predictions against experimental observables sensitive to different phases of the reaction.
NECK EMISSION
Dissipative mid-peripheral collisions, including binary and three-body breakings, offer a unique opportunity to study phenomena occurring in nuclear matter under extreme conditions with respect to shape, intrinsic excitation energy, spin, N/Z ratio, etc., together with the possibility to control these conditions by choosing appropriate entrance and exit channels. Thus, it is possible to probe the mechanisms of nuclear excitation, how intrinsic degrees of freedom are converted into collective modes, how these modes decay and how relaxation processes occur within a small quantal system that is initially far from equilibrium. The velocity and the angular distribution of the reaction products furnish natural clocks from which it is possible to determine the equilibration times of the various degrees of freedom (e.g. N/Z ratio, mass, excitation energy) and discuss whether non-equilibrium features in light particle and IMF emissions are present [21].
Neck emission at Fermi energies has been widely investigated, revealing the presence of features that characterize it as an independent IMF source, clearly distinguishable from the statistical emission of projectile-like (PLF) and target-like (TLF) fragments [21]. In particular, the IMF’s coming from the neck source have a velocity that deviates from the Viola systematics and are aligned, i.e. emitted with a scall angle ĭ with respect to the direction connecting PLF and TLF velocities. It is interesting to study correlations between the fragment N/Z and the alignment. This is presented in Fig.3, for the reaction
124Sn +
64Ni at 35 MeV/u, b = 6 fm. As
already seen for the central reactions, a pronounced decreasing trend of the N/Z is observed in the asystiff case. In this case (semi-peripheral reactions) this can be attributed to the migration of the neutron-richness of the system towards the low-density neck region, influencing especially the properties of IMF’s that interact with the system for a longer time (small ĭ angles).
227
Fig. 3: The N/Z of IMF’s emitted from the neck region as a function of the alignment. Circles: asystiff. Squares: asysoft.
COMPETITION BETWEEN REACTION
MECHANISMS
For dissipative collisions at low energy,
interaction times are quite long and therefore a large coupling among various mean-field modes is expected. In some cases, due to a combined Coulomb and angular momentum (deformation) effect, some instabilities can show up, like in fission decays [22]. This can lead to three-body breakings, where a light cluster is emitted from the neck region, similarly to what is observed at larger beam energy.
For instance, a significant probability for preferential alpha-particle emission perpendicular to the symmetry axis of a fissioning heavy-ion system was reported in Ref.[23] for the system
165Ho +
56Fe at 465 MeV
(see also [24]). In the same energy range, TDHF calculations show a rich variety of dynamical behavior, including deep-inelastic scattering, fusion and three-body break-up (see for instance Ref.[25], where the reaction
86Kr +
139La at 505,
610, 710 MeV is analyzed). Three-body processes, in heavy-ion reactions with exotic systems, can certainly provide a new access to the dynamics of nuclear scission in new conditions, allowing to investigate the role of the isovector part of the nuclear interaction. In particular, one can investigate whether the
development of surface (neck-like) instabilities, that would help ternary breaking, is sensitive to the structure of the symmetry term.
This study has been undertaken in the case of the reaction
132Sn+
64Ni at 10 MeV/n. Semi-
peripheral reactions, corresponding to impact parameters b=6, 7, 8 fm have been considered, for which one observes mostly binary exit channels.
It appears that the neck dynamics is rather different when one considers the asysoft or the asystiff parameterization.
Fig. 4: Density contour plots on the reaction plane obtained in several runs of the reaction 132Sn+64Ni at 10 MeV/n, b = 7 fm, at t = 500 fm/c. Asystiff interaction.
Fig. 5: Density contour plots on the reaction plane obtained in several runs of the reaction 132Sn+64Ni at 10 MeV/n, b = 7 fm, at t = 500 fm/c. Asysoft interaction.
This can be qualitatively seen on Figs. 4-5, where density contour plots of events obtained
228
with the two iso-EOS are represented. Large deformations, strongly suggesting a final
three-body outcome, are observed in the majority of the events in the asystiff case. In fact, in this case, due to the lower value of the symmetry energy, the neutron-rich neck connecting the two systems survives a longer time, leading to deformed primary products, from which eventually small clusters can be dynamically emitted.
To perform a quantitative analysis, one can evaluate the quadrupole or octupole moment of PLF and/or TLF, that are related to the degree of deformation of the di-nuclear system and, hence, to the probability to get a ternary break-up. The distribution of the octupole moment over an ensemble of events is shown in Fig. 6 for the two iso-EOS (the dashed hysto corresponds to asystiff and the full hysto to asysoft) and three impact parameters. In conclusion an asystiff symmetry term leads to more dissipative events, due to lower value of the symmetry energy.
Fig. 6: Distribution of the octupole moment of primary fragments obtained in the reaction 32Sn + 64Ni at 10 MeV/u at b = 6 fm (left), 7 fm (middle), 8 fm (right). Full line: asysoft; dashed line: asystiff.
CONCLUSIONS AND PERSPECTIVES
We have discussed properties of the fragmentation path, in collisions of charge-asymmetric systems at Fermi energies, that can be related to the behavior of the symmetry energy below normal density, thus allowing to extract important information on fundamental quantities of the nuclear interaction.
We focus on the analysis of correlations between fragment isotopic content and kinematical properties, performing simulations based on SMF approaches. This study also allows one to get a deeper insight into the fragmentation mechanism. In fact, the analysis of correlations between fragment composition and
velocity can be used as a clock of fragment formation and as an indicator of the underlying dynamics.
This kind of investigation is extended also to mid-peripheral collisions at energies around 10 MeV/u. Also at these relatively low energies, ternary (neck) break-up is observed in neutron-rich systems, as a manifestation of the degree of dissipation reached, with a good sensitivity to the iso-EOS adopted.
We expect to see effects of the different interaction times and dissipation degree also on the charge equilibration mechanism, probed starting from entrance channels with large N/Z asymmetries, like
132Sn (N/Z=1.64) +
58Ni
(N/Z=1.07). Moreover, the equilibration mechanism is also directly linked to the strength of the symmetry term. For more central collisions this can be studied via the direct measurement of the prompt Dynamical Dipole emission, nucleus-nucleus collective bremsstrahlung radiation during the charge equilibration path, see Refs.[26,27]. Nice experimental features of such dipole radiation are the angular anisotropy, with maximum emission orthogonal to the beam axis, and the gamma spectrum, with centroid at energies well below the expected GDR emission from the residues. The energy range around 10 MeV/u seems to optimize the effect, see the recent data of Ref.[28] with stable beams. From this class of phenomena one can access new independent information on the low-density behavior of the symmetry energy.
[1] Isospin Physics in Heavy-ion Collisions at Intermediate Energies, Eds. Bao-An Li and W. Udo Schroeder, Nova Science Publishers (2001, New York). [2] V. Baran, M.Colonna, V.Greco, M.Di Toro, Phys. Rep. 410 (2005) 335. [3] H.Mueller and B.D.Serot, Phys.Rev. C52 (1995) 2072 [4] Bao-An Li and C.M.Ko, Nucl.Phys. A618 (1997) 498 [5] Ph. Chomaz, M. Colonna, J. Randrup, Phys. Rep. 389, (2004) 263 [6] H.S.Xu et al., Phys. Rev. Lett. 85 (2000) 716. [7] M.B. Tsang, W.A. Friedman, C.K. Gelbke et al., Phys. Rev. Lett. 86 (2001) 5023 [8] A.S. Botvina, O.V. Lozhkin and W. Trautmann, Phys. Rev. C65 (2002) 044610. [9] E. Geraci et al., Nucl. Phys. A732 (2004) 173 [10] D.V.Shetty, S.J.Yennello, G.A.Souliotis, Phys Rev. C75 (2007) 034602; S.Kowalski et al.,
229
Phys Rev. C75 (2007) 014601 [11] M.Colonna and M.B.Tsang, Eur. Phys. J. A30 (2006) 165 [12] M.Famiano er al., Phys. Rev. Lett. 97 (2006) 052701 [13] G.Tabacaru et al., Nucl. Phys. A764 (2006) 371 [14] J.D. Frankland et al., Nucl. Phys. A689 (2001) 940; J.Colin et al., Phys. Rev. C67 (2003) 064603 [15] S.Ayik, C.Gregoire, Phys. Lett. B212 (1998) 269 and refs. therein. [16] J.Randrup and B.Remaud, Nucl. Phys. A514 (1990) 339 [17] M. Colonna et al, Nucl. Phys. A642 (1998) 449 [18] A.Guarnera, M.Colonna, Ph.Chomaz, Phys. Lett. B373 (1996) 297. [19] V. Baran et al., Nucl. Phys. A703 (2002) 603 [20] B-A Li, C.Ko, and Z. Ren, Phys. Rev. Lett. 78
(1997) 1644; T.X.Liu et al., Phys. Rev. C69
(2004) 014603 [21] V. Baran, M. Colonna, M. Di Toro, Nucl. Phys. A730 (2004) 329; E. De Filippo et al., Phys. Rev. C71 (2005) 044602 [22] M.Colonna, M.Di Toro, A.Guarnera, Nucl .Phys. A589 (1995) 160 [23] W.W.Wilcke et al., Phys. Rev. Lett. 51 (1983) [24] U.Brosa et al., Phys. Rep. 197(1990)167 [25] K.T.R.Davies et al., Phys. Rev. C20 (1979) 1372 [26] C.Simenel, Ph. Chomaz, G.de France, Phys. Rev. Lett. 86 (2000) 2971 [27] V.Baran, D.M.Brink, M.Colonna, M.Di Toro, Phys. Rev. Lett. 87 (2001) 182501 [28] D.Pierroutsakou et al., Phys. Rev. C71 (2005) 054605
230
PROPERTIES OF HEAVY ION COLLISIONS AT FERMI
ENERGIES
S.Piantelli1 for the FIASCO Collaboration1,2
1 INFN Sezione di Firenze, 2 Dipartimento di Fisica Universita di Firenze
INTRODUCTION
Heavy ion collisions with beam energybetween 10 and 50AMeV are usually in-dicated as reactions at Fermi energies be-cause the Fermi energy for nucleons insidenuclei is of the same order of magnitude(around 30MeV). In this energy domain pe-ripheral and semi-peripheral collisions showbinary character, with two heavy remnants(the Quasi-Projectile QP and the Quasi-Target QT) in the exit channel. The bestway to put into evidence this behaviouris to present the experimental yields ofthe emitted Light Charged Particles (LCPs,Z = 1, 2) and Intermediate Mass Fragments(IMFs, 3 ≤ Z ≤ 7) as a function of the par-allel and perpendicular components of theircenter of mass velocity with respect to QP-QT separation axis; an example of such rep-resentation is presented in Fig.1 (from [1])for the symmetric reaction 93Nb +93 Nb at38AMeV. The figure shows clearly two in-tensified circular regions located around thevelocity of QP and QT for protons (top) andα particles (middle), corresponding to theso-called Coulomb rings. The events withtwo heavy remnants in the exit channel con-stitute more than 50% of the total reactioncross section.
Another characteristic property of theFermi energy domain is the large amountof IMFs and LCPs emitted with velocity in-termediate between those of QP and QT,the so called “midvelocity” emission [1–11].Their presence clearly emerges if we com-pare the experimental (v‖, v⊥) plots to those
020406080
TKEL=200MeV TKEL=500MeV TKEL=800MeV
020406080
020406080
-50 0 50
V⊥ (
mm
/ns)
-50 0 50-50 0 50
E/A=38MeV
FIG. 1: Efficiency corrected experimental yieldsin the plane (v‖, v⊥) with respect to the QP-QTseparation axis with the origin in the center ofmass reference frame; data refer to the symmet-ric system 93Nb +93 Nb at 38AMeV and theyhave been collected by the FIASCO setup. Rowscorrespond, respectively, from top to bottom, toprotons, α particles and IMFs with 3 ≤ Z ≤ 7.Each column corresponds to a different central-ity of the collision. From [1].
obtained for a pure evaporative simulationmainly based on the GEMINI code [12] (apure evaporative code based on the statis-tical model), as shown in Fig.2 (from [8]).Especially the fourth row, corresponding tothe IMFs case, shows that while the simu-lation (right column) predicts an emissiononly located around the Coulomb rings, theexperimental emission pattern (left column)is mainly concentrated in the central re-gion between the velocity of the QP andof the QT. An emission in the midvelocityregion, superimposed to the emission alongthe Coulomb rings, is present also for the
Conference Proceedings Vol. 96“The Nuclear Physics from the f7/2 to the Quark - Gluon Plasma”F. Gramegna, M. Cinausero, D. Fabris (Eds.)SIF, Bologna 2008
231
LCPs. The origin of this phenomenon is stilldebated, but the usual interpretation at-tributes it to the rupture (in the first phaseof the reaction) of the neck of nuclear mat-ter which is formed between QP and QT inthe interaction phase.
0
50
100Experiment (corr.)
p
Statistical simulation
p
0
50d
v perp
(m
m/n
s) d
0
50Z=2 Z=2
0
50
-50 0 50
Z=3-7
-50 0 50
Z=3-7
vpar (mm/ns)
FIG. 2: Left column: efficiency corrected exper-imental yields in the plane (v‖, v⊥) with respectto the QP-QT separation axis with the origin inthe center of mass reference frame; data referto the system 116Sn +93 Nb at 29.5AMeV andthey have been collected by the FIASCO setup.Right column: same kind of data for a purelyevaporative simulation. From [8].
This work concerns the presentation ofthe physical analysis developed by the FI-ASCO experiment [13] in the past eightyears; the discussed data concern the sym-metric systems 93Nb +93 Nb at 17, 23, 30and 38AMeV and 116Sn +116 Sn at 23,30, and 38AMeV; the asymmetric reaction116Sn +93 Nb at 29.5AMeV is included too.The experiments were performed at Labo-
ratori Nazionali del Sud of INFN in Cata-nia. The goals of our data analysis con-cern: i) the separation of the midvelocitycomponent from the evaporation from theexcited QP and QT; ii) the characterizationof both kinds of emission (evaporative andmidvelocity) from the point of view of par-ticle multiplicities and isotopic composition(for Z=1 only) as a function of the impactparameter; iii) the comparison among dif-ferent beam energies; iv) the average energyand mass balance for the whole reaction; v)the estimate of the time scale associated tothe midvelocity process.
THE EXPERIMENTAL SETUP
As it has been already pointed out, thesetup we used for our data collection iscalled FIASCO (Florentine Initiative Af-ter Superconducting Cyclotron Opening);this setup is described in a detailed wayin [13]; here only its main characteristicsare reminded. FIASCO was specially de-signed for the investigation of peripheraland semi-peripheral heavy ion collisions; infact, for such purposes, it includes 24 posi-tion sensitive Parallel Plate Avalanche De-tectors (PPADs), covering about 70% ofthe forward hemisphere (see Fig.3, wherethe frames of the PPADs are displayed inpolar representation), which measure thevelocity vector of heavy fragments (Z >10) with very low detection thresholds (<0.1AMeV ); as a consequence, they can de-tect the low energy QT also in peripheraland semi-peripheral collisions. In this wayit is possible to obtain a natural clean se-lection of two-body events, which, for ouranalysis, are defined as events with only twofragments with Z > 10 in the exit chan-nel. The setup includes also 96 Silicon tele-scopes (∆E = 200µm, Eres = 500µm),located behind the six most forward gas
232
detectors, which measure charge, energyand mass (this last point was obtained byadding the information concerning the timeof flight given by the coincident PPAD)for the QP. Concerning LCPs and IMFs,FIASCO is equipped with 182 three-layerphoswich telescopes (covering about 30% ofthe forward hemisphere) which identify pro-tons, deuterons, tritons and particles withcharge from 2 up to 15-20 and they measuredirectly their time of flight; in this way theparticle velocities can be obtained withoutenergy calibration of the phoswiches whichis always difficult (and requires dedicatedbeams). The three scintillator layers con-sist of a thin (∼ 180µm thick) fast plas-tic scintillator (Bicron BC404, decay con-stant τ = 1.8ns), a 5mm-thick slower plas-tic scintillator (Bicron BC444, τ = 180ns)and a CsI(Tl) (τ = 600 − 3500ns; thick-ness: 3 − 5cm); in the first measurementcampaign performed by FIASCO some ofthe phoswiches were without the slow plas-tic scintillator (two-layer phoswiches). Fi-nally, the setup includes also the hodoscopeHODO-CT [14], whose data were not usedfor the presented analysis.
-50
0
50
-50 0 50
13
1415
1617
18
19
2021
22
23
24
θ sin φ
θ c
os φ
θ=900
-10
0
10
-10 0 10
1
23
4
5
6
7
8
9
10
11
12
θ sin φ
∗
FIG. 3: Frame of the gas detectors of the FI-ASCO setup in polar representation. From [13].
The flight path of the most forwardPPADs is very long, about 3.5m, as it is ev-ident from Fig.4, where the side view of thesetup is presented; in this way it is possible
to obtain the time of flight of the forwardflying QP in an accurate way. Fig.5 and
-100
-50
0
50
100
-50 0 50 100 150 200 250 300 350 400Beam-axis Z (cm)
X (
cm)
BEAM
side view
FIG. 4: Side view of the FIASCO setup. From[13].
Fig.6 show two photographs of FIASCO asit was mounted inside the Ciclope scatteringchamber at LNS in Catania. In particular,Fig.5 shows the most forward ring (that at3.5m) and Fig.6 presents the target region,with some PPADs in foreground.
An example of the experimental two-bodyevents detected by the PPADs for the sys-tem 116Sn +93 Nb at 29.5AMeV is pre-sented in polar representation in Fig.7. Theforward-backward enhancement due to elas-tic and quasi-elastic collisions is clearly ev-ident. The empty circular zone on the leftside of the figure is due to the shadow ofthe target holder, which was tilted at about45 in order to reduce the material encoun-tered by the very slow QTs flying at about90 in the laboratory frame and to allowthem to reach the detectors escaping the tar-get. The target itself was very thin, about200µg/cm2.
The efficiency of the PPADs for the dif-ferent ions was obtained from the coinci-dences with the phoswich telescopes locatedbehind them; an example of the obtainedresults is presented in Fig.8 as a functionof the velocity in the laboratory frame. Itis evident that while for the Ne (Z = 10)and Mg (Z = 12) the efficiency falls down
233
FIG. 5: Photograph of FIASCO as it wasmounted inside the Ciclope scattering chamberat LNS in Catania. View from the most forwardring. From [13].
very quickly when the ion velocity increases,for the Si (Z = 14) the efficiency is around100% in almost the whole velocity range. Inany case it is worthwhile to note that QPand QT reach such small values of charge(they start from Z = 50 or Z = 41) onlyfor the most dissipative collisions, which areexcluded from the presented analysis.
Concerning the phoswich telescopes, anexample of the obtained particle identifica-tion is presented in Fig.9 for LCPs and inFig.10 for IMFs. The left side of each figurerefers to the identification obtained for thetwo-layer configuration, while the right sideconcerns a three-layer phoswich. The verygood charge resolution up to Z = 25 − 30for the three-layer configuration is evidentfrom Fig.10; the performances are some-what worse for the two-layer case. Con-cerning the LCPs, the isotopic resolution isvery good for the Hydrogen, while it is quite
FIG. 6: Photograph of FIASCO as it wasmounted inside the Ciclope scattering chamberat LNS in Catania. The target region. From[13].
-50 0 50θ sin ϕ
-50
0
50
θ cos ϕ
-5 0 5θ sin ϕ
-5
0
5θ cos ϕ
1
10000
FIG. 7: Experimental two-body events detectedby the PPADs of FIASCO for the system116Sn +93 Nb at 29.5AMeV in polar represen-tation. From [13].
marginal for the Helium and this fact is truefor both kinds of configurations. The iden-tification thresholds are due to the punchthrough of the first layer of scintillator; forthe LCPs they are about 3AMeV.
As it has been already pointed out, the
234
0
20
40
60
80
100NEON
40 50 60 70 80
Effi
cien
cy (
%)
MAGNESIUM
40 50 60 70 80vlab (mm/ns)
SILICON
40 50 60 70 80
FIG. 8: Detection efficiency for the PPADs ofFIASCO for different ions as a function of theirvelocity in the laboratory frame; the arrow cor-responds to the beam velocity. From [13].
1 1.5 2 2.5 3PI
0
1000
2000
3000
4000
5000
countsDouble phoswich
p
d
t
He−4
Li
PI1 1.5 2 2.5 3
Triple phoswich
He−4
LiHe−3
t
d
p
FIG. 9: LCP identification for a phoswichtelescope (typical case). Left side: two-layerphoswich; right side: three-layer phoswich.From [13].
angular coverage of the phoswich telescopesis only a fraction (about 30%) of the forwardhemisphere, as it can be seen from Fig.11,where the experimental counts acquired bythe phoswiches and by the hodoscope inthe reaction 93Nb +93 Nb at 38AMeV arepresented in polar representation. Countshave been uniformly distributed on the ac-tive area of each detector. Because of thisfinite coverage, all the data discussed in the
0 5 10
HHe
Li
Be
B
C
N
O
FCou
nts
(a.
u.)
0 5 10 15 20 25
H
HeLi
Be
B
CN
OF
NeMg S Ca Fe
Particle Identification
Double Triple Phoswich
FIG. 10: IMF identification for a phoswichtelescope (typical case). Left side: two-layerphoswich; right side: three-layer phoswich.From [13].
following sections concerning LCP and IMFmultiplicities have been corrected for geom-etry and detection thresholds of the setup.
-50 0 50
-50
0
50
-10 -5 0 5 10 15
-10
-5
0
5
10θ =90
ϕθsin ϕθsin
θcosϕθcosϕ
FIG. 11: Experimental counts acquired by thephoswich telescopes and the hodoscope in polarrepresentation. From [13].
As last point, the charge identification forthe QP, obtained from the Silicon telescopeswith the ∆E-Eres technique for the reaction116Sn +93 Nb at 29.5AMeV, is presented inFig.12. An unit charge resolution is appar-ent up to the projectile charge.
235
Z
1
10
102
103
10 20 30 40 50
FIG. 12: Charge identification for the QP asobtained from the Silicon telescopes. From [13].
EXPERIMENTAL RESULTS
The impact parameter estimate
As it has been already pointed out, thefirst problem we have to face is the estimateof the impact parameter; since this quantityis not directly accessible, we need an exper-imental observable which is monotonicallycorrelated to it. We used the observableTKEL = Ec.m.
in − 1
2µv2
rel under the hypoth-esis of two-body kinematics, where Ec.m.
in isthe available energy in the center of mass inthe entrance channel, µ is the reduced massof the primary QP-QT system, obtainedfrom the Kinematic Coincidence Method(KCM) [15] and vrel is the reconstructedprimary relative velocity between QP andQT (given by the KCM). It is well knownthat in the low energy domain the TKELis indeed the Total Kinetic Energy Loss, i.e.the amount of kinetic energy of the entrancechannel which is converted into excitationenergy of QP and QT (and rotational mo-tion); as a consequence, it is strictly corre-lated to the centrality of the reaction. Thsmaller the impact parameter, the more vi-olent the collision, with an higher degree ofdissipation of the translational kinetic en-
ergy (higher TKEL) and, as a consequence,an higher excitation of QP and QT. In theFermi energy domain, where the collision isno more strictly binary, such identificationof the TKEL with the energy dissipated inthe reaction is lost (at least partially, aswe will see later), but we can still use theTKEL as an order parameter to classify thecollisions in order of increasing centrality,as we have verified by means of a simula-tion based on the QMD model CHIMERA[16]. The results of the simulation are pre-sented in the top part of Fig.13 and theyclearly show that the relationship betweenthe TKEL and the impact parameter is ef-fectively monotonic even at Fermi energies.Moreover, the simulation told us that forperipheral and semi-peripheral collisions therelationship between the impact parameterb and the TKEL is independent of the beamenergy for a given system (see for examplethe case of the 93Nb +93 Nb at 23, 30 and38AMeV), while there is a difference whenwe move from one system (93Nb +93 Nb) toan other one (116Sn+116Sn). The differenceis of the order of 1fm.
We have also performed an experimentalestimate of the relationship between b andthe TKEL (bottom part of Fig.13) by inte-grating the experimental cross section start-ing from the elastic scattering, as in [17] and[18]; a detailed description of the adoptedtechnique is presented in [1]. The agreementbetween the results given by the experimen-tal evaluation and those obtained from thesimulation is very satisfactory.
Separation of the QP evaporation from
the midvelocity emission
The second problem to solve is how to sep-arate the midvelocity component from theQP evaporation. In order to achieve this re-sults, we take advantage of the emission pat-
236
0
2
4
6
8
10
12
b (
fm)
QMD
0
2
4
6
8
10
12
0 200 400 600 800 1000 1200 1400 1600
TKEL (MeV)
b (
fm)
↓↓↓
EXP
NbNb38NbNb30NbNb23NbNb17
SnSn38SnSn30
FIG. 13: Relationship between the impact pa-rameter (b, fm) and the TKEL. Top: resultscoming from the QMD simulation CHIMERA[16]. Bottom: experimental results. Arrows in-dicates the Ec.m.
in for each reaction. From [1].
tern of the particles on the plane (v‖, v⊥).On the base of the comparison of the experi-mental pattern with that expected for a pureevaporative emission (see Fig.2) we can as-sume that the most forward emission in theQP reference frame (origin in the QP veloc-ity, black point in the left side of Fig.14) ispurely evaporative. As a consequence, wecan separate the two components if we lookat the angular distribution of the emittedparticles with respect to the QP referenceframe (right side of Fig.14). A spin 0 sourceevaporates particles in an isotropic way; forthis reason the angular distribution in theQP reference frame displays a sine-like be-
haviour, as it is shown by the dashed-dottedcurve on the right side of Fig.14. In presenceof a non-zero spin, the emission tends toconcentrate on the reaction plane and fromthe out-of-plane distribution it is possible toestimate the spin of the source (in our case,it increases up to 30h for less peripheral col-lisions); the corresponding angular distri-bution in the QP reference frame flattensand becomes lower than a sine-like function(dotted curve on the figure), but it remainsforward-backward symmetric. Therefore itis possible to evaluate the QP evaporationstarting from the emission with θem below30 − 45 (where θem is the emission anglein the QP reference frame) and extendingit to the whole angular range following theproper curve according to the estimated spinof the QP. The midvelocity emission is ob-tained as the difference between the wholeexperimental angular distribution and theso estimated QP evaporation. With refer-ence to the right side of Fig.14, the differ-ence between the experimental distributionand the dotted curve clearly indicates thatthe midvelocity distribution extends fromthe backward region with respect to the QP(towards the center of mass) well below 90.
Particle multiplicities
Once the separation of the QP evapora-tion from the midvelocity emission has beenachieved, we can look at the particle mul-tiplicities (i.e. the average number of emit-ted particles per event) as a function of theTKEL and of the beam energy for the twoinvestigated symmetric systems. Concern-ing the QP evaporation, the obtained resultsare summarised in Fig.15. For all the par-ticle species and for all the beam energiesthe multiplicities tend to increase when thecentrality of the collision increases; this fact
237
0
20
40
60
80
-20 0 20 40 60
v⊥(mm/ns)
v// (mm/ns)
vc.m. vPLF
l
θ
a)
0
200
400
600
800
1000
1200
0 50 100 150
Yield(a.u.)
θ (deg)
l=0h-
l=30h-
expb)
FIG. 14: Left side: efficiency corrected experi-mental yields in the plane (v‖, v⊥) with respectto the QP-QT separation axis with the origin inthe center of mass reference frame; data refer tothe symmetric system 93Nb+93 Nb at 38AMeV.Right side: angular distribution of the experi-mental yields of the left side picture with v‖ ≥ 0;the emission angle is calculated with respect tothe QP velocity (black point on the left side).From [9].
is quite obvious since to a more violent colli-sion corresponds a higher excitation energyof the QP and, as a consequence, a higheramount of particle evaporation. If we com-pare the multiplicities of the 116Sn +116 Snsystem to those of the 93Nb +93 Nb sys-tem, we can observe that the emission ofthe 116Sn +116 Sn system is systematicallysmaller than that of the other system. Suchan effect, which is confirmed also by theGEMINI code, may be brought back to thehigher N/Z of the 116Sn +116 Sn system,which tends to favour the neutron evapora-tion with respect to the LCP emission.
Some interesting information on the be-haviour of the midvelocity emission can beinferred from Fig.16, where the ratio amongthe midvelocity multiplicities and the total(midvelocity plus QP evaporated) multiplic-ities is presented as a function of TKEL for
Evaporative Multiplicity
10-1
1Nb+Nb 38Nb+Nb 30Nb+Nb 23Nb+Nb 17
p
10-2
10-1
1
Sn+Sn 38Sn+Sn 30
d
10-2
10-1
t
10-1
1α
10-3
10-2
10-1
1
0 200 400 600 800 1000
IMF
TKEL (MeV)
FIG. 15: QP evaporation: experimental par-ticle multiplicities as a function of the TKELfor two symmetric systems ( 93Nb +93 Nb and116Sn +116 Sn) at different beam energies be-tween 17 and 38AMeV. From [1].
different beam energies and systems. Theratio tends to decrease in a systematic waywhen the centrality of the collision increases;as a consequence, the best environment forthe investigation of the midvelocity processis constituted by peripheral collisions. Inparticular, in such reactions, for the IMFsthe midvelocity contribution constitutes al-most the whole particle emission. The ra-tio is higher for the tritons than for the
238
deuterons and the protons: the midvelocityemission is richer in bounded neutrons withrespect to the standard QP evaporation (asobserved also in other experiments, for ex-ample [3]). At a given TKEL, the ratio in-creases when the beam energy increases andthe growth is less pronounced for more pe-ripheral collisions. The behaviour is similarfor the two investigated systems.
0.5
1 Nb+Nb 38Nb+Nb 30Nb+Nb 23Nb+Nb 17
p
0.5
1 Sn+Sn 38Sn+Sn 30
d
0.5
1
t
0.5
1
α
0.5
1
0 200 400 600 800 1000
IMF
TKEL (MeV)
FIG. 16: Ratio among the particle multiplicitiescoming from the midvelocity emission and thetotal (midvelocity plus QP evaporated) multi-plicities as a function of the TKEL for two sym-metric systems ( 93Nb +93 Nb and 116Sn +116
Sn) at different beam energies between 17 and38AMeV. From [1].
Average energy and mass balance
We have performed an average energy andmass balance for the reaction 93Nb +93 Nbat 38AMeV by disentangling the contribu-tion of the two emission components (theQP evaporation and the midvelocity emis-sion). The adopted technique, whose detailsare presented in [9], takes advantage of theextracted particle multiplicities, of the mea-sured velocities of the emitted particles andQP and of the measured secondary chargeand mass of the QP. The energy and massconservation between the entrance channeland the final one is imposed. The largestuncertainty is due to the neutron sharingbetween the midvelocity and the QP evapo-rated components (on the contrary, the to-tal multiplicities of the neutrons is muchless uncertain, since it is estimated from themass conservation adopting the hypothesisA = 2Z for the IMFs). Since the reaction issymmetric, all the contributions have beenestimated only in the region with v‖ (withrespect to QP-QT separation axis) ≥ 0. Theobtained results are presented in Fig.17 forthe QP (left column) and for the midve-locity source (right column). The first rowconcerns the average mass emitted by thesource, while the second one is relative tothe average excitation energy of the source.The main features emerging from this pic-ture are: i) the relationship between the ex-citation energy of the source and the TKELis about linear even at Fermi energies (theslope parameter is obviously smaller than0.5, since part of the available energy goesin the midvelocity emission); ii) the exci-tation energy of the midvelocity source is ofthe same order than the excitation energy ofthe QP; iii) since the mass of the QP sourceis of the order of the mass of the Nb, theenergy density of the QP is ≤ 2MeV/nucl;iv) on the contrary, since the mass of themidvelocity source, although not clearly de-
239
fined, is considerably smaller than the QPmass, the energy density of the midveloc-ity source is considerably higher: it rangesfrom 7 to 14 MeV/nucl, depending on theadopted hypothesis on the source size (wecan identify it with the emitted mass atmidvelocity (≤ 20amu) or we can includea part of the QP); such high values are wellabove the threshold for the multifragmen-tation process (3 − 5MeV/nucl, [19]). Asa consequence, from one side we can con-clude that a large amount of excitation en-ergy remains localized in the contact regionbetween QP and QT and from the otherwe can see the midvelocity emission as afirst example of multifragmentation limitedto the contact region [20].
0
10
20
30
amu
Aevap Amidv
0
100
200
0 200 400 600 800
TKEL (MeV)
MeV
Eevap
200 400 600 800
TKEL (MeV)
Emidv
FIG. 17: Average mass (top) emitted from thesource and average excitation energy (bottom)of the source for the QP (left column) and forthe midvelocity source (right column) for the re-action 93Nb +93 Nb at 38AMeV.
Comparison with GEMINI
If we compare the experimental QP evap-orated particle multiplicities to the predic-tion of the GEMINI code for a source ofthe proper excitation energy (deduced asdescribed in the previous subsection), wecan obtain a very nice agreement for theabsolute values for all the particle species(see Fig.18). Neutrons are obviously presentonly in the GEMINI data.
10-2
10-1
1
n p d t α IMFn p d t α IMFn p d t α IMFn p d t α IMF
E*=100MeV
n p d t α IMF
Gemini,L=30,A=93
n p d t α IMF
Gemini,L=0,A=93
n p d t α IMF
Gemini,L=30,A=76
n p d t α IMF
expGemini,L=30,A=93
E*=200MeV
FIG. 18: Experimental QP evaporated particlesmultiplicities (full circles) for two TKEL bins(corresponding to the excitation energy of theQP source indicated in each picture) for the sys-tem 93Nb +93 Nb at 38AMeV. Open symbolsrefer to the particle multiplicities predicted byGEMINI for a source of the same excitation en-ergy (and the proper mass). From [1].
If we look at the particle multiplicities asa function of 1/
√E∗ (where E∗ is the exci-
tation energy of the source) for the exper-imental QP evaporation and for the GEM-INI code (Fig.19), we can see that the gen-eral agreement is very good, both from thepoint of view of the general trend (which islinear in a semilogarithmic plot, as expectedfor a system ruled by statistical laws, wherethe emission probability is proportional toexp(−E∗/B); B is the emission barrier) and
240
from the point of view of the absolute valuesof the multiplicities.
10-2
10-1
1
0.06 0.08 0.1 0.12
b)
GeminiL=30 A=93
p
d
t
α
IMF
1/√E*
FIG. 19: Semilogarithmic plot of the particlemultiplicities as a function of 1/
√E∗ (where
E∗ is the excitation energy of the source) forthe experimental QP evaporation for the system93Nb +93 Nb at 38AMeV (left side) and for theGEMINI code. From [1].
These facts allow to conclude that the QPemission is fully compatible with the stan-dard evaporation of an equilibrated sourceat normal density.
A similar analysis can be applied to themidvelocity emission (with the proper ex-citation energy of the source, as estimatedfrom the energy balance); the obtained re-sults are presented in Fig.20. The generaltrend is still linear and this fact suggeststhat also the midvelocity process is ruledby statistical laws; but the particle hierar-chy is completely different with respect to
the QP emission (left side of Fig.19): forexample, there is an inversion between pro-tons and α particles and between tritons andIMFs. Moreover, the whole dynamics is in-cluded within one order of magnitude, to becompared with the three orders of magni-tude observed for the QP evaporation. Thisevidence brings to the conclusion that themidvelocity emission can not be interpretedin terms of a standard evaporation from anequilibrated source at normal density.
10-1
1
0.06 0.08 0.1 0.12 0.14
Nb+Nb 38
pd
t
α
IMF
1/√E*midv
FIG. 20: Semilogarithmic plot of the particlemultiplicities as a function of 1/
√E∗ (where E∗
is the excitation energy of the source) for the ex-perimental midvelocity emission for the system93Nb +93 Nb at 38AMeV. From [1].
A similar conclusion can be drawn if wecompare the N/Z ratio for the Hydrogen iso-topes coming from the QP evaporation tothat obtained for the midvelocity emission(Fig.21). While the ratio for the QP emis-sion (full points) is in substantial agreementwith the prediction of the GEMINI code(non-continuous lines), i.e. with what weexpect for the standard evaporation froma source at normal density, the ratio ob-tained for the midvelocity part is consider-ably higher. This is a further confirmationof the richness in bounded neutrons of themidvelocity emission.
241
0
0.2
0.4
0.6
0.8
1
0 200 400 600 800 1000
N/Z for Z=1Nb+Nb 38AMeV
exp mid-velocity
exp PLF-emission
GeminiL=30,20,0
TKEL (MeV)
N/Z
FIG. 21: N/Z for the Hydrogen isotopes for thesystem 93Nb +93 Nb at 38AMeV: open pointsmidvelocity emission, full points QP evapora-tion; uncontinuous lines refer to different GEM-INI calculations. From [1].
Estimate of the time scale of the
midvelocity process
In order to estimate the time scale asso-ciated to the midvelocity process, we havetried to reproduced the experimental emis-sion pattern of the IMFs for peripheralcollisions (where the IMF emission comes,almost completely, from the midvelocitysource) by means of a three-body Coulombtrajectory calculation including two heavyfragments (QP and QT) and an IMF. Re-sults are presented in Fig.22 as yields on the(v‖, v⊥) plane. In the framework of this sim-ulation, experimental data (d) can be verywell reproduced only if we couple an emis-sion from the middle of QP and QT (a) de-veloping over times of the order of 100fm/c(compatible with the neck rupture mecha-nism in the first phase of the reaction) to alater emission (∼ 200fm/c) from the pos-sibly deformed surface of QP and QT (b).This latter process can be seen as an evolu-tion of the fast oriented fission process [17]for extreme mass asymmetries. More details
on the used simulation can be found in [8].
0
50Mid-vel.
a)
v perp
(m
m/n
s)
Surfaceb)
0
50
-50 0 50
Mid-vel. + Surfacec)
-50 0 50
Expd)
vpar (mm/ns)
10
10 2
10 3
-50 0 50
yiel
d
vpar (mm/ns)
e)
0 25 50 75
f)
vperp (mm/ns)
FIG. 22: a), b) and c): simulations based on athree-body Coulomb trajectory calculation aimedto reproduce the experimental d) emission pat-tern of the IMFs for peripheral collisions for thereaction 116Sn +93 Nb at 29.5AMeV; the pre-sented pictures are yields on the (v‖, v⊥) plane.e) and f): v‖ and v⊥ distributions obtained fromthe pictures a)-d). From [8].
The existence of a midvelocity surfaceemission is furtherly confirmed by the ex-perimental kinetic energy spectra of par-ticles emitted around 90 in the QP ref-erence frame (first raw of Fig.23). It isvery clear the presence of two components,which can be fitted simultaneously with twoMaxwellian-shaped curves with very differ-ent inverse slope parameters. The compo-nent with smaller slope parameter (the sloperanges between 2 and 4MeV and it increaseswith the TKEL) can be easily identified withthe standard QP evaporation, since the ob-tained value of the slope is equal (within theerrors) to that obtained for forward emit-ted particles in the QP reference frame (sec-ond raw of Fig.23), where, as we have seen,
242
only the QP evaporation contribution is ex-pected. The second component shows anslope parameter of the order of 8-10MeV forthe Hydrogen isotopes and a higher value(about 12-13MeV) for α particles; the trendis substantially constant as a function ofTKEL for all the particles. In the frame-work explained in this work, we interpretthis second component as due to an emission(on a faster time scale with respect to thestandard QP evaporation) from the locallyhot and highly excited surface region of theQP which, in the first phase of the collision,was in contact with the QT. This explana-tion is in agreement with the previous ob-servation, coming from the energy balance,that the excitation energy is strongly local-ized in the contact region.
cou
nts
10
210
310 °-95°=85θprotons
TKEL=450-550MeV
°-95°=85θα
TKEL=550-650MeV
(MeV)kinE0 20 40 60 80
cou
nts
10
210
310 °-25°=5θprotons
TKEL=450-550MeV
(MeV)kinE0 20 40 60 80 100 120
°-25°=5θα
TKEL=550-650MeV
FIG. 23: Experimental kinetic energy spec-tra for protons (left column) and α particles(right column) for the system 93Nb +93 Nb at38AMeV. First row refers to particles emittedbetween 85 and 95 in the QP reference frame;second raw refers to particles emitted between5 and 25 in the QP reference frame.
CONCLUSIONS
In this work we have presented a sum-mary of the physical analysis developed bythe FIASCO experiment in the past eightyears, concerning the characterization of pe-ripheral and semi-peripheral heavy ion col-lisions at Fermi energies; in particular, wefocused on the investigation of the LCP andIMF emission.
We separated the two contributions whichcan be identified in the particle emissionpattern, i.e. the QP emission and the mid-velocity contribution. We investigated theirevolution as a function of the centrality ofthe reaction (estimated from the TKEL)and of the beam energy (between 17 and38AMeV ). From the comparison with theprediction of the GEMINI code we have seenthat the QP emission can be very well de-scribed in terms of standard evaporationfrom an equilibrated source at normal den-sity. On the contrary, the midvelocity emis-sion shows a very different behaviour fromthe point of view of particle multiplicities(see, for example, the N/Z ratio for the Hy-drogen isotopes or the general trend as afunction of 1/
√E∗). As a consequence, the
midvelocity emission is not an evaporativeprocess from an equilibrated source at nor-mal density; it may be of statistical nature,after a dynamical phase responsible for thesource formation.
Moreover, the midvelocity emission itselfcan be seen as a two component process: aprompt emission from the central region be-tween QP and QT on very fast time scales(∼ 100fm/c) reminding of the neck rupturemechanism in the first phase of the reac-tions, and a later emission from the possiblydeformed surface of QP and QT, which canbe interpreted as an evolution of the fast ori-ented fission process for extreme mass asym-metries.
An extremely clear evidence for the ex-
243
istence of this surface emission comes fromthe kinetic energy spectra of particles emit-ted around 90 in the QP reference frame:they clearly show the presence of two com-ponents with very different slope parame-ters; the softer one can be identified with thestandard QP evaporation, while the harderone may come from the locally hot surface ofthe QP, whose excitation is due to the con-tact with the QT in the first phase of thecollision.
The energy density is strongly localizedin the contact region between QP and QTand according to the fact that its value forthe midvelocity source is greater than thethreshold for the multifragmentation pro-cess, we can see the midvelocity emission asa first appearance of the multifragmentationphenomenon limited to the contact zone.
As last remark, we must observe thatperipheral collisions are the best environ-ment for the investigation of the midveloc-ity process; in fact from one side we havethe largest midvelocity-to-evaporative ratioin the particle emission and from the otherthe relative velocity between QP and QT ismaximal and therefore the separation of themidvelocity contribution from the QP/QTevaporation is easier.
Many thanks are due to all the per-manent and temporary members of theFIASCO collaboration (A.Mangiarotti,P.R.Maurenzig, A.Olmi, M.Bini, G.Casini,G.Pasquali, G.Poggi, A.A.Stefanini,N.Taccetti, L.Bardelli, A.Bartoli, L.Bidini,C.Coppi, S.Poggi, E.Vanzi); in particular toP.R.Maurenzig, A.Olmi and A.Mangiarottiwho contributed in a significant way to thepresented analysis.
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Conference Proceedings Vol. 96
“The Nuclear Physics from the f7/2 to the Quark - Gluon Plasma”
F. Gramegna, M. Cinausero, D. Fabris (Eds.)
SIF, Bologna 2008
ULTRARELATIVISIC NUCLEUS-NUCLEUS COLLISIONS: STATUS AND
PERSPECTIVES
F. Antinori
Dipartimento di Fisica and INFN Padova, Italy
ABSTRACT
The study of ultrarelativistic heavy-ion collisions has become one of the centre-stage subjects in
nuclear physics. The first round of discoveries at CERN-SPS has been followed by a series of
exciting new results from RHIC-BNL. I give a bird’s-eye overview of the current status of the field
and of the perspectives for the jump to the LHC energy.
INTRODUCTION
Despite its remarkable quantitative successes, the Standard Model (SM) of particle physics still presents us with a few puzzles. Two reside in the strong interaction sector of the SM; they have to do with the phenomenon of confinement and with the generation of the masses of the hadrons: i) one-half of the fundamental fermions of
the SM – the six quarks – are not observable as free particles: they seem to be permanently confined inside hadrons. We think that this behaviour derives from the properties of Quantum Chromo-Dynamics (QCD), but of this there is actually no rigorous proof
ii) most of the mass of the hadrons is unaccounted for in terms of those of their valence quarks. If, for instance, we add together the current masses of the three quarks making up a proton, we account for only 1% or so of the proton’s mass, How about the remaining 99%?
The two puzzles are generally thought to be related – the mechanism that confines the quarks to the interior of hadrons is presumably responsible for the generation of the bulk of the hadrons’ mass as well – and to originate in the non-perturbative behaviour of QCD.
The prime experimental tool for the exploration of this region of the SM is provided by ultrarelativistic nucleus-nucleus collisions. In this presentation, I will try to give a short overview of where we stand today in this relatively young and very lively field of nuclear physics, which had Prof. Ricci as one of its early backers in Italy, and to illustrate some of the
perspectives for the field’s near future.
THE QCD PHASE DIAGRAM AND AA
COLLISIONS
In QCD, non-perturbative problems are treated by discretization on a space-time lattice. This allows to avoid ultraviolet (i.e. large momentum scale) divergences, and to recover finite results. Lattice QCD predicts that as the temperature and/or the baryon density of a system of hadrons is increased, the confining effects of strong interaction will at some point disappear, as the individual, colourless hadrons dissolve into a Quark-Gluon Plasma (QGP), where coloured quarks and gluons can freely roam. As an example, figure 1 shows the predicted behaviour of the energy density ε of a strongly interacting system with 3 active quark flavours and zero net baryon density as a function of the system’s temperature T [1]. The energy density, divided here by the T
4 factor of the Stefan-Boltzmann
law, is proportional to the number of degrees of freedom in the system. A rapid rise is seen as the temperature crosses a critical value TC, estimated to be around 170 MeV (in units where the Boltzmann constant k is set equal to 1), due to the activation of the partonic degrees of freedom, much more numerous than the hadronic ones. The energy density at T = TC is expected to be of the order of the GeV/fm
3.
In the deconfined phase, the quark masses are expected to go down from the effective, constituent value they take inside hadrons to the current value of the fundamental Lagrangian, thereby restoring, at least partially, the chiral
245
symmetry which is normally broken in the world of hadrons.
Ultrarelativistic collisions of heavy nuclei allow us to reach values of the energy density in that range, over a relatively extended strongly interacting system, thereby opening up a window for the experimental exploration of the phenomenology of confinement and chiral symmetry breaking.
Fig. 1: Energy density (divided by T
4) versus
temperature (in units of critical temperature) from a lattice calculation with 3 active flavours and zero net baryon number.
SPS: THE EARLY EVIDENCE
The first pieces of evidence for the formation of partonic matter where collected at the CERN Super Proton Synchrotron (SPS) accelerator, with collisions of lead nuclei.
After a first round of experiments with relatively light ions (oxygen and sulphur), an upgrade of the CERN SPS accelerator facility allowing the acceleration of heavy ions was approved in 1990. It involved the construction of a new facility upstream of the Proton Synchrotron Booster (PSB) and modifications to the remaining existing accelerator chain, by a collaboration between CERN and external laboratories (figure 2) [2]. In particular, the Low Energy Beam Transport (LEBT) line and the Radio Frequency Quadrupole (RFQ), accelerating ions to 250 keV/u (figure 3) were built by Laboratori Nazionali di Legnaro (with Prof. Ricci very much supporting the whole operation). The CERN Heavy-Ion Facility started operating in 1994. In total, 9 experiments collected data between 1994 and 2003, with a spectrum of
different physics focuses (photons, low mass dileptons, particle spectra, interferometry, strange particles, high mass dileptons, charmonium, …) and experimental techniques (silicon microdetectors, time projection chambers, photon detectors, muon chambers, Cherenkov detectors, to name but a few).
The programme was a success. A harvest of results was reaped on many features of the new, peculiar strongly interacting system formed in Pb-Pb collisions at a centre-of-mass energy per nucleon-nucleon collision NNs = 17.3 GeV. Doing justice to the outcome of such a rich physics programme would be largely beyond the scope of the present paper. I will concentrate on two topics only: the hyperon enhancements and the J/ȥ suppression, two of the oldest, historic proposed signatures of deconfinement.
Fig. 2: Scheme of the complex of the CERN Heavy-Ion Facility. As briefly discussed above, deconfinement into the QGP phase is believed to be accompanied by a partial restoration of chiral symmetry. For the strange quark this implies a reduction of the value of the mass from around 500 MeV to about 150 MeV. This is comparable with the estimated value of the deconfinement temperature: copious production of strange quark-antiquark pairs, enhanced with respect to elementary collisions, is therefore expected in the QGP [3,4]. This enhancement is predicted to be stronger for particles containing multiple strange quarks, which can be built at the hadronization stage by recombining s quarks produced in independent microscopic reactions [5].
In the QGP phase the interaction potential is expected to be screened for distances larger than a certain value (the Debye length λD), analogously to what happens in an electromagnetic plasma. As a consequence, it is
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predicted that charmonium ( cc ) and bottomonium ( bb ) states with a radius larger than λD will not bind, and their production in the plasma will be suppressed [6]. The value of λD, and therefore which quarkonium states will be suppressed, depends on the temperature.
Fig. 3: Layout of the first stages of the CERN Heavy-Ion Facility. Fig. 4: Hyperon enhancements in Pb-Pb collisions relative to p-Be collisions at the SPS, as a function of the collision centrality (number of wounded nucleons).
Enhancements in the production of hyperons [7], increasing with the hyperon’s strange quark content (figure 4), and an anomalous suppression of the production of the J/ȥ charmonium state [8] (figure 5), were both observed at the SPS. Prof. Ricci was involved in the discovery of the hyperon enhancements, as a member of the WA97 experiment. When these and other results from the SPS lead ion programme are pieced together, the emerging picture is that of a strongly collective system, with a very large
pressure buildup and signature features – like the hyperons enhancements and charmonium suppression patterns discussed above – predicted to characterize the behaviour of a partonic system. Fig. 5: Observed J/ȥ suppression at the SPS (divided by the amount of suppression expected from nuclear absorption) as a function of the collision’s energy density.
HIGHLIGHTS FROM RHIC
The next jump in the field was the coming online in the year 2000 of the Relativistic Heavy Ion Collider (RHIC) at the Brookhaven National Laboratory on Long Island. Built specifically for heavy-ions, RHIC extended by one order of magnitude the centre-of-mass collision energy reach for nucleus-nucleus collisions, to NNs = 200 GeV. Four dedicated experiments were built around the collider’s ring. The programme quickly started pouring out an impressive stream of results. Here, again, I will only mention a few. Perhaps the most spectacular RHIC result was the observation of high-pT suppression. In the absence of medium effects, the production of particles at high transverse momentum (pT) in nucleus-nucleus collisions is expected to scale like the number of binary nucleon-nucleon collisions in the reaction. This can be checked by computing the nuclear modification factor RAA, as the ratio of the particle yields per nucleon-nucleon collision in nucleus-nucleus and proton-proton collisions. As shown in figure 6, approximate scaling of charged particle production at high pT with the number of nucleon-nucleon collisions (RAA ~ 1) is seen for the most peripheral gold-gold collision events (60-80%). For central collisions,
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however, a strong suppression is observed [9]. When looking at two-particle azimuthal correlations using a high-pT “trigger” particle (figure 7), a clear back-to-back jet correlation peak is visible at 180 degrees in pp and deuteron-gold collisions. In central Au-Au collisions, however, the peak has disappeared [10]. These effects can be explained in terms of energy loss of the partons as they attempt to traverse the strongly interacting medium formed in the collision. It looks as though particles created close to the medium boundary manage to escape, while the rest are strongly absorbed in the medium (“jet quenching”). Fig. 6: Nuclear modification factor RAA for the production of charged particles at RHIC, as a function of transverse momentum. Fig. 7: Two-particle correlations at RHIC: distribution of the distance in azimuth from a “trigger” particle – selected with 4 < pT < 6 GeV/c – of associated particles with pT > 2 GeV/c.
One of the early puzzles emerging from RHIC data had to do with the production of baryons at medium pT. Figure 8, for instance, shows the proton, kaon and pion pT spectra in Au-Au collisions at NNs = 200 GeV. Fig. 8: RHIC transverse momentum spectra for pions, kaons, protons and antiprotons, for central (top) and peripheral (bottom) collisions. For central collisions, as many protons as ʌ+
and as many antiprotons as ʌ− are found to be produced at high pT [11]. When looking at the nuclear modification factor Rcp (figure 9; Rcp is calculated in a similar way as RAA, but relative to peripheral Au-Au instead than to pp collisions), it looks like high transverse momentum proton production is not suppressed [12], contrary to what is observed for pions. Fig. 9: Nuclear modification factors Rcp for protons and neutral pions at RHIC. How could this be if the suppression was due to parton energy loss? How would the partons
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“know” if they would end up generating pions or protons? An important clue came with the measurement of the Rcp factors for 0
SK and ȁ [13], which extended the comparison of baryon and meson production to higher transverse momenta (figure 10) than was initially possible for pions and protons. Lambdas, too, were found to be eventually suppressed; only it looked like the effect for them was shifted to a higher pT with respect to kaons.
Fig. 10: Nuclear modification factors Rcp for neutral kaons and lambdas at RHIC. Two different peripheral centrality classes are used in the Rcp definition ( top and bottom plots). Such a behaviour finds a natural explanation within valence quark recombination/coalescence models [14]: if hadrons are formed by recombining quarks from the partonic phase, one expects features of the parton spectrum, such as a suppression at high pT, to end up at different places in the transverse momentum spectrum of mesons and baryons, with momentum scaling factors of 2 and 3 for mesons and baryons respectively, as determined by their respective number of valence quarks/antiquarks. This is in good agreement with the pattern observed in the data. Strong support for the recombination picture came also from the study of the azimuthal dependence of particle production. Due to strong collective expansion effects, for non-central events the distribution of the produced particles retains a memory of the initial azimuthal asymmetry of the nucleus-nucleus collision. This is quantified by measuring the second coefficient
(v2) in the Fourier transform of the azimuthal distribution of particle production. The behaviour of v2 as a function of pT appears – again – to be different for baryons and mesons (figure 11), but the two sets of measurements can be reconciled if both the v2 and the transverse momentum are divided by the number of valence quarks in the hadron (figure 12) [13, 15], as expected, again, if hadron formation in this pT region is dominated by recombination effects.
Fig. 11: Azimuthal asymmetry parameter v2 for strange particles at RHIC.
Fig. 12: v2/n as a function of pT/n for mesons and baryons at RHIC. n being the number of valence quarks/antiquarks.
After the first pieces of evidence for deconfinement where collected at the SPS (incidentally, very similar results on both hyperon enhancements and J/ȥ suppression were later found also at RHIC), RHIC provided us with new evidence for partonic behaviour with the discovery of the valence quark recombination
STAR
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counting rules, and opened up the way to the study of the medium properties with high energy probes with the discovery of high pT suppression.
THE FUTURE: LHC
The Large Hadron Collider (LHC), planned to come online at CERN next year, while designed primarily for the study of proton-proton collisions at s = 14 TeV, will also allow to collide heavy ions. The centre-of-mass energy per nucleon-nucleon collision for the lead-lead system is NNs = 5.5 TeV. With the LHC, a new quantum jump is anticipated, into a region where new, hard probes, such as heavy flavours and fully developed jets will become accessible with high statistics. Here, again, I will limit myself to a few examples, to give a flavour of the physics potential expected at the next machine.
Jet quenching is predicted to be different for heavy and light partons. In the BDMPS framework [16], parton energy loss is calculated in QCD, and found to be mainly due to gluon radiation by bremsstrahlung. The average energy loss for a parton propagating in a QCD medium is computed to be proportional to the parton’s Casimir factor, which measures its colour charge (4/3 for quarks and 3 for gluons), leading to a larger suppression for light hadrons, originating predominantly from gluon jets, than for heavy flavoured hadrons, produced in quark jets. Within the quark sector, then, heavy quarks are predicted to lose less energy than light quarks, due to the so-called dead cone effect, whereby a massive parton cannot lose energy by radiating gluons below a minimum angle, determined by the parton’s mass/energy ratio [17, 18]. Heavy-flavoured particles are therefore expected to be overall less “quenched” than the light-flavoured ones.
The study of the production of heavy flavour in nucleus-nucleus collisions is already being undertaken at RHIC, mainly relying on the extraction of “non-photonic electron” spectra, i.e. electron spectra where the contribution from photon conversions and light hadron decays has been subtracted. When the nuclear modification factor RAA is calculated for such electrons, their suppression seem to be as strong as that of light hadrons (figure 13) [19] contrary to the theoretical expectations discussed above. Attempts at reconciling data and theory are being made, for instance by considering the possibility of a reduced contribution from beauty production, although beauty decays would in
principle be expected to dominate non-photonic electron spectra above a few GeV of pT. Since, due to their lower mass, c quarks are thought to lose more energy than their b counterparts because of the dead-cone effect discussed above, if the production of non-photonic electrons at RHIC were dominated by charm decays across the accessible pT range, it would indeed still be possible to recover some agreement with the theory [20].
Fig. 13: RAA for non-photonic electrons at RHIC as a function of pT. The high pT suppression for charged hadrons (hashed band) and the predictions from various quenching models assuming only c or both c and b contributions are shown for comparison.
Experimentally, this is a rather complicated matter, since the RHIC experiments are not currently equipped with microvertex detectors, which – besides providing an experimental cross-check as to the heavy flavour origin of the non-photonic electron spectra – would allow a separate measurement of their b and c components.
Heavy flavours will be abundantly produced at the LHC, with over a hundred cc pairs and a few
bb pairs per central Pb-Pb collision predicted [21]. ALICE, the LHC experiment dedicated to the study of heavy-ion collisions, is equipped with a silicon pixel microvertex detector (see [22] at this workshop). Good performance for heavy flavour measurements in general and in particular for the b/c separation is anticipated, making it possible to explore the properties of the system with well calibrated probes (see [23] at this workshop).
High energy jets will also be abundantly produced at the LHC [21]. On average, about one 20 GeV jet per central Pb-Pb event is foreseen; even for jet energies as large as 200 GeV, the
non phot.
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estimated statistics is still good: about 100,000 per months at nominal luminosity. Such jets should be well visible even among the large background of low momentum particles of central Pb-Pb collisions at the LHC. The jet fragmentation function, which quantifies the fraction z of the parton’s original momentum ending up in the produced hadrons, is expected to be modified relative to the vacuum case by the parton’s propagation through the medium [24], as shown, for instance, in figure 14 [25] (where the variable ξ = ln(1/z) is used). This is a crucial measurement, for which, again, good performance is expected in ALICE (see figure 14), providing us with yet another tool for exploring the properties of deconfined matter.
Fig. 14: Expected ALICE performance (triangles) for the measurement of the ratio of the fragmentation functions for central (modified) and peripheral (taken to be unmodified) collisions for jets with a mean energy around 125 GeV, as a function of ξ = ln (1/z). The ideal case of perfect jet reconstruction is shown as a histogram. The modification of the fragmentation function was calculated using quenching weights [26] with a medium transport coefficient q = 50 GeV2/fm. R is the jet cone radius. Figure from [25].
CONCLUSION
As was originally hoped, after over a decade of experiments at the SPS and RHIC, good evidence has been collected for the creation of an extended partonic system in the collision of ultrarelativistic heavy ions. As the field matures and prepares for the jump to yet a higher energy regime, the focus is now moving to the study of the properties of this new state of matter, thought to have been that of our Universe a few
microseconds after the Big Bang. The ALICE experiment at the LHC is well equipped to carry on such an ambitious physics programme. Sure enough Professor Ricci, a long-time member of the ALICE Collaboration, is still involved.
[1] U. Heinz, Nucl.Phys. A 685 (2001) 414 [2] N. Angert et al., CERN 93-01 (1993) [3] J. Rafelski, Phys. Rep. 88 (1982) 331 [4] J. Rafelski and B. Müller, Phys. Rev. Lett. 48 (1982) 1066 [5] P. Koch et al., Phys. Rep. 142 (1986) 167 [6] T. Matsui and H. Satz, Phys. Lett. B 178 (1986) 416 [7] E. Andersen et al., Phys. Lett. B 449 (1999) 401 [8] M.C. Abreu et al., Phys. Lett. B 410 (1997) 337 [9] J. Adams et al., Phys. Rev. Lett. 91 (2003) 172302 [10] C. Adler et al., Phys. Rev. Lett 90 (2003) 082302 [11] S.S. Adler et al., Phys. Rev. C 69 (2004) 034909 [12] S.S. Adler et al., Phys. Rev. Lett. 91 (2003) 172301 [13] J. Adams et al., Phys. Rev. Lett. 92 (2004) 052302 [14] See e.g.: R.J. Fries, J. Phys. G 30 (2004) S853 and refererences therein [15] J. Castillo et al., J. Phys. G 30 (2004) S1207 [16] R. Baier et al., Nucl. Phys. B483 (1997) 291 [17] Yu L. Dokshitzer and D.E. Kharzeev, Phys. Lett. B 519 (2001) 199 [18] N. Armesto et al., Phys. Rev. D 69 (2004) 114003 [19] B.I. Abelev et al., Phys. Rev. Lett 98 (2007) 192301 [20] N. Armesto et al., Phys. Lett. B 637 (2006) 362 [21] ALICE Collaboration: Physics Performance Report, Vol. II, J. Phys. G 32 (2006) 1295 [22] S. Moretto, this workshop [23] A. Dainese, this workshop [24] N. Borghini and U.A. Wiedemann, arXiv: hep-ph/0506218 [25] F. Antinori et al., J. Phys. G 34 (2007) S511 [26] C.A. Salgado and U.A. Wiedemann, Phys. Rev. D 68 (2003) 014008
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Conference Proceedings Vol. 96
“The Nuclear Physics from the f7/2 to the Quark - Gluon Plasma”
F. Gramegna, M. Cinausero, D. Fabris (Eds.)
SIF, Bologna 2008
PHYSICS PROGRAM OF THE ALICE EXPERIMENT AT THE LHC
A. Dainese, for the ALICE Collaboration
INFN, Laboratori Nazionali di Legnaro, viale dell’Università 2, 35020 Legnaro (Padova), Italy
1. INTRODUCTION
ALICE [1,2] is a general-purpose heavy-ion experiment designed to study the physics of high-density strongly interacting matter in nucleus–nucleus collisions at the CERN Large Hadron Collider (LHC) at a centre-of-mass energy of 5.5=NNs TeV per nucleon–nucleon collision, for the Pb-Pb system. In these collisions, a system with an energy density hundreds of times larger than that of ordinary atomic nuclei is expected to be produced. Under these conditions, the formation of a thermally-equilibrated medium characterized by partonic, rather than hadronic, degrees of freedom (the so called Quark-Gluon Plasma, QGP) is predicted by the theory of strong interactions (Quantum Chromodynamics, QCD). A discussion on the evidences for QGP formation collected in past and present heavy-ion experiments at CERN-SPS and BNL-RHIC, as well as a description of the most relevant observables for the characterization of the state of strongly-interacting matter formed in high-energy nucleus-nucleus collisions, can be found in Ref. [3].
The ALICE detector has been designed to cope with the highest particle multiplicities among those anticipated for Pb–Pb collisions (dNch/dy up to 8000) and it will be operational at the start-up of the LHC, now expected in summer 2008 with proton–proton (pp) collisions at 14=s TeV. In addition to heavy-ion systems, the ALICE Collaboration will study collisions of lower-mass ions, which are a means of varying the energy density of the system formed in the collision, and protons (both pp and proton–nucleus), which primarily provide reference data for the nucleus–nucleus collisions. In addition, the pp data will allow for a number of genuine pp physics studies.
We briefly summarize the ALICE Physics list in section 2. In section 3 we describe the ALICE experimental setup, and in section 4 we outline
the strategy for event reconstruction, giving some of expected performance figures. In the following sections, we go through the main points of the ALICE Physics program.
2. ALICE PHYSICS LIST AND
OBSERVABLES IN A NUTSHELL
• Energy density of the hot and dense system produced in the collision å measurement of the charged-particle multiplicity and charged-particle rapidity density.
• Temperature and baryon density of the system at the chemical freeze-out and temperature at the kinetic freeze-out å measurement of identified-particle yields (probe chemical freeze-out) and momentum spectra (probe kinetic freeze-out).
• Hadronization mechanism of the system: interplay between quark recombination from a partonic medium and parton fragmentation outside the medium å measurement of the baryon-to-meson ratios as a function of momentum and rapidity.
• Size of the hot particle-emitting source å HBT interferometry with identical bosons (Bose-Einstein correlations).
• Pressure-driven expansion of the system, to be compared to hydrodynamical models å measurement of radial flow and elliptic flow (azimuthal particle production anisotropy in non-central collisions).
• Fluctuations induced by the QCD phase transition å measurement of event-by-event
particle spectra • Effect of parton energy loss via medium-
induced gluon-radiation on heavy quarks (charm and beauty): dependence of energy loss on the parton colour charge (c quarks vs.
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gluons) and on the parton mass (b quarks vs. c quarks) å measurement of transverse momentum spectra of D and B mesons.
• Quarkonium (charmonium and bottomonium) suppression by dissociation due to colour screening in a deconfined medium vs. charmonium enhancement by parton recombination in a charm-rich medium å measurement of charmonium and bottomonium yields.
• Initial temperature of the QGP via thermal photons from the medium å measurement of the transverse momentum spectrum of single photons.
• Effect of parton energy loss on jet structure and jet fragmentation function å measurement of reconstructed jets and photon-tagged jets (provide initial jet energy calibration).
3. ALICE DETECTOR LAYOUT
The detector (see Fig. 1) consists of a central barrel, which measures hadrons, electrons and photons, and of a forward spectrometer to measure muons. The central barrel, which covers polar angles from 45
o to 135
o over the full
azimuth, is embedded in the large L3 solenoidal magnet providing a magnetic field of up to 0.5 T.
Fig. 1: Layout of the ALICE experimental setup.
It consists of: an Inner Tracking System (ITS)
with six cylindrical layers of high-resolution silicon detectors, among which two layers of Silicon Pixel Detectors (SPD) [4]; a cylindrical Time-Projection Chamber (TPC); a single-arm electromagnetic calorimeter (PHOS); and three particle identification arrays of: Time-Of-Flight (TOF) detector, Transition Radiation Detector (TRD), and a single-arm ring imaging Cherenkov (HMPID). The forward muon arm (covering polar angles 171
o–178
o) consists of a
complex arrangement of absorbers, a large dipole magnet, and fourteen planes of tracking and triggering chambers. Several smaller detectors (ZDC, PMD, FMD, T0, V0) for global event characterization and triggering are located at forward angles. An electro-magnetic calorimeter (EMCAL) for jet measurements and jet triggering, covering one third of the central barrel azimuthal acceptance and its full polar acceptance, will be added in 2009-2010.
4. TRACK RECONSTRUCTION AND
PARTICLE IDENTIFICATION
The primary vertex of the collisions is found using the clusters reconstructed in the two innermost ITS layers, made of the Silicon Pixel Detector (SPD) [3]. In central Pb–Pb collisions, the vertex position is reconstructed with a precision of about 5 たm in the beam direction and about 25 たm in the transverse plane. For pp collisions, the precision on the vertex position is about one order of magnitude worse. However, due to the very low track multiplicity in pp events, this deterioration of the vertex precision does not have a significant impact on the reconstruction of physics signals, such as charm and beauty particle decays.
The track finding in the central detectors starts in the TPC. For tracks with a sufficient number of hits and transverse momentum pt above 0.2 GeV/c, the TPC track-finding efficiency is almost 100%, even for the charged-particle densities of central Pb–Pb collisions. The effective TPC track-finding efficiency is lower, around 85% (and around 90% for tracks with pt above 1 GeV/c), because of particle decays and the dead zones between the TPC sectors. The momentum resolution of tracks reconstructed in the TPC is about 0.7% (at pt = 1 GeV/c and the magnetic field 0.5 T), and the specific energy loss (dE/dx) resolution is about 6%. These resolutions depend only slightly on event multiplicity.
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The tracks reconstructed in the TPC are then prolonged to the ITS. Using the ITS measurements, the track impact-parameter (distance of closest approach to the primary vertex) resolution is improved to 60 たm for 1 GeV/c tracks in central Pb–Pb collisions (see Fig. 2). As we will show in section 10, such resolution, mainly provided by the two layers of Silicon Pixel Detectors at r = 4 and 7 cm, allows a good performance for the reconstruction of charm and beauty decay vertices, displaced by a few hundred μm from the primary vertex.
Fig. 2: Track impact parameter resolution in the directions transverse (rφ) and parallel (z) to the beamline, for different particle species, as a function of the transverse momentum pt [2].
Including the ITS measurements and, to a lesser extent, also the TRD data in the track reconstruction significantly improves the momentum resolution at high pt; at pt = 100 GeV/c the momentum resolution is around 3.5% in magnetic field B = 0.5 T. However, in this case the effective tracking efficiency is reduced to about 60%, because of particle absorption in the TRD and in the support structure.
In the last step, the reconstruction algorithm searches for secondary vertices from strange particle decays (V0’s: K
0S→π+π−,
Λ0→pπ−; cascades: Ξ-→Λ0π−, Ω-→Λ0Κ−) and
kinks (i.e. charged pion or kaon decays on the flight, like K
+→μ+νμ). The V0 and cascade decays are reconstructed within the fiducial volume between 1 cm from the primary vertex and the TPC inner radius (85 cm). Typical reconstruction efficiencies are 60% for K
0S’s,
40% for Λ’s, and 5% for Ξ’s. The kinks are
reconstructed inside the TPC in the fiducial volume 120 < r < 220 cm. The kink reconstruction efficiency for charged kaon decays is about 70% in pp collisions and about 40% in central Pb–Pb collisions for kaons with pt up to 20 GeV/c.
The identification of charged hadrons is done by combining the PID information provided by the ITS, TPC, TDR, TOF, and HMPID detectors. The efficiency of the PID algorithm is above 95% up to p = 6 GeV/c for pions, above 60% up to p = 3 GeV/c for kaons, and above 70% up to p = 5 GeV/c for protons, in all cases the contamination with wrongly-identified particles is below 30%. The overall effective PID efficiency is limited by particle decays and absorption in the material. It is about 50% for pions and protons, and about 40% for kaons, integrated over momentum. Electrons with momentum above 1 GeV/c are identified by the TRD with the efficiency above 90% and with the pion-rejection factor of about 100.
The PHOS spectrometer detects and identifies photons with high energy and position resolutions. In the low-momentum range, below 20 GeV/c, the direct-photon spectrum is obtained by subtracting, from the overall identified-photon spectrum, the contribution from decay photons, mainly from the light neutral mesons. The yields of these mesons are measured by an invariant-mass analysis. In the high-momentum range, above 20 GeV/c and up to 100 GeV/c, direct photons are identified on an event-by-event basis, by the shower-shape and the isolation-cut discrimination techniques. The identification efficiency for photons (0.5 GeV < E < 40 GeV) in pp collisions is above 90%. In central Pb–Pb collisions this efficiency is above 50%. The contamination from misidentified particles (electrons, charged hadrons, long-lived neutral mesons, neutrons and antineutrons) remains below 3%. For even higher-energy photons (40 GeV < E < 120 GeV) the detection efficiency decreases to about 40%, however, the contamination from non-resolved π0→γγ is smaller than 10%.
The Photon Multiplicity Detector (PMD) counts photons in the forward pseudorapidity region 2.3 < η < 3.5. The photon-reconstruction efficiency is a function of the pseudorapidity with a maximum of 70% at η = 2.6. The purity of the sample of reconstructed photons is above 60% in the whole pseudorapidity range.
The reconstruction quality in the muon arm depends on the level of the background. However, even for the worst background
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scenario (using the pile-up of two highest multiplicity events), the muon-arm track-finding efficiency is about 95% and the resolution in the reconstructed ϒ (bottomonium) mass is better than 100 MeV/c
2, thus allowing the separation of
the three states ϒ, ϒ’ and ϒ’’.
5. COLLISION CHARACTERIZATION
The initial geometry of the collisions is determined by measuring the global event properties. This measurement allows also to study how the available centre-of-mass energy is redistributed in phase space.
The collision geometry can be estimated using several observables. One way is to use the information from the Zero-Degree Calorimeters (ZDCs). The number Npart of participant nucleons in the collision (Npart
≈ 400 in central Pb–Pb) is determined with the resolution σNpart = 15, roughly independent of centrality.
The charged-particle multiplicity and the charged-particle pseudo-rapidity distribution, which is related to the energy density of the system formed in the collision, can be measured over almost 8 units in pseudorapidity, by means of the Forward Multiplicity Detector (FMD), and of the innermost layers of the ITS (SPD). A simplified tracking algorithm will be used in the ITS to measure multiplicity in a robust way, defining ‘tracklets’ by associating clusters of hits in the two SPD planes. In Pb–Pb collisions, the charged-particle multiplicity is measured with very good accuracy for all centralities. In the mid-rapidity region, even for very peripheral events, the resolution on multiplicity is better than 10%, and it becomes progressively smaller for more central collisions.
6. PARTICLE PRODUCTION
The comprehensive measurements of particle ratios and momentum spectra are an important part of the ALICE physics program. They are important both in the low-pt region, where a thermal and chemical analysis of the system freeze-out conditions is the main aim, and at intermediate and high pt, where the role of radial flow, quark recombination, and, eventually, hard processes, becomes apparent.
Figure 3 illustrates the expected coverages in pt for the different identified particles, for one month of data taking at nominal LHC luminosity
with Pb-Pb. By combining the information from different
PID detectors, stable charged hadrons (pions, kaons, and protons) can be identified and measured from very low momentum (hundreds of MeV) up to at least 50 GeV. Secondary vertices are used to identify charged and neutral kaons as well as hyperons up to, and beyond 10 GeV. Baryon production will be measured in the central region (p, Λ0
, Ξ-, Ω-
, and their anti-particles) to study the baryon number transfer in rapidity both in Pb–Pb and pp collisions.
Resonances bring additional information about the final stages of the collision. Three resonances have been investigated so far, the ρ0
, the K0*,
and the φ. In addition to production spectra, ALICE will be able to measure to some extent variations in the resonance parameters (mass, width, line shape), which may arise from the restoration of chiral symmetry.
Fig. 3: Expected pt ranges for identified particles (one month Pb-Pb at nominal luminosity) [2].
7. TWO-PARTICLE INTERFEROMETRY
(HBT)
The space–time geometry of the particle-emitting source created in ultra-relativistic heavy-ion collisions can be studied by the analysis of two-particle intensity interferometry (HBT).
ALICE will contribute to the existing results of HBT analysis in heavy-ion collisions as well as open the possibility for new analysis, such as direct-photon interferometry or event-by-event HBT analysis. Data from the LHC may help to clarify the ‘RHIC HBT puzzle’ (the expected increase with collision energy of the size of the particles source is not seen in the experimental data) by extending the excitation function to
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much higher energy and particle multiplicities, and by making precise measurements of the shape and the anisotropy of the particle-emitting source as given by azimuthally-sensitive HBT analysis. It will also extend the existing investigations to a larger number of different hadron species, which will help to better understand the particle emission, and therefore the geometry and evolution of the system.
8. FLOW
High-accuracy measurements of anisotropic flow are very important for understanding the dynamics of the heavy-ion collisions at the LHC.
The determination of the reaction plane, a prerequisite for the measurement of anisotropic flow, will benefit from the possibility to be done independently by the different subsystems of the ALICE detector, and by different analysis methods. At mid-rapidity, making use of the elliptic flow signal (v2), we will be able to determine the reaction plane for a very wide range of particle multiplicities and magnitudes of the elliptic flow. At beam-rapidity, using the directed flow signal (v1), we will get an independent determination of the reaction plane from the ZDCs.
The expected precision of the reaction-plane determination will allow for anisotropic flow measurements with unprecedented accuracy for both charged and identified particles in a momentum range from a few hundred MeV/c up to well above 10 GeV/c. These measurements are expected to provide constraints on the equation of state (low pt, below 2 GeV/c), collective motion of the constituent quarks (intermediate pt, 2-7 GeV/c), and path-length dependence of the in-medium parton energy loss (high pt, above 7 GeV/c).
9. EVENT-BY-EVENT FLUCTUATIONS
Fluctuations of thermodynamic quantities are fundamental to the study of the QGP phase transition.
The ALICE experiment is well suited to precise event-by-event measurements of various observables: temperature fluctuations, multiplicity and strangeness fluctuations, fluctuations of conserved quantities including net-charge fluctuation, balance functions, fluctuation in azimuthal anisotropy, fluctuation
in space–time parameters from correlation measurements.
Fluctuations in these observables can be studied in order to understand the physics of bulk properties of matter as well as high-pt particles and jets. Recent lattice QCD calculations have shown that interesting fluctuation patterns might be present also at the small chemical potential, which will prevail at LHC energies.
10. CHARM AND BEAUTY
LHC is the first machine where heavy quarks will be produced abundantly in heavy-ion collisions. The study of heavy-flavour production in both pp and nucleus–nucleus collisions down to almost zero transverse momentum will allow a sensitive comparison with QCD predictions and a study of the in-medium energy loss of heavy quarks compared to massless partons (light quarks and gluons).
Fig. 4: Sketch of the D0→K−π+ decay (top) and example of K−π+ invariant-mass distribution after applying the selection cuts, in central Pb–Pb events, after the subtraction of the combinatorial background in the insert (bottom) [2].
The benchmark decay channel D0→K
−π+ has
π
pointing angle θpointing
secondary vertexprimary vertex
D reconstructed momentum 0
D flight line0
d
d
0
0
K
K
π
impact parameters ~100 mµ
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been studied in detail. Figure 4 shows a sketch of the decay topology and an example K
−π+
invariant-mass distribution in central Pb–Pb collisions, as expected after applying the secondary-vertex selection cuts. In one LHC year at nominal luminosity, we expect to cover, in |η| < 0.9, the transverse-momentum range 1 GeV/c < pt < 18 GeV/c in central Pb–Pb collisions and 0.5 GeV/c < pt < 18 GeV/c in pp and pPb collisions, with statistical errors smaller than 15–20% at high pt in all cases.
Beauty production in central Pb–Pb collisions can be measured via semi-leptonic decays. Identified electron tracks displaced from the primary vertex provide a measurement of the b-hadron cross section above a given pt
min . As
shown in Fig. 5, ALICE can cover the range 2 GeV/c <pt
min < 30 GeV/c (in |η| < 0.9) with
statistical errors of order 10% or less. Single muons and opposite-sign dimuon pairs allow a measurement of open-beauty production with high statistics in the forward pseudorapidity region −4 < η < −2.5 in the transverse-momentum range 2 GeV/c < pt
min < 22 GeV/c.
Fig. 5: Expected performance for the reconstruction of the B-meson production cross section as a function of pt
min, using the semi-electronic decay channel, in one month of Pb–Pb data taking. The statistical errors (inner bars) and combined statistical and systematic errors (outer bars) are shown. The predicted B-meson suppression due to b-quark energy loss in the hot and dense medium is also shown [2].
Additional channels are currently under investigation, such as D
+ reconstruction,
electron–muon and multi-muon correlations,
beauty production via displaced J/ψ’s from B decays and the perspectives for the measurement of W-boson-decay muons (which will be useful as a medium-blind reference to study the in-medium energy loss of heavy flavour).
11. QUARKONIA
At LHC, the complete spectrum of heavy quarkonia states (J/ψ, ψ’, ϒ, ϒ’, and ϒ’’) is accessible and will allow a very detailed study of both suppression phenomena (due to deconfinement, which should affect members of both the charm and beauty family) and possible enhancement (due to recombination, significant only for the charmonium states).
Quarkonia are detected in ALICE at mid-rapidity (−0.9 < η < 0.9) in the di-electron channel, and at backward rapidity (−4.0 < η < −2.5) in the di-muon channel.
Fig. 6: Di-electron (e+e-) invariant-mass spectrum for central Pb-Pb collisions, as expected to measured in the central rapidity region (|η|<0.9) in one month of Pb–Pb data-taking. The uncorrelated (combinatorial background) is not subtracted in the figure [2].
The expected performance is illustrated by the
di-lepton invariant-mass spectra shown in Figs. 6 (di-electrons) and 7 (di-muons).
In the central-rapidity region, the J/ψ production cross section will be measured down to pt = 0 GeV/c in the minimum-bias data sample. The data triggered with high-pt electrons have the pt threshold for J/ψ acceptance of about 5 GeV/c. The production of ϒ states is measured over the full transverse-momentum range in both minimum-bias and triggered data samples.
[GeV/c]mintB p
0 5 10 15 20 25 30
) [m
b]m
int
> p
t/d
y (p
B NN
σd
-610
-510
-410
-310
-210
= 5.5 TeVNNsPb-Pb, 0-5%, e+X→B
/fm2 = 25--100 GeVq
= 0bm
= 4.8 GeVbm
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Fig. 7: Di-muon (μ+μ-) invariant-mass spectrum for central Pb–Pb collisions, as expected to measured in the backward rapidity region (-4<η<-2.5) in one month of Pb–Pb data-taking. The uncorrelated (combinatorial background), evaluated from like-sign combinations, has been subtracted in the figure [2].
The mass resolutions are σm = 30 MeV/c2 for
the J/ψ and σm = 80 MeV/c2 for the ϒ. About
105 J/ψ and 10
3 ϒ will be measured in central Pb–Pb collisions during one year of data taking.
Quarkonia measured at forward rapidity allow measurement of parton distributions at x values as small as 10
−5. The modest transverse-
momentum cut on single muons applied at the trigger level extends quarkonia detection down to zero transverse momentum. The number of detected J/ψ is about 7×10
5 per year, allowing
for a detailed study of J/ψ production as a function of centrality and transverse momentum. Similar studies can be carried out for the ϒ, but with significant statistical errors, since the expected yearly statistics is of about 10
4 ϒ’s.
12. PHOTONS
Direct prompt photons at high pt allow the study of hard processes in the dense medium without any final-state modification. In the low-pt domain, thermal photons trace the thermal evolution of the system and, in particular, of the hot and early phase of the reaction.
The photon spectrum will be measured in ALICE with the PHOS spectrometer. Hard photons will be identified on an event-by-event basis using shower-shape and isolation-cut analyses. In this energy domain, the systematic errors due to misidentified neutral mesons will be of the order of a few per cent. Statistics will limit the measurement in the high-energy part of the spectrum to about 100 GeV both in pp and in Pb–Pb collisions. Prompt photons will be used to tag charged jets emitted in the opposite direction in order to study jet-fragmentation functions
(Fig. 8). In-medium modification of the fragmentation function will be measured with an accuracy of the order of a few per cent (Fig. 9).
Various correlations, such as photon–hadron and photon–photon correlations will provide additional information on the medium modified di-jet structure.
In the low-energy domain direct photons will be identified as an excess of identified photons (with shower-shape analysis) when compared with the spectrum of decay photons
Fig. 8: Photon-tagged jet measurement. The photon provides a measurement of the energy of the parton that originates the jet, thus allowing to study the in-medium modification of the jet energy.
The systematic error on the measurement of the excess will be about 8%. This excess has several origins, including thermal photons from the QGP and hadron gas, photons generated by fast partons traversing the medium, and prompt photons. Various correlations, such as photon–hadron and photon–photon correlations will provide additional information on the medium modified di-jet structure. In the low-energy domain direct photons will be identified as an excess of identified photons (with shower-shape analysis) when compared with the spectrum of decay photons. The systematic error on the measurement of the excess will be about 8%. This excess has several origins, including thermal photons from the QGP and hadron gas, photons generated by fast partons traversing the medium, and prompt photons
259
Fig. 9: Expected performance of the measurement of the nuclear modification, in Pb–Pb (medium) with respect to pp (no medium) collisions, of the fragmentation function of photon-tagged jets. The expected error bars are reported on the curve (RFF = 1) expected if jets are not affect by the medium. The curve below shows the expected modification induced by energy loss (quenching) in the medium: RFF > 1 for z close to 0, RFF << 1 for z close to 1.
13. JET PHYSICS
The properties of the hot and dense medium produced in nucleus–nucleus collisions can be studied via the energy loss experienced by fast partons in the medium (jet quenching). The highest sensitivity to the medium properties is expected when measuring the longitudinal and transverse fragmentation functions of jets both at large and at small relative momentum fraction z.
In central Pb–Pb collisions at LHC, jet rates within the ALICE acceptance are sufficient to map out the energy dependence of jet fragmentation over a very wide kinematic range, up to Et = 200 GeV. However, jet reconstruction in nuclear collisions has to cope with the large background from the underlying event, therefore, jet reconstruction has to be limited to small cone sizes ( 22 ηφ Δ+Δ=cR ) in the range 0.3 < Rc < 0.5. In addition, a transverse momentum cut in the range 1 GeV/c < pt < 2 GeV/c has to be applied to reduce the background. As a consequence, even for perfect calorimetry, the energy resolution is limited to ΔEt/Et = 20%.
To study the ALICE performance, jets with energies in the range from 20 GeV to 200 GeV have been embedded into simulated Pb–Pb events and passed through the full detector
simulation and reconstruction chain. The energy spectrum and jet-structure observables are reconstructed and compared to unmodified jets as measured in pp collisions. Only for cone energies below 50 GeV, fake jets do influence the quality of the reconstruction, as shown in Fig. 10.
In its initial design, ALICE can measure only the charged particles within the jets, limiting the jet-energy resolution to 40–50%. Nevertheless, at high Et, charged-jet reconstruction is shown to be much superior to studying high-pt parton fragmentation using leading particles only, because the bias in the fragmentation function is significantly reduced. Fig. 10: Jet energy spectrum reconstructed with charged tracks only (no calorimetry) in one month of Pb–Pb data taking. The upper curves represents the input spectrum, the lower curve the spectrum reconstructed in a simulation without the Pb–Pb background, the markers represent the spectrum reconstructed in a simulation with the full Pb–Pb background, that causes the reconstruction of fake jets below 50 GeV.
Whereas the high-pt and high-jt (momentum
transverse to the jet axis) regions of the leading parton remnants are essentially background free and will be measured very well in ALICE, the spectra of particles originating from radiated gluons have to be extracted mostly from kinematic regions, where background dominates the signal (S/B = 10
−1-10
−2). In such domain the
low-pt tracking capabilities of ALICE are essential and unique, and allow a study of this region (including PID information) on a statistical basis.
In the low-Et-jet region, jet-structure modifications will be studied with inclusive
260
spectra of identified particles and particle correlations, as shown by the RHIC experiments. These studies require excellent low-pt and PID capabilities and ALICE will extend them to heavy-ion collisions at the LHC.
The planned electromagnetic calorimeter (EMCAL) for ALICE (2009-2010) will improve the jet-energy resolution, increase the selection efficiency and further reduce the bias on the jet fragmentation. Furthermore, it will add a jet trigger which is needed to increase the statistics at high Et. The low- and high-transverse-momentum tracking capabilities combined with electromagnetic calorimetry represent an ideal tool for jet-structure modification studies at the LHC over a wide kinematic region of jet and associated-particle momenta.
14. CONCLUSIONS
In summary, the ALICE detector will allow us to study the properties of strongly-interacting matter in extreme conditions and to enjoy Nuclear Physics at the highest energies.
ACKNOWLEDGEMENTS
The author warmly thanks the organizers of the Workshop for inviting him to give this presentation.
[1] ALICE Collaboration, Physics Performance Report, Volume 1, J. Phys. G30 (2004) 1517. [2] ALICE Collaboration, Physics Performance Report, Volume 2, J. Phys. G32 (2006) 1295 [3] F. Antinori, these proceedings. [4] S. Moretto, these proceedings.
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Conference Proceedings Vol. 96
“The Nuclear Physics from the f7/2 to the Quark - Gluon Plasma”
F. Gramegna, M. Cinausero, D. Fabris (Eds.)
SIF, Bologna 2008
THE SILICON PIXEL DETECTOR FOR ALICE EXPERIMENT
Sandra Moretto
on behalf of ALICE SPD collaboration
Dipartimento di Fisica dell’Universitá and INFN Sezione di Padova, I-35131 Padova, Italy
INTRODUCTION
ALICE (A Large Ion Collider Experiment) is
an experiment under construction at the CERN
Large Hadron Collider (LHC) optimized for the
study of ultra-relativistic nucleus-nucleus
collisions, at a center-of-mass energy of 5.5 TeV
per nucleon. The prime aim of the experiment is
to study in detail the behavior of nuclear matter
at extreme densities and temperatures, in view of
probing deconfinement and chiral symmetry
restoration. For a recent description of the
ALICE experimental apparatus see ref. [1]. The
Inner Tracking System (ITS) [2] will provide
precise tracking information close to the
interaction point. It consists of six concentric
layers of three different types of silicon
detectors, within a radius of about 44 cm: two
innermost layers of Silicon Pixel Detectors
(SPD), two layers of Silicon Drift Detectors
(SDD) and two layers of Silicon Strip Detectors
(SSD). The secondary vertexing capability of the
SPD will allow the detection of charm and
beauty hadrons which are of particular interest to
probe the formation of deconfined matter [3].
An overview of the SPD system and of its
integration inside the ALICE detector is
presented.
THE ALICE SILICON PIXEL DETECTOR
The SPD consists of two barrel layers of hybrid
Silicon Pixel Detectors, mounted on a carbon
fiber support, placed around the beam line at
radii of 3.9 cm and 7.6 cm, respectively. In the
following we describe the main components of
the SPD and how they have been assembled.
The ladder
The heart of the SPD is the ladder, which is an
assembly of a 200 μm thick p+n silicon sensor
flip-chip bonded to five readout chips. In the
following we will use the cylindrical coordinates
as reference system, with the z axis along the
beam direction. The silicon sensor is a matrix
with an active area of 12.8 mm (rφ) x 70.7 mm
(z), arranged in 256 rows (rφ) x 160 columns (z)
of pixels. The size of each pixel is 50 μm (rφ) x
425 μm (z). Each pixel is bump-bonded to a
contact of the ALICE1LHCb read-out chip, a
mixed analogue-digital signal chip developed in
a 0.25 μm CMOS technology, radiation hardened
by design layout [4]. Each chip, 150 μm thick,
contains 8192 readout cells arranged in 256 rows
and 32 columns. Five chips are bump-bonded to
each ladder. A modular test system was
developed based on LabView and VME, which
allows to test individual bare front-end pixel
chips as well as single flip-chip bonded chips and
ladders [5].
Half-Stave
The basic module of the SPD is the Half-Stave
(HS), that is made of two ladders mounted
together, along the beam direction, one
grounding foil, an Al-polyimide 5-layer bus and
a multi-chip-module (MCM). An Al-Kapton foil,
70 μm thick, is glued to the chip side of the
ladder to provide the proper grounding of the
Half-Stave and an electrical shielding with
respect to the mechanical carbon-fiber support.
An Al-polyimide 5-layer bus is glued on the
sensor side of the ladder. The bus incorporates
control and data lines and is connected to the
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front-end read-out chip and to the MCM by
ultrasonic wire-bonding, as shown in figure 1.
The MCM, that carries auxiliary read-out and
control signals, is placed at one end of the Half-
Stave. All signals to and from the counting room
are transmitted via optical fibers. The alignment
constraints and the proper gluing are crucial for
the wire-bonding, consequently the micrometric
alignment of the components with respect to
each other relies on a Mitutoyo coordinate
measuring machine and have been carried out in
a Clean Laboratory.
Fig. 1: The SPD Half-Stave layout and a sketch of
the wire-bonding connections.
The Sector
Two Half-Staves are coupled together to form
a Stave. The Staves are glued on a 200 μm thick
Carbon Fiber Support Sector (CFSS), each sector
carries 6 staves: 4 for the outer layer and 2 for
the inner layer. Ten CFSS are mounted around
the beam line and constitute the mechanical
support of the SPD barrel. Since the front-end
chips may generate a heat load up to 20-25 W
per Stave, to remove the total power dissipated in
the front-end electronics, an evaporative C4F10
based cooling system has been adopted to
maintain the SPD at constant temperature. To
this end the Sectors are equipped with cooling
ducts, made of Phynox, embedded in the CFSS.
Due to the strong requirements on relative
positioning of the components, to the severe
material budget constrains and to fragile nature of
the components, the Sector assembly has
required the development of specific tools and
mounting techniques for the manipulation of all
the components. A dedicated system for the
assembly has been mounted on the working
plane of a JOHANSSON TOPAZ Measuring
Machine, placed in a Clean Laboratory. The
mechanical coupling is obtained by fixing the
Half-Staves directly to the CFSS by means of
UV-curable glue tags and carbon fiber clips for
the outer layers. The thermal coupling between
the Half-Stave and the cooling duct is ensured by
means of thermal grease pads.
Fig. 2: The first Half-Barrel assembled.
Half-Barrel and SPD
Five Sectors have been assembled together to
form an Half-Barrel, as shown in figure 2. Two
Half-Barrels mounted face-to-face around the
beam pipe form the entire SPD, as shown in
figure 3 in which the SPD is mounted on a
specific mechanical support for the final
assembly tests. Due to the severe thermal
stability requirements of the Silicon Drift
Detectors, positioned just outside the SPD barrel,
a thermal shield surrounds and isolates the SPD
volume. The shield is made of two halves, each
consisting of a half-cylinder and a half-cone. It
provides mechanical protection during the
installation procedures and also the structural
support for the final assembly around the beam
pipe.
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Integration
The integration of the SPD around the beam
pipe, inside the ITS, and the installation
procedures have been quite complex. The
presence of the ALICE forward muon arm
complicates the access to the area of the inner
detectors, moreover a minimum distance
between the closest SPD component and the
beam pipe of only 5 mm and the delicate cooling
system connections give additional constrains.
For these reasons the installation procedure is a
sequence of many delicate operations, which
have been first tested with the aid of a 3D CAD
modeling and then performed, in all the details,
in the laboratory before the final installation.
Fig. 3: The entire SPD mounted at CERN.
CONCLUSIONS
The commissioning of the ten Sectors has been
done and the integration of the whole SPD has
been completed. The installation of the SPD in
the ALICE experimental hall and all the cabling
of the detector have been completed. At the
present date the start of the commissioning of the
SPD is scheduled for October 2007.
[1] ALICE Physics Performance Report Vol. I, J.
Phys. G: Nucl. Part. Phys. 30 (2004) 1517.
[2] ITS Technical Design Report, CERN-LHCC 99
12, 1999.
[3] ALICE Physics Performance Report Vol. II, J.
Phys. G: Nucl. Part. Phys. 32 (2006) 1295.
[4] K. Wyllie et al., Front-end pixel chips for tracking
in ALICE and particle identification in LHCb,
Proceeding of PIXEL 2002 Conference, SLAC
Electronic Conference Proceedings, Carmel, USA,
September 2002.
[5] P.Riedler et al., Nucl. Instr. Meth. A568 (2006)
284.
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