symmetry breaking in the pseudogap state and fluctuations about it schematic universal phase diagram...

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breaking in the Pseudogap state and Fluctuations a Schematic Universal phase diagram of high- Schematic Universal phase diagram of high- T T c superconductors superconductors Marginal Marginal Fermi-liquid Fermi-liquid Fermi liquid Fermi liquid T x (doping) x (doping) T* T* Crossover Crossover QCP I II SC III A F M “Pseudo- Gapped” 1. Symmetry and Topology in Region II of the phase diagram? Why no specific heat singularity at T*(x)? 2. Quantum critical fluctuations in Region I. (with Vivek Aji) 3. D-wave pairing.

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Page 1: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

Symmetry breaking in the Pseudogap state and Fluctuations about it

Schematic Universal phase diagram of high-Schematic Universal phase diagram of high-TTcc superconductorssuperconductors

MarginalMarginalFermi-liquidFermi-liquid

Fermi liquidFermi liquid

TT

x (doping)x (doping)

T*T*CrossoverCrossover

QCP

III

SCIII

AFM

“Pseudo- Gapped”

1. Symmetry and Topology in Region II of the phase diagram? Why no specific heat singularity at T*(x)?2. Quantum critical fluctuations in Region I. (with Vivek Aji)3. D-wave pairing.

Page 2: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

Two Principle Themes in the work:

1. Fluctuations due to a Quantum critical point determine the normal state properties as well as leads to superconductivity.2. Cuprates are unique and this is due to their unique solid state Chemistry. A microscopic theory should be built on a model which represents this solid state chemistry.

Page 3: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

AntiferromagnetismAntiferromagnetismMarginal Marginal

Fermi liquidFermi liquid

Fermi liquidFermi liquid

x (doping)x (doping)

T*T*CrossoverCrossover

CPQ

TF€

∝ sgn(ω) , for ωc ff ω ff T.

Phenomenology(1989): Properties in Region I follow if there exists a Quantum Critical Point with scale invariant fluctuations given by

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I

II

SC

From approximate Inversion of ARPES and Optical conductivity: Pairing glue has spectrumconsistent with this. Deriving these fluctuations may be considered the central problem.

Page 4: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

II I

AntiferromagnetismAntiferromagnetism

SuperconductivitySuperconductivity

Pseudogapped metalPseudogapped metal

Marginal Marginal Fermi liquidFermi liquid

Fermi liquidFermi liquid

TT

x (doping)x (doping)

T*T*CrossoverCrossover

CPQ

Broken Symmetry?

Quantum Critical Point in high Tc crystals

If there is a QCP, there might be an ordered phase emanating fromit on one side and a Fermi-liquid below another line emanating from it.

Page 5: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

Microscopic Model:

cu

o

o

Cannot be reduced to a Hubbard Model because the ionization energyof Cu is nearly the same as the ionization energy of oxygen.

Why are Cuprates Unique? (1987)

Page 6: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

Look for symmetry breaking not ruled out by ExperimentsPreserve translational symmetry: severely limits possible phases;

Bond Decomposition of near neighbor interactions.

Page 7: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

Only Possible States not changing Translational and Spin-Rotational symmetries have order parameters:

Time-Reversal and some Reflection Symmetries lost.

Page 8: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

Experiments to look for time-reversal breaking in the pseudogap phase;

Dichroism in Angle-Resolved Photoemission:

Experiment by Kaminski et al. (2002);

Direct Observation by Polarized neutron Diffraction

(Bourges et al. 2005).

Page 9: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

Kaminski et al., Nature (2002)

Dichroism in BISCCO

Page 10: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

Fauques et al. (2005): Polarized Elastic Neutron Scattering in underdoped and overdoped Y(123)

Page 11: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

Fauques et al. (2005):

Polarized Neutron diffraction in YBCuO

Magnetic Diffraction Pattern consistent withLoop Current Phase II just as Dichroic ARPES

Page 12: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

Classical Stat. Mech. Model for the observed Loop Current Phase

Four states per unit-cell.

Why no specific heat singularity at T*(x)?

Time-reversal and 3 of four reflections broken:

Two Ising degrees of freedom per unit-cell

Ashkin-Teller Model :

Observed broken symmetry for -1 < J4/J2 < 1.

Phase diagram obtained by Baxter; Kadanoff et al.

Page 13: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

Phase Diagram of the Ashkin-Teller Model (Baxter, Kadanoff)

Gaussian line

Page 14: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

Specific Heat for the relevant region: (Hove and Sudbo)

Page 15: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

AntiferromagnetismAntiferromagnetism

SuperconductivitySuperconductivity

Marginal Marginal Fermi liquidFermi liquid

Fermi liquidFermi liquid

x (doping)x (doping)

T*T*CrossoverCrossover

CPQ

TF€

∝ sgn(ω) , for ωc ff ω ff T.

Quantum critical Fluctuations : Fluctuations of the order parameter which condenses to give broken symmetry in Region II.

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I

II

SC

Very simple but peculiar Phenomenology:

Page 16: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

Quantum Critical Fluctuations:

Vivek Aji, cmv (Preprint soon)

AT model:

is equivalent by to

Replace constraint with a four-fold anisotropy term

Same classical criticality as AT model. Constraint irrelevant abovethe critical line and relevant below.Add quantum-mechanics: Moment of Inertia plus damping due to Fermions.Model is related to 2+1 dim. Quantum xy models with dissipation.

Page 17: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

Critical Region:Need not consider anisotropy term.For simplicity keep only the xy-term.

Fourier transformed dissipation: Derivable from elimination of current-current coupling of collective modes to fermions:

Without dissipation model is 3d xy ordered at T=0.We also assume J such that it is ordered at finite T of interest.Wish to examine region where dissipation disorders the phase.

Page 18: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

Previous work on the dissipative xy model:

Nagaosa (1999); Tewari, Chakravarti, Toner (2003),…

Below a critical value of , dissipation destroys long range orderat T=0. But no calculation of correlation functions, connection with vortex fluctuations or connection with the classical transition.

Page 19: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

Steps in the derivation:

lives on the bonds of the lattice

2.

1.

3.

i i+x

i+y

Page 20: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

. .

Velocity field due to: decreases as 1/r.

Velocity field due to: spatially independent

Time-independent Time-dependent

Page 21: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

Action in terms of , (schematically):

+ terms which are not singular when integrated over k and omega.

Partition function splits into a product of a space-dependentpart and a time-dependent part. Problem transforms to a K-T problem in space and (mathematically) a Kondo problem in time.

A remarkable simplification which allows a solution!

Page 22: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

RG equations for fugacity y for instantons and for , similar toflows in the Kondo problem or the KT problem:

Instanton field does the disordering:

Page 23: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

Calculate order parameter correlation functions: At

Associate variation of with change in doping. This is then a theory ofcritical fluctuations at x=x_c as a function of temperature.

Gaussian Model : No corrections?

For , proliferates and disorders the velocity field.

This was the Phenomenological Spectrum proposed in 1989 to explainThe anomalous normal state (Marginal Fermi-liquid) and suggested asthe glue for pairing. Fluctuations are of current loops of all sizes and directions.

Crossover for

Page 24: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

Coupling of Fluctuations to Fermions and pairing vertex

k k+q

g(k, k+q)

Leading deviations from MFT allow this calculation:From this calculate Pairing Vertex:

g g

Decompose into different IR’s:S-wave and p-wave are repulsiveD-wave and X-S are attractive,Just as in the old calculation(Miyake, Schmitt-Rink, cmv) for AFMFluctuations.Right energy scale and coupling constant for Tc.Answers why self-energy ind. of q but d-wavePairing.

Inversion of ARPES indicates a broad featureless spectrum is the glue.

Page 25: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

AntiferromagnetismAntiferromagnetism

SuperconductivitySuperconductivity

Marginal Marginal Fermi liquidFermi liquid

Fermi liquidFermi liquid

x (doping)x (doping)

T*T*CrossoverCrossover

CPQ

TF€

∝ sgn(ω) , for ωc ff ω ff T.

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I

II

SC

Summary: It is possible to understand different regions of the phase diagram of the cuprates with a single idea. Interesting Quantum criticality. Probably relevant in several othercontexts. A Possible Theory for the Cuprates if the symmetry breaking in Region II is further confirmed.

Page 26: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

Spectra and thermodynamics in the underdoped cuprates.

BUT, A time-reversal violating state with a normal Fermi-surface is not possible: (PRL (99); PR-B(06))

Quasi-particle velocity ---->

For fluctuations of non-conserved discrete quantities, damping of fluctuations and their coupling of fermions to fluctuations is finite for .

This leads to single-particle self-energy

Time-reversal violation alone does not lead to observed properties.

Observed Phase must be accompanied by a Fermi-surface Instability.

Page 27: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

To see what can happen, look at the same issue as it arisesin another context.

Pomeranchuk Expansion of the free-energy for distortions of theFermi-surface

But

So, no symmetry change possible in the channel

But something must happens since specific heat cannot be allowed to be negative. Look at

0<z<1. Therefore instability due to diverging velocity.

What cures the instability?

Page 28: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

Approach to the Instability

Suggests a state with an anisotropic gap at the chemical potential:

No change in Symmetry, only change in Topology of the Fermi-surface

Page 29: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

Have found a stable state (PRL-99, PRB- 06)with

Ground state has only four fermi-points. No extra change in symmetry, just in topology, (Lifshitz Transition).

is coupling of flucts. at q = 0 to the fermions at the F.S.

Page 30: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

Kanigel et al. (2006) : Define “Fermi-arc length” as the set of angles for which at any , the spectral function peaks at the chemical potential for compounds with different x. The data for 6 underdoped BISCO samples scales with T*(x) and shows four fermi-points as T --->0.

Page 31: Symmetry breaking in the Pseudogap state and Fluctuations about it Schematic Universal phase diagram of high-T c superconductors MarginalFermi-liquid Fermi

Compare calculated “Fermi-arc length” with Experiments(Lijun Zhu and cmv- 2006)

using the spectrum derived plus self-energy calculated using only kinematics. Same D_0/T_g gives the

measured Specific Heat and Magnetic Susceptibility.