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Step-scan time-domain terahertz magneto-spectroscopy D. Molter, 1,2,G. Torosyan, 1 G. Ballon, 3 L. Drigo, 3 R. Beigang, 1,2 and J. L´ eotin 3 1 Fraunhofer Institute for Physical Measurement Techniques IPM, Department of Terahertz Measurement and Systems, Erwin-Schroedinger-Str., Building 56, 67663 Kaiserslautern, Germany 2 University of Kaiserslautern, Department of Physics and Research Center OPTIMAS, Erwin-Schroedinger-Str., Building 46, 67663 Kaiserslautern, Germany 3 Laboratoire National des Champs Magn´ etiques Intenses, UPR 3228, CNRS-UJF-UPS-INSA, 143 avenue de Rangueil, 31400 Toulouse, France [email protected] Abstract: We present a novel approach for terahertz time-domain spectroscopy of magneto-optic phenomena. The setup used in this work combines a tabletop pulsed magnet and a standard terahertz time-domain spectroscopy system. The approach is based on repetitive operation of the pulsed magnet and step-wise increment of the delay time of the time-domain spectroscopy system. The method is demonstrated by plotting the magneto-transmission spectra of linearly polarized THz pulses through the hole gas of a Ge sample and the electron gas of GaAs, InSb and InAs samples. Cyclotron resonance spectra are displayed in the frequency range from 200 GHz to 2 THz and for a magnetic field up to 6 T. The GaAs spec- tra are analyzed in more detail using simulations based on the Drude model. © 2012 Optical Society of America OCIS codes: (300.6495) Spectroscopy, terahertz; (230.3810) Magneto-optic systems. References and links 1. D. Some and A. Nurmikko, “Real-time electron cyclotron oscillations observed by terahertz techniques in semi- conductor heterostructures,” Appl. Phys. Lett. 65, 3377–3379 (1994). 2. S. A. Crooker, “Fiber-coupled antennas for ultrafast coherent terahertz spectroscopy in low temperatures and high magnetic fields,” Rev. Sci. Instrum. 73, 3258–3264 (2002). 3. X. Wang, D. J. Hilton, L. Ren, D. M. Mittleman, J. Kono, and J. L. Reno, “Terahertz time-domain magnetospec- troscopy of a high-mobility two-dimensional electron gas,” Opt. Lett. 32, 1845–1847 (2007). 4. X. Wang, A. A. Belyanin, S. A. Crooker, D. M. Mittleman, and J. Kono, “Interference-induced terahertz trans- parency in a semiconductor magneto-plasma,” Nat. Phys. 6, 126–130 (2010). 5. X. Wang, D. J. Hilton, J. L. Reno, D. M. Mittleman, and J. Kono, “Direct measurement of cyclotron coherence times of high-mobility two-dimensional electron gases,” Opt. Express 18, 12354–12361 (2010). 6. Y. Ikebe, T. Morimoto, R. Masutomi, T. Okamoto, H. Aoki, and R. Shimano, “Optical Hall Effect in the Integer Quantum Hall Regime,” Phys. Rev. Lett. 104, 256802 (2010). 7. T. Arikawa, X. Wang, D. J. Hilton, J. L. Reno, W. Pan, and J. Kono, “Quantum control of Landau-quantized two- dimensional electron gas in a GaAs quantum well using coherent terahertz pulses,” Phys. Rev. B 84, 241307(R) (2011). 8. J. Kono, “Cyclotron Resonance,” in Methods in Materials Research, E. N. Kaufmann, ed. (John Wiley & Sons, New York, 2001). 9. D. Molter, F. Ellrich, T. Weinland, S. George, M. Goiran, F. Keilmann, R. Beigang, and J. L´ eotin, “High-speed terahertz time-domain spectroscopy of cyclotron resonance in pulsed magnetic field,” Opt. Express 18, 26163– 26168 (2010). #161190 - $15.00 USD Received 10 Jan 2012; revised 17 Feb 2012; accepted 17 Feb 2012; published 27 Feb 2012 (C) 2012 OSA 12 March 2012 / Vol. 20, No. 6 / OPTICS EXPRESS 5993

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Page 1: Step-scan time-domain terahertz magneto …nanojapan.rice.edu/Downloads/Papers/2012_Leotin_Optical Society_THz...Step-scan time-domain terahertz magneto-spectroscopy ... then give

Step-scan time-domain terahertzmagneto-spectroscopy

D. Molter,1,2,∗ G. Torosyan,1 G. Ballon,3 L. Drigo,3

R. Beigang,1,2 and J. Leotin3

1Fraunhofer Institute for Physical Measurement Techniques IPM,Department of Terahertz Measurement and Systems,

Erwin-Schroedinger-Str., Building 56, 67663 Kaiserslautern, Germany2University of Kaiserslautern, Department of Physics and Research Center OPTIMAS,

Erwin-Schroedinger-Str., Building 46, 67663 Kaiserslautern, Germany3Laboratoire National des Champs Magnetiques Intenses, UPR 3228, CNRS-UJF-UPS-INSA,

143 avenue de Rangueil, 31400 Toulouse, France∗[email protected]

Abstract: We present a novel approach for terahertz time-domainspectroscopy of magneto-optic phenomena. The setup used in this workcombines a tabletop pulsed magnet and a standard terahertz time-domainspectroscopy system. The approach is based on repetitive operation ofthe pulsed magnet and step-wise increment of the delay time of thetime-domain spectroscopy system. The method is demonstrated by plottingthe magneto-transmission spectra of linearly polarized THz pulses throughthe hole gas of a Ge sample and the electron gas of GaAs, InSb and InAssamples. Cyclotron resonance spectra are displayed in the frequency rangefrom 200 GHz to 2 THz and for a magnetic field up to 6 T. The GaAs spec-tra are analyzed in more detail using simulations based on the Drude model.

© 2012 Optical Society of America

OCIS codes: (300.6495) Spectroscopy, terahertz; (230.3810) Magneto-optic systems.

References and links1. D. Some and A. Nurmikko, “Real-time electron cyclotron oscillations observed by terahertz techniques in semi-

conductor heterostructures,” Appl. Phys. Lett. 65, 3377–3379 (1994).2. S. A. Crooker, “Fiber-coupled antennas for ultrafast coherent terahertz spectroscopy in low temperatures and

high magnetic fields,” Rev. Sci. Instrum. 73, 3258–3264 (2002).3. X. Wang, D. J. Hilton, L. Ren, D. M. Mittleman, J. Kono, and J. L. Reno, “Terahertz time-domain magnetospec-

troscopy of a high-mobility two-dimensional electron gas,” Opt. Lett. 32, 1845–1847 (2007).4. X. Wang, A. A. Belyanin, S. A. Crooker, D. M. Mittleman, and J. Kono, “Interference-induced terahertz trans-

parency in a semiconductor magneto-plasma,” Nat. Phys. 6, 126–130 (2010).5. X. Wang, D. J. Hilton, J. L. Reno, D. M. Mittleman, and J. Kono, “Direct measurement of cyclotron coherence

times of high-mobility two-dimensional electron gases,” Opt. Express 18, 12354–12361 (2010).6. Y. Ikebe, T. Morimoto, R. Masutomi, T. Okamoto, H. Aoki, and R. Shimano, “Optical Hall Effect in the Integer

Quantum Hall Regime,” Phys. Rev. Lett. 104, 256802 (2010).7. T. Arikawa, X. Wang, D. J. Hilton, J. L. Reno, W. Pan, and J. Kono, “Quantum control of Landau-quantized two-

dimensional electron gas in a GaAs quantum well using coherent terahertz pulses,” Phys. Rev. B 84, 241307(R)(2011).

8. J. Kono, “Cyclotron Resonance,” in Methods in Materials Research, E. N. Kaufmann, ed. (John Wiley & Sons,New York, 2001).

9. D. Molter, F. Ellrich, T. Weinland, S. George, M. Goiran, F. Keilmann, R. Beigang, and J. Leotin, “High-speedterahertz time-domain spectroscopy of cyclotron resonance in pulsed magnetic field,” Opt. Express 18, 26163–26168 (2010).

#161190 - $15.00 USD Received 10 Jan 2012; revised 17 Feb 2012; accepted 17 Feb 2012; published 27 Feb 2012(C) 2012 OSA 12 March 2012 / Vol. 20, No. 6 / OPTICS EXPRESS 5993

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10. F. Ellrich, T. Weinland, D. Molter, J. Jonuscheit , and R. Beigang, “Compact fiber-coupled terahertz spectroscopysystem pumped at 800 nm wavelength,” Rev. Sci. Instrum. 82, 053102 (2011).

11. D. Molter, F. Ellrich, T. Weinland, S. George, M. Goiran, F. Keilmann R. Beigang, and J. Leotin, “Terahertztime-domain magneto-optics using pulsed magnetic fields,” Proc. IEEE, IRMMW-THz 2011 (2011).

12. E. D. Palik and J. K. Furdyna, “Infrared and microwave magnetoplasma effects in semiconductors,” Rep. Prog.Phys. 33, 1193 (1970).

13. B. L. Cardozo, “GaAs Blocked-Impurity-Band Detectors for Far-Infrared Astronomy,” Ph.D. thesis, Universityof Berkeley, California (2004).

14. X. Wang, “Time-Domain Terahertz Magneto-Spectroscopy of Semiconductors,” Ph.D. thesis, Rice University(2009).

15. K. Suzuki and J. C. Hensel, “Quantum resonances in the valence bands of germanium,” Phys. Rev. B 9, 4184–4218 (1974).

16. I. Vurgaftman, J. R. Meyer, and L. R. Ram-Mohan, “Band parameters for III-V compound semiconductors andtheir alloys,” J. Appl. Phys. 89, 5815 (2001).

1. Introduction

Terahertz (THz) time-domain spectroscopy (TDS) is becoming most attractive for measuringoptical properties of condensed matter systems at THz frequencies and particularly under ex-posure to high magnetic fields [1–7]. Such measurements are of fundamental importance sincethey ultimately provide the possibility to determine the magneto-optic tensors that govern dy-namical properties of metallic, semiconducting, dielectric and magnetic systems [8]. Recently,we have measured a set of cyclotron resonance spectra in p-doped germanium (p-Ge) in the timedomain and at very high speed during a single sweep of a long-duration pulsed magnet [9]. Forthis experiment, a portable, fiber-coupled THz TDS system [10] employing a high-speed delayline was operated at a pulsed magnet facility. In the present paper, we present a novel approachto measure magneto-optical phenomena, that is based on the repetitive operation of a portable,short-duration (FWHM pulse duration of about 2.5 ms) pulsed magnet placed in a standardTHz TDS system [11]. Instead of high-speed TDS measurements, the transmitted electric fieldis measured step-wise with increments of the delay time after each pulse of the magnet. Inthe following, we first compare the previous fast-scan with the present step-scan approach. Wethen give a detailed presentation of the step-scan method, describe the experimental setup anddisplay cyclotron resonance spectra of electrons in n-GaAs, n-InSb, n-InAs and holes in p-Ge.Two-dimensional plots representing the relative change of THz transmittance versus frequencyand magnetic field are presented for a frequency range from 200 GHz to 2 THz and a magneticfield up to 6 T.

2. Step-scan approach

A side by side methodology of the step-scan approach introduced in this paper and the fast-scanapproach used in [9] is presented in Fig. 1.

In the fast-scan method, a high-speed delay line was used, enabling repetitive measurementof the THz pulses during a single and long-duration shot of the pulsed magnet. Magnetic fieldpulses of durations in the order of some hundreds of milliseconds were used. In this situa-tion, the scan speed ensures a quasi-constant magnetic field during the measurement of eachindividual THz time trace. In contrast, the new method bases on the repetitive operation of ashort-duration pulsed magnet. As the pulse duration of the used miniature magnet is in the orderof a few milliseconds, single-shot or fast-scan measurements are not feasible with the availablehigh-speed delay lines. So, a different approach is introduced here. After each shot (or a de-finable number of shots) of the magnet, the delay time is incremented. During the magneticpulse, a voltage induced in a pickup coil providing magnetic field calibration data as well as theelectric field detected by the photoconductive detector, amplified and filtered by a lock-in am-plifier is recorded. With these data, the electric field of the THz pulse at a given delay time can

#161190 - $15.00 USD Received 10 Jan 2012; revised 17 Feb 2012; accepted 17 Feb 2012; published 27 Feb 2012(C) 2012 OSA 12 March 2012 / Vol. 20, No. 6 / OPTICS EXPRESS 5994

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fast-scan approach step-scan approach

real (measurement) time [arb. u.] real (measurement) time [arb. u.]

real (measurement) time [arb. u.] real (measurement) time [arb. u.]

�FWHM�FWHM�FWHMTrep

Fig. 1. Comparison of the step-scan approach with the fast-scan approach from [9]. Insteadof repetitive measurements of the time-domain traces during a single shot of the magnet, theelectric field of the THz pulse is measured during repetitive operation of a short-durationpulsed magnet. The traces presented here are real measurement data, but trimmed for betterreadability. Typical values for τFWHM and Trep are 2.5 ms and about 7 s respectively.

be assigned to the magnetic field strength by interpolation algorithms. By doing so repetitivelywith successively incrementing the delay time, the (delay) time dependent electric field of theTHz pulse for a given magnetic field strength can be extracted.

3. Experimental setup

The experimental setup of the system is shown in Fig. 2.A Ti:sapphire laser (MaiTai from Spectra Physics) is employed as pump source for a standard

THz TDS system. Only a small fraction of the available optical output of the laser is usedto pump the emitter and detector photoconductive antennas with an average optical power of20 mW each. In one of the arms, a linear translation stage is implemented as delay line. TwoLT-GaAs photoconductive antennas with dipole metallization (dipole length of about 30 µm)are used as emitter and detector. The dipole structure results in a linear polarized emission ofTHz radiation as well as the detection of (mainly) only one polarization state. Standard Si lensesare utilized to couple the THz radiation from and to the antennas. The THz beam path is builtby four off-axis parabolic mirrors providing a focus at which the center of the magnet coil isplaced. The emitter antenna is biased by a 50 V RMS AC voltage with a modulation frequencyof 57 kHz. The detector antenna is connected to a transimpedance amplifier (amplification of107 V/A, 3 dB bandwidth of 200 kHz), which is then connected to a lock-in amplifier (StanfordResearch Systems SR830). Typical time-constants are set to 30 µs to be able to observe fastdynamics during a shot of the magnet. This is close to the modulation period of 17.5 µs, butfeasible for stable modulation techniques (as it is in the case of using a frequency generator).The output of the lock-in amplifier as well as the signal detected by the pick-up coil is read byan A/D card with a sampling rate of 100 kHz and a resolution of 16 bit. For data acquisition, a

#161190 - $15.00 USD Received 10 Jan 2012; revised 17 Feb 2012; accepted 17 Feb 2012; published 27 Feb 2012(C) 2012 OSA 12 March 2012 / Vol. 20, No. 6 / OPTICS EXPRESS 5995

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�delay

pump laser

Ti:sapphire100 fs

80 MHz780 nm

Tx RxA / DA / D PC

lock-inE (t , )THz meas delay�

dB/dt (t )meas measmagnet coilwith sample

AMP

Fig. 2. Experimental setup used in this work. The output of a mode-locked Ti:sapphire laserwith a center emission wavelength of 780 nm is used. LT-GaAs photoconductive switchesare used as emitter and detector and are pumped with an average optical power of 20 mWeach. Four off-axis mirrors are used to guide the THz beam and to provide a focus, in whichthe magnet is placed.

measurement program was implemented in LabVIEWTM. Each time a magnet pulse is detected,a 50 ms section of relevant data (10 ms section before and 40 ms section after the main peakof the magnetic field) is stored. After this, the delay line is incremented by a certain step size(0.1 ps in the experiments presented here). In the experiments presented in the following, onlyone shot of the magnet is used for each time delay, but SNR improvements are straightforwardby averaging several shots before proceeding to the next time-delay step.

The assembled and disassembled magnet and cryostat are shown in Fig. 3.

magnetcoil

glass fibretube

polycarbonatecylinder

innervessel(b)(a)(a) (b)

Fig. 3. Photos of the assembled (a) and disassembled (b) magnet cryostat. The magnetcoil is held by two glass fibre tubes, which are themselves attached to the walls of a smallpolycarbonate container. This transparent polycarbonate tube is intended to hold the liquidnitrogen during operation and has a slit in the top part for refilling and leakage of nitro-gen gas. The outer polycarbonate tube serves as thermal isolation and is flooded by theevaporated nitrogen in the experiment.

The magnet is immersed in liquid nitrogen using a very crude double wall polycarbonatecryostat. The coil itself is 16 mm long and has an inner diameter of 6 mm. It is built of 400turns of copper wire (with a diameter of 0.4 mm) wounded around a fiber glass tube. It provides

#161190 - $15.00 USD Received 10 Jan 2012; revised 17 Feb 2012; accepted 17 Feb 2012; published 27 Feb 2012(C) 2012 OSA 12 March 2012 / Vol. 20, No. 6 / OPTICS EXPRESS 5996

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a magnetic field up to 10 T with a field inhomogeneity less than 1 % along a distance of 3mm.The coil is held by a pair of wider fiber glass tubes with a diameter of 20 mm and a length of70 mm, that are capped with a double layer foil window (plastic warp) for thermal isolation.This set of tubes ensures a wide enough optical access to the sample at the coil center. Nitrogenfilling of the cryostat is achieved through an upper hole in the outer cylinder and a slit in theinner. Vaporized nitrogen is flooded around the inner vessel and evacuated through a hole at thebottom. This transparent cryogenic system actually provides an efficient cooling of the magnetcoil with visual control of nitrogen level. The sample holder consists of a tube of 6 mm outerdiameter on which an o-ring with an inner diameter of 3 mm is glued. On top of this o-ring,the semiconductor samples are glued with varnish. In the vicinity of the sample, a resistancethermometer (Pt100) is placed for monitoring of the temperature. This sample holder is insertedto the glass fibre tube supporting the magnet coil.

The magnet coil is electronically fed by a supply connected to a conventional wall plug.It delivers current pulses of several hundred amperes with a pulse duration of about 2.5 ms(FWHM pulse duration, depending on the peak current). Two capacitors of 1 mF each, store amaximum energy of 250 J at a peak voltage of 500 V. This energy is converted into magneticenergy by controlled discharge of the capacitors to provide pulses with peak magnetic fields ofup to 10 T. At the same time, the energy ends up into Joule heating and then finally into nitrogenevaporation directly observed after each shot. Photos of the tabletop electric supply, refilling ofthe pulsed magnet during operation and the sample holder with pickup coil and sample areshown in Fig. 4.

(b)

20 cm20 cm

6 mm6 mm

samplesample

pickupcoilpickupcoilpickupcoil

(a)(a) (b) (c)(c)(c)

Fig. 4. (a) Tabletop power supply of the pulsed magnet employing two 500 V, 1 mF capaci-tors. (b) Liquid nitrogen refilling of the pulsed magnet during operation. (c) Sample holderwith pickup coil.

4. Results

The change in the detected THz electric field amplitude for a n-doped GaAs sample and ap-doped Ge sample are shown in Fig. 5 and Fig. 6, respectively. In these intensity plots thedifference ΔE(tmeas,τdelay) = E(tmeas,τdelay)− E(0,τdelay) is displayed together with themagnetic field B(tmeas). The temperature measured by the resistance thermometer was about120 K in both cases.

The change of the THz waveform induced by the magnetic field is clearly visible and ingeneral follows the trend of the magnetic field. For both samples, the first etalon echo (whichis of course also influenced by cyclotron resonance) is observed. Even already in this time-domain data it is obvious, that p-Ge possesses a more complex behavior. This can be deductedmost clearly from the down-sweep (of the magnetic field, starting from 5 ms magnet time)characteristics. In the p-Ge data, a low frequency component (heavy hole resonance as will be

#161190 - $15.00 USD Received 10 Jan 2012; revised 17 Feb 2012; accepted 17 Feb 2012; published 27 Feb 2012(C) 2012 OSA 12 March 2012 / Vol. 20, No. 6 / OPTICS EXPRESS 5997

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0 2 4 6 86 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 223

4

5

6

7

8

9

delay time [ps]

mea

sure

men

t/

mag

net

time

[ms]

magnetic field [T]

n-GaAsn-GaAs

change of THz electricfield amplitude [arb. u.]

0 2 4 6 86 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22

E(B)

-E(0

)[ar

b.u.

]

0.5 T1.0 T1.5 T2.0 T2.5 T3.0 T3.5 T4.0 T4.5 T5.0 T5.5 T6.0 T6.5 T

Fig. 5. Change of the detected THz electric field amplitude as a function of delay timeand magnet time for n-GaAs displayed as an intensity plot as well as conventional plotsextracted thereof. The THz amplitude values for no magnetic field are subtracted from themeasured data to obtain these differential plots. In addition, the magnetic field pulse isshown.

shown later) is present at the highest field and is accompanied by a high frequency componentin the down-sweep, starting from about 7 ms magnet time. In the n-GaAs sample data, thefrequency of the resonance seems to change up to a magnetic field of 4 T and then builds aplateau. This feature is not caused by cyclotron resonance, it occurs at frequencies lower thanthe collision frequency, where featureless absorption decreases at increasing magnetic fields.

To obtain the change of the THz transmittance induced by the magnetic field, the THz wave-forms E(tmeas,τdelay) were numerically transformed to waveforms dependent on the magneticfield E(B,τdelay). Afterwards, they were Fourier-transformed and referenced to the data at nomagnetic field.

For magneto-optical transmission spectroscopy measurements of dilute plasma systems, therelevant information can be displayed by two-dimensional plots representing the relative changeof the transmitted intensity dependent on the frequency and the magnetic field

(E(ω,B)E(ω,0)

)2

−1. (1)

In the limit of low-density plasma, where the sample reflectance does not vary significantly inthe measured THz frequency range, such transmittance spectra are proportional to the changeof absorbed power in the sample under exposure to the magnetic field [12]. In these systems theabsorbed power is dissipated by the current Jx driven by the linearly incident polarized waveEx=E0e−iωt . In this case, the power absorbed per unit volume is

P =12

Re(JE∗) =12

Re(σxx)E20 . (2)

#161190 - $15.00 USD Received 10 Jan 2012; revised 17 Feb 2012; accepted 17 Feb 2012; published 27 Feb 2012(C) 2012 OSA 12 March 2012 / Vol. 20, No. 6 / OPTICS EXPRESS 5998

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6 8 10 12 14 16 18 20 22 24 26 28 30 32 34 36 38 403

4

5

6

7

8

9

delay time [ps]

mea

sure

men

t/

mag

net

time

[ms]

0 2 4 6 8magnetic field [T]

0 1 2 3 4 5 6 7 86 8 10 12 14 16 18 20 22 24 26 28 30 32 34 36 38 40

E(B)

-E(0

)[ar

b.u.

]

0.5 T1.0 T1.5 T2.0 T2.5 T3.0 T3.5 T4.0 T4.5 T5.0 T5.5 T6.0 T6.5 T

change of THz electricfield amplitude [arb. u.]

p-Gep-Ge

Fig. 6. Change of the detected THz electric field amplitude as a function of delay time andmagnet time for p-Ge displayed as an intensity plot as well as conventional plots extractedthereof. The THz amplitude values for no magnetic field are subtracted from the measureddata to obtain these differential plots. In addition, the magnetic field pulse is shown.

It turns out, that the transmittance spectra of a wave polarized along the x-axis directly dis-play the real part of the diagonal conductivity tensor Re(σxx). In the following, we present THztransmittance spectra for bulk n-GaAs, p-Ge, n-InSb and n-InAs quantum well. The results forGaAs will be analyzed using the low-density limit approximation, while the ones of the othersamples are only briefly commented.

Figure 7 shows experimental and numerical results of the relative change of THz transmit-tance dependent on the frequency and magnetic field for a bulk n-type GaAs thick layer. Thissample was grown by liquid phase epitaxial technique for implementing sensitive photoconduc-tive detectors with high THz absorption from 1s to 2p impurity transition at liquid-helium tem-perature [13]. The layer thickness was 60 µm with an electron concentration of 1.5·1015 cm−3.Measurement was performed at 120 K. Obviously, two striking features appear in both plots ofFig. 7. A broad line of decreased transmission that saturates at 50 % of the zero field transmis-sion value and a green area below a threshold frequency that displays increased transmission.The average slope of the absorption line and the resonance equation

m∗ =eBωc

(3)

yield an effective mass m∗ of of (0.075± 0.005) m0. This value is higher than the acceptedvalue of 0.067 m0 for electrons at the bottom of the conduction band, but nevertheless consis-tent with recent temperature-dependent measurements [14]. The above spectral features can beexplained by numerical simulations based on the Drude model. The absorbed power per unitvolume is given by

P =14

σ0E2

(1

1+(ωc −ω)2τ2 +1

1+(ωc +ω)2τ2

). (4)

#161190 - $15.00 USD Received 10 Jan 2012; revised 17 Feb 2012; accepted 17 Feb 2012; published 27 Feb 2012(C) 2012 OSA 12 March 2012 / Vol. 20, No. 6 / OPTICS EXPRESS 5999

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n-GaAs(simulation)n-GaAs(simulation)n-GaAs(simulation)

n-GaAs(experimental)n-GaAs(experimental)n-GaAs(experimental)

relative change of THztransmittance

0 +0.83-0.5 0 +0.83-0.5

relative change of THztransmittance

0 1 2 3 4 5 60.00.20.40.60.81.01.21.41.61.82.0

freq

uenc

y[T

Hz]

magnetic field [T]0 1 2 3 4 5 6

0.00.20.40.60.81.01.21.41.61.82.0

freq

uenc

y[T

Hz]

magnetic field [T]

0.2 0.4 0.6 0.8 1.0 1.2 1.4 1.6 1.8 2.0

rela

tive

chan

geof

THz

tran

smitt

ance

frequency [THz]

0.2 0.4 0.6 0.8 1.0 1.2 1.4 1.6 1.8 2.0

rela

tive

chan

geof

THz

tran

smitt

ance

frequency [THz]

1.0 T

2.0 T

3.0 T

4.0 T

5.0 T

6.0 T

1.0 T

2.0 T

3.0 T

4.0 T

5.0 T

6.0 T

Fig. 7. Experimental and simulation results of the relative change in the THz transmittancefor n-GaAs. Black values indicate no change of THz transmittance when the sample isexposed to the magnetic field. Red, yellow and white indicate absorption (here causedby cyclotron resonance), green denotes an increase of transmission. Grayed out areas areneglected due to poor SNR (included in the simulation to preserve comparability).

This expression includes two contributions, which correspond to the two circularly polarizedwaves of equal amplitude that combine in the linearly polarized wave. For the case ωτ > 1,according to Eq. (4), the wave mode that rotates in the same sense as the electrons gets reso-nantly absorbed and therefore called cyclotron resonance active (CRA) mode, while the othermode, denoted cyclotron resonance inactive (CRI), is practically unchanged by the magneticfield. This is shown in Fig. 7, where, however, the CR line develops a saturated plateau. Indeed,the numerical simulation demonstrates that, after crossing the 60 µm thick layer, the transmittedpower of the CRA wave vanishes in a wide frequency range around the resonance peak. In thiscase, because the CRI is not changed by the magnetic field, the transmitted THz intensity dropsto 50 % near the resonance peak and a saturated plateau is observed around the CR line. Onthe other hand, at low frequencies (ωτ < 1), the absorption of both CRA and CRI waves de-creases with magnetic field according to Eq. (4) and gives rise to the green area. The thresholdfrequency gives a fair estimate of the reciprocal collision time τ , which is about 4 ps here, inagreement with the measured mobility value at this temperature of about 8·104 cm2

Vs .Figure 8 shows experimental results of the measured relative change in the THz transmit-

tance for p-Ge, n-InAs and n-InSb (with the same scale for the magnetic field for comparison).The free holes concentration is 2·1014 cm−3 for the p-Ge sample, free electrons concentration3·1014 cm−3 for n-InSb and 5·1011 cm−2 for the InAs quantum well. As before, the intensity ata given frequency is normalized to its zero magnetic field value.

For the p-Ge data, two hole cyclotron resonances (light and heavy) and a weak resonancein between due to quantum mechanical effects [15] are observed. The lines slopes give lightand heavy hole effective masses of 0.04 m0 and 0.3 m0, respectively. The absence of green area

#161190 - $15.00 USD Received 10 Jan 2012; revised 17 Feb 2012; accepted 17 Feb 2012; published 27 Feb 2012(C) 2012 OSA 12 March 2012 / Vol. 20, No. 6 / OPTICS EXPRESS 6000

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p-Gep-Ge

InAsInAs InSbInSb

relative change of THztransmittance

0 +1.25-0.75

relative change of THztransmittance

0 +0.6-0.36

relative change of THztransmittance

0 +0.83-0.5

0 1 2 3 4 5 60.00.20.40.60.81.01.21.41.61.82.0

freq

uenc

y[T

Hz]

magnetic field [T]0 1 2 3 4 5 6

0.00.20.40.60.81.01.21.41.61.82.0

freq

uenc

y[T

Hz]

magnetic field [T]

0 1 2 3 4 5 60.00.20.40.60.81.01.21.41.61.82.0

freq

uenc

y[T

Hz]

magnetic field [T]

Fig. 8. Experimental results of the relative change in the THz transmittance for p-Ge, n-InAs and n-InSb. Black values indicate no change of spectral THz intensity when the sam-ple is exposed to the magnetic field. Red, yellow and white indicate absorption (here causedby cyclotron resonance), green denotes an increase of transmission. Grayed out areas areneglected due to poor SNR. The same scale is kept for comparison of all plots.

indicates a lower value of collision frequency that falls in the grayed out area of poor SNR. Theobtained results agree very well with the results from the fast-scan measurements with a long-duration pulsed magnetic field up to 12 T [9], but provide a broader frequency range as well asan improved SNR. Again, only single shots of the magnet between step-wise increments of thedelay line were used. Due to the use of lock-in technique and a longer effective measurementtime, the results presented here have a higher SNR (in the order of 102) and provide access to abroader spectrum compared to the fast-scan technique (SNR in the order of 10).

The plots for InSb and InAs are limited to fields below 1 T and 2.8 T and they are onlypresented here for illustrating the step-scan technique. The average slope effective masses of0.02 m0 and 0.035 m0 for InSb and InAs, respectively, deviate significantly from acceptedvalues of 0.014 m0 and 0.026 m0 [16]. However, detailed analysis explaining the deviations,including magneto-plasma effects [4, 12], is outside the scope of this paper.

5. Conclusion

We have demonstrated a novel and simple approach for THz magneto-optical spectroscopy,which is based on a portable, repetitive pulsed magnet combined with a standard THz time-domain spectroscopy system. Magneto-transmission spectra of linearly polarized THz pulsesthrough semiconductor layers of GaAs, Ge, InSb and InAs were displayed in the frequencyrange from 200 GHz to 2 THz and for magnetic field up to 6 T. The data were obtained witha single magnet shot between step-wise increments of the TDS delay line. It is straightforwardto improve the signal to noise ratio of the measured THz electric field amplitude by averagingmultiple shots between delay line increments or by increasing the magnet duty cycle. This

#161190 - $15.00 USD Received 10 Jan 2012; revised 17 Feb 2012; accepted 17 Feb 2012; published 27 Feb 2012(C) 2012 OSA 12 March 2012 / Vol. 20, No. 6 / OPTICS EXPRESS 6001

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tabletop step-scan time-domain THz magneto-spectrometer based on a liquid-nitrogen cooledresistive mini-coil can be implemented at higher magnetic fields and broadly used for furthermagneto-optics experiments.

Acknowledgments

Part of this work has been supported by EuroMagNET II under the EU contract number 228043.We gratefully acknowledge discussions with Oleksiy Drachenko and Junichiro Kono. We aregrateful to E.E. Haller for the gift of a GaAs epilayer and to Anne Ahrens and Oliver Hans forliquid nitrogen provision.

#161190 - $15.00 USD Received 10 Jan 2012; revised 17 Feb 2012; accepted 17 Feb 2012; published 27 Feb 2012(C) 2012 OSA 12 March 2012 / Vol. 20, No. 6 / OPTICS EXPRESS 6002