soontae kim and daewon w. byun comparison of emission estimates from smoke and eps2 used for...
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Soontae Kim and Daewon W. ByunSoontae Kim and Daewon W. ByunSoontae Kim and Daewon W. ByunSoontae Kim and Daewon W. Byun
Comparison of Emission Estimates from SMOKE Comparison of Emission Estimates from SMOKE and EPS2 Used for Studying Houston-Galveston and EPS2 Used for Studying Houston-Galveston
Air QualityAir Quality
Comparison of Emission Estimates from SMOKE Comparison of Emission Estimates from SMOKE and EPS2 Used for Studying Houston-Galveston and EPS2 Used for Studying Houston-Galveston
Air QualityAir Quality
Institute for Multidimensional Air Quality Institute for Multidimensional Air Quality
Studies (IMAQS)Studies (IMAQS)
University University ofof Houston Houston
Institute for Multidimensional Air Quality Institute for Multidimensional Air Quality
Studies (IMAQS)Studies (IMAQS)
University University ofof Houston Houston
- Based on Area/Nonroad, Point and Biogenic - Based on Area/Nonroad, Point and Biogenic emissions in Texas Emissions Inventoryemissions in Texas Emissions Inventory
Spatial allocationSpatial allocation
BackgroundsBackgrounds
OutlineOutline
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
Emissions processing with SMOKE & Emissions processing with SMOKE &
EPS2EPS2
Biogenic emissionsBiogenic emissions
Examples of CMAQ Examples of CMAQ
resultsresults
Chemical speciationChemical speciation
Temporal allocationTemporal allocation
Houston-Galveston area, Houston-Galveston area,
Texas EITexas EI
BEIS3 & GloBEIS3BEIS3 & GloBEIS3
Non-attainment area due to high ground-level ozone concentrations
Several air quality modeling studies
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
The Houston-Galveston AreaThe Houston-Galveston Area
LouisianaLouisiana
HGAHGA
The Gulf The Gulf of Mexicoof Mexico
The ship channel area
Downtown Houston
Offshore emissions
Major NEGU point sources
Available Emissions Inventories
CMAQ, CAMx and etc.CMAQ, CAMx and etc.
National - NET96, NEI99 from U.S. EPANational - NET96, NEI99 from U.S. EPA
State - Texas Emissions Inventory from State - Texas Emissions Inventory from TCEQ (Texas Commission on TCEQ (Texas Commission on Environmental Quality)Environmental Quality)
Emissions processing systemsSMOKE - NET96, NEI99SMOKE - NET96, NEI99
EPS2 - Texas Emission Inventory (TEI) EPS2 - Texas Emission Inventory (TEI)
Source typeSource typeNOx (tons/day)NOx (tons/day) VOC (tons/day)VOC (tons/day)
NEI99 NEI99 1)1) TEI TEI 2)2) NEI99NEI99 TEITEI
On-road mobileOn-road mobile 353353 246246 255255 156156
Area/Nonroad mobileArea/Nonroad mobile 192192 193193 227227 241241
Point Point 521521 490490 152152 327 (178) 327 (178) 3)3)
8-County total 8-County total anthropogenic anthropogenic emissionsemissions
10661066 929929 633633 724 (575)724 (575)
Data sources: Data sources: 1)1) National – Calculated based on U.S. EPA NEI 1999 final version 2 National – Calculated based on U.S. EPA NEI 1999 final version 2 2)2) State – TCEQ documents (available at State – TCEQ documents (available at ftp://ftp.tnrcc.state.tx.us/pub/OEPAA/ TAD/ftp://ftp.tnrcc.state.tx.us/pub/OEPAA/ TAD/
Modeling/HGAQSE/Modeling/Doc/TSD_PHASE1/attachment3-emissions_inventory.pdf )Modeling/HGAQSE/Modeling/Doc/TSD_PHASE1/attachment3-emissions_inventory.pdf ) 3)3) Parenthesis presents regular case emissions. Parenthesis presents regular case emissions.
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
NEI99 & Texas EINEI99 & Texas EI
For the HGA 8-countyFor the HGA 8-county
<<>>
Emissions Inventory ProcessingEmissions Inventory Processing
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
AQMs input-ready AQMs input-ready emissionsemissions
Temporal allocationTemporal allocation
Spatial Spatial allocationallocationChemical Chemical speciationspeciation
Emissions InventoryEmissions Inventory
Depend on Depend on cross-reference cross-reference
& profile files& profile files
Same Same processes in processes in SMOKE & EPS2SMOKE & EPS2
Different Different inputs for inputs for SMOKE & EPS2SMOKE & EPS2Present Present different AQM-different AQM-ready ready emissionsemissions
ObjectivesObjectives
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
Texas EI was processed Texas EI was processed for the HGA 2-km grid for the HGA 2-km grid domain (166 x 130 cells) during the period of domain (166 x 130 cells) during the period of the TexAQS 2000 Experiment (Aug. 23the TexAQS 2000 Experiment (Aug. 23rdrd - Sept. - Sept. 11stst, 2000) , 2000) ..Focusing on the effects of differences in Focusing on the effects of differences in cross-reference and profile files.cross-reference and profile files.
SMOKESMOKE and and EPS2EPS2 used used U.S. EPA’sU.S. EPA’s and and TCEQ’sTCEQ’s cross-reference and profile files, respectively.cross-reference and profile files, respectively.
CompareCompare two emission modeling systems, two emission modeling systems,SMOKE and EPS2SMOKE and EPS2, to identify uncertainties , to identify uncertainties arising during each step of processing; arising during each step of processing; spatial spatial griddinggridding, , chemical speciationchemical speciation and and temporal temporal allocationallocation
BEIS3BEIS3 and and GloBEIS3GloBEIS3 were also were also compared.compared.
SMOKE & EPS2: General comparisonSMOKE & EPS2: General comparison
ProcessProcess EPS2EPS2
Spatial Spatial allocationallocation
ChemicalChemicalspeciationspeciation
TemporalTemporalallocationallocation
BiogenicBiogenic
U.S. EPA’s 15 surrogates. New surrogating system (64 srgs) are applicable.No surrogates for off-shore emissions.
Nationwide spilt factors.Mostly depends on SCC.Separate treatments for PO and hourly emissions.Additional profiles for hourly emissions prepared.BEIS3, BELD3 / MM5
SMOKESMOKE
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
TCEQ has developed 27 surrogates. Unique surrogates for the HGA including off-shore surrogates.
Uses Plant ID, Stack ID, SCC & FIPS for points.PO/hourly emissions at the same time. No diurnal variation for NEGU point emissions.GloBEIS3, Texas LULC / Observed met. data
Surrogates used for EPS2Surrogates used for EPS2
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
SurrogateSurrogate Surrogate Surrogate
PopulationPopulationUrban populationUrban populationRural populationRural populationCommercial airportsCommercial airportsGeneral airportsGeneral airports
SMOKESMOKE1)1)
Gas stationsGas stationsDry cleanerDry cleanerRestaurantsRestaurantsResidential areaResidential areaForestForest
Military airportsMilitary airportsCounty yardsCounty yardsWaterWaterShipsShipsHarborsHarbors
CanalCanalRailroadRailroadAuto body shopsAuto body shopsMarine coating facilitiesMarine coating facilities
Offshore Offshore Shipping lanesShipping lanesPlatformsPlatforms
AgricultureAgricultureCommercial & industrial Commercial & industrial Commercial & residentialCommercial & residentialOil and gas wells (Inland)Oil and gas wells (Inland)Offshore oil and gas wellsOffshore oil and gas wells
SMOKE SMOKE
AA, , BBAA, , BBAA, , BB--AA, , BB
BBAA, , BBAA, , BBBBAA, , BB
--AA, , BB----
BBBBBBBBAA, , BB
AA, , BBBBBB----
------
Note: Note: 1)1) AA – Included in U.S. EPA’s 15 surrogates. – Included in U.S. EPA’s 15 surrogates. BB – Included in U.S. EPA’s 64 surrogates (New – Included in U.S. EPA’s 64 surrogates (New surrogating system).surrogating system).
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
Difference in SurrogatesDifference in Surrogates
PopulationPopulation
TCEQTCEQ(US Census Bureau, (US Census Bureau,
2000)2000)
SMOKETOOLSMOKETOOL(Shp1996; US (Shp1996; US Census Bureau, Census Bureau, 1990)1990)
MIMSMIMSSpatial allocatorSpatial allocator(Shp2003; US Census (Shp2003; US Census Bureau, 2000)Bureau, 2000)
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
Unique surrogates for the HGAUnique surrogates for the HGA
Offshore oil and gas wellsOffshore oil and gas wells PlatformsPlatforms Shipping lanesShipping lanes
Marine coating facilitiesMarine coating facilities Auto body shopsAuto body shops RestaurantsRestaurants
From TCEQ’s surrogatesFrom TCEQ’s surrogates
EPS2EPS2 SMOKESMOKE
Example of Spatial AllocationExample of Spatial Allocation
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
Without offshore surrogates from TCEQWithout offshore surrogates from TCEQ
Area/Nonroad mobile emissions: NOArea/Nonroad mobile emissions: NO
EPS2EPS2 SMOKESMOKE
Example of Spatial AllocationExample of Spatial Allocation
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
After implementing TCEQ’s surrogates for offshore emissions.After implementing TCEQ’s surrogates for offshore emissions.
Area/Nonroad mobile emissions: NOArea/Nonroad mobile emissions: NO
EPS2EPS2 SMOKESMOKE
Example of Spatial AllocationExample of Spatial Allocation
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
Area/Nonroad mobile emissions: ETHArea/Nonroad mobile emissions: ETH
Chemical SpeciationChemical Speciation
11Split factors (Chemical speciation profile) Split factors (Chemical speciation profile)
Applied to lumped VOC species (CB-IV mechanism).
SMOKE assigns SCC-related profile codes provided by U.S. EPA.EPS2 uses SCC, FIPS code, Plant ID and Stack ID to assign profile codes developed by TCEQ.
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
22Example of split factorsExample of split factors
3.72E-023.72E-02--------------5.54E-055.54E-052.95E-022.95E-02--EPA EPA (TOG)(TOG)
--1.61E-051.61E-050.00E+000.00E+001.09E-041.09E-041.55E-021.55E-022.37E-042.37E-041.07E-051.07E-053.64E-053.64E-051.69E-041.69E-041.57E-021.57E-028.04E-038.04E-03TCEQTCEQ(VOC)(VOC)
NRNRISOPISOPETOHETOHMEOHMEOHETHETHALD2ALD2FORMFORMXYLXYLTOLTOLPARPAROLEOLE
NEGU point - SCC 30118701: Chemical Manufacturing, Ethylene: General (FIPS 48000)NEGU point - SCC 30118701: Chemical Manufacturing, Ethylene: General (FIPS 48000)
Split factors for point source emissions show large differences.
Units: mol/kgUnits: mol/kg
Example of Chemical SpeciationExample of Chemical Speciation
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
NEGU point emissionsNEGU point emissions
0.00.0
0.20.2
EP
S2
/S
MO
KE e
mis
sio
ns r
ati
os
EP
S2
/S
MO
KE e
mis
sio
ns r
ati
os
CO
ETH
FORM
OLE
PAR
0.40.4
0.60.6
0.80.8
1.01.0
1.21.2
1.41.4
1.61.6
NOx
ALD2
TOL
XYL
SpeciesSpecies
NEGU point emissionsNEGU point emissions
0.00.0
0.20.2
EP
S2
/S
MO
KE e
mis
sio
ns r
ati
os
EP
S2
/S
MO
KE e
mis
sio
ns r
ati
os
CO
ETH
FORM
OLE
PAR
0.40.4
0.60.6
0.80.8
1.01.0
1.21.2
1.41.4
1.61.6
NOx
ALD2
TOL
XYL
SpeciesSpecies
Area emissionsArea emissions
0.00.0
0.20.2
EP
S2
/S
MO
KE e
mis
sio
ns r
ati
os
EP
S2
/S
MO
KE e
mis
sio
ns r
ati
os
CO ETH
FORM
OLE
PAR
0.40.4
0.60.6
0.80.8
1.01.0
1.21.2
1.41.4
1.61.6
NOx
ALD2
TOL
XYL
Area emissionsArea emissions
0.00.0
0.20.2
EP
S2
/S
MO
KE e
mis
sio
ns r
ati
os
EP
S2
/S
MO
KE e
mis
sio
ns r
ati
os
CO ETH
FORM
OLE
PAR
0.40.4
0.60.6
0.80.8
1.01.0
1.21.2
1.41.4
1.61.6
NOx
ALD2
TOL
XYL
Nonroad mobile emissionsNonroad mobile emissions
0.00.0
0.20.2
CO ETH
FORM OLE
PAR
Ratio =1Ratio =1
0.40.4
0.60.6
0.80.8
1.01.0
1.21.2
1.41.4
1.61.6
NOx
ALD2 TOL
XYL
Nonroad mobile emissionsNonroad mobile emissions
0.00.0
0.20.2
CO ETH
FORM OLE
PAR
Ratio =1Ratio =1
0.40.4
0.60.6
0.80.8
1.01.0
1.21.2
1.41.4
1.61.6
NOx
ALD2 TOL
XYL
EGU point emissionsEGU point emissions
0.00.0
0.20.2
CO
ETH
FORM
OLE
PAR
Ratio =1Ratio =1
0.40.4
0.60.6
0.80.8
1.01.0
1.21.2
1.41.4
1.61.6
NOx
ALD2
TOL
XYL
SpeciesSpecies
2.9
EGU point emissionsEGU point emissions
0.00.0
0.20.2
CO
ETH
FORM
OLE
PAR
Ratio =1Ratio =1
0.40.4
0.60.6
0.80.8
1.01.0
1.21.2
1.41.4
1.61.6
NOx
ALD2
TOL
XYL
SpeciesSpecies
2.9
Temporal AllocationTemporal Allocation
11Peak ozone day and annual average emissions
Area & nonroad mobile and regular point emissions. SMOKE uses U.S. EPA’s profiles.EPS2 uses Texas-specified profiles.
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
22Hourly emissions
Supplementary and special point emissions.
No Profiles are used. No difference in SMOKE and EPS2.
Source- and hour-specific profiles are prepared for SMOKE based on emission patterns.
Example of Temporal AllocationExample of Temporal Allocation
Area emissionsArea emissions
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 120
1000
2000
3000
4000
5000
6000
OLE_SMK OLE_EPS2
Em
issi
on r
a te s
(m
o le s
/ hr )
Aug22 Aug23 Aug24 Aug25 Aug26 Aug27 Aug28 Aug29 Aug30 Aug31 Sep01
Hour (CST)
0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 120
2000
4000
6000
8000
10000
ETH_SMK ETH_SMK
Em
issi
on r
a te s
(m
o le s
/ hr )
Aug22 Aug23 Aug24 Aug25 Aug26 Aug27 Aug28 Aug29 Aug30 Aug31 Sep01
Hour (CST)
0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 120
100000
200000
300000
400000
500000
600000
CO_SMK CO_EPS2
Em
issi
on r
a te s
(m
o le s
/ hr )
Aug22 Aug23 Aug24 Aug25 Aug26 Aug27 Aug28 Aug29 Aug30 Aug31 Sep01
Hour (CST)
0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 120
20000
40000
60000
80000
100000
NO_SMK NO_EPS2
Em
issi
on r
a te s
(m
o le s
/ hr )
Aug22 Aug23 Aug24 Aug25 Aug26 Aug27 Aug28 Aug29 Aug30 Aug31 Sep01
Hour (CST)
Example of Temporal AllocationExample of Temporal Allocation
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
Nonroad mobile emissionsNonroad mobile emissions
0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 120
1000000
2000000
3000000
4000000
5000000
6000000
CO_SMK CO_EPS2
Em
issi
on r
a te s
(m
o le s
/ hr )
Aug22 Aug23 Aug24 Aug25 Aug26 Aug27 Aug28 Aug29 Aug30 Aug31 Sep01
Hour (CST)
0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 120
50000
100000
150000
200000
250000
NO_SMK NO_EPS2
Em
issi
on r
a te s
(m
o le s
/ hr )
Aug22 Aug23 Aug24 Aug25 Aug26 Aug27 Aug28 Aug29 Aug30 Aug31 Sep01
Hour (CST)
0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 120
5000
10000
15000
20000
25000
ETH_SMK ETH_EPS2
Em
issi
on r
a te s
(m
o le s
/ hr )
Aug22 Aug23 Aug24 Aug25 Aug26 Aug27 Aug28 Aug29 Aug30 Aug31 Sep01
Hour (CST)
0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 120
5000
10000
15000
20000
OLE_SMK OLE_EPS2
Em
issi
on r
a te s
(m
o le s
/ hr )
Aug22 Aug23 Aug24 Aug25 Aug26 Aug27 Aug28 Aug29 Aug30 Aug31 Sep01
Hour (CST)
Example of Temporal AllocationExample of Temporal Allocation
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
EGU point emissionsEGU point emissions
0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 120
50000
100000
150000
CO_SMK CO_EPS2
Em
issi
on r
a te s
(m
o le s
/ hr )
Aug22 Aug23 Aug24 Aug25 Aug26 Aug27 Aug28 Aug29 Aug30 Aug31 Sep01
Hour (CST)
0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 120
50000
100000
150000
200000
250000
300000
350000
NO_SMK NO_EPS2
Em
issi
on r
a te s
(m
o le s
/ hr )
Aug22 Aug23 Aug24 Aug25 Aug26 Aug27 Aug28 Aug29 Aug30 Aug31 Sep01
Hour (CST)
0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 120
5
10
15
20
25
30
ETH_SMK ETH_EPS2
Em
issi
on r
a te s
(m
o le s
/ hr )
Aug22 Aug23 Aug24 Aug25 Aug26 Aug27 Aug28 Aug29 Aug30 Aug31 Sep01
Hour (CST)
0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 120
5
10
15
20
25
30
OLE_SMK OLE_EPS2
Em
issi
on r
a te s
(m
o le s
/ hr )
Aug22 Aug23 Aug24 Aug25 Aug26 Aug27 Aug28 Aug29 Aug30 Aug31 Sep01
Hour (CST)
Example of Temporal AllocationExample of Temporal Allocation
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
NEGU point emissionsNEGU point emissions
0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12250000
270000
290000
310000
330000
350000
CO_SMK CO_EPS2
Em
issi
on r
a te s
(m
o le s
/ hr )
Aug22 Aug23 Aug24 Aug25 Aug26 Aug27 Aug28 Aug29 Aug30 Aug31 Sep01
Hour (CST)
0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12250000
270000
290000
310000
330000
350000
NO_SMK NO_EPS2
Em
issi
on r
a te s
(m
o le s
/ hr )
Aug22 Aug23 Aug24 Aug25 Aug26 Aug27 Aug28 Aug29 Aug30 Aug31 Sep01
Hour (CST)
0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 120
10000
20000
30000
40000
ETH_SMK ETH_EPS2
Em
issi
on r
a te s
(m
o le s
/ hr )
Aug22 Aug23 Aug24 Aug25 Aug26 Aug27 Aug28 Aug29 Aug30 Aug31 Sep01
Hour (CST)
0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 120
5000
10000
15000
20000
25000
30000
OLE_SMK OLE_EPS2
Em
issi
on r
a te s
(m
o le s
/ hr )
Aug22 Aug23 Aug24 Aug25 Aug26 Aug27 Aug28 Aug29 Aug30 Aug31 Sep01
Hour (CST)
Biogenic emissions: different inputsBiogenic emissions: different inputs
11Land use land cover data
SMOKE uses BELD3 provided by U.S. EPA for BEIS3.TCEQ developed Texas LULC data for GloBEIS3. ( e.g. Texas Forest Service, …)
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
22Meteorological data
SMOKE uses MM5 / MCIP output.
GloBEIS3 uses the observed temperatures.
TCEQ uses Photosynthetically Active Solar Radiation fields processed thru GOES satellite data analysis.
Split factors in BEIS3 and GloBEIS3Split factors in BEIS3 and GloBEIS3
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
11MONOTERPINESMONOTERPINES
22 OVOCsOVOCs
SpeciesSpecies BEIS3 BEIS3 2)2) (mole/kg) (mole/kg)
OLEOLEPARPARXYLXYLALD2ALD2NRNR
GloBEIS3 GloBEIS3 1)1) (mole/kg) (mole/kg)
4.174.1770.8370.83 -- -- 4.174.17
7.47.453.253.2 0.3290.329 6.26.2 0.3110.311
SpeciesSpecies BEIS3 (mole/kg)BEIS3 (mole/kg)
OLEOLEPARPARFORMFORMALD2ALD2ETHETHMEOHMEOHETOHETOHNRNRTERPBTERPB
GloBEIS3 (mole/kg) GloBEIS3 (mole/kg)
4.174.1750.0050.00 --12.5012.50 -- -- -- -- 8.338.33
4.34.312.812.8 1.21.2 33 2.12.145452121 1.291.29 --
Data sources: Data sources: 1)1) Texas Commission on Environmental Quality, 2002: Attachment 3 – Emissions Texas Commission on Environmental Quality, 2002: Attachment 3 – Emissions Inventory Inventory Development and Modeling for the August 25-September 1, 2000 Episode Development and Modeling for the August 25-September 1, 2000 Episode November 15, 2002. November 15, 2002. 2)2) Calculated based on GSPRO profiles for ‘BV309’ Calculated based on GSPRO profiles for ‘BV309’..
Biogenic emissions: ISOPBiogenic emissions: ISOP
GloBEIS3 (TCEQ)GloBEIS3 (TCEQ) BEIS3BEIS3
Biogenic 4km, GloBEIS3 & BEIS3, TexAQS 2000
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
Biogenic emissions: OLEBiogenic emissions: OLE
GloBEIS3 (TCEQ)GloBEIS3 (TCEQ) BEIS3BEIS3
Biogenic 4km, GloBEIS3 & BEIS3, TexAQS 2000
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
Biogenic emissions: ETHBiogenic emissions: ETH
GLOBEIS3 (TCEQ)GLOBEIS3 (TCEQ) BEIS3BEIS3
Biogenic 4km, GloBEIS3 & BEIS3, TexAQS 2000
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
No No speciation speciation No No emissions!!emissions!!
Biogenic emissionsBiogenic emissions
Biogenic 4km, GLOBEIS3 & BEIS3, TexAQS 2000Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
ISOP (TCEQ 4km Domain)
0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 120
1000
2000
3000
4000
5000
6000BEIS3 GloBEIS3
Em
issi
on r
a te s
(K
mo l
e /h r
)
Aug22 Aug23 Aug24 Aug25 Aug26 Aug27 Aug28 Aug29 Aug30 Aug31
Hour (CST)
ALD2 (TCEQ 4km Domain)
0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 120
200
400
600
800BEIS3 GloBEIS3
Em
issi
on r
a te s
(K
mo l
e /h r
)
Hour (CST)
Aug22 Aug23 Aug24 Aug25 Aug26 Aug27 Aug28 Aug29 Aug30 Aug31
OLE (TCEQ 4km Domain)
0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 120
200
400
600
800
1000BEIS3 GloBEIS3
Em
issi
on r
a te s
(K
mo l
e /h r
)
Hour (CST)
Aug22 Aug23 Aug24 Aug25 Aug26 Aug27 Aug28 Aug29 Aug30 Aug31
PAR (TCEQ 4km Domain)
0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 120
2000
4000
6000
8000BEIS3 GloBEIS3
Em
issi
on r
a te s
(K
mo l
e /h r
)
Hour (CST)
Aug22 Aug23 Aug24 Aug25 Aug26 Aug27 Aug28 Aug29 Aug30 Aug31
0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12
0
200
400
600
800
1000
1200Area/Nonroad Mobile Point Biogenic Total
OLE
Em
i ss i
o n r
a tes
(K
mol
e /hr
)
Aug23 Aug24 Aug25 Aug26 Aug27 Aug28 Aug29 Aug30 Aug31 Sep01
Hour (CST)
0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 120
200
400
600
800
1000
1200Area/Nonroad Mobile Point Biogenic Total
OLE
Em
i ss i
o n r
a tes
(K
mol
e /hr
)
Domain total emissions: OLEDomain total emissions: OLE
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
The SMOKEThe SMOKEsystem system (BEIS3)(BEIS3)
The The EPS2EPS2system system (GloBEIS(GloBEIS3)3)
BiogenicBiogenicemissionsemissions
0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12
0
50
100
150
200
250
300Area/Nonroad Mobile Point Biogenic Total
ET
H E
mi s
sion
ra t
e s (
Km
o le /
h r)
Aug23 Aug24 Aug25 Aug26 Aug27 Aug28 Aug29 Aug30 Aug31 Sep01
Hour (CST)
0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 12 0 120
50
100
150
200
250
300Area/Nonroad Mobile Point Biogenic Total
ET
H E
mi s
sion
ra t
e s (
Km
o le /
h r)
Domain total emissions: ETHDomain total emissions: ETH
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
The SMOKEThe SMOKEsystem system (BEIS3)(BEIS3)
The The EPS2EPS2system system (GloBEIS(GloBEIS3)3)
No biogenicNo biogenicemissions!!emissions!!
BiogenicBiogenicemissionsemissions
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
CMAQ results: Daily Max. O3 Concentration CMAQ results: Daily Max. O3 Concentration
0
20
40
60
80
100
120
140
160EPS2+GloBEIS3 SMOKE+BEIS3 SMOKE+GloBEIS3
Aug23 Aug24 Aug25 Aug26 Aug27 Aug28 Aug29 Aug30 Aug31
Dai
ly m
a xim
um c
once
n tra
t ion
(ppb
)
Ambient O3 (TCEQ 4km Domain)
Hour (UTC)
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
06AM (CST)06AM (CST) 09AM09AM NoonNoon
03PM03PM 06PM06PM 09PM09PM
CMAQ results: O3(EPS2+GB3) – O3(SMOKE+B3)CMAQ results: O3(EPS2+GB3) – O3(SMOKE+B3)
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
06AM (CST)06AM (CST) 09AM09AM NoonNoon
03PM03PM 06PM06PM 09PM09PM
CMAQ results: O3(EPS2+GB3) – O3(SMOKE+GB3)CMAQ results: O3(EPS2+GB3) – O3(SMOKE+GB3)
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
06AM (CST)06AM (CST) 09AM09AM NoonNoon
03PM03PM 06PM06PM 09PM09PM
CMAQ results: O3(SMOKE+B3) – O3(SMOKE+GB3)CMAQ results: O3(SMOKE+B3) – O3(SMOKE+GB3)
ConclusionsConclusions
After CMAQ simulations using TEI, the SMOKE and EPS2 systems present more than 20 ppb differences in localized ambient ozone concentrations for the HGA.
Different VOC split factors including land use land cover and meteorological data present different biogenic emissions in BEIS3 and GloBEIS3.
Surrogates, chemical split factors and temporal Surrogates, chemical split factors and temporal profiles will be harmonized to test the system profiles will be harmonized to test the system algorithm differencesalgorithm differences in SMOKE and EPS2 in the in SMOKE and EPS2 in the near future. near future.
SMOKE and EPS2 present different emission rates of each VOC species for Texas EI after spatial allocation, chemical speciation, and temporal allocation due to different inputs of cross-reference and profile data.
Institute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality StudiesInstitute for Multi-dimensional Air Quality Studies
BEIS3 will reprocessed with PAR, LULC and BEIS3 will reprocessed with PAR, LULC and temperature data used in GloBEIS3. temperature data used in GloBEIS3.