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Page 1: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 1

Ionization Imaging:a better way to search for

0-v decay?

David Nygren

LBNL Physics Division

Page 2: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 2

Two Types of Double Beta Decay

This process not yet observedparticle = antiparticle

Neutrinoless double beta decay lifetime

Neutrino effective

mass

A known background process and an important calibration tool

Z

0

2

22

2

1

1mG

T×Μ×=

.1019

2

1 yrsT ≈

Page 3: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 3

0-v Decay

• If 0-v decays occur, then:– Neutrino mass ≠0 (now we know this!)

– Decay rate measures effective mass mv

– Neutrinos are Majorana particles– Lepton number is not conserved

• Because the physics impact is so great, the experimental result must be robust.

Page 4: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 4

Uncertainties…

• Hierarchy uncertaino Determines needed sensitivity

• Matrix element calculations uncertaino Order of magnitude in rate

• Effective mass uncertaino Phases enter: mv

= |∑ |Uei|2 imi |• Direct tests by 3H kinematics uncertain

o For mv << 1 eV, technically very difficult!

• Best experimental approach: uncertain!

Page 5: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 5

A “Robust” Experiment:

Only

2-v decays!

Rate

Energy Q-value

Only

0-v decays!

No backgrounds above Q-value!

The experimental result is a spectrum of all events, with very small or negligible backgrounds.

0

Page 6: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 6

A robust experiment:

• Has negligible overlap of 0- and 2- events – excellent energy resolution is essential!

• Selects 0-v and 2-v events identically– does not depend solely on end-point energy!

• Scales to large active mass – M ~ 1/ mv2 >1000 kg needed?

• Rejects all backgrounds effectively– no insensitive surfaces!

Page 7: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 7

Energy Resolution

Germanium Detectors:– Excellent electron and hole mobilities

• Complete charge collection

– Small level of recombination• Charge collection independent of track topology

– Small energy per ion/electron pair • Fluctuations small

The Gold Standard:

Energy resolution with Germanium detector:

E/E ~ 1.25 x 10-3 FWHM at 2.6 MeV

Page 8: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 8

Energy Resolution

“Extra margin in energy resolution is very desirable because non-gaussian characteristics are often present in the tails of the experimental distribution.”

“To realize an energy resolution near the limit imposed by physical processes, the detector and target must be the same.”

Page 9: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 9

Using Energy to Detect

Spectra from Ludwig DeBraekeleer

1. Get a large quantity of candidate nuclei2. Put them in an electron detector3. Shield and purify4. Acquire data for a few years (“plug and pray”)5. Cut on energy to select out the neutrinoless events

100’s of kg target - Condensed matter strongly preferred

Theory

Practice

Spectra from Klapdor Kleingrothaus et. al.

positive signal claim is disputed!

Background rejection is essential - energy resolution may not be enough !

Esum of 2 final state electrons

Page 10: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 10

Present Status

• Heidelberg-Moscow (H-M) claim:

mv = 0.44 +0.14-0.20 eV (best value) disputed!

0v1/2 = (8 — 18.3) x 1024 y (95% c.l.)

Scale: ~11 kg of 76Ge, for ~7 years

No other claim for a positive result exists

Page 11: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 11

Worldwide Activity• CAMEO.........• CANDLES.....• COBRA.........• CUORE.........• DCBA............• EXO..............• GERDA.........• GSO..............• Majorana.......• MOON...........• Nano-crystals• Super-NEMO• Xe.................• XMASS.........

CdWO4 crystals in liquid scintillator

CaF2 crystals in liquid scintillatorCdTe semiconductors

TeO2 bolometers, Cuoricino nowNd foils and tracking chambersXe TPC; liquid now, maybe gas laterGermanium crystals in LN

Gd2SiO5 crystals in liquid scintillatorSegmented Ge crystalsMo foils and plastic scintillatorsSuspended nanoparticlesFoils with trackingXe dissolved in liquid scintillatorLiquid xenon

Page 12: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 12

Present Perspective…

• Cuoricino (130Te): background-limited

E/E only Cuore needs factor of ~20

• Majorana (76Ge): pre-construction stage

E/E + multi-site rejection (x10), but – a factor of several 100 needed beyond HM

• Common to both:– Multi-detector coincidences can reject many

backgrounds, but:– Large rejection factor needed for success

Page 13: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 13

Xenon

• Qv = 2.49 MeV (136Xe)• Previous experiments inconclusive

– HPXe TPC in Gotthard tunnel (5 bar, no start time)

– Russian experiments with various MWPC

• EXO– EXO-200 underway with LXe @ WIPP– No laser tagging of barium daughter: R&D stage – Strong anti-correlation of ionization/scintillation– Results eagerly awaited

Page 14: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 14

NUSAG Recommendations:

• “…support research in two or more 0-v experiments to explore the region of degenerate neutrino masses (mv > 100 meV)…”

• “The knowledge gained and the technology developed in the first phase should then be used in a second phase to extend exploration into the inverted hierarchy region of (mv > 10 - 20 meV) with a single experiment.”

But: no explicit encouragement for new ideas!

Page 15: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 15

Experimental Approach

“We believe that an

Imaging Ionization Chamber is most likely to meet all criteria imposed

for a robust experiment.”

An Imaging Ionization Chamber (IIC) is

a TPC without gain at the readout plane

Page 16: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 16

Imaging Ionization Chamber

-HV planePixel Readout planePixel Readout plane

.

ionselectrons

~99%Xe + ~1% CH4

@ 20 bars

Page 17: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 17

Proportional Gain: good results for low-energy x-rays

MWPC, GEM, micromegas all work well...

but:why are there so many events below the peak?

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SCIPP - November 14, 2006 18

Proportional Gain: poor resolution for MeV energies

Typical E/E: 4 - 6.6% FWHM @ 2.5 MeV– Gain variations?

• gas density, composition • mechanics, calibration maps

– Extended tracks? • ballistic deficit in signal processing• impact of space charge on gain

– Intrinsic physical phenomena?• sensitivity to dE/dx density variations

• large scintillation/ionization fluctuations

Page 19: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

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Ionization Chamber Mode

• Reason # 1:– “Best energy resolution can only be

obtained through direct charge integration”• There is a lot to learn here...

• Reason # 2:– “Gain may be needed at HV plane…”

• This is a new, but very speculative aspect

Page 20: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 20

Imaging Ionization Chamber is filled with 136Xe gas

• Xe is relatively safe and easy to enrich• EXO has 200 kg highly enriched in 136Xe

• high density is desirable to contain event• But there is an upper limit: < 0.55 g/cm3

• working density: ~ 0.1 g/cm3 (LXe = 2.95 g/cm3)• ~20 bars; critical point P = 58 bars, T = 290° K• 1000 kg in ~10 m3 : = 200 cm, L =300 cm• dn/dx ~ 1 fC/cm = 6000 electron/ion pairs/cm

Page 21: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 21

UV Scintillation in HPXe

• N ~ Nelectron/ion pairs ~ 118,000 at Q = 2.49 MeV – can use for event start time– ratio depends on E field

– spectrum peaks at ~170 nm ~ 7 eV

• However, small amount of “CH4” is necessary– to cool electron drift and keep diffusion low for tracking

• Does methane absorb 170 nm light? - No• Does methane quench scintillation? - don’t know, but

– 2% added to LXe without loss! – Does HPXe behave similarly? maybe...

Page 22: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 22

Imaging Ionization Chamber…

• “provides adequate S/N for good tracking”– detailed imaging of event topologies

• “provides fully closed, active fiducial surface”– ex post facto variable definition with mm resolution

• “provides energy resolution of 1% FWHM”– avoids scintillation/ionization anti-correlation

• “may permit detection of birth of Ba daughter”– automatic process tags both space and time

Page 23: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 23

Event Characteristics in IIC

– High density of xenon constrains event:• Total track length ~10 - 20 cm max

– Multiple scattering will be prominent in xenon• Unclear if B-field would help identification

– True events will have two “blobby” ends• Shown to reject background by ~30 in Gotthard TPC

– Bremsstrahlung and fluorescence ’s• Distinct satellite “blobs” may be visible

Page 24: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 24

Imaging Ionization Chamber

has a fully “decorated” pixel readout plane – no grids or wires: eliminates microphonics

– pixel size is 5 mm x 5 mm (4 x 104 /m2)• ~ 40 - 80 contiguous “hit” pixels for E = Q

• dn/dx = ~3000 electrons/(5mm)

– ultra-low noise readout electronics - BNL ASIC• <n> = ~30 e– rms for 4 s shaping time, with pixel!

• Other noise terms must be included <n>= 60 e– rms?

– “waveform capture” essential for extended tracks

Page 25: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 25

Pixel geometry

A low capacitance solution: a 7-pixel hexagonal sub-module:

Or, a 16 channel 4x4 rectangular array…

Page 26: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 26

Imaging Ionization Chamber

collects electrons on pixel readout plane– all energy information is derived from q = Idt– current is very small until electrons approach pixel– pixels with no net charge have bipolar currents

– drift velocity is small, 0.1< Vd <0.5 cm/s

– diffusion after 1.5 m drift is ~ 2 mm rms– event is reconstructed from contiguous hit pixels– noise adds only from hit pixels + some neighbors

Page 27: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

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Energy Resolution…

Q-value of 136Xe = 2.48 MeVW = E per ion/electron pair = 21 eVN = number of ion pairs = Q/WN 2.49 x 106 eV/21 eV = 118,350

N2 = FN (0.05 < F < 0.17)

F = 0.17 for pure noble gases (theory)

N = (FN)1/2 ~ 140 electrons rms

Page 28: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 29

Energy Resolution…

• If ionization were the only issue:E/E = 2.9 x 10-3 FWHM

• Other contributions:– electronic noise from N = 49 pixels in event

• N1/2 x <n> if noise is gaussian ~ 7 x 60 = 430 e–

– ballistic deficit in signal processing – “locked” charge caused by slow-moving ions

E/E < 10.0 x 10-3 FWHM

Page 29: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 31

IIC and Imaging Power

• The 3-D imaging of the IIC provides:– Topology reconstruction– Energy resolution independent of scale– Active and continuous fiducial surfaces– Variable fiducial surfaces ex post facto

Rejection of ionizing backgrounds from surfaces can be essentially 100%

Page 30: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 32

Perspective

• The basic IIC concept offers:– Stable operation: ionization mode– Excellent energy resolution: ~1% FWHM– Good scaling: active mass ~1000 kg– No dead surfaces: 3-D event placement– Active, adjustable fiducial boundaries– Topological rejection of backgrounds– Possibility to evolve further…

Page 31: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 33

Barium Daughter Atom

– In a volume of ~1027 xenon atoms, a event creates one barium atomic ion.

– The Ba ion drifts out to the HV plane, and in ~ 1 second, the ion will be lost!

– Is this a hopeless situation?

Page 32: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 34

Barium Daughter Atom

– In xenon/CH4, the Ba++ ion will survive:

• IP(Xe) = 12.13 eV, IP(CH4) = 13.0 eV• First IP(Ba+) = 5.212 eV• Second IP(Ba++) = 10.004 eV

– if impurities exist with IP less than 10 eV:• Ba++ becomes Ba+ through charge exchange

Page 33: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 35

Ion Mobilities

Is there a straightforward way to detect and identify the barium daughter?

• Ba and Xe ion masses are ~identical…

• Ba+ and Xe+ ion charges are identical…

• Ion mobilities should be the ~same, Right??

Page 34: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 36

Ion Mobilities…

• But: Ion mobilities are quite different!– The cause is resonant charge exchange– RCE is macroscopic quantum mechanics

• occurs only for ions in their parent gases • no energy barrier exists for Xe+ in xenon • energy barrier exists for Ba ions in xenon• resonant charge exchange is a long-range

process; glancing collisions = back-scatter

– RCE increases viscosity of ions

Page 35: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 37

Ion Mobilities in Xenon

– Mobility differences have been measured at low pressures, where clustering effects are small: (Xe+) = 0.6 cm2/V-sec (Cs+) = 0.88 cm2/V-sec (Cs is between Ba and Xe)

– So, the barium ion should move faster by ~50%! (maybe even faster if Ba++ is stable)

RCE can provide a way to detect Ba daughter!

Page 36: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 38

Ion mobility in dense gases?

• Ion mobility data at high pressure does not apparently exist in the literature.– Clustering may be prominent at 20 bars.– Clustering phenomena are complex, and

may introduce very different behavior• Not clear whether this will help or hurt!• Low pressure measurements not adaptable to

high pressures like 20 bars - need new method

Page 37: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 39

Ba Daughter Detection

• If we assume that barium ion mobility is not identical to xenon ion mobility, then:

• A barium ion will arrive at the HV plane at a different time than the Xe+ ion track image.

• If event time origin and mobilities of the barium and xenon ions are known, an arrival time for the barium daughter at HV plane is predicted.

• The unique t between Xe+ and Ba+ ions is a robust signature for a true event.

Page 38: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 40

Arrival Time Separation

• Assume low-pressure data…– Assume drift distance: L= T = 250 mm– Thermal transport diffusion: ~ .25 mm

/L = 0.25/250 = 1/1000

/(L) = 21/2/(Ba - Xe)T ~ 1/235

– Arrival times are very precisely determined

Page 39: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 41

Detection of Ion Arrival

• Detection of ion arrival may be possible:– Ions drift at thermal energies to HV plane…

Then: – Ions are attracted to “high field pore (HFP)”

• Very high electric field inside HFP • Ions can enter, but electrons are blocked• High energy tail of M-B distribution relevant• Ba++ may be critical for desired outcome • Hoped-for outcome: ≥1 electron appears

Page 40: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 42

Blind GEM or “Microwell”

Drift region: Low E-field

ions

Very High E-field inside pore; low work-function surface?

Resistive back side blocked to electrons

HV plane

Page 41: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 43

The barium daughter “Echo”

– If a single electron appears, high E-field in blind GEM causes electron avalanche.

– Electron avalanche will saturate, producing a large pulse of electrons, more than 103.

– Electron pulse returns to pixel plane, at a spot on the projected event track.

– This spot on the projected track is very close to origin of the barium daughter.

Page 42: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 44

“Birth Detection”

Because the echo tagging is so precise

in space and time

(if it can be done at all)

I refer to this process as

“Birth detection”

Page 43: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 45

The Return Image Echo

• The Xe+ ions will also enter HFP, producing an “echo” of the track.

• The track echo time will be distinct from the pulse due to the barium daughter.

• Maybe: transfer charge to C2H4: IP =11.6 eV– Complex organic molecule may be much less

likely to liberate electrons than Ba++ or Ba+

– Will a mobility difference still exist?

Page 44: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 46

Event Quality

• strong primary UV scintillation gives to

– Enough intensity, even at low visible energy

• electron track image provides topology– Energy resolution limited by electronic noise

• ion track echo also places event in space– Don’t need all 115,000 echoes from HV plane

• barium daughter echo is elegant tag method– Can some detection scheme be found?

• an over-constrained reconstruction possible.

Page 45: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 47

Imaging Ionization Chamber

-HV planePixel Readout planePixel Readout plane

.

ionselectrons

Page 46: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 48

What to do?

• An R&D (and library) effort is needed to:– Develop good simulation tools– Optimize S/N with real electronics– Measure E/E in HPXe IIC with rays– Investigate benefits of organic additives– Determine ion mobilities in HPXe.– Explore ion-induced avalanche processes

Page 47: SCIPP - November 14, 20061 Ionization Imaging: a better way to search for 0- v  decay? David Nygren LBNL Physics Division

SCIPP - November 14, 2006 49

What to do?

• An R&D (and library) effort is needed to:– Develop good simulation tools– Optimize S/N with real electronics– Measure E/E in HPXe IIC with rays– Investigate benefits of organic additives– Determine ion mobilities in HPXe.– Explore ion-induced avalanche processes

• A proposal has been rejected by DOE!

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Summary

• A novel concept for a robust 0- decay search has been developed: E/E ~ 1% FWHM – Detailed & constrained 3-D event topology – Active, variable fiducial boundaries– Identification of Ba daughter possible, in

principle, by exploitation of macroscopic quantum mechanical phenomenon, RCE

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SCIPP - November 14, 2006 54

Acknowledgments

• Azriel Goldschmidt - LBNL

• Adam Bernstein - LLNL

• Mike Heffner - LLNL

• Jacques Millaud - LLNL/LBNL

• Leslie Rosenberg - UW