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Loss compensation in long-range dielectric- loaded surface plasmon-polariton waveguides Sonia M. García-Blanco, 1,* Markus Pollnau, 1 and Sergey I. Bozhevolnyi 2 1 Integrated Optical MicroSystems Group, MESA+ Institute for Nanotechnology, University of Twente, P.O. Box 217, 7500 AE Enschede, The Netherlands 2 Institute of Technology and Innovation, University of Southern Denmark, DK-5230 Odense, Denmark * [email protected] Abstract: Loss compensation in long-range dielectric-loaded surface plasmon-polariton waveguides is theoretically analyzed when rare-earth- doped double tungstate crystalline material is used as the gain medium in three different waveguide configurations. We study the effect of waveguide geometry on loss compensation at the telecom wavelength of 1.55 μm, and demonstrate that a material gain as small as 12.5 dB/cm is sufficient for lossless propagation of plasmonic modes with sub-micron lateral confinement when using waveguide ridges with gain. 2011 Optical Society of America OCIS codes: (250.5403) Plasmonics; (230.7370) Waveguides; (160.5690) Rare-earth doped materials; (230.4480) Optical amplifiers. References and links 1. Q. Min, C. Chen, P. Berini, and R. Gordon, “Long range surface plasmons on asymmetric suspended thin film structures for biosensing applications,” Opt. Express 18, 19009-19019 (2010). 2. M. Mansuripur, A. R. Zakharian, A. Lesuffleur, S.-H. Oh, R. J. Jones, N. C. Lindquist, H. Im, A. Kobyakov, and J. V. Moloney, “Plasmonic nano-structures for optical data storage,” Opt. Express 17, 14001-14014 (2009). 3. H. A. Atwater and A. Polman, “Plasmonics for improved photovoltaic devices,” Nat. Mater. 9, 205-213 (2010). 4. S. I. Bozhevolnyi, Plasmonic Nanoguides and Circuits (Pan Stanford Publishing Pte. Ltd, Singapore, 2009). 5. J. Gosciniak, S. I. Bozhevolnyi, T. B. Anndersen, V. S. Volkov, J. Kjelstrup-Hansen, L. Markey, and A. Dereux, “Thermo-optic control of dielectric-loaded plasmonic waveguide components,” Opt. Express 18, 1207- 1216 (2010). 6. O. Tsilipakos, E. E. Kriezis, and S. I. Bozhevolnyi, “Thermo-optic microring resonator switching elements made of dielectric-loaded plasmonic waveguides,” J. Appl. Phys. 109, 0703111 (2011). 7. A. V. Krasavin and A. V. Zayats, “Silicon-based plasmonic waveguides,” Opt. Express 18, 11791-11799 (2010). 8. S. A. Maier, “Plasmonics: The promise of highly integrated optical devices,” IEEE J. Sel. Top. Quantum Electron. 12, 1671-1677 (2006). 9. R. F. Oulton, V. J. Sorger, D. A. Genov, D. F. P. Pile, and X. Zhang, “A hybrid plasmonic waveguide for subwavelength confinement and long-range propagation,” Nat. Photonics 2, 496-500 (2008). 10. J. A. Dionne, L. A. Sweatlock, H. A. Atwater, and A. Polman, “Plasmon slot waveguides: Towards chip-scale propagation with subwavelength-scale localization,” Phys. Rev. B 73, 035407 (2006). 11. S. I. Bozhevolnyi, V. S. Volkov, E. Devaux, J.-Y. Laluet, and T. W. Ebbesen, “Channel plasmon subwavelength waveguide components including interferometers and ring resonators,” Nature 440, 508-5011 (2006). 12. A. Degiron, S.-Y. Cho, C. Harrison, N. M. Jokerst, C. Dellagiacoma, O. J. F. Martin, and D. R. Smith, “Experimental comparison between conventional and hybrid long-range surface plasmon waveguide bends,” Phys. Rev. A 77, 021804 (2008). 13. T. Holmgaard and S. I. Bozhevolnyi, “Theoretical analysis of dielectric-loaded surface plasmon-polariton waveguides,” Phys. Rev. B 75, 245405 (2007). 14. P. Berini, “Plasmon-polariton waves guided by thin lossy metal films of finite width: Bound modes of symmetric structures,” Phys. Rev. B 61, 10484-10503 (2000). 15. T. Holmgaard, J. Gosciniak, and S. I. Bozhevolnyi, “Long-range dielectric-loaded surface plasmon polariton waveguides,” Opt. Express 18, 23009-23015 (2010). 16. J. Gosciniak, T. Holmgaard, and S. I. Bozhevolnyi, “Theoretical analysis of long-range dielectric-loaded surface plasmon polariton waveguides,” J. Lightwave Technol. 29, 1473-1481 (2011). #154169 - $15.00 USD Received 6 Sep 2011; revised 29 Sep 2011; accepted 29 Sep 2011; published 23 Nov 2011 (C) 2011 OSA 5 December 2011 / Vol. 19, No. 25 / OPTICS EXPRESS 25298

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Page 1: Loss compensation in long-range dielectric- loaded surface plasmon-polariton waveguides · 2017-04-01 · Loss compensation in long-range dielectric-loaded surface plasmon-polariton

Loss compensation in long-range dielectric-loaded surface plasmon-polariton waveguides

Sonia M. García-Blanco,1,* Markus Pollnau,1 and Sergey I. Bozhevolnyi2 1Integrated Optical MicroSystems Group, MESA+ Institute for Nanotechnology,

University of Twente, P.O. Box 217, 7500 AE Enschede, The Netherlands 2Institute of Technology and Innovation,

University of Southern Denmark, DK-5230 Odense, Denmark *[email protected]

Abstract: Loss compensation in long-range dielectric-loaded surface

plasmon-polariton waveguides is theoretically analyzed when rare-earth-

doped double tungstate crystalline material is used as the gain medium in

three different waveguide configurations. We study the effect of waveguide

geometry on loss compensation at the telecom wavelength of 1.55 µm, and

demonstrate that a material gain as small as 12.5 dB/cm is sufficient for

lossless propagation of plasmonic modes with sub-micron lateral

confinement when using waveguide ridges with gain.

2011 Optical Society of America

OCIS codes: (250.5403) Plasmonics; (230.7370) Waveguides; (160.5690) Rare-earth doped

materials; (230.4480) Optical amplifiers.

References and links

1. Q. Min, C. Chen, P. Berini, and R. Gordon, “Long range surface plasmons on asymmetric suspended thin film

structures for biosensing applications,” Opt. Express 18, 19009-19019 (2010).

2. M. Mansuripur, A. R. Zakharian, A. Lesuffleur, S.-H. Oh, R. J. Jones, N. C. Lindquist, H. Im, A. Kobyakov,

and J. V. Moloney, “Plasmonic nano-structures for optical data storage,” Opt. Express 17, 14001-14014 (2009).

3. H. A. Atwater and A. Polman, “Plasmonics for improved photovoltaic devices,” Nat. Mater. 9, 205-213 (2010).

4. S. I. Bozhevolnyi, Plasmonic Nanoguides and Circuits (Pan Stanford Publishing Pte. Ltd, Singapore, 2009).

5. J. Gosciniak, S. I. Bozhevolnyi, T. B. Anndersen, V. S. Volkov, J. Kjelstrup-Hansen, L. Markey, and A.

Dereux, “Thermo-optic control of dielectric-loaded plasmonic waveguide components,” Opt. Express 18, 1207-

1216 (2010).

6. O. Tsilipakos, E. E. Kriezis, and S. I. Bozhevolnyi, “Thermo-optic microring resonator switching elements

made of dielectric-loaded plasmonic waveguides,” J. Appl. Phys. 109, 0703111 (2011).

7. A. V. Krasavin and A. V. Zayats, “Silicon-based plasmonic waveguides,” Opt. Express 18, 11791-11799

(2010).

8. S. A. Maier, “Plasmonics: The promise of highly integrated optical devices,” IEEE J. Sel. Top. Quantum

Electron. 12, 1671-1677 (2006).

9. R. F. Oulton, V. J. Sorger, D. A. Genov, D. F. P. Pile, and X. Zhang, “A hybrid plasmonic waveguide for

subwavelength confinement and long-range propagation,” Nat. Photonics 2, 496-500 (2008).

10. J. A. Dionne, L. A. Sweatlock, H. A. Atwater, and A. Polman, “Plasmon slot waveguides: Towards chip-scale

propagation with subwavelength-scale localization,” Phys. Rev. B 73, 035407 (2006).

11. S. I. Bozhevolnyi, V. S. Volkov, E. Devaux, J.-Y. Laluet, and T. W. Ebbesen, “Channel plasmon subwavelength

waveguide components including interferometers and ring resonators,” Nature 440, 508-5011 (2006).

12. A. Degiron, S.-Y. Cho, C. Harrison, N. M. Jokerst, C. Dellagiacoma, O. J. F. Martin, and D. R. Smith,

“Experimental comparison between conventional and hybrid long-range surface plasmon waveguide bends,”

Phys. Rev. A 77, 021804 (2008).

13. T. Holmgaard and S. I. Bozhevolnyi, “Theoretical analysis of dielectric-loaded surface plasmon-polariton

waveguides,” Phys. Rev. B 75, 245405 (2007).

14. P. Berini, “Plasmon-polariton waves guided by thin lossy metal films of finite width: Bound modes of

symmetric structures,” Phys. Rev. B 61, 10484-10503 (2000).

15. T. Holmgaard, J. Gosciniak, and S. I. Bozhevolnyi, “Long-range dielectric-loaded surface plasmon polariton

waveguides,” Opt. Express 18, 23009-23015 (2010).

16. J. Gosciniak, T. Holmgaard, and S. I. Bozhevolnyi, “Theoretical analysis of long-range dielectric-loaded surface

plasmon polariton waveguides,” J. Lightwave Technol. 29, 1473-1481 (2011).

#154169 - $15.00 USD Received 6 Sep 2011; revised 29 Sep 2011; accepted 29 Sep 2011; published 23 Nov 2011(C) 2011 OSA 5 December 2011 / Vol. 19, No. 25 / OPTICS EXPRESS 25298

Page 2: Loss compensation in long-range dielectric- loaded surface plasmon-polariton waveguides · 2017-04-01 · Loss compensation in long-range dielectric-loaded surface plasmon-polariton

17. M. A. Noginov, V. A. Podolskiy, G. Zhu, M. Mayy, M. Bahoura, J. A. Adegoke, B. A. Ritzo, and K. Reynolds,

“Compensation of loss in propagating surface plasmon polariton by gain in adjacent dielectric medium,” Opt.

Express 16, 1385-1392 (2008).

18. M. C. Gather, K. Meerholz, N. Danz, and K. Leosson, “Net optical gain in a plasmonic waveguide embedded in

a fluorescent polymer,” Nat. Photonics 4, 457-461 (2010).

19. J. Grandinier, G. Colas des Francs, S. Massenot, A. Bouhelier, L. Markey, J.-C. Weeber, C. Finot, and A.

Dereux, “Gain-assisted propagation in a plasmonic waveguide at telecom wavelength,” Nano Lett. 9, 2935-2939

(2009).

20. I. De Leon and P. Berini, “Amplification of long-range surface plasmons by a dipolar gain medium,” Nat.

Photonics 4, 382-387 (2010).

21. X. Zhang, Y. Li, T. Li, S. Y. Lee, C. Feng, L. Wang, and T. Mei, “Gain-assisted propagation of surface plasmon

polaritons via electrically pumped quantum wells,” Opt. Lett. 35, 3075-3077 (2010).

22. M. Z. Alam, J. Meier, J. S. Aitchison, and M. Mojahedi, “Gain assisted surface plasmon polaritons in quantum

wells structures,” Opt. Express 15, 176-182 (2007).

23. A. V. Krasavin, T. P. Vo, W. Dickson, P. M. Bolger, and A. V. Zayats, “All-plasmonic modulation via

stimulated emission of copropagating surface plasmon polaritons on a substrate with gain,” Nano Lett. 11,

2231-2235 (2011).

24. P. M. Bolger, W. Dickson, A. V. Krasavin, L. Liebscher, S. G. Hickey, D. V. Skryabin, and A. V. Zayats,

“Amplified spontaneous emission of surface plasmon polaritons and limitations on the increase of their

propagation length,” Opt. Lett. 35, 1197-1199 (2010).

25. I. P. Radko, M. G. Nielsen, O. Albrektsen, and S. I. Bozhevolnyi, “Stimulated emission of surface plasmon

polaritons by lead-sulphide quantum dots at near infra-red wavelengths,” Opt. Express 18, 18633-18641 (2010).

26. R. M. Ma, R. F. Oulton, V. J. Sorger, G. Bartal, and X. Zhiang, “Room-temperature sub-diffraction-limited

plasmon laser by total internal reflection,” Nat. Materials 10, 110-113 (2011).

27. R. A. Flynn, C. S. Kim, I. Vurgaftman, M. Kim, J. R. Meyer, A. J. Mäkinen, K. Bussmann, L. Cheng, F. S.

Choa, and J. P. Long, “A room temperature semiconductor spaser operating near 1.5 µm,” Opt. Express 19,

8954-8961 (2011).

28. M. T. Hill, Y.-S. Oei, B. Smalbrugge, Y. Zhu, T. De Vries, P. J. Van Veldhoven, F. W. M. Van Otten, T. J.

Eijkemans, J. P. Turkiewicz, H. De Waardt, E. Jan Geluk, S.-H. Kwon, Y.-H. Lee, R. Notzel, and M. K. Smit,

“Lasing in metallic-coated nanocavities,” Nat. Photonics 1, 589-594 (2007).

29. D. Geskus, S. Aravazhi, S. M. García-Blanco, and M. Pollnau, “Giant optical gain in a rare-earth-ion-doped

microstructure,” Adv. Mater., accepted (2011).

30. J. D. B. Bradley, M. Costa e Silva, M. Gay, L. Bramerie, A. Driessen, K. Wörhoff, J. C. Simon, and M. Pollnau,

“170 Gbit/s transmission in Al2O3:Er3+ integrated amplifiers,” Opt. Express 17, 22201-22208 (2009).

31. E. H. Bernhardi, H. A. G. M. van Wolferen, L. Agazzi, M. R. H. Khan, C. G. H. Roeloffzen, K. Wörhoff, M.

Pollnau, and R. M. de Ridder, “Ultra-narrow-linewidth, single-frequency distributed feedback waveguide laser

in Al2O3:Er3+ on silicon,” Opt. Lett. 35, 2394-2396 (2010).

32. N. V. Kuleshov, A. A. Lagatsky, A. V. Podlipensky, V. P. Mikhailov, and G. Huber, “Pulsed laser operation of

Yb-doped KY(WO4)2 and KGd(WO4)2,” Opt. Lett. 22, 1317-1319 (1997).

33. M. L. Theye, “Investigation of the optical properties of Au by means of thin semitransparent films,” Phys. Rev.

B 2, 3060-3078(1970).

34. R. H. French, J. M. Rodríguez-Parada, M. K. Yang, R. A. Derryberry, and N. T. Pfeiffenberger, “Optical

properties of polymeric materials for concentrator photovoltaic systems,” Sol. Energ. Mat. Sol. C. 95, 2077-

2086 (2011).

35. PhoeniX B.V., Hengelosestraat 705, 7521PA, Enschede, Netherlands.

1. Introduction

Surface plasmon polaritons (SPPs), evanescent electromagnetic waves propagating along

metal-dielectric interfaces, have been the subject of numerous studies due to their unique

properties promising applications in a variety of fields, such as optical biosensing [1], data

storage [2], photovoltaic cells [3], and highly integrated photonic circuits [4]. The great

interest in plasmonic waveguides is largely due to their capability to confine the

electromagnetic field below the diffraction limit, which can potentially lead to photonic

circuits suitable for very large scale integration [4]. Another interesting feature of SPP

waveguides is the high sensitivity to their immediate environment that makes them very

attractive for realizing ultra-sensitive optical sensors [1]. Furthermore, the presence of metal

in the midst of propagating mode fields enables a direct and very efficient electrical control of

their propagation characteristics by making use of, for example, thermo-optic effects [5, 6].

#154169 - $15.00 USD Received 6 Sep 2011; revised 29 Sep 2011; accepted 29 Sep 2011; published 23 Nov 2011(C) 2011 OSA 5 December 2011 / Vol. 19, No. 25 / OPTICS EXPRESS 25299

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Many different plasmonic waveguiding configurations have been proposed and

demonstrated over the past few years [7-16]. In general, SPP waveguides are subject to a

trade-off between mode-field confinement and propagation loss due to absorption in the

metal, exhibiting either good optical confinement but short propagation distances, typically in

the few tens of micrometers (e.g., dielectric-loaded SPP waveguides [13]), or long

propagation distances (in the millimeter range) that necessitate large mode profiles (e.g., long-

range SPP waveguides [14]). Recently, a novel type of plasmonic waveguide configuration

was proposed, long-range dielectric-loaded surface plasmon-polariton (LR-DLSPP)

waveguides that combine the millimeter-range propagation with a relatively strong mode

confinement [15, 16]. Reduced propagation losses provided by this novel structure (albeit at

the expense of higher tolerances and increased complexity of configuration) permit enlarging

the range of gain materials that can be selected for loss compensation.

Many efforts have been directed towards compensating propagation losses in plasmonic

waveguides by use of different gain materials [17-25]. Although providing very high gain,

laser dyes exhibit a limited lifetime due to photo-bleaching, which forces continuous

refreshment of a dye in the solution, making them unpractical for integrated devices.

Semiconductor quantum wells, which are capable of providing exceptionally high material

gain, also encounter difficulties for their integration into plasmonic structures. On the one

hand, a thin insulating layer is needed between the metal and the semiconductor gain material,

which limits the gain available for very confined plasmonic modes. On the other hand, in the

case of larger plasmonic modes, the overlap between this larger mode and the nanometer-

scale quantum well gain region limits the resulting modal gain. Nevertheless, compensation of

plasmonic losses by semiconductor gain materials, leading to lasing, has recently been

demonstrated [26-28].

Very large optical gain, ~950 dB/cm, has recently been achieved in a rare-earth (RE)-

doped double tungstate crystalline waveguide [29]. RE-doped gain materials do not exhibit

the limitations of laser dyes or semiconductor gain materials discussed above. Furthermore,

the optical gain provided by RE ions possesses very interesting features. RE gain materials

can amplify very-high-rate signals in the small-signal-gain regime without distortion [30].

They provide a large gain bandwidth up to a few tens of nanometers, which is interesting for

broadband optical amplification and the generation of ultra-short laser pulses. Finally, they

enable the production of very-narrow-linewidth lasers due to the lack of detrimental linewidth

broadening effects characteristic of semiconductor lasers [31]. When RE ions are doped into a

double tungstate crystal, very large gain can be obtained due to the large absorption and

emission cross-sections of RE ions in these materials [32] and the large dopant concentrations

possible without significant luminescence quenching because of the large inter-ionic

separation provided by the crystalline structure of double tungstates [29].

In this paper, loss compensation in LR-DLSPP waveguides due to optical gain provided

by a RE-doped double tungstate material incorporated into the LR-DLSPP configuration is

theoretically studied. Several structures are discussed in detail. The effect of different

waveguide parameters on the efficiency of the material gain to compensate propagation losses

is evaluated. Lossless propagation is predicted for material gain as low as 12.5 dB/cm, while

maintaining a mode size comparable to conventional dielectric-loaded surface plasmon-

polariton waveguides [13].

2. Proposed structures

The generic LR-DLSPP structure includes a low-refractive-index substrate material, a buffer

layer of a high-refractive-index material, a metal stripe and a dielectric ridge, the dimensions

and refractive index of which should be chosen to balance the electric fields at both sizes of

the gold stripe in order to ensure long-range propagation [15, 16]. The three waveguide

geometries studied in this paper are shown in Fig. 1 and their corresponding material

#154169 - $15.00 USD Received 6 Sep 2011; revised 29 Sep 2011; accepted 29 Sep 2011; published 23 Nov 2011(C) 2011 OSA 5 December 2011 / Vol. 19, No. 25 / OPTICS EXPRESS 25300

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properties are summarized in Table 1. The radiation wavelength utilized throughout this study

is chosen in the telecom wavelength range and equal to 1.55 µm.

The materials considered in this study are selected for their availability in a standard

microfabrication facility. They should be easy to deposit and pattern and the temperatures

involved in the processes should be compatible with previous fabrication steps and integration

onto a CMOS platform. In an attempt to stay as close as possible to the passive structures

proposed in [15, 16], the substrate material chosen is SiO2 (n ~ 1.46) and the metal selected is

gold (ngold = 0.55+j11.5 [33]). The dimensions of the gold stripe were fixed in all cases to a

thickness of 15 nm [15, 16] and a width of 200 nm. In Structures 1 and 2, the gain material,

RE-doped double tungstate with refractive index ~2.05, is added as the buffer layer by direct

bonding . The ridge is made of the photo-patternable polymer benzocyclobutene (BCB) in

Structure 1 (nBCB ~ 1.535) and of polyimide (n ~ 1.9 [34]) in Structure 2. The effect of ridge

material and dimensions on the efficiency of material gain to compensate the plasmonic losses

was analyzed. Finally, in the third structure, the buffer layer is chosen as Si3N4 (nSi3N4 ~2.05)

and the gain is added to the ridge instead of the buffer layer. A 100-nm-thin BCB adhesive

layer is introduced between the buffer layer and the ridge as part of the integration of the gain

material to the structure. Although this configuration leads to a more involved fabrication and

integration process, it drastically reduces the necessary material gain for lossless propagation.

Fig. 1. Layout of the LR-DLSPP structures with gain analyzed in this work. (a) Gain material, RE-doped double

tungstate, as buffer layer and ridge in BCB. (b) Gain material in the buffer and polyimide ridge. (c) Gain material in

the ridge, buffer layer in silicon nitride and 100-nm-thin BCB adhesive layer between buffer and ridge.

Table 1. Parameters of the structures used for the simulations.

Structure 1 Structure 2 Structure 3

Buffer Material RE double tungstate RE double tungstate Si3N4

hbuffer [µm] 0.04-0.13 0.25-0.4 0.2-0.5

nbuffer 2.05 2.05 2.05

Ridge Material BCB Polymide RE double tungstate

hridge [µm] 1-1.6 0.6-1.6 0.5-0.8

wridge [µm] 1-1.6 0.6-1.6 0.5-0.8

nridge 1.535 1.9 2.05

Metal Material Gold

ngold 0.55+j11.5

Substrate Material SiO2

ns 1.45

3. Finite difference calculations

Finite difference (FD) calculations with perfect magnetic conductor (PMC) boundary

conditions were carried out using the FieldDesigner module of PhoeniX B.V. [35]. A

perfectly matched layer (PML), which absorbs both outgoing and reflected radiation, was also

#154169 - $15.00 USD Received 6 Sep 2011; revised 29 Sep 2011; accepted 29 Sep 2011; published 23 Nov 2011(C) 2011 OSA 5 December 2011 / Vol. 19, No. 25 / OPTICS EXPRESS 25301

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applied around the calculation window. A sufficiently large calculation window, 20 µm by

20 µm, was used. Special attention was paid to the grid size due to the large difference in

dimension between the different parts of the simulated structure (i.e., thickness of the gold

layer, 15 nm, and buffer layer, 40-500 nm, versus height of the ridge in the micrometer range).

FieldDesigner permits the utilization of a dynamic grid. In order to ensure that enough grid

points were assigned to the thinner layers (i.e., buffer and gold layer) present in the y-

direction, these thin structures were artificially divided in the required number of sublayers. In

such configuration, the software assigns at least a grid point at the interface between two such

sublayers. The number of layers was selected so that the addition of more layers only

produced negligible variation in the results. Such construction permits using 129 × 129 grid

points without loss of accuracy when compared with the results obtained with a mesh of

129 × 1025 grid points (i.e., denser grid in the y-direction), but drastically reducing the

computation time. In the x-direction, the dimensions are relatively large and, therefore, such

construction was not necessary. Fig. 2 shows an example of the mesh utilized in the

simulations for Structure 1. In the metal, a grid size of 0.75 nm was utilized (i.e., the metal

stripe of 15 nm thickness was represented by 20 sublayers). Such a fine mesh size sufficiently

resolves the electromagnetic field inside the metal.

Fig. 2. Mesh utilized in the simulations. (a) General view of Structure 1, i.e., BCB ridge and double tungstate buffer

layer. (b) Zoom into the gold stripe region, marked as the red dashed rectangle in (a).

The different modes supported by the structures were calculated for a vacuum wavelength

of 1.55 µm. The structures were verified to support a long-range SPP mode (TM polarized)

and, in some cases, radiative TE modes with much shorter propagation distance than the main

long-range SPP mode (i.e., typically less than a few tens of micrometers). From the imaginary

part of the effective refractive index of the long-range SPP mode, the propagation losses (or

gain when the sign is negative) of the different structures were calculated as:

[ ] ( )02 Im 4.34

effdB cm k nα = × × × (1)

Here k0 is the vacuum wavevector, 2π/λ, where λ is the vacuum wavelength in cm, neff is the

effective refractive index of the propagating SPP mode, and the factor 4.34 converts the loss

value from 1/cm to dB/cm. The imaginary part of neff is positive for lossy materials, and

becomes eventually negative for materials exhibiting sufficiently large optical gain. The

absorption losses of RE-doped double tungstates responsible for the optical gain have been

ignored in the simulations. In the case of passive structures, it has been assumed that the

necessary optical pump power has been applied to the gain material in order to compensate for

the absorption losses and obtain gain = loss = 0 (i.e., zero imaginary part of the refractive

index). It has also been assumed that the gain achieved in the material is uniform. The

anisotropy of the double tungstate materials has not been considered, as it was assumed that

the waveguides are aligned along one of the major axes of the optical indicatrix.

#154169 - $15.00 USD Received 6 Sep 2011; revised 29 Sep 2011; accepted 29 Sep 2011; published 23 Nov 2011(C) 2011 OSA 5 December 2011 / Vol. 19, No. 25 / OPTICS EXPRESS 25302

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The optical power confinement in the gain region is an important parameter, as it

determines how effective the material gain is in compensating the propagation losses. Another

important parameter is the mode size, especially in the x-direction, as it indicates the mode

confinement in the different configurations. Depending on the application, a mode size as

small as possible in one or both directions can be an important design parameter. The mode

size has been calculated as the width of a Gaussian fit to the major component of the H-field

at the level of 1/e of its maximum value.

4. Effect of waveguide structure on loss compensation

A number of waveguide parameters must be taken into account for optimization of the

waveguide structure. These parameters comprise the ridge material, ridge size (width and

height), buffer layer material and thickness, metal stripe material, thickness, and width, and

substrate material. In this work, the metal was fixed to gold with a width of 200 nm and a

thickness of 15 nm. The effect of the remaining parameters on the net gain finally achieved in

the LR-DLSPP waveguides will be discussed in this section.

4.1 LR-DLSPP waveguide with BCB ridge

Structure 1 was simulated as described in Section 3. Fig. 3 shows the transverse mode profile

of the long-range SPP mode supported by the structure. A propagation loss of 3.6 dB/cm and

mode width of 1.7 µm in the horizontal x-direction and 2.5 µm in the vertical y-direction were

calculated for hbuffer = 60 nm and hridge = wridge = 1.4 µm. This structure exhibits two main

drawbacks. Firstly, the thickness of the buffer layer is too thin to be easily realized in a double

tungstate gain material. Secondly, as can be clearly seen in Fig. 3, the optical power

confinement in the gain region (buffer layer) is very small (~2 %). The much lower refractive

index of the ridge structure is more favorable for the plasmonic mode than the high refractive

index of the buffer, pulling a large fraction of the optical power above the metal stripe. As a

consequence, this structure is not very efficient to obtain lossless propagation or propagation

with net gain. In order to permit penetration of the mode into the gain region, a structure with

a better balanced refractive index profile is desirable. This goal can be achieved by selecting a

high-refractive-index material for the ridge, such as polyimide.

Fig. 3. (a) Mode profile for Structure 1 with hbuffer = 60 nm and hridge = wridge = 1.4 µm. (b) Vertical line scan of the

mode profile across the center of the metal stripe (x ~ 0). It can be seen that the electric field hardly penetrates inside

the gain buffer material.

4.2 LR-DLSPP waveguide with polyimide ridge

Using polyimide (n ~ 1.9 at 1.55 µm wavelength [34]) as the ridge material, the effective

refractive indices on both sides of the metal stripe are better balanced than in the previous

case (Structure 1), permitting the LR-SPP mode field to penetrate much stronger into the gain

buffer layer. Fig. 4 shows the evolution of net loss versus buffer layer thickness for a fixed

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ridge height (0.6 µm) and several ridge widths (0.8 to 1.6 µm) for several material gain values

of the buffer layer [(a)-(d)]. Fig. 5 shows the same evolution, however for a fixed ridge width

(1.6 µm) and several ridge heights (0.6 to 1.6 µm). Note that the occurrence of net modal gain

corresponds to the net loss of LR-SPP mode being negative.

Fig. 4. Effect of ridge width in Structure 2. Net optical loss versus thickness of buffer layer for a fixed ridge height

(0.6 µm) and several ridge widths (0.8-1.6 µm). Several buffer layer material gain values have been studied. (a)

0 dB/cm. (b) 35 dB/cm. (c) 106 dB/cm. (d) 246 dB/cm. (e) Power confinement to the gain region (buffer layer). (f)

Lateral mode width in the x-direction.

For a passive structure (i.e., a material gain of 0 dB/cm), as the ridge width increases for a

given ridge height [Fig. 4 (a)], the losses decrease and the location of the minimum loss shifts

towards larger buffer thicknesses that balance increasing ridge widths. As the ridge width

increases, the field intensity close to the metal layer decreases, because the mode is pulled

both into the ridge and buffer layers, increasing the ratio between the mode power

concentrated in dielectric regions and that in the (absorptive) metal region. The propagation

losses are, therefore, reduced. For each ridge dimension, the waveguide structure providing

minimum losses corresponds to the configuration for which the mode is balanced on the top

and bottom of the metal stripe [15]. For a given ridge height, as the ridge width increases, this

#154169 - $15.00 USD Received 6 Sep 2011; revised 29 Sep 2011; accepted 29 Sep 2011; published 23 Nov 2011(C) 2011 OSA 5 December 2011 / Vol. 19, No. 25 / OPTICS EXPRESS 25304

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condition is met for thicker buffer layers, as can be appreciated in Fig. 4 (a). As the ridge

width increases, both the mode confinement to the active layer [Fig. 4 (e)] and the mode width

in the x-direction [Fig. 4 (f)] increases. Comparison of Fig. 4 (a) to (d) indicates that with

increasing material gain of the buffer layer the parameter space for which net gain is obtained

increases. For a buffer layer material gain of 246 dB/cm [Fig. 4(d)] practically all investigated

geometrical configurations exhibit net gain. A similar physical behavior governs the influence

of ridge height on net loss (Fig. 5).

Fig. 5. Net optical loss versus thickness of buffer layer in Structure 2 for a fixed ridge width of the ridge (1.6 µm) and

several ridge heights (0.6-1.6 µm). Several buffer layer material gain values have been studied. (a) 0 dB/cm; (b)

35 dB/cm. (c) 106 dB/cm. (d) 246 dB/cm. (e) Confinement to active buffer layer. (f) Lateral mode width in the

horizontal x-direction.

Two distinct zones can be observed. In the first zone (i.e., small buffer thickness), losses

increase as the ridge height increases. In the second zone (i.e., large buffer thickness), the

opposite behavior is observed. The behavior in both zones can again be qualitatively

explained by the fact that the losses decrease, as the effective refractive indices above and

below the metal stripe approach the point of balance. For small buffer layer thickness and

#154169 - $15.00 USD Received 6 Sep 2011; revised 29 Sep 2011; accepted 29 Sep 2011; published 23 Nov 2011(C) 2011 OSA 5 December 2011 / Vol. 19, No. 25 / OPTICS EXPRESS 25305

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fixed ridge width, as the height of the ridge increases, the structure moves farther away from

this low-loss condition. For large buffer thickness, the opposite occurs: as the ridge height

increases, the structure moves closer to the balanced condition. In all cases, the minimum

propagation loss as a function of buffer thickness shifts to larger buffer thicknesses, as the

height of the ridge increases. An increase of ridge height forces both the mode confinement to

the active layer [Fig. 5 (e)] and the lateral mode width in the x-direction [Fig. 5 (f)] to

decrease. Again, with increasing material gain of the buffer layer the parameter space for

which net gain is obtained increases, and, for the highest investigated buffer layer material

gain of 246 dB/cm [Fig. 5 (d)] practically all investigated geometrical configurations provide

net gain.

The net modal loss (or gain) is determined by two contributions, the LR-SPP mode

propagation loss and the optical gain of the mode fraction confined within the gain material,

and can be evaluated as follows:

net loss matgα α= −Γ (2)

where αnet is the net modal loss in dB/cm, αloss is the propagation loss of the passive structure

in dB/cm [Eq. (1)], Γ is the fraction of optical power overlapping with the gain region (in this

case the buffer layer), and gmat is the material gain provided by the material utilized in the gain

region. One can qualitatively explain the dependencies shown in Fig. 5 (a)-(d) by combining

the loss dependencies in the absence of material gain [Fig. 5 (a)] with the corresponding

dependencies of the mode confinement within the gain material [Fig. 5 (e)] in accordance with

Eq. (2). Indeed, for a given ridge dimension, the mode fraction confined within the active area

increases as the thickness of the buffer layer increases [Fig. 5 (e)]. Therefore, the

compensation of propagation losses is more efficient for larger buffer layer thicknesses, a

circumstance that results in shifting the location of minimum losses [Fig. 5 (b)-(d)]. It is,

therefore, apparent that not only the waveguide dimensions but also the expected material

gain should be considered in the design of the optimized structures. For example, although the

combination hridge = 1.6 µm and wridge = 1.6 µm provides the lowest net loss [Fig. 5 (a)], this

ridge structure is the one providing the lowest net gain for the material gain of 106 dB/cm due

to lower confinement of the optical power to the gain region [Fig. 5 (e)]. If lossless

propagation should be achieved, a material gain of ~37 dB/cm in a 375-nm-thick buffer layer

would be sufficient for a ridge with hridge = wridge = 1.6 µm, resulting in the LR-DLSPP mode

being 1.4-µm wide. Fig. 6 shows the 2-dimensional mode profiles and vertical mode profile

across the center of the metal stripe for Structure 2 for a 1.6-µm-wide ridge and two different

ridge heights, 0.6 µm [Fig. 6 (a)] and 1.6 µm [Fig. 6 (b)].

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Fig. 6. Two-dimensional mode profile and vertical mode profile across the center of the metal stripe for Structure 2 at

zero gain. (a) Ridge height 0.6 µm, ridge width 1.6 µm, buffer thickness 0.25 µm. (b) Ridge height 1.6 µm, ridge

width 1.6 µm, buffer thickness 0.375 µm.

4.3 LR-DPSPP with Si3N4 buffer layer and gain ridge

As was discussed in the previous sections, substantial mode confinement in the gain material

is necessary in order to enhance the net modal gain. In all the cases described above, the

optical power confinement to the ridge region was larger than that to the buffer layer. It is,

therefore, desirable to fabricate the ridge in the gain material whenever the application permits

(Structure 3 in Fig. 1 (c)).

The net loss of such a structure was simulated as a function of thickness of the buffer

layer for several ridge dimensions. The power confinement to the active region (in this case

the ridge) and lateral mode dimension in the horizontal x-direction were also calculated. In

Fig. 7 (a), (c), and (e), the effect of ridge width is shown for a given ridge height. As the ridge

width increases, the propagation loss minimum shifts towards thicker buffer layers, consistent

with the balancing of the effective refractive indices above and below the metal stripe.

Furthermore, increasing the ridge width leads to a decrease of the minimum of the

propagation losses, slight increase in mode waist in the horizontal x-direction, and increase of

mode confinement to the active area (ridge). The latter effect improves the exploitation of

available material gain, which is shown in Fig. 8 for two values of material gain. The

influence of the ridge height is shown in Fig. 7 (b), (d), and (f). As the ridge height increases,

the propagation loss minimum shifts towards thicker buffer layers, again as a result of

balancing the refractive indices at both sides of the metal. The mode size in the x-direction

increases, as the ridge height decreases. This phenomenon can be intuitively explained by the

squeezing out of the optical mode, as the ridge height decreases, forcing the mode to widen in

the x-direction. The mode confinement to the ridge also decreases, because the mode is

pushed towards the metal by a reduction of the ridge height.

#154169 - $15.00 USD Received 6 Sep 2011; revised 29 Sep 2011; accepted 29 Sep 2011; published 23 Nov 2011(C) 2011 OSA 5 December 2011 / Vol. 19, No. 25 / OPTICS EXPRESS 25307

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Fig. 7. Structure 3: Net optical loss as a function of hbuffer for (a) hridge = 0.8 µm and various wridge and (b)

wridge = 0.8 µm and various hridge. Confinement of the optical power to the active material region (ridge) as a function

of hbuffer for (c) hridge = 0.8 µm and several wridge and (d) wridge = 0.8 µm and several hridge. Mode width in the x-

direction as a function of hbuffer for (e) hridge = 0.8 µm and various wridge and (f) wridge = 0.8 µm and various hridge. The

material gain was considered to be zero in all cases (passive structure).

Finally, for obtaining a manufacturable design it is important that the waveguide behavior

does not change drastically if the ridge height or width or thicknesses of the buffer and

adhesive layer vary within typical fabrication tolerances. In Fig. 8, the minima for the ridge

dimensions 0.8 µm × 0.8 µm are flatter than those for the ridge dimensions 0.8 µm × 0.5 µm.

Therefore, the larger ridge will be more tolerant to small variations of the buffer thickness (in

this case determined by control of the Si3N4 deposition process). Furthermore, at the target

buffer thickness, hbuffer = 0.35 µm, the curves corresponding to ridge widths of 0.8 µm and

0.7 µm are very close to each other. Thus, a small variation of the ridge width, controlled by

the lithography and etching processes, should have very little influence on the characteristics

of the final devices. The same applies for the ridge height [Fig. 7 (b)]. The influence of

thickness of the adhesive layer has been analyzed for a passive structure with

0.8 µm × 0.8 µm ridge size. As the thickness of the adhesive increases, the mode becomes

#154169 - $15.00 USD Received 6 Sep 2011; revised 29 Sep 2011; accepted 29 Sep 2011; published 23 Nov 2011(C) 2011 OSA 5 December 2011 / Vol. 19, No. 25 / OPTICS EXPRESS 25308

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more confined in the ridge, losing its plasmonic character. A tolerance of ~50 nm around the

100-nm target can, however, be tolerated.

Fig. 8. Net optical loss in Structure 3 for hridge = 0.8 µm and various wridge when assuming a material gain of (a) 35

dB/cm and (b) 106 dB/cm.

Table 2. Waveguide dimensions and mode profiles for a large ridge structure (Waveguide 1) and for a smaller ridge

structure (Waveguide 2).

Waveguide 1 Waveguide 2

Ridge height [µm]: 0.8 Ridge height [µm]: 0.8

Ridge width [µm]: 0.8 Ridge width [µm]: 0.5

Buffer height [µm]: 0.35 Buffer height [µm]: 0.25

Mode width X [µm]: 0.92 Mode width X [µm]: 0.78

Mode width Y [µm]: 1.1 Mode width Y [µm]: 1.08

Gain for lossless propagation [dB/cm]: 12.5 Gain for lossless propagation [dB/cm]: 26

Fig. 9. (a) and (b) Vertical and 2-D mode profile (Re[Ey]) of Waveguide 1 described in Table 2. (c) and (d) Vertical

and 2-D mode profile (Re[Ey]) of Waveguide 2 described in Table 2.

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6. Conclusions

Loss compensation in plasmonic waveguides will pave the road toward utilization of these

structures in a wide range of novel devices by permitting full exploitation of their potential. In

this paper, a detailed investigation of the compensation of propagation loss in LR-DLSPP

waveguides using RE-doped double tungstates as the gain material has been presented for

three different configurations that were selected keeping in mind manufacturability using

fabrication and assembly equipment commonly available in standard microfabrication

cleanrooms. In the first two structures, the gain material is integrated as a buffer layer. We

found that only a small fraction of the mode power is confined within the material gain region,

making this approach not very favorable for loss compensation. Nevertheless, using a high-

refractive-index ridge made of polyimide (n ~ 1.9) resulted in an increased mode confinement

to the gain material. It was also found that, in the design of optimized structures, one should

consider simultaneously the LR-SPP waveguide dimensions and the available material gain.

For example, it was demonstrated that a material gain of 37 dB/cm is sufficient to achieve

lossless propagation in a LR-DLSPP waveguide structure with a 1.6×1.6 µm2 ridge and a 375-

nm-thick buffer layer. In general, configurations with larger mode fractions within the gain

(buffer) layer resulted in larger lateral mode widths, which are detrimental with respect to the

bend loss (that increases with the mode width) and maximum achievable density of

waveguide components [15, 16].

In the third structure, the gain material was integrated as the ridge material. A 100-nm-

thin BCB layer was introduced between the gold stripe and the waveguide ridge in order to

ease manufacturability. This structure ensures a considerably higher confinement of the mode

optical power in the active material region, making the LR-DLSPP waveguide configuration

much more amenable with respect to loss compensation. A material gain as low as

12.5 dB/cm is sufficient to allow for lossless propagation in a waveguide structure with a

0.8×0.8 µm2 ridge and 350-nm-thick buffer layer. Simultaneously, the hybrid LR-DLSPP

mode supported by this structure has a lateral width of only 0.92 µm.

The structures considered in this paper show a great potential to reach the goal of loss

compensation in plasmonic waveguides and are promising for plasmon amplification and

lasing. The low material gain required to compensate propagation losses broadens the range of

gain materials that can be utilized. RE-doped double tungstate gain materials were selected in

this study due to their very good match of refractive index with the materials utilized in the

structure and the elevated gain they can provide. Experimental demonstration of LR-DLSPP

waveguides corresponding to the considered structures will constitute the next milestone on

the way towards lossless plasmonic waveguides.

Ackowledgements The authors acknowledge support from the COST Action MP0702: Towards functional sub-

wavelength photonic structures. Dr. García-Blanco acknowledges support from the FP7 Marie

Curie Career Integration Grant PCIG09-GA-2011-29389, technical support and useful

discussions with from PhoeniX B.V., and useful discussions with Manfred Hammer and Hugo

Hoekstra. The financial support of the Danish Council for Independent Research (FTP-project

No. 09-072949 ANAP) is also appreciated (SIB).

#154169 - $15.00 USD Received 6 Sep 2011; revised 29 Sep 2011; accepted 29 Sep 2011; published 23 Nov 2011(C) 2011 OSA 5 December 2011 / Vol. 19, No. 25 / OPTICS EXPRESS 25310