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Funding : Quantum Coherent Properties of Spins II, PITP, 6 th December 2009

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Long-lived spin coherence in silicon with electrical readout Gavin W Morley London Centre for Nanotechnology and Department of Physics and Astronomy, UCL. Funding:. Quantum Coherent Properties of Spins II, PITP, 6 th December 2009. Introduction. People Involved in this Work. - PowerPoint PPT Presentation

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Page 1: Long-lived spin coherence in silicon with electrical readout Gavin  W Morley London Centre for Nanotechnology  and Department of Physics and Astronomy, UCL

Funding:

Quantum Coherent Properties of Spins II, PITP, 6th December 2009

Page 2: Long-lived spin coherence in silicon with electrical readout Gavin  W Morley London Centre for Nanotechnology  and Department of Physics and Astronomy, UCL

People Involved in this Work

University of UtahChristoph BoehmeDane R McCameyHeather A Seipel

National High Magnetic Field LaboratoryHans van TolLouis-Claude Brunel

Introduction

Page 3: Long-lived spin coherence in silicon with electrical readout Gavin  W Morley London Centre for Nanotechnology  and Department of Physics and Astronomy, UCL

Phosphorus dopants in silicon

- Long spin coherence (A M Tyryshkin et al, PRB 68, 193207 2003)

- Atomic positioning(S R Schofield et al, PRL 91, 136104 2003)

- Control wavefunction size (N Q Vinh et al, PNAS 105, 10649 2008)

Introduction

Page 4: Long-lived spin coherence in silicon with electrical readout Gavin  W Morley London Centre for Nanotechnology  and Department of Physics and Astronomy, UCL

Introduction

Experimental challenges:

1. Initialization2. Control superposition and entanglement3. Decoherence4. Readout

Introduction Our research

Towards quantum computing

we have a plan

Page 5: Long-lived spin coherence in silicon with electrical readout Gavin  W Morley London Centre for Nanotechnology  and Department of Physics and Astronomy, UCL

Pulsed ESR at 4, 8 and 12 T

Nuclear Spin Polarization: GWM, J van Tol, A Ardavan, K Porfyrakis, J Zhang and G A D Briggs, Phys Rev Lett 98, 220501 (2007)

CW ESR: J van Tol, L C Brunel and R J Wylde, Rev Sci Inst 76, 074101 (2005)

Introduction Our research

GWM, L-C Brunel and J van Tol, Rev Sci Instrum 79, 064703 (2008)

Page 6: Long-lived spin coherence in silicon with electrical readout Gavin  W Morley London Centre for Nanotechnology  and Department of Physics and Astronomy, UCL

A

DC current source reacts slowly

Fast current detector measures signal

1 mm overlap

silicon

Circularly polarized 240 GHz radiation manipulates electron spins

Visible light creates electron-hole pairs

B0 = 8.6 T

T = 2.8 K10 micron

Introduction Our research

Page 7: Long-lived spin coherence in silicon with electrical readout Gavin  W Morley London Centre for Nanotechnology  and Department of Physics and Astronomy, UCL

Continuous-wave electrically-detected magnetic resonance

8.56 8.57 8.58 8.59

-1.5

-1.0

-0.5

0.0

I/I

(%)

Magnetic Field (T)

Our papers: PRL 101, 207602 (2008),

PRL 102, 027601 (2009), PRB 78, 045303 (2008)

Introduction Our research

Page 8: Long-lived spin coherence in silicon with electrical readout Gavin  W Morley London Centre for Nanotechnology  and Department of Physics and Astronomy, UCL

A

DC current source reacts slowly

Fast current detector measures signal

1 mm overlap

silicon

Circularly polarized 240 GHz radiation manipulates electron spins

Visible light creates electron-hole pairs

10 micron

B0 = 8.6 T

T = 2.8 K

Introduction Our research

Page 9: Long-lived spin coherence in silicon with electrical readout Gavin  W Morley London Centre for Nanotechnology  and Department of Physics and Astronomy, UCL

e

h

e

h

10 micron

Circularly polarized 240 GHz radiation manipulates electron spins

Visible light creates electron-hole pairs

DD Thornton & A Honig, PRL 30 909 (1973)

A Honig & M Moroz, RSI 49 183 (1978)

GWM, DR McCamey, HA Seipel, LC Brunel, J van Tol & C. Boehme, PRL 101, 207602,(2008)

e

B0 = 8.6 T

T = 2.8 K

Sensitivity: need (100 nm)3 sample

Introduction Our research

Page 10: Long-lived spin coherence in silicon with electrical readout Gavin  W Morley London Centre for Nanotechnology  and Department of Physics and Astronomy, UCL

Continuous-wave electrically-detected magnetic resonance

8.56 8.57 8.58 8.59

-1.5

-1.0

-0.5

0.0

I/I

(%)

Magnetic Field (T)

Our papers: PRL 101, 207602 (2008),

PRL 102, 027601 (2009), PRB 78, 045303 (2008)

Introduction Our research

Page 11: Long-lived spin coherence in silicon with electrical readout Gavin  W Morley London Centre for Nanotechnology  and Department of Physics and Astronomy, UCL

Continuous-wave electrically-detected magnetic resonance

8.56 8.57 8.58 8.59

mI = -1/2

I

Magnetic Field (T)

mI = +1/2

Temperature = 1.37 K

Polarization = -68±1 %

Our papers: PRL 101, 207602 (2008),

PRL 102, 027601 (2009), PRB 78, 045303 (2008)

Introduction Our research

DR McCamey, J van Tol, GWM & C. Boehme, PRL 102, 027601 (2009)

Page 12: Long-lived spin coherence in silicon with electrical readout Gavin  W Morley London Centre for Nanotechnology  and Department of Physics and Astronomy, UCL

Continuous-wave electrically-detected magnetic resonance

1. Thermal Equilibrium

2. Flip-flop, X

3. Capture-emission, CE

1. Thermal Equilibrium

2. Flip-flop, X

1. Thermal Equilibrium

P = 0P < 0

Our papers: PRL 101, 207602 (2008),

PRL 102, 027601 (2009), PRB 78, 045303 (2008)

Introduction Our research

DR McCamey, J van Tol, GWM & C. Boehme, PRL 102, 027601 (2009)

Page 13: Long-lived spin coherence in silicon with electrical readout Gavin  W Morley London Centre for Nanotechnology  and Department of Physics and Astronomy, UCL

Continuous-wave electrically-detected magnetic resonance

8.56 8.57 8.58 8.59

-1.5

-1.0

-0.5

0.0

I/I

(%)

Magnetic Field (T)

Our papers: PRL 101, 207602 (2008),

PRL 102, 027601 (2009), PRB 78, 045303 (2008)

Introduction Our research

Page 14: Long-lived spin coherence in silicon with electrical readout Gavin  W Morley London Centre for Nanotechnology  and Department of Physics and Astronomy, UCL

Transient response to a 240 GHz pulse

-10 0 10 20

-1.2

-1.0

-0.8

-0.6

-0.4

-0.2

0.0

0.2

time

current measurement

GWM, DR McCamey, HA Seipel, LC Brunel, J van Tol & C. Boehme, PRL 101, 207602 (2008)

Introduction Our research

Page 15: Long-lived spin coherence in silicon with electrical readout Gavin  W Morley London Centre for Nanotechnology  and Department of Physics and Astronomy, UCL

Rabi Oscillations

GWM, DR McCamey, HA Seipel, LC Brunel, J van Tol & C. Boehme, PRL 101, 207602 (2008)

Introduction Our research

Isidor Isaac Rabi (1898 – 1988)

time

integrated current measurement

Page 16: Long-lived spin coherence in silicon with electrical readout Gavin  W Morley London Centre for Nanotechnology  and Department of Physics and Astronomy, UCL

Rabi Oscillations

GWM, DR McCamey, HA Seipel, LC Brunel, J van Tol & C. Boehme, PRL 101, 207602 (2008)

Introduction Our research

time

integrated current measurement

Page 17: Long-lived spin coherence in silicon with electrical readout Gavin  W Morley London Centre for Nanotechnology  and Department of Physics and Astronomy, UCL

Spin echo animation by Chris Noble

Spin echo

GWM, DR McCamey, HA Seipel, LC Brunel, J van Tol & C. Boehme, PRL 101, 207602 (2008)

Introduction Our research

Erwin L Hahn (born 1921)

Page 18: Long-lived spin coherence in silicon with electrical readout Gavin  W Morley London Centre for Nanotechnology  and Department of Physics and Astronomy, UCL

Electrically-detected spin echo

0 1 2 3 4 5 6

0

1

2

3

4

5

2 s 2 stime

integrated current

measurement

22

22

2222

GWM, DR McCamey, HA Seipel, LC Brunel, J van Tol & C. Boehme, PRL 101, 207602 (2008)

Introduction Our research

Page 19: Long-lived spin coherence in silicon with electrical readout Gavin  W Morley London Centre for Nanotechnology  and Department of Physics and Astronomy, UCL

Decay of electrically-detected spin echoes

0 100 200 300 400

-0.1

0.0

0.1

0.2

0.3

0.4

0.5

0.6

time

integratedmm - wave

echo

time

integrated current

measurement2

22

integrated electrically-

detected echo

2

GWM, DR McCamey, HA Seipel, LC Brunel, J van Tol & C. Boehme, PRL 101, 207602 (2008)

Introduction Our research

Page 20: Long-lived spin coherence in silicon with electrical readout Gavin  W Morley London Centre for Nanotechnology  and Department of Physics and Astronomy, UCL

Decay of electrically-detected spin echoes

0 100 200 300 400

-0.1

0.0

0.1

0.2

0.3

0.4

0.5

0.6

time

integratedmm - wave

echo

time

integrated current

measurement2

22

integrated electrically-

detected echo

2

GWM, DR McCamey, HA Seipel, LC Brunel, J van Tol & C. Boehme, PRL 101, 207602 (2008)

Introduction Our research

Page 21: Long-lived spin coherence in silicon with electrical readout Gavin  W Morley London Centre for Nanotechnology  and Department of Physics and Astronomy, UCL

Decay of electrically-detected spin echoes

GWM, DR McCamey, HA Seipel, LC Brunel, J van Tol & C. Boehme, PRL 101, 207602 (2008)

Introduction Our research

Page 22: Long-lived spin coherence in silicon with electrical readout Gavin  W Morley London Centre for Nanotechnology  and Department of Physics and Astronomy, UCL

Entangling multiple qubits: theoryA M Stoneham, A J Fisher & P T Greenland, J Phys CM 15 L477 (2003)

R Rodriquez, A J Fisher, P T Greenland & A M Stoneham, J Phys CM 16 2757 (2004)

A M Stoneham, A H Harker & GWM, in press at J Phys CM, arXiv:0904.4895

Qubit 1 Qubit 2Control

light

Introduction Our research

Page 23: Long-lived spin coherence in silicon with electrical readout Gavin  W Morley London Centre for Nanotechnology  and Department of Physics and Astronomy, UCL

Entangling multiple qubitsBismuth is a good as phosphorus

5 10 15 20 25 30 35 40 45 501E-5

1E-4

1E-3

0.01

0.1

1

10

100

1000

4 x 1016 Bi cm-3 (ref 25) : T1

28Si:P (ref 9): T1

T2

Rel

axat

ion

time

(ms)

Temperature (K)

Our data for ~3 x 1015 Bi cm-3 Monoexponential T

2

T2 from fit to exp(-/T

2-3/T3

S)

TS from fit to exp(-/T

2-3/T3

S)

CPMG decay T

1

Fit to T1

Introduction Our research

Page 24: Long-lived spin coherence in silicon with electrical readout Gavin  W Morley London Centre for Nanotechnology  and Department of Physics and Astronomy, UCL

Conclusions

Experimental challenges:

1. Initialization2. Control superposition and entanglement3. Decoherence4. Readout

Introduction Our research Conclusions and future work

we have a plan