jrjc 2009 30/11/09 barbara sulignano jrjc 2009 cea saclay key questions how do protons and neutrons...

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30/11/09 Barbara Sulignano JRJC 2009 JRJC 2009 CEA SACLAY Key questions Key questions How do protons and neutrons make stable nuclei and rare isotopes? How many neutrons can a nucleus hold? What are the heaviest nuclei that can exist?

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Page 1: JRJC 2009 30/11/09 Barbara Sulignano JRJC 2009 CEA SACLAY Key questions How do protons and neutrons make stable nuclei and rare isotopes? How many neutrons

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Key questionsKey questions

How do protons and neutrons make stable nuclei and rare isotopes?

How many neutrons can a nucleus hold?

What are the heaviest nuclei that can exist?

How do protons and neutrons make stable nuclei and rare isotopes?

How many neutrons can a nucleus hold?

What are the heaviest nuclei that can exist?

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1934 – Liquide drop model (Bethe, Von 1934 – Liquide drop model (Bethe, Von Weizsäcker):Weizsäcker):

Nuclear fissionNuclear fission

1949 – Shell model (Maria Goeppert-1949 – Shell model (Maria Goeppert-Mayer, Mayer,

Hans Jensen)Hans Jensen)Magic NumbersMagic Numbers

1960 - …Microscopic Models1960 - …Microscopic Models

EHFB = Emacro + Eshell + EpairingEHFB = Emacro + Eshell + Epairing

1934 – Liquide drop model (Bethe, Von 1934 – Liquide drop model (Bethe, Von Weizsäcker):Weizsäcker):

Nuclear fissionNuclear fission

1949 – Shell model (Maria Goeppert-1949 – Shell model (Maria Goeppert-Mayer, Mayer,

Hans Jensen)Hans Jensen)Magic NumbersMagic Numbers

1960 - …Microscopic Models1960 - …Microscopic Models

EHFB = Emacro + Eshell + EpairingEHFB = Emacro + Eshell + Epairingstable nucleistable nuclei

known nucleiknown nuclei

terra incognitaterra incognita

N=Z

pro

ton

s

neutrons

50

82

50

28

28

82

2082

28

20

126

The Nuclear LandscapeThe Nuclear Landscape

Page 3: JRJC 2009 30/11/09 Barbara Sulignano JRJC 2009 CEA SACLAY Key questions How do protons and neutrons make stable nuclei and rare isotopes? How many neutrons

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Evidence for shell structureEvidence for shell structureEven-even nuclei: 2+

1 state energy as an indicator of shell structure

Page 4: JRJC 2009 30/11/09 Barbara Sulignano JRJC 2009 CEA SACLAY Key questions How do protons and neutrons make stable nuclei and rare isotopes? How many neutrons

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Magicity is a

fragile concept

Near stabilityNear stability N>>ZN>>Z

Nuclear shell structureNuclear shell structureIs nuclear shell strucuture modified away from the line of stability?

As we add neutrons, traditional shell closures are changed, and may

even disappear!

Page 5: JRJC 2009 30/11/09 Barbara Sulignano JRJC 2009 CEA SACLAY Key questions How do protons and neutrons make stable nuclei and rare isotopes? How many neutrons

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N=28 is not a good shell closure anymore

Experimental proof of disappearing of shell gap for neutron rich nuclei

Page 6: JRJC 2009 30/11/09 Barbara Sulignano JRJC 2009 CEA SACLAY Key questions How do protons and neutrons make stable nuclei and rare isotopes? How many neutrons

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protons

neutrons

82

5028

28

50

82

2082

28

20

126

stable double-magic nuclei4He, 16O, 40Ca, 48Ca, 208Pb

radioactive: 56Ni, 132Sn, magic ? 48Ni, 78Ni, 100Sn

70Ca ?48Ca

40Ca42Si32Mg

?4040

Shell structure of atomic nucleiShell structure of atomic nuclei

Page 7: JRJC 2009 30/11/09 Barbara Sulignano JRJC 2009 CEA SACLAY Key questions How do protons and neutrons make stable nuclei and rare isotopes? How many neutrons

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Tools we have to investigate shell Tools we have to investigate shell structurestructure

• Evidence for nuclear shell structure from :

– Nuclear masses.

– Spectroscopy of excited states

– Reaction cross sections Corinne’s Talk

Page 8: JRJC 2009 30/11/09 Barbara Sulignano JRJC 2009 CEA SACLAY Key questions How do protons and neutrons make stable nuclei and rare isotopes? How many neutrons

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Masses can be measured in different way:

• Time of flight

• Storage ring

• Penning trap Mass measurement via determination ofCyclotron frequency:

fc=qB/2п mFrom characteristic motion of stored ions

Masses measurementMasses measurement

Page 9: JRJC 2009 30/11/09 Barbara Sulignano JRJC 2009 CEA SACLAY Key questions How do protons and neutrons make stable nuclei and rare isotopes? How many neutrons

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SpectroscopySpectroscopy

Particle detector

TargetBeam

γ

Reacted beam

stable beam and target

Fusion evaporationCoulomb excitationsOne and two nucleon knockoutCoulomb break upCharge exchange reactions

Only access to stable or neutron deficient nuclei

Page 10: JRJC 2009 30/11/09 Barbara Sulignano JRJC 2009 CEA SACLAY Key questions How do protons and neutrons make stable nuclei and rare isotopes? How many neutrons

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Spectroscopy

Particle detector

TargetBeam

γ

Reacted beam

radioactive beam:

Coulomb excitationsOne and two nucleon knockoutCoulomb break upCharge exchenge reactions

Access to neutron rich nuclei

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• Projectile Fragmentation

•Isol technique

How to produce radioactive beamHow to produce radioactive beam

Page 12: JRJC 2009 30/11/09 Barbara Sulignano JRJC 2009 CEA SACLAY Key questions How do protons and neutrons make stable nuclei and rare isotopes? How many neutrons

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Key questionsKey questions

How do protons and neutrons make stable nuclei and rare isotopes?

What are the heaviest nuclei that can exist?

How do protons and neutrons make stable nuclei and rare isotopes?

What are the heaviest nuclei that can exist?

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Z = 100

island of stability

?

black: stable isotopered: +-unstable isotopeblue: --unstable isotope yellow: -instable isotopegreen: spontan fission

Pb (lead) and Bi (bismuth)

U (uranium) and Th (thorium)

What is the next magic nucleus beyond What is the next magic nucleus beyond 208208Pb? Pb?

Page 14: JRJC 2009 30/11/09 Barbara Sulignano JRJC 2009 CEA SACLAY Key questions How do protons and neutrons make stable nuclei and rare isotopes? How many neutrons

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1934Enrico Fermi proposes to irradiate Uranium with neutrons in order to synthesise Even heavier elements

1938Otto Hahn andFritz Straßmanndiscover the neutron-inducednuclear fission

193960-inch-cyclotron group:Cooksey, Corson, Ernest O. LawrenceThornton, Backus, Salisbury,Luis Alvarez und Edwin McMillan

With Fermi’s method and the 60’’-cyclotron 7 Transurane could (Z=93-98) Be synthesised. By irradiation of actinides with light ions the elements up Z=106 could beProduced in Berkeley (CA, U.S.A.)and in Dubna (Rußland).

The linear acceleratorUNILAC and thevelocity filter SHIP at GSI allowed for the synthesis of elements with Z=107-112.

Synthesis of SHE via fusion of heavy target nuclei with light projectiles1952 1974

Neutron period1940 1952

1896Discovery of radioactivity by A.H. Becquerel

Radioactivity period1896 1940

Synthesis of SHE via fusion (Pb and Bi as target nuclei)1974 1996

1899Actinium (Z=89) 1908

Radon (Z=86) 1939Francium (Z=87)

1917Protactinium (Z=91)

1952Einsteinium (Z=99)Fermium (Z=100)

1940Astatin (Z=85)Neptunium (Z=93)

1944Americium (Z=95)Curium (Z=96)

1941Plutonium (Z=94)

1950Californium (Z=98)

1949Berkelium (Z=97)

1996Copernicium(Z=112)

1994Darmstadium(Z=110) Rontgenium(Z=111)

1982Meitnerium (Z=109)

1981Bohrium (Z=107) 1984

Hassium (Z=108)

1969Rutherfordium (Z=104)

1965Nobelium (Z=102)Lawrencium (Z=103)

1974Seaborgium (Z=106)

1970Dubnium (Z=105)

1955Mendelevium (Z=101)

1898 Polonium (Z=84) Radium (Z=88)

History of the synthesis and History of the synthesis and discovery of super heavy elementsdiscovery of super heavy elements

Synthesis of SHE via fusion (48Ca beam and actinide targets)1999 2005

2005Element 118

2000 Element 1161999

Element 114 2003Element 113 element 115

Dubna

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How to produce super heavy elementsHow to produce super heavy elements

Neutron capture up to Z=100

reactors

bomb

in stars?

ee--

αα

αα

DésexcitationDésexcitation

Chaîne de Chaîne de DésintégrationDésintégration

T ~10T ~10-15-15ss

T >10T >10-6-6ss

Elément Elément superlourdsuperlourd

ee--

nn nnFusionFusion

CompétitionCompétition- fission- fission- évaporation- évaporation

Noyau Noyau composécomposé

T ~10T ~10-20/-17-20/-17ss

Fusion evaporation

Cold fusion X+ 208Pb, 209Bi

Hot fusion 48Ca+X

See Fabien’s talk

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Status of SHE researchCold fusion (GSI, RIKEN) based on Pb and Bi targets

Cold fusion (GSI, RIKEN) based on Pb and Bi targets

1second

1 minute

1 hour

1 day

10 days

GSIRIKEN

1 pb

Hot fusion (JINR) based on actinide targets

Hot fusion (JINR) based on actinide targets

DUBNA

1 pb35fb3 events250days

2pb6 events (Dubna)44days

Needs for- Higher Z- More events for studies

Beam:High intensity beamSpectrometer:High rejection powerWide angular acceptanceGood mass resolution

Needs for- Higher Z- More events for studies

Beam:High intensity beamSpectrometer:High rejection powerWide angular acceptanceGood mass resolution

Proton

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Reaction synthesisReaction synthesis

DAVID’s talk