coincidence simulation of a two-channel czt-based

1
INTRODUCTION The Comprehensive Test Ban Treaty Organization makes use of radioxenon detection systems in the International Monitoring System stations to watch for signs of nuclear weapons testing and undeclared facilities. Systems using beta-gamma coincidence detection have been shown to have significantly reduced background counts, and are thus able to detect trace amounts of atmospheric radioxenon. A prototype of a multi- element coplanar CZT that uses two face-to-face coplanar CZT crystals to measure beta-gamma coincidence events from atmospheric radioxenon was developed at OSU. OBJECTIVES The CZT-based detection system was simulated using MCNP to find the response of the detector to the xenon radioisotopes of interest and also calculate the coincidence detection efficiency of the device for these radioisotopes. In this work, modeling results from 131m Xe, 133m Xe, and 135 Xe are reported. MCNP MODELING 1. DETECTOR GEOMETRY Geometry of the CZT-based radioxenon detection system simulated in MCNP. 2. PTRAC CARD To model β-γ coincidence events in the CZT crystals, the PTRAC card was used. PTRAC follows each particle individually and writes an output file containing the entire history of that particle including position of interaction, energy of the particle, and the history number. A Python code was . developed to parse the PTRAC files and extract the position of . . interaction, energy released in each CZT crystal, and the . history number of each event from the PTRAC files. β-γ . coincidence events were then extracted for events with the . same history number ( NPS number). COINCIDENCE DETECTION PYTHON ALGORITHMS RESULTS 135 Xe 135 Xe emits 250 keV gammas in coincidence with beta particles (maximum energy ~ 910 keV) 133m Xe 133m Xe emits 30 keV x-rays in coincidence with 199 keV conversion electrons. (a) Simulated beta/gamma coincidence spectrum of 133m Xe (b) energy deposited by 133m Xe coincident events in CZT1. 131m Xe 131m Xe emits 30 keV x-rays in coincidence with 129 keV conversion electrons. (a) Simulated beta/gamma coincidence spectrum of 131m Xe (b) energy deposited by 131m Xe coincident events in CZT1. Radioxenons coincidence detection efficiencies calculated using MCNP. Coincidence Simulation of a Two-Channel CZT-based Radioxenon Detector Lily Ranjbar*, Abi T. Farsoni, Eric M. Becker, David M. Hamby Oregon State University, Corvallis, OR Abi Farsoni, [email protected] Consortium for Verification Technology (CVT) Radioxenon Gas Cell Coplanar CZT1 Radioxenon Injection Tube Start Load β / CE PTRAC file Load γ / X- rays PTRAC file Interaction in CZT1/CZT2? Yes Full Energy absorption? Yes Calculate Partial Energy Absorption No Save β /CE and γ/x-ray Partial Energy Absorption Save β/CE and γ/x-ray Full Energy Finish No Last NPS Next NPS Ignore First 10 Lines Flowchart of the Python algorithm to parse the PTRAC output files. Flowchart of the Python algorithm to extract coincident events. CZT 1 CZT 2 β/CE γ/x-ray γ/x-ray β/CE Scenario No.1 Scenario No.2 Coincidence scenarios considered in this simulation. Isotope Half-life Coincident Energies (keV) Type Intensity (%) 131m Xe 11.9 d 30 129 K X-ray CE 54.1 60.7 133m Xe 2.19 d 30 199 K X-ray CE 56.3 63.1 133 Xe 5.245 d 31 81 45 346 K X-ray Gamma CE Beta (endpoint) 48.9 37 54.1 99 135 Xe 9.1 h 250 910 Gamma Beta (endpoint) 99 97 250 keV γ-rays 134 keV Compton edge γ-γ coincidence events x-rays escape peak (a) (b) (a) (b) (a) (b) This work was funded in-part by the Consortium for Verification Technology under Department of Energy National Nuclear Security Administration award number DE-NA0002534. Save γ Energy in Array1, β Energy in Array 2 Equal NPS? Yes Finish No Start Last NPS Next NPS Load β / CE Energy Data in CZT2 Load γ / X-rays Energy Data in CZT1 Yes Next NPS Equal NPS? Load β / CE Energy Data in CZT1 Load γ / X-rays Energy Data in CZT2 No Finish Last NPS Save γ Energy in Array 2, β Energy in Array 1 Radioxenon Coincidence Efficiency (%) 131m Xe 3.1 133m Xe 2.7 135 Xe 1.7 (a) Simulated beta/gamma coincidence spectrum of 135 Xe (b) energy deposited by 135 Xe coincident events in CZT1. Unclassified

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Page 1: Coincidence Simulation of a Two-Channel CZT-based

INTRODUCTION The Comprehensive Test Ban Treaty Organization makes use of radioxenon detection systems in the International Monitoring System stations to watch for signs of nuclear weapons testing and undeclared facilities. Systems using beta-gamma coincidence detection have been shown to have significantly reduced background counts, and are thus able to detect trace amounts of atmospheric radioxenon. A prototype of a multi-element coplanar CZT that uses two face-to-face coplanar CZT crystals to measure beta-gamma coincidence events from atmospheric radioxenon was developed at OSU.

OBJECTIVES The CZT-based detection system was simulated using MCNP to find the response of the detector to the xenon radioisotopes of interest and also calculate the coincidence detection efficiency of the device for these radioisotopes. In this work, modeling results from 131mXe, 133mXe, and 135Xe are reported.

MCNP MODELING 1. DETECTOR GEOMETRY

Geometry of the CZT-based radioxenon detection system simulated in MCNP.

2. PTRAC CARD

To model β-γ coincidence events in the CZT crystals, the PTRAC card was used. PTRAC follows each particle individually and writes an output file containing the entire history of that particle including position of interaction, energy of the particle, and the history number. A Python code was . developed to parse the PTRAC files and extract the position of . . interaction, energy released in each CZT crystal, and the . history number of each event from the PTRAC files. β-γ . coincidence events were then extracted for events with the . same history number ( NPS number).

COINCIDENCE DETECTION

PYTHON ALGORITHMS RESULTS

135Xe 135Xe emits 250 keV gammas in coincidence with beta particles (maximum energy ~ 910 keV)

133mXe 133mXe emits 30 keV x-rays in coincidence with 199 keV conversion electrons. (a) Simulated beta/gamma coincidence spectrum of 133mXe (b) energy deposited by 133mXe coincident events in CZT1.

131mXe 131mXe emits 30 keV x-rays in coincidence with 129 keV conversion electrons.

(a) Simulated beta/gamma coincidence spectrum of 131mXe (b) energy deposited by 131mXe coincident events in CZT1.

Radioxenons coincidence detection efficiencies calculated using MCNP.

Coincidence Simulation of a Two-Channel CZT-based Radioxenon Detector Lily Ranjbar*, Abi T. Farsoni, Eric M. Becker, David M. Hamby

Oregon State University, Corvallis, OR

Abi Farsoni, [email protected]

Consortium for Verification Technology (CVT)

Radioxenon

Gas Cell

Coplanar CZT1

Radioxenon

Injection Tube

Start

Load β / CE

PTRAC file

Load γ / X-

rays PTRAC

file

Interaction in

CZT1/CZT2?

Yes Full Energy

absorption?

Yes

Calculate

Partial Energy

Absorption

No

Save β /CE

and γ/x-ray

Partial Energy

Absorption

Save β/CE

and γ/x-ray

Full Energy

Finish

No

Last NPS Next NPS

Ignore First

10 Lines

Flowchart of the Python algorithm to parse

the PTRAC output files.

Flowchart of the Python algorithm to extract coincident events.

CZT 1 CZT 2

β/CE γ/x-ray

γ/x-ray β/CE

Scenario No.1

Scenario No.2

Coincidence scenarios considered in

this simulation.

Isotope Half-life Coincident Energies

(keV) Type Intensity (%)

131mXe 11.9 d 30

129

K X-ray

CE

54.1

60.7

133mXe 2.19 d 30

199

K X-ray

CE

56.3

63.1

133Xe 5.245 d

31

81

45

346

K X-ray

Gamma

CE

Beta (endpoint)

48.9

37

54.1

99

135Xe 9.1 h 250

910

Gamma

Beta (endpoint)

99

97

250 keV γ-rays

134 keV Compton edge

γ-γ

coincidence

events

x-rays escape peak

(a) (b)

(a) (b)

(a) (b)

This work was funded in-part by the Consortium for Verification Technology under Department of Energy National Nuclear Security Administration award number DE-NA0002534.

Save γ Energy in

Array1, β Energy

in Array 2

Equal NPS?

Yes

Finish

No

Start

Last NPS Next NPS

Load β / CE

Energy Data in

CZT2

Load γ / X-rays

Energy Data in

CZT1

Yes

Next NPS

Equal NPS?

Load β / CE

Energy Data in

CZT1

Load γ / X-rays

Energy Data in

CZT2

No

Finish Last NPS

Save γ Energy in

Array 2, β Energy

in Array 1

Radioxenon Coincidence Efficiency (%)

131mXe 3.1

133mXe 2.7

135Xe 1.7

(a) Simulated beta/gamma coincidence spectrum of 135Xe (b) energy deposited by 135Xe coincident events in CZT1.

Unclassified