a life cycle evaluation of wood pellet gasification for district heating

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  • 8/11/2019 A Life Cycle Evaluation of Wood Pellet Gasification for District Heating

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    A life cycle evaluation of wood pellet gasification for district heating

    in British Columbia

    Ann Pa a, Xiaotao T. Bi a,, Shahab Sokhansanj a,b

    a Clean Energy Research Centre for University of British Columbia, 2360 East Mall Vancouver, BC, Canada, V6T 1Z3b Environmental Sciences Division, Oak Ridge National Laboratory, Oak Ridge, TN 37831, USA

    a r t i c l e i n f o

    Article history:

    Received 23 November 2010

    Received in revised form 28 January 2011

    Accepted 1 February 2011

    Available online 5 February 2011

    Keywords:

    Life cycle analysis (LCA)

    Wood pellets

    British Columbia

    District heating

    Gasification

    a b s t r a c t

    The replacement of natural gas combustion for district heating by wood waste and wood pellets gasifi-cation systems with or without emission control has been investigated by a streamlined LCA. While stack

    emissions from controlled gasification systems are lower than the applicable regulations, compared to

    the current base case, 12%and 133% increases areexpected in the overall human health impacts for wood

    pellets and wood waste, respectively. With controlled gasification, external costs and GHG emission can

    be reduced by 35%and 82%on average, respectively. Between wood pellets andwoodwaste, wood pellets

    appear to bethe better choice as it requires less primary energy and has a much lower impact on the local

    air quality.

    2011 Elsevier Ltd. All rights reserved.

    1. Introduction

    As climate change due to greenhouse gas (GHG) emissions is

    gaining recognitions, various methods of climate change adapta-

    tion and GHG emission mitigation have been proposed, discussed

    and explored. Replacing a fraction of the current fossil fuel by

    alternative energy sources such as bioenergy is one of the many

    approaches recommended by policy makers. For instance, ethanol

    blending requirement in transport fuel in the United States

    reaches 1.14 EJ in 2010 and will increase to 3.18 EJ by 2022 while

    the European Union target for renewable energy in the transport

    sector in 2020 is set to 10%, or 1.29 EJ of biofuel (IEA and OECD,

    2009; European Commission, 2007). Other than in the transport

    sector, there are numerous studies that emphasize the potentials

    of renewable energy, or more specifically bioenergy, in district or

    residential heating and in combined heat and power systems

    (CHP) (Difs et al., 2010; Bjrklund et al., 2001). The importanceof policy developments to promote the use of bioenergy in these

    sectors is also discussed (Kopetz, 2007; Rickerson et al., 2009).

    However, the use of biomass for district heating has been quite

    controversial due to concerns with possible increase in health im-

    pact (Ries et al., 2009). This concern is especially true when the

    fossil fuel to be replaced is natural gas and when the community

    is densely populated. There are currently a few major district

    heating systems in Vancouver. These include one located in the

    stadium and entertainment district in the core of downtown

    (Davis, 2004) and three in Vancouvers largest hospital sites (Roger

    Bayley Inc., 2009; Ministry of Energy of British Columbia, 2010).

    The most recent establishment is the Southeast False Creek Neigh-

    bourhood Energy Utility (NEU) which provides hot water and heat

    for all new buildings in the area, including the Olympic Village that

    was built to accommodate Olympic athletes participating in the

    2010 Winter Olympic (City of Vancouver, 2010). The downtown

    system operates on natural gas while the NEU operates on a

    base-load system utilizing sewer heat recovery pump along with

    a natural gas peaking/back-up boiler. There was a debate at the

    beginning on the energy source to be chosen for the base-load sys-

    tem and the two contenders were biomass and sewer heat (Roger

    Bayley Inc., 2009). In the end sewer heat recovery heat pump sys-

    tem was selected because of the public concerns on local air qual-

    ity and traffic inconvenience that may arise from biomassutilization.

    Another district heating system in Vancouver is at the Univer-

    sity of British Columbia (UBC), where more than 99% of the heat

    is generated fromnatural gas and the rest fromfuel oil during peak

    season. With UBCs ambitious plan of reducing GHG to 33%, 67%

    and 100% below the 2007 level by 2015, 2020 and 2050, respec-

    tively, the University has devised a detailed plan of action. Replac-

    ing natural gas with renewable energy is an important part of the

    actions to be taken (University of British Columbia, 2010a). In fact,

    $26 million CAD has been allocated for the establishment of a bio-

    mass gasification cogeneration system on campus for research and

    0960-8524/$ - see front matter 2011 Elsevier Ltd. All rights reserved.

    doi:10.1016/j.biortech.2011.02.009

    Corresponding author. Tel.: +1 604 822 4408; fax: +1 604 822 6003.

    E-mail address: [email protected](X.T. Bi).

    Bioresource Technology 102 (2011) 61676177

    Contents lists available at ScienceDirect

    Bioresource Technology

    j o u r n a l h o m e p a g e : w w w . e l s e v i e r . c o m / l o c a t e / b i o r t e c h

  • 8/11/2019 A Life Cycle Evaluation of Wood Pellet Gasification for District Heating

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    demonstration purposes (University of British Columbia, 2010b).

    Given UBCs strong motive to become green and the large amount

    of GHG emissions from the boiler house, it is interesting to inves-

    tigate the complete replacement of fossil fuels in its boiler house

    with bio-based fuels. Wood pellets, made of sawmill residue, burn

    cleaner than biomass residue and are produced in large quantity in

    BC are thus consideredas a potential candidate. In 2008, 9 out of 30

    pellet plants in operations in Canada are located in BC and about 35

    Canadian pellet mills are in the planning stage with 13 of them tobe located in BC (Melin, 2008, unpublished data). Overall, about

    90% of the pellets produced in Canada were exported and 78% of

    these pellets were shipped to Europe (Melin, 2008, unpublished

    data; Spelter and Toth, 2009). Finding domestic applications for

    these pellets would result in less transportation-related GHG emis-

    sions. The technology to be evaluated is gasification as it is cleaner

    than direct combustion.

    The replacement of UBCs current natural gas boiler house

    with a wood pellet gasification system is evaluated by a stream-

    lined life cycle analysis (LCA). LCA is a powerful tool for scenario

    comparisons as the incremental variation between each scenario

    would provide valuable insights for decision making. Up to date,

    LCA has been used to examine the benefits and impacts of various

    new projects such as the wastewater treatment and reuse system

    in China (Zhang et al., 2010). As there have been many concerns

    on the true impacts and degree of sustainability of biomass en-

    ergy systems, LCA has been used extensively in recent years to

    evaluate a wide range of bioenergy systems and, sometimes for

    comparison purposes, fossil fuel energy systems. Some examples

    include the study on lignocellulosic ethanol production (Spatari

    et al., 2010; Gonzlez-Garca et al., 2010), biofuel production from

    microalgae (Campbell et al., 2011; Collet et al., 2011) and biomass

    district heating systems (Eriksson et al., 2007). Eriksson et al.

    (2007) conducted a LCA study of district heating and CHP system

    in Sweden using three different fuels: waste incineration, biomass

    combustion and natural gas combustion. Another study at-

    tempted to use LCA to investigate which of natural gas combus-

    tion, wood pellet combustion, sewer heat recovery and

    geothermal recovery would be the best choice for a district heat-ing system in Vancouver, BC, Canada (Ghafghazi et al., in press).

    The study reveals that none of the energy sources has absolute

    advantages over the others in all the impact categories considered

    although by using renewable energy at least 200 kg of CO2-eqv

    can be avoided per MWh of heat produced. Furthermore, the per-

    formance of each type of energy source depends on many factors

    such as electricity mix and types of energy utilized for producing

    pellets.

    For this study, an in-house life cycle inventory (LCI) database of

    BC pellets (Pa et al., 2009) is utilized to evaluate a total of five sce-

    narios for district heating at UBC. The base scenario is the current

    installation and the others are wood waste gasification, wood pel-

    let gasification and each of the two gasification operations with

    emission controls. The wood waste gasification scenario utilizes

    emission factors from the industry for wood waste gasificationwhile the pellet scenario uses estimated wood pellet gasification

    emission factors based on literature values and wood waste gasifi-

    cation emission factors from industry. For the scenarios with emis-

    sion controls, an electrostatic precipitator (ESP) for dust control

    and a selective catalytic reduction (SCR) unit for NOXcontrol are

    included. The overall impacts on human health, ecosystem quality

    and primary energy consumption in addition to GHG reduction

    resulting from using wood waste and wood pellets are compared

    to demonstrate the pros and cons of wood waste and wood pellet

    utilization when replacing natural gas. The externality analysis

    based on variations in emission profiles in different scenarios is

    also performed to quantify the economical benefits for each

    option.

    2. Method and calculation

    2.1. In-house BC pellet LCI Database

    The functional unit for the in-house BC pellet LCI database is

    one tonne (t) of wood pellets. Allocations are mass-based. The

    streamlined life cycle consists of harvesting, transportation of har-

    vested material to sawmill, sawmill processing, transportation of

    sawmill by-products such as planer shavings and sawdust to pelletmill, pellet mill operations, pellet transportation in bulk via heavy

    duty trucks (HDV, class 8, which has a gross vehicle weight rating

    of above 15 t) and train to port in North Vancouver. For this study,

    the transportation of pellets from port in North Vancouver to UBC

    campus and the pellet usage in the UBC gasification/combustion

    boiler are also included. The 20.2 km transportation from port in

    North Vancouver to UBC is by HDV. Emissions from infrastructures

    and land use changes are not included in the database in view that

    pellets in BC are made from sawmill residue and forest residue.

    The pollutants investigated are CO2, CH4, N2O, CO, non-methane

    volatile organic compound (NMVOC), NOX, SOX and particulate

    matters (PM). Other pollutants in trace amounts, although avail-

    able in some databases, are not included in this study for consis-

    tency reasons. CO2

    is categorized as either fossil or biogenic.

    However, CH4and CO are separated into biogenic or generic where

    generic may contain a small amount of biogenic emissions as not

    all emission data used segregated fossil and biogenic emissions

    of CH4 and CO. Note that all indirect emissions are also included

    in the analysis. For instances, emissions produced during produc-

    tion and transportation of fuels are all accounted for in the

    database.

    Energy consumption data during harvesting and sawmill oper-

    ations are obtained from Sambos (2002) and Nyboers (2008)

    work, respectively. Information gathered from a few member com-

    panies of Wood Pellet Association of Canada provided energy con-

    sumption data for pellet mill and port operations. The different

    types of energy considered are electricity, natural gas, heavy fuel

    oil (HFO), middle distillates (diesel), propane, steam, wood waste

    and gasoline. The primary energy consumptions are included inthis database and the electricity mix used is specific to BC. Details

    regarding various transportation segments are also obtained from

    the surveys.

    The pellet LCI database was presented in the 8th World Con-

    gress of Chemical Engineering in Montral (Pa et al., 2009) and will

    be released in a follow-up publication with more details. The

    methodology used to establish this database is used to construct

    all the scenarios in this study.

    2.2. UBC district heating system

    For this study, a total of five scenarios will be investigated. The

    base case is the current operation and the four woody biomass gas-

    ification systems are wood waste, wood pellets and each of these

    two systems equipped with ESPs with 99% PM removal efficiencyand SCR with 80% NOXremoval efficiency.

    The values presented in this work are either per MJ of fuel input

    or per year of operation. The annual operation is based on the

    amount of heat that is currently generated in the base scenario

    on a yearly basis, which is 974 TJ. This is chosen as the functional

    unit because the amount of heat to be produced in a year is iden-

    tical for all scenarios thus allowing for scenario comparison, which

    is also equivalent to the functional unit of per unit of energy

    produced.

    2.2.1. Base scenario

    The current facility configuration consists of boilers where the

    fuels (natural gas and fuel oil) are fed into. The fuels are combusted

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    to heat up the entering water stream to produce steam at 165 psig

    (1138 kPa) that is then distributed around the campus. The flue gas

    from the boilers is directed to an economizer to preheat the water

    entering the boiler before the flue gas exits the facility. For the base

    case, the stages in the LCA of both natural gas and oil include pro-

    duction of fuels, their transportation or transmission to UBC, and

    emissions during the end usage at the current facility. The emis-

    sion factors for natural gas and fuel oil production and transmis-

    sion are obtained from GHGenius v3.17 (Delucchi and Levelton,2010) and are referred to as upstream emission factors. In GHGe-

    nius, CH4 and CO emissions from both fossil and biomass origins

    are not segregated and are both reported simply as CH4 and CO.

    By default, GHGenius does not display biogenic emissions of CO 2but this can be altered so biogenic CO2emission values can be ex-

    tracted. The combustion emission factors for the current installa-

    tion are from the Combustion Test Report provided by UBC boiler

    house (Northwest Instrument Systems Inc., 2009), EMEP CORINAIR

    Emission Inventory Guidebook (European Environment Agency,

    2007) and US EPA AP-42 documents (US Environmental Protection

    Agency, 1995). For the CombustionTest Report, the boiler was fired

    with different fuels and at different capacities. The emissions were

    higher if the equipment was operated at a lower capacity. For the

    purpose of this study, the emission factors at 50% capacity are se-

    lected. The emissions were reported as concentrations (in ppmv) of

    the flue gas so material balance is carried out to determine the flue

    gas flow rate. For natural gas firing, SOXemission is assumed to be

    0 as sulfur content in the BC natural gas is negligible. Table 1lists

    the total emission factors of the UBC boiler running on natural gas

    and fuel oil with the sources of emission factors specified. The cur-

    rent amount of steam production is further explained in detail in

    the following section for easy comparison with the woody biomass

    scenarios.

    2.2.2. Woody biomass gasification scenarios

    The system boundary and stages for the wood pellet scenario

    have already been described earlier in the In-house BC pellet LCI

    Database section. The life cycle stages for the wood waste gasifi-

    cation scenarios include the production of two types of wood res-idues and their transportation, and the final usage at UBC. The two

    types of wood residues are forest harvesting residues and sawmill

    residues.

    The forest residue production started from harvesting operation

    with data taken fromSambo (2002). The forest residue is chopped

    in the forest using mobile chopper andthe emissions related to this

    process are from US-EI (Swiss Centre for Life Cycle Inventories

    et al., 2008). The chopped residue is then transported to railhead

    via HDV over a distance of 150 km. From the railhead to the North

    Vancouver shipping port, the train would travel 350 km. From the

    shipping port, the forest residue would be delivered to UBC district

    heating facility via HDV over a distance of 20.2 km.

    For the sawmill and planer mill residue, the harvesting of wood

    for the forest and sawmill operations are all included and emission

    data are based on literature used for the pellet LCI but convertedaccordingly so that the functional units are per tonne of wood res-

    idue with 51% moisture content, dry basis. The sawmill residue

    would be transported to the railhead via HDV over a distance of

    25 km. The residue then travel by train for 350 km before arriving

    the North Vancouver port. The residue is then delivered to UBC via

    HDV over a distance of 20.2 km. The distances used in the calcula-

    tions are estimated based on harvest field and sawmill locations in

    BC, Canada (Natural Resources of Canada, 2003a,b) and opinions

    from the local industry (Melin, 2010, personal communication).

    The final wood waste to be gasified is assumed to have a mois-

    ture content of 60%, dry basis, as that is maximum moisture con-

    tent allowed for smooth operation of the gasifier. Due to this

    limitation, some natural drying/aging is assumed to happen at

    UBC and the moisture content difference between the fuel deliv-

    ered and the fuel fed into the system is taken into account.

    The proposed biomass utilization system for woody biomass

    gasification is a retrofitted air gasification system because gasifica-

    tion generally produces lower PM, CO, VOC (volatile organics) and

    NOXemissions compared to direct combustion (European Environ-

    ment Agency, 2007; Sparica, 2009, personal communication). The

    syngas produced is combusted in the existing natural gas combus-

    tor to heat up water in the boiler to generate steam. The flue gas

    can be treated with an ESP to remove PM and/or a SCR unit to re-

    move NOXif required.

    The thermal efficiency of this system depends on the moisture

    content of the biomass fuel. Typical thermal efficiency for biomass

    fuel with approximately 60% moisture content (dry basis) is 62%

    (Sparica, 2009, personal communication) and this is the thermal

    efficiency assumed for the wood waste scenarios. For biomass with10% moisture content, the thermal efficiency is 78% (Sparica, 2009,

    personal communication). This number is used for wood pellet sce-

    narios despite the moisture content of BC wood pellets is actually

    around 6%. Combining thermal efficiency and the amount of steam

    produced in 2008, it is deduced that 126,015 t of wood waste, with

    a gross calorific energy content at 12.50 MJ/kg (Forest Product

    Table 1

    Estimated total emission factors for UBC boiler house and their sources.

    Fuel oil-firing boiler Natural gas-firing boiler

    Total emission

    factor (g/GJ of

    fuel used)

    Source of emission factor Total emission

    factor (g/GJ of

    fuel used)

    Source of emission factor

    Upstream Combustion Upstream Combustion

    CO2, fossi l 88,593 Delucchi and

    Levelton (2010)

    European Environment

    Agency (2007)

    53,393 Delucchi and

    Levelton (2010)

    Northwest Instrument Systems

    Inc. (2009)

    CO2, biogenic 475 0 79.9 0

    CH4 120 European Environment

    Agency (2007)

    72.3 European Environment

    Agency (2007)N2O 7.97 1.67

    CO 26.1 US Environmental Protection

    Agency (1995)

    9.14 Northwest Instrument Systems

    Inc. (2009)

    NMVOCa 22.8 European Environment

    Agency (2007)

    5.05 European Environment

    Agency (2007)

    NOX 89.8 Northwest Instrument Systems

    Inc. (2009)

    36.1 Northwest Instrument Systems

    Inc. (2009)

    SOX 245 Mass balance based on input S

    content fromPodolski et al. (2008)

    6.09 Mass balance based on input S

    content

    PM 5.73 European Environment Agency (2007) 0.49 European Environment

    Agency (2007)

    a Non-methane volatile organic compounds.

    A. Pa et al. / Bioresource Technology 102 (2011) 61676177 6169

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    Laboratory, 2004), is required annually to produce the same

    amount of steam as the base case. For the wood pellet scenarios,

    64,257 t of wood pellets, with a gross calorific energy content at

    19.4 GJ/t (Accredited Laboratory, 2007), is required. Just for com-

    parison, in 2008 the boiler house consumed 1034 TJ of natural

    gas and 7.84 TJ of fuel oil to generate 350 kt of steam at 165 psig

    (1138 kPa), translating to 974 TJ of heat produced (UBC Utilities,

    2009). These numbers correspond to a 93% overall thermal

    efficiency.

    2.2.1.2. Woody biomass gasification emission factors. For the wood

    waste scenarios, the gasification emission factors utilized were

    based on wood waste gasification in a commercial fixed bed gas-

    ifier. The biogenic CO2 emission is calculated based on the carbon

    content of wood. It was assumed that the carbon content in dry

    wood is 50% and the moisture content of wood waste, a mixture

    of forest residue and sawmill and planner mill residue, is 60%,

    dry basis, which is the maximum moisture allowed for the gasifier.

    At 60% moisture content, the mixed waste would give off 0.092 kg

    of biogenic CO2 emission per MJ of pellets gasified. The CH4, N2O

    and SOXemission factors are not available so they are estimated

    by the emissions of wood waste combustion in boiler from US

    AP42 document (US Environmental Protection Agency, 1995). The

    annual emissions are obtained by multiplying the emission factors

    by the annual fuel consumption.

    It is speculated that wood pellet gasification emission factors

    may vary quite substantially given that the combustion emission

    for wood waste and wood pellets do vary considerably as shown

    in the literature or published database (Swiss Centre for Life Cycle

    Inventories, 2008; Johansson et al., 2004; Wierzbicka et al., 2005;

    Lillieblad et al., 2004). In attempt to better represent wood pellet

    gasification emissions in the wood pellet scenarios, which are not

    available in the literature, the emission factors are estimated using

    two types of ratios. The first ratio is the ratio between wood and

    pellet combustion emission factors from literature and database.

    This first ratio together with the wood gasification emission factors

    from the industry can yield a set of estimated emission factors for

    the wood pellet gasification system. The second ratio is the ratiobetween published wood combustion emissions and the wood gas-

    ification emission from the industry. This ratio can then be applied

    to pellet combustion emission factors from literature and database,

    resulting in another set of estimated emission factors for pellet

    gasification, provided that the values of pellet and wood combus-

    tion emissions are different from those used to calculate the first

    ratio, as that would yield two identical sets of wood pellet gasifica-

    tion emission factors.

    In order to carry out this approximation process based on ratios,

    it is crucial to compare data with similar set-up in terms of emis-

    sion controls, system type and type of biomass used. Different

    emission data are matched based on considerations mentioned

    and whenever possible, data from the same article or database

    are compared. For the calculation of the first type of ratio, no unit

    conversion is required as the units used are usually consistentwithin a single source. However, when calculating the second type

    of ratios, unit conversions need to be performed as industrial emis-

    sion data for wood gasification are provided in mass of pollutant

    per energy unit of wood utilized while most literature report their

    data in mass of pollutant per volume of flue gas with the O2% or

    CO2% of flue gases provided along with the specification on dry

    or wet gas basis. Conversions of units are performed as described

    in The Handbook of Biomass Combustion and Co-firing (van Loo

    and Koppejan, 2007). Since gasification emission factors from the

    industry do not include CH4and N2O, their ratios are not calculated

    and pellet combustion emission factors from the US-EI database

    are used in the estimated pellet gasification emission data.Table 2

    lists all the emission factors used in the calculation of the ratios. Table

    2

    Listofpelletandwoodcombustionemissionfac

    torsfrom

    literatureinkgofpollutantemittedperMJoffuelutilized.

    Source

    Wierzbickaetal.

    (2005

    )

    Pagelsetal.

    (2003)

    Johanssonetal.

    (2004)

    USEnviron

    mental

    ProtectionAgency

    (1995)

    SwissCentrefor

    LifeCycleInventories

    etal.

    (2008)

    Lilliebladetal.

    (2004)

    Fuel

    Forestresidue

    Pellet

    Forestresidue

    Mixedwood

    Pellet

    Wetwood

    Mixedwood

    chip

    fromforest

    Pellet

    Shaving

    chips,

    andsawdust

    Pellet

    Load

    Medium

    High

    Medium

    80%

    60%

    45%

    Low

    Low

    Emissioncontrol

    Multicyclone

    Multicyclone

    None

    Multi

    cyclone

    M

    ulticyclone

    Typeofequipment

    1.5

    MW,

    movinggrate

    1MW,

    movinggrate

    Emission

    median

    forpelletboiler

    Emission

    median

    forpelletboiler

    Furnace,

    50kW

    1.5

    MW,

    m

    ovinggrate

    BiogenicCO2

    9.1

    7E02

    9.1

    7E02

    1.0

    3E01

    9.6

    5E028.9

    3E02

    7.8

    5E02

    BiogenicCH4

    4.3

    5E05

    1.7

    7E06

    9.0

    3E06

    9.0

    3E06

    7.0

    0E07

    3.0

    0E07

    N2O

    5.5

    9E06

    5.5

    9E06

    3.0

    0E06

    2.5

    0E06

    BiogenicCO

    4.1

    0E03

    3.2

    0E04

    2.5

    8E04

    2.5

    8E04

    1.1

    8E04

    6.5

    0E054.0

    0E04

    3.4

    4E05

    NMVOC

    2.8

    5E05

    2.5

    0E06

    7.3

    1E06

    7.3

    1E06

    9.0

    0E07

    1.5

    0E06

    NO

    X

    7.2

    0E05

    6.7

    0E05

    9.4

    6E05

    9.4

    6E05

    1.1

    0E04

    7.4

    0E053.3

    1E05

    4.6

    7E05

    SOX

    1.0

    7E05

    1.0

    7E05

    2.5

    0E06

    2.5

    0E06

    PM2.5

    3.4

    0E05

    2.0

    0E05

    PM

    4.4

    6E05

    6.8

    8E05

    1.8

    7E05

    8.1

    0E05

    5.5

    9E05

    4.5

    4E05

    8.8

    0E05

    1.9

    0E05

    1.4

    2E04

    9.4

    6E05

    4.3

    0E05

    2.3

    7E052.1

    6E05

    2.1

    6E05

    6170 A. Pa et al./ Bioresource Technology 102 (2011) 61676177

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    Table 3 summarizes the two set of emission factors obtained

    from the two types of ratios and their average values. The average

    estimated pellet gasification emission factors are used for the cal-

    culation in uncontrolled pellet scenario in this study. Note that SOXis manually set to zero since SOXemission depends mostly on the

    sulfur content of the fuel and wood pellet contains negligible sulfur

    at less than 0.01%, dry basis (Johansson et al., 2004).

    2.2.1.3. Emission controlled woody biomass gasification scenarios.

    Table 3also includes the current air emission limits, in kg per MJof fuel consumed, for biomass boilers and heaters in Metro Van-

    couver (Metro Vancouver, 2008) and the wood waste gasification

    emission factors used in this study. It is apparent that emission

    control units need to be in place in order to stay below the local

    air emission limit. The numbers show that NOX and PM need to

    be reduced by 37% and 66%, respectively for wood pellet and 44%

    and 87% for wood waste gasification. Both can be easily achieved

    by technologies such as SCR for NOXreduction and ESP for PM re-

    moval as the typical removal efficiencies for these units are

    approximately 80% and 99%, respectively (Forzatti, 2001; De

    Nevers, 2000). These efficiencies are applied for the controlled

    woody biomass gasification emission scenarios.

    2.3. Life cycle impact assessments of the scenarios

    Biogenic CO, CO2 and CH4 have the same impacts as non-bio-

    genic emissions in terms of human and ecosystem quality as the

    chemical structure does not depend on the origin of emissions.

    However, in terms of climate change impact, biogenic CO, CO2and CH4are considered to have less impact than their fossil-origin

    counterparts as biogenic carbon emissions are considered to be

    carbonneutral and do not result in net-increase in the carbon con-

    tent of the atmosphere. By definition PM is for all particulate mat-

    ters while PM2.5 refers to those less than 2.5lm and PM10 are

    those less than 10 lm. PM2.5 are the ones with significant health

    impacts (Humbert et al., 2005). The impact factors for PM are esti-

    mated based on an average PM2.5to PMratio in ambient air of 0.33

    (Humbert et al., 2005; Dockery and Pope, 1994). Throughout this

    study, care was taken to avoid double accounting. When only PMemission factors are available, such as from GHGenius database

    (Delucchi and Levelton, 2010), they are used and the impacts are

    calculated using PM impact factors. When both PM and PM2.5emission factors are available, only the PM2.5 emission factors

    and thus impacts are utilized. In the result section, sometimes both

    PMand PM2.5are listed, but it is important to acknowledge that for

    each process, only one of the PM or PM2.5 emission factors, and

    thus their respective impact factors, is used, not both.

    The emission factors and energy consumption data are im-

    ported into a commercial LCA software, SimaPro, to allow for the

    use of various life cycle impact assessment (LCIA) methods. IM-

    PACT 2002+ (Jolliet et al., 2003) is selected for impact assessment

    in this case study. IMPACT 2002+ includes both midpoint and

    end point impacts by linking all life cycle inventory data via 15

    midpoint categories to four damage, or end point, categories, as

    illustrated inFig. 1. The dashed lines indicate that the conversion

    into damage categories has not yet been properly established.

    The units used for each impact category, such as DALY and

    PDFm2 yr, are defined inFig. 1.

    The most current version of IMPACT 2002+ at time of analysis

    (v2.06) is adapted for analysis with two extra categories added to

    keep track of the primary energy consumption and external costs

    throughout the entire life cycle. These two new end point catego-ries are also presented inFig. 1. The impacts of biogenic CH4 and

    CO are added under the categories of respiratory organic and inor-

    ganic, respectively, using the impact values of their fossil fuel ori-

    gin counterparts. Six endpoint categories, human health,

    ecosystem quality, climate change, primary energy consumption,

    external cost and resources can be obtained. Only the first five will

    be evaluated in this study. It is important to keep in mind that IM-

    PACT 2002+ was developed in Europe so the values of parameters

    used for the compilation of human toxicity are at a continental le-

    vel for Western Europe. Due to this reason, the final values to be

    presented here only serve as indicators for scenario comparisons

    as the absolute values may not be so meaningful due to geograph-

    ical and geological differences in Western Canada and Western

    Europe.

    External cost, also known as externality, is the unaccounted anduncompensated impact on a group arising from the social or eco-

    nomic activities of other groups (European Commission, 2003).

    Table 3

    Estimated wood pellet gasification emission factors and air emission limits for biomass boilers in Vancouver, Canada.

    Pol lutant Wood waste

    gasification emission

    factors (kg/MJ)

    Estimated pellet gasification

    emission factors based on

    ratio 1 (kg/MJ)

    Estimated pellet gasification

    emission factors based on

    ratio 2 (kg/MJ)

    Average estimated pellet

    gasification emission

    factors (kg/MJ)

    Vancouver air emission

    limit for biomass boilers

    (kg/MJ)

    Biogenic CO2 9.17E02 8.50E02 8.22E02 8.36E02

    Biogenic CH4 9.03E06 3.00E07 3.00E07 3.00E07

    N2O 5.59E06 2.50E06 2.50E06 2.50E06

    Biogenic CO 1.46E05 1.26E06 1.14E06 1.20E06 1.59E04

    NMVOC 4.30E06 3.77E07 3.02E07 3.39E07

    NOX 7.31E05 6.80E05 6.33E05 6.56E05 4.10E05

    PM 4.00E05 1.92E05 1.14E05 1.53E05 5.13E06

    Fig. 1. Overall scheme of the IMPACT 2002+ framework, linking LCI results via the

    midpoint categories to damage categories with modifications implemented for this

    study (based onJolliet et al., 2003).

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    Therefore, externality reflects the impact on environment and hu-

    man health. Table 4 lists three sets of reported external costs for air

    pollutants investigated in this study. The costs for biogenic CO2,

    CH4 and CO are estimated using the impact factors for different

    pollutants in IMPACT 2002+. The global warming factors listed in

    IMPACT 2002+ are mostly based on IPCC 2001s 500-year time

    horizon values. Since CO2 only has an effect on climate change

    and biogenic CO2 has no impact, biogenic CO2 has been assigned

    a zero external cost. It is noted that the average external cost for

    CH4 in the literature is close to $0.23, which is equal to the cost

    of CO2 multiplied by the impact factor of CH4, a value of seven.

    The same observation is made for N2O where the calculated valuebased on its impact factor of 156 is $5.15. Based on these observa-

    tions, the external cost of biogenic CH4is estimated by multiplying

    its impact factor of 4.25 by the cost of CO2 to yield $0.14. This is

    plausible as CH4 only has effects on global warming according to

    IMPACT 2002+. For biogenic CO, it also has impact on human

    health, which is the total cost of CO minus the cost of climate

    change. With the cost of climate change for CO being estimated

    as the cost of CO2 multiplied by the climate change impact factor

    for CO in IMPACT 2002+, which is 1.57, the health cost for CO is

    found to be $0.67, which applies to CO from all sources. Since

    the climate change impact factor of biogenic CO is 0, the total cost

    of biogenic CO is equal to the health cost of CO. The emission

    reduction achieved from replacing natural gas and fuel oil with

    wood pellets can then be combined with external cost for each pol-

    lutant inTable 4to derive the reduction in external costs.Since health impact depends heavily on the emission location

    and its proximity to population, the health impact associated with

    end usage alone for all five scenarios are compared as the point of

    usage is at UBC campus, where the risk of exposure to pollutant is

    much higher compared to pellet mills in suburban areas. The end

    stage health impacts for all scenarios are normalized by the value

    of the base scenario as it is the relative, not the absolute, values of

    the health impact that are relevant for this comparison.

    3. Results and discussion

    Using values presented inTable 1, the current annual emissions

    from UBC boiler house are calculated and presented in Table 5,

    together with the emissions from all the biomass gasification sce-

    narios. The emission factor for PM instead of PM2.5is provided for

    all processes in the life cycle except for steam generation, where

    the PM2.5 emission factor is provided instead of PM. Due to this

    reason, there are both PM and PM2.5emissions reported inTable 5

    but there is no overlapping between them as the emission factor

    for PM during steam generation was not used in the calculation.

    From Table 5 it is apparent that the estimated biogenic CO,

    NMVOC, NOXand PM emissions for pellet gasification are lower

    than wood waste gasification, as observed in pellet and wood

    waste combustion. It appears that the most obvious advantage of

    switching to woody biomass gasification is the drastic reductionof CO2emissions of fossil fuel origin. However, this is coupled with

    a substantial increase in biogenic CO2emission, particularly due to

    lower thermal efficiency for the biomass gasification system and

    the high carbon intensity of biomass energy. Another emission

    reduction lies in generic CH4. Even though there is a slight increase

    of biogenic CH4 emission, there is a net CH4 reduction of 64% and

    77% when accounting CH4from all origins for wood waste and pel-

    let gasification, respectively. The high CH4emission from the cur-

    rent scenario arises from the upstream processing of natural gas

    as well as the leakage and loss during pipeline transmission. This

    observation is more noticeable inFig. 2where the stage-wise dis-

    tribution of each pollutant for the current scenario is illustrated. It

    is evident from the same figure that natural gas burns very cleanly

    with most of the emissions from upstream, with the exception of

    fossil CO2, N2O and NMVOC. Despite that natural gas combustionand upstream operations seem to be contributing the most to the

    emissions and environmental impacts, it is important to note that

    more than 99% of the energy input was from natural gas thus Fig. 2

    does not suggest that fuel oil burning is cleaner than natural gas.

    However, it is noted that there is a significant SOXemission from

    oil combustion despite that only less than 1% of the energy input

    was from fuel oil.

    Other than generic CH4emission and CO2emission of fossil ori-

    gins, all other emissions would increase when the boiler is

    switchedfrom natural gas to woody biomass gasification. The most

    significant increase, other than in biogenic CO2, is in PM emissions,

    reaching approximately 130- and 77-folds for wood waste and

    wood pellets, respectively. Even with an ESP unit, the increase

    Table 4

    Summary of external costs from literature and the external costs used in this study.

    Bi and Wang (2006) Average values from various

    states in the US a Golay (2005)

    Dones et al. (2005) Values used in this analysis Calculation and remarks

    CAD $/kg CAD $/kg CAD $/kg CAD $/kg

    CO2, fossil 0.04 0.03 0.03 0.03 Average of all values

    CO2, biogenic 0 Estimated using impact factors in

    IMPACT 2002+ method

    CH4 1.05b 0.25 NA 0.25 State average value is used as it is

    not just estimation based on GWP

    CH4, biogenic 0.14 Estimated using impact factors in

    IMPACT 2002 + method

    N2O 12.52b 4.73 NA 4.73 State average value is used as it is

    not just estimation based on GWP

    CO 0.41 1.02 NA 0.72 Average of all values

    CO, biogenic 0.67 Estimated using impact factors in

    IMPACT 2002 + method

    NMVOC NA NA 1.78 1.78

    VOC NA 3.76 NA 3.76

    NOX 5.23 6.41 4.59 5.41 Average of all values

    SOX 5.46 2.30 4.64 4.14 Average of all values

    PM 14.70 3.14 18.52c 12.12 Average of all values

    PM2.5 NA NA 30.87 30.87

    a Based on values from New York State Public Service Commission, Department of Public Utilities of Massachusetts, Public Service Commission of Nevada and

    California Public Utilities Commission and presented in Golays lecture slides (Golay, 2005).b Estimated by source based on CO2cost multiplied by specific pollutants 100 years time horizon GWP (global warming potential) value from the 2007 IPCC report.c Estimated by source based on typical PM2.5/PM ratio.

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    would still be approximately 17- and 43-folds for wood waste and

    pellet, respectively. ESP appears to be less effective for the pellet

    scenario because a large portion of PM emission is released from

    the upstream fuel preparation process, which is not controlled by

    the ESP installed for the gasification plant. For wood pellet sce-

    nario, approximately 31% of the total PM emission is from pellet

    mill where wood residue is burned for biomass drying. Thus,

    removing PM from gasification process alone would achieve a less

    significant PM reduction over the entire life cycle. However, it isimportant to point out that the zero emission of PM2.5under cur-

    rent natural gas operation results from the fact that all emission

    factors related to base scenario are only for PM but not for PM2.5specifically. With emission controls in place, the increase in other

    pollutant emissions ranges from 215% (for NMOVC) to 448% (for

    N2O) for wood waste and 42% (for SOX) to 393% (for all CO), for

    wood pellets.

    InFig. 3, the stage-wise contributions to the total emissions are

    illustrated for wood waste gasification (Fig. 3a), wood pellet gasifi-

    cation (Fig. 3b), wood waste gasification with emission controls

    (Fig. 3c) and wood pellet gasification with emission controls

    (Fig. 3d), respectively.Fig. 3 reveals that the top contributor to bio-

    genic CO2and N2O emissions is the gasification stage for all woody

    biomass gasification scenarios. For the uncontrolled wood waste

    scenario, more than 80% of the generic CO and approximately

    50% of the NMVOC emissions are emitted during the harvesting

    stage. The gasification stage is the main contributor to the remain-

    ing pollutants except for fossil-origin CO2and generic CH4as more

    than 40% of each of these pollutants are emitted during harvesting.

    For wood waste gasification with emission control units, the har-

    vesting stage also becomes the main contributing stage for NOXand PM emissions throughout the life cycle and remains to be

    the main contributor for fossil-origin CO2 and generic CH4.

    For both uncontrolled and controlled wood pellet scenarios, the

    harvesting stage is the main contributor to fossil-origin CO2, gener-

    ic CO, NMVOC, and SOXwhile pellet mill is where the majority of

    biogenic CH4and CO is emitted due to the burning of wood residue

    within the mill. In the uncontrolled pellet scenario, 42% of the NOX

    emission in the life cycle is emitted in the harvesting stage and 40%from gasification. Moreover, gasification is responsible for 44% of

    the life cycle PM emission. However, with emission control, gasifi-

    cation stages contribution to PM and NOXare reduced to 0.8% and

    12%, respectively, with pellet mill becoming the new hot-spot for

    PMemission. Note that the PM categories in both Figs. 2 and 3 refer

    to All PM inTable 5.

    The external costs from each scenario are also presented inTa-

    ble 5. By switching to wood waste gasification, there is actually an

    increase of $450,000 CAD in external costs while wood pellet gas-

    ification would result in an $87,000 CAD saving. It was stated ear-

    lier that in order to satisfy the air emission limits in Vancouver for

    biomass boiler theNOX and PMemissions need to be reduced. With

    the installation of SCR and ESP units, these two pollutants can be

    reduced by 80% and 99% thus achieving emissions much lower

    than what is required. With the emission control units, the exter-nal costs can be reduced by 38% and 31% from the base case for

    wood waste and wood pellets, respectively. Note that no spatial

    variation of the external cost has been considered in the current

    analysis in which the emissions released in densely populated ur-

    ban area and less populated remote area are given the same exter-

    nal cost for each gas pollutant.

    Since emissions are increased for all major pollutants when the

    boiler house is switched from natural gas to wood pellet gasifica-

    tion, it is hard to comprehend the relative overall impacts from

    each scenario based on emission inventories only.Fig. 4compares

    each of the five scenarios impacts on human health, ecosystem

    quality and climate change, as well as a breakdown of these

    Table

    5

    Annualairemissionsfrom

    currentandwoodpe

    lletscenarios.

    Uncontrolledwoodybiomassgasification

    Controlledwoodybiomassgasificationa

    Emissionsforbase

    Scenario(t/yr)

    Emissionsfor

    woodwaste(t/yr)

    Reductioninexternal

    cost($1000CAD)

    Emission

    sfor

    woodpe

    llet(t/yr)

    Reductioninexternal

    cost($1000CAD)

    Emissionsfor

    woodwaste(t/yr)

    Reductioninexternal

    cost($1000CAD)

    Emissionsfor

    woodpellets(t/

    yr)

    Reductioninexternal

    cost($1000CAD)

    AllCO2

    55,9

    97

    154

    ,205

    1,5

    06

    121,5

    52

    1,5

    52

    154,2

    05

    1,5

    06

    121,5

    52

    1,5

    52

    CO2,

    fossil

    55,9

    11

    8

    ,629

    1,5

    06

    8,8

    77

    1,5

    52

    8,6

    29

    1,5

    06

    8,8

    77

    1,5

    52

    CO2,

    biogenic

    86.3

    0

    145

    ,575

    0.0

    0

    112,6

    76

    0.0

    0

    145,5

    75

    0.0

    0

    112,6

    76

    0.0

    0

    AllCH4

    75.7

    0

    27.1

    8

    13.8

    3

    17.5

    2

    14.7

    9

    27.1

    8

    13.8

    3

    17.5

    2

    14.7

    9

    CH4

    75.7

    0

    12.8

    5

    15.8

    4

    16.3

    6

    14.9

    6

    12.8

    5

    15.8

    4

    16.3

    6

    14.9

    6

    CH4

    b,b

    iogenic

    0.0

    0

    14.3

    3

    2.0

    1

    1.1

    7

    0.1

    6

    14.3

    3

    2.0

    1

    1.1

    7

    0.1

    6

    N2O

    1.7

    9

    9.8

    1

    37.8

    9

    4.6

    3

    13.4

    0

    9.8

    1

    37.8

    9

    4.6

    3

    13.4

    0

    AllCO

    9.6

    5

    47.7

    3

    25.9

    7

    47.6

    0

    25.9

    8

    47.7

    3

    25.9

    7

    47.6

    0

    25.9

    8

    COb

    9.6

    5

    21.6

    2

    8.5

    9

    23.4

    3

    9.8

    9

    21.6

    2

    8.5

    9

    23.4

    3

    9.8

    9

    CO,b

    iogenic

    0.0

    0

    26.1

    0

    17.3

    8

    24.1

    7

    16.1

    0

    26.1

    0

    17.3

    8

    24.1

    7

    16.1

    0

    NMVOC

    5.4

    0

    17.0

    1

    20.6

    2

    11.7

    9

    11.3

    4

    17.0

    1

    20.6

    2

    11.7

    9

    11.3

    4

    NOX

    38.0

    4

    219

    980

    203

    893

    127.0

    0

    481

    137.5

    6

    539

    SOX

    8.2

    2

    127.0

    0

    77.8

    1

    11.6

    4

    14.1

    1

    27.0

    4

    77.8

    1

    11.6

    4

    14.1

    1

    AllPM

    0.5

    6

    72.5

    5

    882

    43.5

    5

    522

    10.1

    8

    126

    24.6

    3

    292

    PM

    0.5

    6

    72.0

    6

    867

    43.5

    2

    521

    9.6

    9

    111

    24.5

    9

    291

    PM2.5

    c

    0.0

    0

    0.4

    9

    15.2

    0

    0.0

    3

    1.0

    1

    0.4

    9

    15.2

    0

    0.0

    3

    1.0

    1

    Totalchangesin

    externalcost

    450

    87

    804

    671

    aselectivecatalyticreduction(SCR)hasaremovalefficiencyof80%whileelectrostaticprecipit

    atorhasaPMremovalefficiencyof99%.

    bmayincludesomebiogenicemissionsasw

    ell.

    cfromsteamgenerationonlyasnoPMem

    issionfactorwasavailableforthisprocess.

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    impacts into different stages to signal out hot-spots throughout

    their life cycles.

    By switching to woody biomass, both impacts on human health

    and ecosystem quality increase significantly. For human health, the

    current impact is 4 DALY and it would increase by 6.2- and 8.6-

    folds for wood pellets and wood waste, respectively. Even with

    emission control units, the increase would still be 3.3-folds on

    average for both woody biomass fuels. Since the parameters used

    in the impact assessment method are based on Western Europe,care should be exercised in the interpretation of human health

    impact.

    The current impact on ecosystem quality is 2.26E5 PDF m2 yr

    and it would increase by around 4.7 and 4.2 times when switched

    from natural gas to wood waste and wood pellet gasification sys-

    tems, respectively. With SCR and ESP, the increase can be lowered

    to an average of 2.4-folds for both fuel types.

    FromFig. 4it becomes apparent that the harvesting of woody

    material and the gasification stage contribute greatly to humanFig. 2. Stage-wise emission distribution for current natural gas boiler scenario.

    Fig. 3. Stage-wise emission distribution for (a) wood waste gasification, (b) wood pellet gasification, (c) wood waste gasification with SCR and ESP units with 80% NOXand

    99% PM removal efficiency, respectively, and (d) wood pellet gasification with identical emission control units.

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    health impact. It is evident that by adding emission control units,

    the pellet scenarios human health impact for the entire life cycle

    can be further reduced by 35% while the health impact associated

    with gasification alone can be further reduced by 87%. However,

    since wood waste requires little upstream processing, the addition

    of emission control can effectively reduce the overall health impact

    by 59% and the reduction in gasification stage alone would be 88%.

    For the effect on ecosystem quality, the main contributions are

    from the harvesting and gasification stages as well. With emissioncontrol, gasification only contributes 20% and 12% to the entire life

    cycles impact on ecosystem quality for wood waste and pellet,

    respectively. Moreover, with emission controls the ecosystem

    quality impact for the entire pellet gasification life cycle can be fur-

    ther lowered by 32% while impacts associated with gasification

    alone can be reduced by 80% when compared to uncontrolled pel-

    let scenario.

    Lastly,Fig. 4 confirms that the key advantage associated with

    switching to woody biomass is the reduction in GHG emissions.

    Fig. 4c clearly illustrates that impact on climate change can be re-

    duced by 82% and 83% from the current 56.7 kt of CO2-equvalent

    per year when wood waste and wood pellets are used, respectively.

    Another scenario performance indicator is primary energy con-

    sumption. To generate 974 TJ of usable heat annually, the current

    natural gas scenario consumes 1284 TJ of primary energy and this

    number is slightly higher for the pellet scenarios at 1516 and 1725

    TJ for wood waste scenarios. Primary energy takes into account the

    energy resource required to produce fuels, power or products.

    These include the heating value of raw materials such as harvested

    wood and crude oil, energy required to produce fuels such as die-

    sel, and energy required to convert different fuels, such as natural

    gas or diesel, to electricity.

    It is important to acknowledge that human health impact is

    more of local concern as compared to theglobal climate change im-

    pact. As the UBC district heating systemis located in a densely pop-

    ulated area, the stack emissions from the boiler house will have the

    most significant impact on human health. The end usage contribu-

    tions to human health impact for all five scenarios are normalizedby the base case value andare comparedin Fig. 5. It is apparent that

    the human health impact directly linked to the end usage increases

    substantially when switched from natural gas to woody biomass as

    it would be augmentedby 18- and7.7- folds for uncontrolled wood

    waste and pellet gasification, respectively. Thisvalueis lowered to a

    133% increase for controlled wood waste scenario and a mere 12%

    increase for controlled wood pellet scenario. As a result, it is

    strongly recommended that both the PM and NOXemission control

    units be installed in biomass combustion/gasification district heat-

    ing systems to prevent the deterioration of local air quality and

    drastic increase in local health impact, in addition to meeting the

    local emission standards. It should be noted that adopting wood

    pellet gasification may have other impacts on the community that

    are not accounted for in this study, such as the noise and inconve-

    nience associated with pellet delivery traffics.

    In this study, the gasification plant produces only heat so the

    LCA study of a CHP plant in place of the existing boiler house might

    yield different results. As UBC also aims to become a net energy

    exporter by 2050, the CHP option is readily pursued as UBC has

    Fig. 4. Stage-wise impact analysis in terms of (a) human health, (b) ecosystem quality, and (c) climate change for curren t and woody biomass gasification with and without

    emission control units.

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    already decided to establish a CHP demonstration unit on campus

    using a system developed by Nexterra and GE to provide green

    heat and electricity while serving as a research facility.

    4. Conclusions

    Replacing fossil fuels with biomass may not always be desirable

    and the decision would depend heavily on the priorities of the spe-

    cific project. Natural gas combustion outperforms emission-con-

    trolled woody biomass gasification scenarios in primary energy

    consumption and all impact categories considered other than cli-

    mate change while all woody biomass gasification scenarios yield

    significant reduction on GHG and external costs. Pellet gasification

    is superior to wood waste as it has lower primaryenergy consump-

    tion and the health impact associated with stack emission for the

    controlled waste wood gasification is 133% higher than the base

    scenario, compared to 12% for pellets.

    Acknowledgements

    The authors would like to thank UBC Sustainability office, UBC

    Utility, and Dr. Anthony Lau for providing the air emission data

    for the existing natural gas district heating facility. The authors

    are also grateful to the financial support from Agriculture Canadas

    ABIN program and the UBC Graduate Fellowship (UGF) program.

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