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    Scattering of partially coherent electromagnetic beams

    by water droplets and ice crystals

    Jianping Liu a,n, Lei Bi b, Ping Yang b, George W. Kattawar a

    a Department of Physics and Astronomy, Texas A&M University, College Station, TX 77843, USAb Department of Atmospheric Sciences, Texas A&M University, College Station, TX 77843, USA

    a r t i c l e i n f o

    Article history:

    Received 31 August 2013

    Received in revised form

    6 November 2013

    Accepted 8 November 2013Available online 16 November 2013

    Keywords:

    Partially coherent light

    LorenzMie

    Mueller matrix

    Water droplet

    Ice crystal

    a b s t r a c t

    The conventional LorenzMie theory is generalized for a case when the light source is

    partially spatially coherent. The influence of the degree of coherence of the incident field

    on the generalized Mueller matrix and the spectral degree of coherence of the scattered

    light is analytically studied by using the vector field instead of the scalar field to extend

    previous results on the angular intensity distribution. The results are compared with the

    Mueller matrix obtained from the Discrete Dipole Approximation (DDA) method, which is

    an average over an ensemble of stochastic incident beams. Special attention is paid to the

    Mueller matrix elements in the backward direction, and the results show some Mueller

    matrix elements, such as P22, depend monotonically on the coherence length of the

    incident beam. Therefore, detecting back scattering Mueller matrix elements may be a

    promising method to measure the degree of coherence. The new formalism is applied to

    cases of large spherical droplets in water clouds and hexagonal ice crystals in cirrus

    clouds. The corona and glory phenomena due to spheres and halos associated with

    hexagonal ice crystals are found to disappear if the incident light tends to be highly

    incoherent.

    & 2013 Elsevier Ltd. All rights reserved.

    1. Introduction

    In the conventional theories of light scattering, such as

    LorenzMie theory[1], Discrete Dipole Approximation (DDA)

    [2,3], and Finite-Difference Time-Domain (FDTD) method[4],

    the incident light is generally assumed to be fully coherent in

    both space and time. However, the assumption is not always

    justified. In reality, light acquires some degree of incoherence

    due to light source fluctuations or to interactions with randommedia such as a turbulent atmosphere. Although the general

    framework of optical coherence theory has long been well

    established[57], scarcely any attention has been paid to the

    effect of coherence on light scattering by deterministic media.

    The influence of spatial coherence on scattering by a particle

    was partially investigated by Cabaret et al. [8]and Greffet[9].

    The extinction cross section of rotationally invariant scatterers

    was found not to depend on the transverse (or spatial)

    coherence length, but the extinction cross section of aniso-

    tropic scatterers did depend on the state of coherence of the

    illuminating field. Further research on the topic was con-

    ducted by van Dijk [10] and Fischer [11] who studied the

    effects of spatial coherence on the angular distribution of

    radiant intensity scattered by a sphere. By using the angular

    spectrum representation of a random field[6]and half wave

    expansion of the scattering amplitude, the intensity of ascattered field was analytically obtained. The angular distribu-

    tion of radiant intensity depends strongly on the degree of

    coherence, but the extinguished power does not. Sukhov [12]

    numerically studied the effect of spatial coherence by a

    random medium on the properties of scattered fields, and

    the DDA method was used to demonstrate that the statistical

    properties of the scattered light from an inhomogeneous

    medium were altered due to coherence effects.

    Previous theories have been limited to the study of the

    scattered field intensity, which does not fully describe

    a scatterer with respect to light scattering. A common

    Contents lists available atScienceDirect

    journal homepage: www.elsevier.com/locate/jqsrt

    Journal of Quantitative Spectroscopy &Radiative Transfer

    0022-4073/$ - see front matter & 2013 Elsevier Ltd. All rights reserved.http://dx.doi.org/10.1016/j.jqsrt.2013.11.002

    n Corresponding author. Tel.: 1 979 587 9918.

    E-mail address: [email protected] (J. Liu).

    Journal of Quantitative Spectroscopy& Radiative Transfer 134 (2014) 7484

    http://www.sciencedirect.com/science/journal/00224073http://www.elsevier.com/locate/jqsrthttp://dx.doi.org/10.1016/j.jqsrt.2013.11.002mailto:[email protected]:[email protected]://dx.doi.org/10.1016/j.jqsrt.2013.11.002http://dx.doi.org/10.1016/j.jqsrt.2013.11.002http://dx.doi.org/10.1016/j.jqsrt.2013.11.002http://dx.doi.org/10.1016/j.jqsrt.2013.11.002http://dx.doi.org/10.1016/j.jqsrt.2013.11.002http://dx.doi.org/10.1016/j.jqsrt.2013.11.002mailto:[email protected]://crossmark.crossref.org/dialog/?doi=10.1016/j.jqsrt.2013.11.002&domain=pdfhttp://crossmark.crossref.org/dialog/?doi=10.1016/j.jqsrt.2013.11.002&domain=pdfhttp://crossmark.crossref.org/dialog/?doi=10.1016/j.jqsrt.2013.11.002&domain=pdfhttp://dx.doi.org/10.1016/j.jqsrt.2013.11.002http://dx.doi.org/10.1016/j.jqsrt.2013.11.002http://dx.doi.org/10.1016/j.jqsrt.2013.11.002http://www.elsevier.com/locate/jqsrthttp://www.sciencedirect.com/science/journal/00224073
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    generalization is to study the Mueller matrix, which relates

    the Stokes vector of the incident beam to the Stokes vector of

    the scattered beam. For a large class of light beams such as

    the so-called Gaussian Schell-model beam, the Mueller

    matrix for a sphere is derived analytically by extending the

    LorenzMie theory. We developed a DDA code [3] by

    modifying the source field to incorporate incoherence, and

    the Mueller matrix was obtained by averaging over anensemble of stochastic incident fields. In addition, we

    investigated the spectral degree of coherence of the scat-

    tered light. As applications of the formalism developed, we

    performed the computation of light scattering by water

    droplets and hexagonal ice crystals, which are the major

    scatterers inside atmospheric clouds. The coherence effects

    of spherical water droplets were studied by modifying the

    LorenzMie theory. With the Invariant Imbedding T-matrix

    method (see[13]and references cited therein), we were able

    to study the coherence effects on halos of large hexagonal ice

    crystals.

    2. Scattering of partially coherent light by a sphere

    We consider the scattering of electromagnetic beams of

    an arbitrary state of spatial coherence by a homogenous

    sphere on the basis of a generalization of previous results

    in[10,11]. Note that the procedure is quite similar to that

    used by Lahiri and Wolf [14], where the refraction and

    reflection of partially coherent electromagnetic beams

    were considered.

    2.1. Theory of coherence

    We use some of the important results from the coher-

    ence theory of electromagnetic beams [7]. The stochasticnature of incoherent monochromatic light is represented

    by an ensemble of random fields fEr;g, where is the

    frequency, and for each realization, the field component is

    transverse to the direction of propagation. By choosing the

    same plane of reference as in the previous section, each

    random field can be expressed as

    Er; Elr;

    Err;

    !: 1

    Following the same formalism used by Wolf [7], the

    second-order correlation properties of the stochastic field

    are fully characterized by the 22 cross-spectral density

    matrix (CSDM) defined by

    Wr1; r2; Enr1;UE

    Tr2;

    Enl r1;Elr2; E

    n

    l r1;Err2;

    Enrr1;Elr2; En

    rr1;Err2;

    !;

    2

    where denotes the ensemble average. From the CSDM,

    the spectral density can be derived at point r and at

    frequency

    Sr; TrWr; r;; 3

    which can be interpreted as a contribution to the intensity

    at point r from the field component of frequency .The spatial degree of coherence of the random field is

    defined by[7]

    r1; r2; TrWr1; r2;ffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi

    Sr1;p ffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi

    Sr2;p ; 4

    which unifies both polarization and coherence. 0r j

    r1; r2;jr1 with 0 representing complete incoherence

    and 1 representing complete coherence.

    2.2. Incident light

    Incoherent beams can be represented by an ensemble

    of random fields and are realized using the angular

    spectrum representation [6]. A partially coherent beam

    propagating in the zdirection can be expressed as

    Eir;

    Zju

    ?jo1

    eiu? ;expikuUr d2

    u? ; 5

    where the coefficient eiu? ; is a two-component ran-

    dom vector defined by

    eiu? ; eil u

    ? ;

    eir u

    ? ;

    0@ 1A; 6k =cis the wavenumber, u is the direction of propaga-

    tion of each plane wave component, u? ux; uy is the

    projection ofuonto thez0 plane, and the unit vector u

    points into the z40 half space, i.e. uzffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi

    1ju? j2

    q . The

    scattering plane is chosen as the reference plane.

    The incident field is uniquely defined by the source at

    thez0 plane, which is characterized by the CSDM

    Wi1;2; E

    in1;UEiT2;; 7

    where 1 and 2 are 2D vectors in the z0 plane. UsingEq.(5), we have

    Wi1;2;

    Z d

    2u? d

    2u?

    ~W

    iu? ; u

    ? ;expiku

    ? U1u

    ? U2;

    8

    where the angular correlation matrix ~W

    i

    u? ; u

    ? ;

    einu? UeiTu? is defined as a four-dimensional

    Fourier transformation of the CSDM at thez0 plane, i.e.

    ~W

    i

    u?

    ; u?

    ;

    k

    2

    4 Z d

    21d

    22W

    i

    1;2;expiku

    ? U1u

    ? U2:

    9

    We consider a widely used class of partially coherent

    beams, the so-called Gaussian Schell-model beams, which

    have the following CSDM elements

    Wilm1;2; alamblmexp

    2122

    4s2S

    !exp

    122

    2s2

    !:

    10

    The independently chosen parameter sS can be inter-

    preted as the width of the beam, and s as the coherencelength. The remaining parameters in Eq. (10) have the

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    following constraints[7]

    bij 1 when i j; 11

    bij r1 when iaj; 12bij b

    n

    ji; 13

    ai Z0: 14

    By substituting Eq.(10)into Eq.(9)and performing the

    four dimensional integration, one can obtain the angular

    correlation matrix[10]

    ~Wi

    lmu

    ? ; u

    ? ; alamblmk

    2ssef f

    2

    !2

    exp k

    2

    2 u? u

    ? 2s

    2Su

    ? u

    ? 2s

    2ef f

    4

    " #( ); 15

    where

    1

    s2ef f

    1

    s2

    1

    4s2S: 16

    In order to obtain the Mueller matrix, knowledge of the

    Stokes vector of the incident beam is required. According

    to the definition, the Stokes vector is closely related to the

    22 polarization matrix[7]

    Wir; r; Einr;UEiTr;

    E

    in

    l r;Eil r; E

    in

    l r;Eir r;

    Ein

    r r;Eil r; E

    in

    r r;Eir r;

    0

    @

    1

    A:

    17

    From Eq.(17),we get the Stokes vector I ir; at point r

    Iir;

    Will r;Wirrr;

    Will r;Wirrr;

    Wirl r;Wirl r;

    iWirlr;W

    ilrr;

    0BBBBBB@

    1CCCCCCA

    : 18

    However, such a Stokes vector is spatially dependent

    and would make the Mueller matrix ill defined. One

    solution is to define the Stokes vector of the incident beam

    at the z0 plane and let the width of the beam go toinfinity. From Eq.(10), we immediately have the Gaussian

    Schell-model beam

    Wilm;; alamblm; 19

    which is a constant 22 matrix. Analogously, the angular

    correlation matrix in the same limit can written as

    ~Wi

    lmu

    ? ; u

    ? ; alamblmk

    2s

    2

    2

    exp 1

    2k

    2s

    2 u

    ? j2

    2u? u

    ? :

    20

    Thus, under this condition, we can generalize theMueller matrix to the case of incoherent beam scattering.

    2.3. Scattered light

    In the previous section, the incident field amplitude is

    defined with reference to the main scattering plane, which is

    defined with respect to the whole incoherent beam. How-

    ever, for each plane wave component of the incident beam,

    the scattering plane is different from the main scattering

    plane because the wave vector is different from that of theincident beam (the comparison with Mie scattering is

    illustrated in Figs. 1 and 2). Therefore, each plane wave

    component must experience a series of coordinate rotations

    in order to be placed in the fixed scattering plane.

    Due to the rotational symmetry of homogenous

    spheres and the incident beam about the z axis, the

    scattering direction can be chosen to be

    u sin ; 0; cos; 21

    which implies the main scattering plane coincides with

    the meridian plane that contains vector u (see Fig. 2).

    Now consider the plane wave component ei

    u? ;exp

    ikuUr, where the amplitude is defined with reference to

    the meridian plane ofu. First, we transform the reference

    plane to the meridian plane of u, which can be done

    X Y

    Z

    u u'

    r'

    l'

    r

    l

    Fig. 1. The geometry of Mie scattering, where uis the incident direction,

    u is the scattering direction, and is the scattering angle.

    XY

    Z

    u u'

    i2 i1

    l'r'

    lr

    Fig. 2. Scattering of one plane wave component of the partially coherent

    beam, where Z is the direction of whole incident beam,uis the incident

    direction,u is the scattering direction, and is the scattering angle. i1 is

    the angle between the meridian plane containing u and the scattering

    plane, and i2 is the angle between the meridian plane containing u andthe scattering plane.

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    through a rotation about the zaxis, i.e.

    eil

    eir

    0@

    1A-

    cos sin

    sin cos

    ! e

    il

    eir

    0@

    1A; 22

    or in a more compact form ei-Rei, where the fact is

    used that the unit vector u has a spherical coordinate

    ;

    . Second, we consider the scattering of a plane wave

    from direction uinto direction u. Since in the LorenzMie

    scattering the change of amplitude is defined with respect

    to the scattering plane, the incident field amplitude has to

    be transformed from the meridian plane to scattering

    plane by a counterclockwise rotation about vector uwith

    an angle i1 (see Fig. 2), which is the angle between the

    meridian plane of uand the scattering plane spanned by

    vectors uand u. Thus, the amplitude of the incident field

    can be written as

    Ri1Rei: 23

    By applying the results of the LorenzMie theory, we

    obtain the scattered field in the scattering plane ofuand u

    SRi1Rei; 24

    where is the angle between u and u, and S is the

    scattering amplitude matrix of LorenzMie scattering,

    which is given by[15]

    S S2 0

    0 S1

    !: 25

    Third, the scattered field has to be expressed with

    respect to the main scattering plane, and is obtained by a

    clockwise rotation about vector u with an angle i2,

    where i2 is the angle between the scattering plane

    spanned by vector u and u. The resulting scattered field

    reads

    R1

    i2SRi1Rei; 26

    which is equivalent to

    Ri2SRi1Rei; 27

    when using the relation R1

    i2 Ri2.

    Note that the above argument only works when o

    or u uU ^z40. When u uU ^zo0, the scattered field

    in the main scattering plane is given by

    R1

    i2SRi1Rei R i2SRi1Re

    i;

    28

    which is essentially the same as Eq. (27) except that the

    signs of sin i1 and sin i2 are reversed. Therefore, after

    obtaining cos i1 and cos i2 from spherical trigonometry,

    namely

    cos i1 cos cos cos

    sin sin ; 29

    cos i2 cos cos cos

    sin sin ; 30

    sin i1 and sin i2 are given by

    sin i1 ^

    u ^

    u

    U ^

    zju uU ^zjffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi ffiffiffiffi

    1 cos 2i1p

    ; 31

    sin i2 u uU ^z

    ju uU ^zj

    ffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi ffiffiffiffi1 cos 2i2

    p ; 32

    where cos uUu.

    We obtain the total scattered field referenced to the

    main scattering plane

    Esru; expikr

    ikrZ Au; uUeiu? ; d2u? ; 33

    where the 22 matrix Au; u is defined by

    Au; u Ri2SRi1R: 34

    2.4. Mueller matrix

    Once the scattered field is known, we can calculate the

    CSDM

    Wsr1 u1; r2 u2;

    exp ikr1r2

    k2

    r1r2

    Z d

    2u? d

    2u?

    An

    u1; uU ~W

    i

    u? ; u

    ? ;UATu2; u; 35

    with the definition of the angular correlation matrix of the

    incident field given by

    ~W

    i

    u? ; u

    ? ; einu? ;Ue

    iTu? ;: 36

    Taking the limit that the width of the Gaussian Schell-

    model beam goes to infinity, which implies that Eq. (20)

    holds, we obtain

    Wsr1 u1; r2 u2;

    exp ikr1r2

    k2

    r1r2

    k2s

    2

    2

    Z d

    2u?A

    n

    u1; uUWiz 0UA

    Tu2 u

    exp 12

    k2s

    2 u

    ? j2

    ; 37where W

    iz 0 is the CSDM of the incident beam

    defined at the z0 plane. From Eq. (37), we have the

    polarization matrix at point ru

    Wsru; ru;

    1

    k2

    r2

    k2s

    2

    2

    Z d

    2u?A

    n

    u; uU

    Wiz 0UA

    Tu; u exp

    1

    2k

    2s

    2ju

    ? j2

    : 38

    Using the relation between the Stokes vector and the

    polarization matrix(18), and the definition of the Mueller

    matrix

    Isu 1

    k2

    r2PuUIiz 0; 39

    we get the 44 Mueller matrix Pu, given by

    Pu k

    2s

    2

    2

    Z d

    2u? exp

    1

    2k

    2s

    2ju

    ? j2

    Mu; u: 40

    Here, the 44 matrix Mu; u is the Mueller matrix

    defined from the effective amplitude matrix Au; u. Some

    selected matrix elements ofMu; uare listed below

    M11 jA1j2jA2j

    2jA3j2jA4j

    2=2;

    M12 jA2j2jA2j

    2jA4j2jA3j

    2=2;

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    M22 jA1j2jA2j

    2jA3j2jA4j

    2=2;

    M33 ReA1An

    2A3An

    4;

    M43 ImA1An

    2A3An

    4;

    M44 ReA1An

    2A3An

    4; 41

    whereA1 A22, A2 A11,A3 A12, andA4 A21. Substitut-

    ing Eq.(34)into Eq.(41), we find the relation between the

    matrixMu; u and the Mueller matrix of a sphere in the

    fully coherent case P0

    M11 P011 ;

    M12 P011 cos 2i1;

    M22 P011 cos 2i2 cos 2i1P

    033 sin 2i2 sin 2i1;

    M33 P011 sin 2i2 sin 2i1 P

    033 cos 2i2 cos 2i1;

    M43 P043 cos 2i1;

    M44 P044 : 42

    Together with Eq. (40), we can calculate the Mueller

    matrix of a sphere when the incident light has an arbitrary

    degree of coherence.

    2.5. Spectral degree of coherence

    Once the CSDM is obtained, we can study the spectral

    degree of coherence of the scattered field. According to

    definition (4), the degree of coherence sr1 u1; r2 u2;

    between two directions in the far field zone can be written as

    sr1 u1; r2 u2; TrW

    sr1 u1; r2 u2;

    ffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi ffiffiffiffiSsr1 u1;q ffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiS

    sr2 u2;q

    : 43

    We consider a special case where the incident beam is

    completely unpolarized, i.e. the CSDM at z 0 has the

    value

    Wi

    lmz 0 Ilm: 44

    Therefore, the CSDM of the scattered field is given by

    Wsr1 u1; r2 u2; I

    expikr1r2

    k2

    r1r2

    k2s

    2

    2

    Z d

    2u?A

    n

    u1; uUATu2; u exp

    1

    2k

    2s

    2 ju

    ? j2

    ;

    45

    from which one can obtain the spectral density at point

    ru by

    Ssru; I 2

    k2r2

    k2s

    2

    2

    Z d

    2u? P

    011 uU uexp

    1

    2k

    2s

    2 ju

    ? j2

    :

    46

    P011 has the same meaning as in the previous section, and

    the numerical results of the spectral degree of coherence

    will be presented inSection 4.

    2.6. Water droplets and ice crystals

    We apply the developed formalism to randomlyoriented ice crystals. In general, the scattering amplitude

    matrix in Eq. (25)is no longer diagonal but is given by

    SS2 S3

    S4 S1

    !: 47

    Following the same procedure as inSection 2.4,one can

    derive similar results in Eqs. (40) and(42), with Eq. (42)

    modified to be

    M11 P011 ;

    M12 P011 cos 2i1P

    013 sin 2i1;

    M22 P022 cos 2i2P

    032 sin 2i2 cos 2i1

    P033 sin 2i2P

    023 cos 2i2 sin 2i1;

    M33 P022 sin 2i2P

    032 cos 2i2 sin 2i1

    P033 cos 2i2P023 sin 2i2 cos 2i1;

    M43 P043 cos 2i1P

    042 sin 2i1;

    M44 P044 : 48

    After orientation averaging,P0

    becomes block-diagonal,

    which means the Mueller matrix elements P013 , P

    023 , P

    032 ,

    andP042 in the previous equation vanish. Therefore, we get

    the same formalism as for the sphere, except that P0

    is the

    orientation averaged Mueller matrix in the fully coherent

    case.

    As an application, we studied the coherence effects on

    light scattering by spherical water droplets and hexagonal

    ice crystals. Here, the coherent Mueller matrix for an ice

    crystal was obtained by using the invariant imbedding

    T-matrix method[13]. The numerical results are presented

    inSection 4.

    3. DDA simulation

    We present a general numerical method to calculate

    the Mueller matrix of a particle of arbitrary shape and

    refractive index when the incident light is partially coher-

    ent. To link the numerical simulations to the analytical

    results in the previous section, we limit the incident beam

    to the Gaussian Schell-model beam with infinite width.

    Thus, the only free parameter of the incident beam is the

    coherence length. Moreover, the incident field can have an

    arbitrary polarization state because the Mueller matrix isindependent of the CSDM at the source plane (z0). In the

    simulation, we choose to linearly polarize the incident

    field. After simplification, the electric field is essentially

    reduced to a scalar random field, and the second-order

    correlation matrix is reduced to a scalar function. The first

    step of the problem is to generate a 2D source that satisfies

    the required correlation function, and once the source is

    known, the field at any point in space can be obtained by

    propagating the source using the Green's function [7].

    Several numerical methods are available, such as the

    random pulse method[16], random phase screens method

    [17], and shift-invariant filter method [18], but we use a

    more straightforward general method. As an example, letus consider the second-order correlation function on the

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    z0 plane

    1;2; Un2; tU1; t A1A221;

    49

    where A is the spatial profile, 21 is the spatial

    degree of coherence, and is the temporal degree of

    coherence. The goal is to express the random field U; t as

    a superposition of some random variables that havepredefined correlation functions, i.e.

    U; t Ak

    hkheikUe itIkxIkyI; 50

    where Ikx, Iky, and I are complex random numbers

    with correlation functions

    InkxInkyI

    nIkxIkyI kxkxkyky: 51

    From Eqs.(49) to(51), one can obtain

    1;2; A1A2k

    jhkj2eikU 2 1

    jhj2e i;

    52

    which implies that

    k

    jhkj2eikU 2 1 21; 53

    jhj2e : 54

    Thus, the coefficients hk and h in the random field

    U; t can be obtained by solving the two equations.

    For the monochromatic case, the correlation function is

    given by

    1;2 exp 12

    2

    2s2

    !12; 55

    and the random field is written as

    U k

    hkeikUIkxIky: 56

    The coefficient hk in Eq. (50)can be easily solved from

    Eq.(53). In the actual DDA simulation, the incident field

    Ei;z; can be obtained directly from the above results,

    i.e.

    Ei;z; jk? jrkhk? IkxIky

    exp i k? U

    ffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffik

    2jk? j

    2

    q z

    ei; 57

    whereei is a unit vector denoting the polarization of the

    incident field. For a specific realization of the random field,

    one can get the scattering amplitude matrix Su and

    corresponding Mueller matrix Mu in the direction u.

    After averaging over the ensemble of the incident fields,

    one can get the Mueller matrix for a sphere. Numeric

    results are discussed inSection 4.

    4. Results

    We applied the analytical formalism to calculate the

    Mueller matrix of a sphere when the incident light is

    partially coherent. The results are shown in Fig. 3. The

    sphere has a refractive index of n 1:5 and a radius ofa , where is the wavelength of the incident light. The

    coherence length shas values fromto 10. Note thatP11is essentially the intensity reported in [10,11]based on a

    scalar incident field and similar conclusions were reached.

    One of the most important conclusions is that the phase

    function tends to be more isotropic as the incident field

    becomes less coherent and gradually approaches the

    coherent case as the coherence length increases. Other

    Mueller matrix elements also become more isotropic ascoherence deteriorates. Moreover, the reduced Mueller

    matrix elements P22=P11, P33=P11, and P44=P11 in the

    backward direction are much more sensitive to the coher-

    ence length than those in the forward direction, and can

    be explained by the fact that interference in the forward

    direction is more robust to random phases than that in the

    backward direction.

    To validate the formalism we derived, we compared the

    analytical results with DDA simulations. The comparisons

    of Mueller matrix elements are shown inFig. 4. The sphere

    has the same parameters as before and two cases, s

    and 4, are computed. In the DDA simulations, 160 plane

    waves components are used to construct the incident field,a total of 1000 ensemble averages are taken, and the inter-

    dipole spacing used isd =20. The results show that DDA

    simulations agree very well with the analytical formalism.

    We investigated the Mueller matrix elements in

    the backward direction (1801 degree scattering). The

    sphere has the same parameters as before, and the

    coherence length is chosen from 0 to 10. As can be seen

    from Fig. 5, for Mueller matrix elements P12=P11 and

    P43=P11, no significant dependence on coherence length

    is observed. In comparison, other Mueller matrix elements

    all change monotonically and gradually plateau as the

    coherence length increases. Evidently, all approach coher-

    ent values when the coherence length reaches a largeenough value.

    In addition, we computed the spectral degree of coher-

    ence of the scattered field. The results are shown in Fig. 6,

    where the sphere has the same parameters as previously

    and the coherence length is chosen fromto 10. Here, the

    spectral degree of coherence is defined as the correlation

    between two directions, the zand the polar angle . We

    find that at any angle, the norm of the degree of coherence

    always decreases as the incident light becomes less coher-

    ent. Note that jj is not always unity even when the

    coherence length approaches infinity due to the comple-

    tely unpolarized special form of the incident beam. A

    simple calculation gives the degree of coherence whenthe coherence length is infinitely large

    1; 2 jSn21S22Sn11S12jffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi ffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi

    jS11j2jS21j

    2q ffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi

    jS12j2jS22j

    2q ;

    58

    whereS1 and S2 are defined in Eq. (25). It can be shown

    that Eq.(58) is not always equal to unity.

    As applications of the formalism developed, we com-

    puted the Mueller matrix elements for water droplets and

    hexagonal ice crystals that are the constituents for atmo-

    spheric clouds. The results for a water droplet are shown in

    Fig. 7. The water droplet has a size parameter x 80 and arefractive index n 1:33. The coherence length parameter

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    kshas values from 5 to 100. Apart from similar conclusions

    to the case of a small sphere, we found that both the coronaand glory phenomena will be eliminated as the incident

    field becomes incoherent. Since both are consequences of

    interference, which can be extinguished by the introductionof incoherence, the elimination is reasonable. The results for

    Fig. 3. Mueller matrix elements for a sphere of radius a and refractive index n1.5. The coherence length s has values of, 4, and 10.

    Fig. 4. Comparison of Mueller matrix elements computed from DDA and Mie methods. Two cases, s and 4are simulated. The remaining parameters

    are the same asFig. 3.

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    the hexagonal ice crystal are shown inFig. 8. The ice crystal

    has a size parameter kL 2ka 150, whereL is the height

    andais the semi-width, and a refractive indexn 1:31. The

    coherence length parameter ks has the values 5, 10, and

    100. The results show that both the 221 and 461 halos

    gradually disappear as the coherence length decreases,

    which can be explained by the same reasoning as used for

    the corona and glory for water droplets. The Mueller matrix

    elements for the water droplet and ice crystal in the

    backward direction are shown in Figs. 9 and 10, respec-tively. We found similar results to those of small spheres.

    5. Conclusions and discussions

    The conventional LorenzMie formalism is generalized

    to the case when the incident light is partially coherent.For the Gaussian Schell-model beams, the Mueller matrix

    and spectral degree of coherence for the scattered field is

    derived analytically and the formalism is validated by DDA

    simulation. The results suggest that the reduced Mueller

    matrix elements P22=P11, P33=P11, and P44=P11 in the

    backward direction strongly depend on the degree of

    coherence of the incident light. The same formalism is

    applied to randomly orientated water droplets and hex-

    agonal ice crystals. We find that the corona and glory

    phenomena associated with water droplets and halos with

    hexagonal ice crystals disappear if the incident light is

    highly incoherent.

    The relevance of these results to atmospheric radiationis three-fold. First, despite the fact that the solar source is

    completely incoherent, which is presumably thermal

    emission, the sunlight reaching the surface of the earth

    acquires a certain degree of correlation through the

    process of propagation. This is a straightforward result of

    the van CittertZernike theorem, and a rough estimation

    reveals that the sunlight has a spatial coherence length of

    about 60mm [7]. Given the size of large atmospheric

    particles, the finite coherence length of sunlight will have

    observable effects on the pattern of the scattered field.

    Second, when using a laser beam instead of natural solar

    light in remote sensing, the light beam becomes partially

    coherent when passing through atmospheric turbulence.Therefore, it is of practical interest to investigate the effect

    Fig. 5. Mueller matrix elements for a sphere in the backward direction (1801). The coherence length s is from 0 to 10. The remaining parameters are the

    same asFig. 3.

    0 45 90 135 180

    0

    0.1

    0.2

    0.3

    0.4

    0.5

    0.6

    0.7

    0.8

    0.9

    1

    Fig. 6. The spectral degree coherence of the scattered field from a sphere.

    is the angle between scattering direction and the z direction. Five

    cases, including the coherent case are simulated. The parameters are the

    same asFig. 3.

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    of spatial coherence in light scattering. Third, even though

    there is not a variant of the radiative transfer equation inwhich the scattering matrix derived in this paper can be

    inserted, the results obtained here shed light on what

    results can be expected in a multiple scattering situation.As it is shown here, all Muller matrix elements become

    Fig. 7. Mueller matrix elements for a water droplet of size parameter x80 and refractive indexn 1:33. The coherence length parameter ks has values of

    5, 10 and 100.

    Fig. 8. Mueller matrix elements for a hexagonal ice crystal with size parameterkL2ka150, whereLis the height andais the semi-width, and refractive

    indexn 1:31. The coherence length parameter ks has values of 5, 10 and 100.

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    Thus our results provide a potential method to deter-

    mine coherence length and for possible applications in

    atmospheric remote sensing.

    Acknowledgments

    George Kattawar acknowledges support by the National

    Science Foundation (OCE-1130906). Ping Yang acknowl-

    edges support by NASA (NNX11AK37G).

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