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Scattering of partially coherent electromagnetic beams
by water droplets and ice crystals
Jianping Liu a,n, Lei Bi b, Ping Yang b, George W. Kattawar a
a Department of Physics and Astronomy, Texas A&M University, College Station, TX 77843, USAb Department of Atmospheric Sciences, Texas A&M University, College Station, TX 77843, USA
a r t i c l e i n f o
Article history:
Received 31 August 2013
Received in revised form
6 November 2013
Accepted 8 November 2013Available online 16 November 2013
Keywords:
Partially coherent light
LorenzMie
Mueller matrix
Water droplet
Ice crystal
a b s t r a c t
The conventional LorenzMie theory is generalized for a case when the light source is
partially spatially coherent. The influence of the degree of coherence of the incident field
on the generalized Mueller matrix and the spectral degree of coherence of the scattered
light is analytically studied by using the vector field instead of the scalar field to extend
previous results on the angular intensity distribution. The results are compared with the
Mueller matrix obtained from the Discrete Dipole Approximation (DDA) method, which is
an average over an ensemble of stochastic incident beams. Special attention is paid to the
Mueller matrix elements in the backward direction, and the results show some Mueller
matrix elements, such as P22, depend monotonically on the coherence length of the
incident beam. Therefore, detecting back scattering Mueller matrix elements may be a
promising method to measure the degree of coherence. The new formalism is applied to
cases of large spherical droplets in water clouds and hexagonal ice crystals in cirrus
clouds. The corona and glory phenomena due to spheres and halos associated with
hexagonal ice crystals are found to disappear if the incident light tends to be highly
incoherent.
& 2013 Elsevier Ltd. All rights reserved.
1. Introduction
In the conventional theories of light scattering, such as
LorenzMie theory[1], Discrete Dipole Approximation (DDA)
[2,3], and Finite-Difference Time-Domain (FDTD) method[4],
the incident light is generally assumed to be fully coherent in
both space and time. However, the assumption is not always
justified. In reality, light acquires some degree of incoherence
due to light source fluctuations or to interactions with randommedia such as a turbulent atmosphere. Although the general
framework of optical coherence theory has long been well
established[57], scarcely any attention has been paid to the
effect of coherence on light scattering by deterministic media.
The influence of spatial coherence on scattering by a particle
was partially investigated by Cabaret et al. [8]and Greffet[9].
The extinction cross section of rotationally invariant scatterers
was found not to depend on the transverse (or spatial)
coherence length, but the extinction cross section of aniso-
tropic scatterers did depend on the state of coherence of the
illuminating field. Further research on the topic was con-
ducted by van Dijk [10] and Fischer [11] who studied the
effects of spatial coherence on the angular distribution of
radiant intensity scattered by a sphere. By using the angular
spectrum representation of a random field[6]and half wave
expansion of the scattering amplitude, the intensity of ascattered field was analytically obtained. The angular distribu-
tion of radiant intensity depends strongly on the degree of
coherence, but the extinguished power does not. Sukhov [12]
numerically studied the effect of spatial coherence by a
random medium on the properties of scattered fields, and
the DDA method was used to demonstrate that the statistical
properties of the scattered light from an inhomogeneous
medium were altered due to coherence effects.
Previous theories have been limited to the study of the
scattered field intensity, which does not fully describe
a scatterer with respect to light scattering. A common
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n Corresponding author. Tel.: 1 979 587 9918.
E-mail address: [email protected] (J. Liu).
Journal of Quantitative Spectroscopy& Radiative Transfer 134 (2014) 7484
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generalization is to study the Mueller matrix, which relates
the Stokes vector of the incident beam to the Stokes vector of
the scattered beam. For a large class of light beams such as
the so-called Gaussian Schell-model beam, the Mueller
matrix for a sphere is derived analytically by extending the
LorenzMie theory. We developed a DDA code [3] by
modifying the source field to incorporate incoherence, and
the Mueller matrix was obtained by averaging over anensemble of stochastic incident fields. In addition, we
investigated the spectral degree of coherence of the scat-
tered light. As applications of the formalism developed, we
performed the computation of light scattering by water
droplets and hexagonal ice crystals, which are the major
scatterers inside atmospheric clouds. The coherence effects
of spherical water droplets were studied by modifying the
LorenzMie theory. With the Invariant Imbedding T-matrix
method (see[13]and references cited therein), we were able
to study the coherence effects on halos of large hexagonal ice
crystals.
2. Scattering of partially coherent light by a sphere
We consider the scattering of electromagnetic beams of
an arbitrary state of spatial coherence by a homogenous
sphere on the basis of a generalization of previous results
in[10,11]. Note that the procedure is quite similar to that
used by Lahiri and Wolf [14], where the refraction and
reflection of partially coherent electromagnetic beams
were considered.
2.1. Theory of coherence
We use some of the important results from the coher-
ence theory of electromagnetic beams [7]. The stochasticnature of incoherent monochromatic light is represented
by an ensemble of random fields fEr;g, where is the
frequency, and for each realization, the field component is
transverse to the direction of propagation. By choosing the
same plane of reference as in the previous section, each
random field can be expressed as
Er; Elr;
Err;
!: 1
Following the same formalism used by Wolf [7], the
second-order correlation properties of the stochastic field
are fully characterized by the 22 cross-spectral density
matrix (CSDM) defined by
Wr1; r2; Enr1;UE
Tr2;
Enl r1;Elr2; E
n
l r1;Err2;
Enrr1;Elr2; En
rr1;Err2;
!;
2
where denotes the ensemble average. From the CSDM,
the spectral density can be derived at point r and at
frequency
Sr; TrWr; r;; 3
which can be interpreted as a contribution to the intensity
at point r from the field component of frequency .The spatial degree of coherence of the random field is
defined by[7]
r1; r2; TrWr1; r2;ffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi
Sr1;p ffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi
Sr2;p ; 4
which unifies both polarization and coherence. 0r j
r1; r2;jr1 with 0 representing complete incoherence
and 1 representing complete coherence.
2.2. Incident light
Incoherent beams can be represented by an ensemble
of random fields and are realized using the angular
spectrum representation [6]. A partially coherent beam
propagating in the zdirection can be expressed as
Eir;
Zju
?jo1
eiu? ;expikuUr d2
u? ; 5
where the coefficient eiu? ; is a two-component ran-
dom vector defined by
eiu? ; eil u
? ;
eir u
? ;
0@ 1A; 6k =cis the wavenumber, u is the direction of propaga-
tion of each plane wave component, u? ux; uy is the
projection ofuonto thez0 plane, and the unit vector u
points into the z40 half space, i.e. uzffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi
1ju? j2
q . The
scattering plane is chosen as the reference plane.
The incident field is uniquely defined by the source at
thez0 plane, which is characterized by the CSDM
Wi1;2; E
in1;UEiT2;; 7
where 1 and 2 are 2D vectors in the z0 plane. UsingEq.(5), we have
Wi1;2;
Z d
2u? d
2u?
~W
iu? ; u
? ;expiku
? U1u
? U2;
8
where the angular correlation matrix ~W
i
u? ; u
? ;
einu? UeiTu? is defined as a four-dimensional
Fourier transformation of the CSDM at thez0 plane, i.e.
~W
i
u?
; u?
;
k
2
4 Z d
21d
22W
i
1;2;expiku
? U1u
? U2:
9
We consider a widely used class of partially coherent
beams, the so-called Gaussian Schell-model beams, which
have the following CSDM elements
Wilm1;2; alamblmexp
2122
4s2S
!exp
122
2s2
!:
10
The independently chosen parameter sS can be inter-
preted as the width of the beam, and s as the coherencelength. The remaining parameters in Eq. (10) have the
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following constraints[7]
bij 1 when i j; 11
bij r1 when iaj; 12bij b
n
ji; 13
ai Z0: 14
By substituting Eq.(10)into Eq.(9)and performing the
four dimensional integration, one can obtain the angular
correlation matrix[10]
~Wi
lmu
? ; u
? ; alamblmk
2ssef f
2
!2
exp k
2
2 u? u
? 2s
2Su
? u
? 2s
2ef f
4
" #( ); 15
where
1
s2ef f
1
s2
1
4s2S: 16
In order to obtain the Mueller matrix, knowledge of the
Stokes vector of the incident beam is required. According
to the definition, the Stokes vector is closely related to the
22 polarization matrix[7]
Wir; r; Einr;UEiTr;
E
in
l r;Eil r; E
in
l r;Eir r;
Ein
r r;Eil r; E
in
r r;Eir r;
0
@
1
A:
17
From Eq.(17),we get the Stokes vector I ir; at point r
Iir;
Will r;Wirrr;
Will r;Wirrr;
Wirl r;Wirl r;
iWirlr;W
ilrr;
0BBBBBB@
1CCCCCCA
: 18
However, such a Stokes vector is spatially dependent
and would make the Mueller matrix ill defined. One
solution is to define the Stokes vector of the incident beam
at the z0 plane and let the width of the beam go toinfinity. From Eq.(10), we immediately have the Gaussian
Schell-model beam
Wilm;; alamblm; 19
which is a constant 22 matrix. Analogously, the angular
correlation matrix in the same limit can written as
~Wi
lmu
? ; u
? ; alamblmk
2s
2
2
exp 1
2k
2s
2 u
? j2
2u? u
? :
20
Thus, under this condition, we can generalize theMueller matrix to the case of incoherent beam scattering.
2.3. Scattered light
In the previous section, the incident field amplitude is
defined with reference to the main scattering plane, which is
defined with respect to the whole incoherent beam. How-
ever, for each plane wave component of the incident beam,
the scattering plane is different from the main scattering
plane because the wave vector is different from that of theincident beam (the comparison with Mie scattering is
illustrated in Figs. 1 and 2). Therefore, each plane wave
component must experience a series of coordinate rotations
in order to be placed in the fixed scattering plane.
Due to the rotational symmetry of homogenous
spheres and the incident beam about the z axis, the
scattering direction can be chosen to be
u sin ; 0; cos; 21
which implies the main scattering plane coincides with
the meridian plane that contains vector u (see Fig. 2).
Now consider the plane wave component ei
u? ;exp
ikuUr, where the amplitude is defined with reference to
the meridian plane ofu. First, we transform the reference
plane to the meridian plane of u, which can be done
X Y
Z
u u'
r'
l'
r
l
Fig. 1. The geometry of Mie scattering, where uis the incident direction,
u is the scattering direction, and is the scattering angle.
XY
Z
u u'
i2 i1
l'r'
lr
Fig. 2. Scattering of one plane wave component of the partially coherent
beam, where Z is the direction of whole incident beam,uis the incident
direction,u is the scattering direction, and is the scattering angle. i1 is
the angle between the meridian plane containing u and the scattering
plane, and i2 is the angle between the meridian plane containing u andthe scattering plane.
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through a rotation about the zaxis, i.e.
eil
eir
0@
1A-
cos sin
sin cos
! e
il
eir
0@
1A; 22
or in a more compact form ei-Rei, where the fact is
used that the unit vector u has a spherical coordinate
;
. Second, we consider the scattering of a plane wave
from direction uinto direction u. Since in the LorenzMie
scattering the change of amplitude is defined with respect
to the scattering plane, the incident field amplitude has to
be transformed from the meridian plane to scattering
plane by a counterclockwise rotation about vector uwith
an angle i1 (see Fig. 2), which is the angle between the
meridian plane of uand the scattering plane spanned by
vectors uand u. Thus, the amplitude of the incident field
can be written as
Ri1Rei: 23
By applying the results of the LorenzMie theory, we
obtain the scattered field in the scattering plane ofuand u
SRi1Rei; 24
where is the angle between u and u, and S is the
scattering amplitude matrix of LorenzMie scattering,
which is given by[15]
S S2 0
0 S1
!: 25
Third, the scattered field has to be expressed with
respect to the main scattering plane, and is obtained by a
clockwise rotation about vector u with an angle i2,
where i2 is the angle between the scattering plane
spanned by vector u and u. The resulting scattered field
reads
R1
i2SRi1Rei; 26
which is equivalent to
Ri2SRi1Rei; 27
when using the relation R1
i2 Ri2.
Note that the above argument only works when o
or u uU ^z40. When u uU ^zo0, the scattered field
in the main scattering plane is given by
R1
i2SRi1Rei R i2SRi1Re
i;
28
which is essentially the same as Eq. (27) except that the
signs of sin i1 and sin i2 are reversed. Therefore, after
obtaining cos i1 and cos i2 from spherical trigonometry,
namely
cos i1 cos cos cos
sin sin ; 29
cos i2 cos cos cos
sin sin ; 30
sin i1 and sin i2 are given by
sin i1 ^
u ^
u
U ^
zju uU ^zjffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi ffiffiffiffi
1 cos 2i1p
; 31
sin i2 u uU ^z
ju uU ^zj
ffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi ffiffiffiffi1 cos 2i2
p ; 32
where cos uUu.
We obtain the total scattered field referenced to the
main scattering plane
Esru; expikr
ikrZ Au; uUeiu? ; d2u? ; 33
where the 22 matrix Au; u is defined by
Au; u Ri2SRi1R: 34
2.4. Mueller matrix
Once the scattered field is known, we can calculate the
CSDM
Wsr1 u1; r2 u2;
exp ikr1r2
k2
r1r2
Z d
2u? d
2u?
An
u1; uU ~W
i
u? ; u
? ;UATu2; u; 35
with the definition of the angular correlation matrix of the
incident field given by
~W
i
u? ; u
? ; einu? ;Ue
iTu? ;: 36
Taking the limit that the width of the Gaussian Schell-
model beam goes to infinity, which implies that Eq. (20)
holds, we obtain
Wsr1 u1; r2 u2;
exp ikr1r2
k2
r1r2
k2s
2
2
Z d
2u?A
n
u1; uUWiz 0UA
Tu2 u
exp 12
k2s
2 u
? j2
; 37where W
iz 0 is the CSDM of the incident beam
defined at the z0 plane. From Eq. (37), we have the
polarization matrix at point ru
Wsru; ru;
1
k2
r2
k2s
2
2
Z d
2u?A
n
u; uU
Wiz 0UA
Tu; u exp
1
2k
2s
2ju
? j2
: 38
Using the relation between the Stokes vector and the
polarization matrix(18), and the definition of the Mueller
matrix
Isu 1
k2
r2PuUIiz 0; 39
we get the 44 Mueller matrix Pu, given by
Pu k
2s
2
2
Z d
2u? exp
1
2k
2s
2ju
? j2
Mu; u: 40
Here, the 44 matrix Mu; u is the Mueller matrix
defined from the effective amplitude matrix Au; u. Some
selected matrix elements ofMu; uare listed below
M11 jA1j2jA2j
2jA3j2jA4j
2=2;
M12 jA2j2jA2j
2jA4j2jA3j
2=2;
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M22 jA1j2jA2j
2jA3j2jA4j
2=2;
M33 ReA1An
2A3An
4;
M43 ImA1An
2A3An
4;
M44 ReA1An
2A3An
4; 41
whereA1 A22, A2 A11,A3 A12, andA4 A21. Substitut-
ing Eq.(34)into Eq.(41), we find the relation between the
matrixMu; u and the Mueller matrix of a sphere in the
fully coherent case P0
M11 P011 ;
M12 P011 cos 2i1;
M22 P011 cos 2i2 cos 2i1P
033 sin 2i2 sin 2i1;
M33 P011 sin 2i2 sin 2i1 P
033 cos 2i2 cos 2i1;
M43 P043 cos 2i1;
M44 P044 : 42
Together with Eq. (40), we can calculate the Mueller
matrix of a sphere when the incident light has an arbitrary
degree of coherence.
2.5. Spectral degree of coherence
Once the CSDM is obtained, we can study the spectral
degree of coherence of the scattered field. According to
definition (4), the degree of coherence sr1 u1; r2 u2;
between two directions in the far field zone can be written as
sr1 u1; r2 u2; TrW
sr1 u1; r2 u2;
ffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi ffiffiffiffiSsr1 u1;q ffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiS
sr2 u2;q
: 43
We consider a special case where the incident beam is
completely unpolarized, i.e. the CSDM at z 0 has the
value
Wi
lmz 0 Ilm: 44
Therefore, the CSDM of the scattered field is given by
Wsr1 u1; r2 u2; I
expikr1r2
k2
r1r2
k2s
2
2
Z d
2u?A
n
u1; uUATu2; u exp
1
2k
2s
2 ju
? j2
;
45
from which one can obtain the spectral density at point
ru by
Ssru; I 2
k2r2
k2s
2
2
Z d
2u? P
011 uU uexp
1
2k
2s
2 ju
? j2
:
46
P011 has the same meaning as in the previous section, and
the numerical results of the spectral degree of coherence
will be presented inSection 4.
2.6. Water droplets and ice crystals
We apply the developed formalism to randomlyoriented ice crystals. In general, the scattering amplitude
matrix in Eq. (25)is no longer diagonal but is given by
SS2 S3
S4 S1
!: 47
Following the same procedure as inSection 2.4,one can
derive similar results in Eqs. (40) and(42), with Eq. (42)
modified to be
M11 P011 ;
M12 P011 cos 2i1P
013 sin 2i1;
M22 P022 cos 2i2P
032 sin 2i2 cos 2i1
P033 sin 2i2P
023 cos 2i2 sin 2i1;
M33 P022 sin 2i2P
032 cos 2i2 sin 2i1
P033 cos 2i2P023 sin 2i2 cos 2i1;
M43 P043 cos 2i1P
042 sin 2i1;
M44 P044 : 48
After orientation averaging,P0
becomes block-diagonal,
which means the Mueller matrix elements P013 , P
023 , P
032 ,
andP042 in the previous equation vanish. Therefore, we get
the same formalism as for the sphere, except that P0
is the
orientation averaged Mueller matrix in the fully coherent
case.
As an application, we studied the coherence effects on
light scattering by spherical water droplets and hexagonal
ice crystals. Here, the coherent Mueller matrix for an ice
crystal was obtained by using the invariant imbedding
T-matrix method[13]. The numerical results are presented
inSection 4.
3. DDA simulation
We present a general numerical method to calculate
the Mueller matrix of a particle of arbitrary shape and
refractive index when the incident light is partially coher-
ent. To link the numerical simulations to the analytical
results in the previous section, we limit the incident beam
to the Gaussian Schell-model beam with infinite width.
Thus, the only free parameter of the incident beam is the
coherence length. Moreover, the incident field can have an
arbitrary polarization state because the Mueller matrix isindependent of the CSDM at the source plane (z0). In the
simulation, we choose to linearly polarize the incident
field. After simplification, the electric field is essentially
reduced to a scalar random field, and the second-order
correlation matrix is reduced to a scalar function. The first
step of the problem is to generate a 2D source that satisfies
the required correlation function, and once the source is
known, the field at any point in space can be obtained by
propagating the source using the Green's function [7].
Several numerical methods are available, such as the
random pulse method[16], random phase screens method
[17], and shift-invariant filter method [18], but we use a
more straightforward general method. As an example, letus consider the second-order correlation function on the
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z0 plane
1;2; Un2; tU1; t A1A221;
49
where A is the spatial profile, 21 is the spatial
degree of coherence, and is the temporal degree of
coherence. The goal is to express the random field U; t as
a superposition of some random variables that havepredefined correlation functions, i.e.
U; t Ak
hkheikUe itIkxIkyI; 50
where Ikx, Iky, and I are complex random numbers
with correlation functions
InkxInkyI
nIkxIkyI kxkxkyky: 51
From Eqs.(49) to(51), one can obtain
1;2; A1A2k
jhkj2eikU 2 1
jhj2e i;
52
which implies that
k
jhkj2eikU 2 1 21; 53
jhj2e : 54
Thus, the coefficients hk and h in the random field
U; t can be obtained by solving the two equations.
For the monochromatic case, the correlation function is
given by
1;2 exp 12
2
2s2
!12; 55
and the random field is written as
U k
hkeikUIkxIky: 56
The coefficient hk in Eq. (50)can be easily solved from
Eq.(53). In the actual DDA simulation, the incident field
Ei;z; can be obtained directly from the above results,
i.e.
Ei;z; jk? jrkhk? IkxIky
exp i k? U
ffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffik
2jk? j
2
q z
ei; 57
whereei is a unit vector denoting the polarization of the
incident field. For a specific realization of the random field,
one can get the scattering amplitude matrix Su and
corresponding Mueller matrix Mu in the direction u.
After averaging over the ensemble of the incident fields,
one can get the Mueller matrix for a sphere. Numeric
results are discussed inSection 4.
4. Results
We applied the analytical formalism to calculate the
Mueller matrix of a sphere when the incident light is
partially coherent. The results are shown in Fig. 3. The
sphere has a refractive index of n 1:5 and a radius ofa , where is the wavelength of the incident light. The
coherence length shas values fromto 10. Note thatP11is essentially the intensity reported in [10,11]based on a
scalar incident field and similar conclusions were reached.
One of the most important conclusions is that the phase
function tends to be more isotropic as the incident field
becomes less coherent and gradually approaches the
coherent case as the coherence length increases. Other
Mueller matrix elements also become more isotropic ascoherence deteriorates. Moreover, the reduced Mueller
matrix elements P22=P11, P33=P11, and P44=P11 in the
backward direction are much more sensitive to the coher-
ence length than those in the forward direction, and can
be explained by the fact that interference in the forward
direction is more robust to random phases than that in the
backward direction.
To validate the formalism we derived, we compared the
analytical results with DDA simulations. The comparisons
of Mueller matrix elements are shown inFig. 4. The sphere
has the same parameters as before and two cases, s
and 4, are computed. In the DDA simulations, 160 plane
waves components are used to construct the incident field,a total of 1000 ensemble averages are taken, and the inter-
dipole spacing used isd =20. The results show that DDA
simulations agree very well with the analytical formalism.
We investigated the Mueller matrix elements in
the backward direction (1801 degree scattering). The
sphere has the same parameters as before, and the
coherence length is chosen from 0 to 10. As can be seen
from Fig. 5, for Mueller matrix elements P12=P11 and
P43=P11, no significant dependence on coherence length
is observed. In comparison, other Mueller matrix elements
all change monotonically and gradually plateau as the
coherence length increases. Evidently, all approach coher-
ent values when the coherence length reaches a largeenough value.
In addition, we computed the spectral degree of coher-
ence of the scattered field. The results are shown in Fig. 6,
where the sphere has the same parameters as previously
and the coherence length is chosen fromto 10. Here, the
spectral degree of coherence is defined as the correlation
between two directions, the zand the polar angle . We
find that at any angle, the norm of the degree of coherence
always decreases as the incident light becomes less coher-
ent. Note that jj is not always unity even when the
coherence length approaches infinity due to the comple-
tely unpolarized special form of the incident beam. A
simple calculation gives the degree of coherence whenthe coherence length is infinitely large
1; 2 jSn21S22Sn11S12jffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi ffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi
jS11j2jS21j
2q ffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi
jS12j2jS22j
2q ;
58
whereS1 and S2 are defined in Eq. (25). It can be shown
that Eq.(58) is not always equal to unity.
As applications of the formalism developed, we com-
puted the Mueller matrix elements for water droplets and
hexagonal ice crystals that are the constituents for atmo-
spheric clouds. The results for a water droplet are shown in
Fig. 7. The water droplet has a size parameter x 80 and arefractive index n 1:33. The coherence length parameter
J. Liu et al. / Journal of Quantitative Spectroscopy & Radiative Transfer 134 (2014) 7484 79
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kshas values from 5 to 100. Apart from similar conclusions
to the case of a small sphere, we found that both the coronaand glory phenomena will be eliminated as the incident
field becomes incoherent. Since both are consequences of
interference, which can be extinguished by the introductionof incoherence, the elimination is reasonable. The results for
Fig. 3. Mueller matrix elements for a sphere of radius a and refractive index n1.5. The coherence length s has values of, 4, and 10.
Fig. 4. Comparison of Mueller matrix elements computed from DDA and Mie methods. Two cases, s and 4are simulated. The remaining parameters
are the same asFig. 3.
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the hexagonal ice crystal are shown inFig. 8. The ice crystal
has a size parameter kL 2ka 150, whereL is the height
andais the semi-width, and a refractive indexn 1:31. The
coherence length parameter ks has the values 5, 10, and
100. The results show that both the 221 and 461 halos
gradually disappear as the coherence length decreases,
which can be explained by the same reasoning as used for
the corona and glory for water droplets. The Mueller matrix
elements for the water droplet and ice crystal in the
backward direction are shown in Figs. 9 and 10, respec-tively. We found similar results to those of small spheres.
5. Conclusions and discussions
The conventional LorenzMie formalism is generalized
to the case when the incident light is partially coherent.For the Gaussian Schell-model beams, the Mueller matrix
and spectral degree of coherence for the scattered field is
derived analytically and the formalism is validated by DDA
simulation. The results suggest that the reduced Mueller
matrix elements P22=P11, P33=P11, and P44=P11 in the
backward direction strongly depend on the degree of
coherence of the incident light. The same formalism is
applied to randomly orientated water droplets and hex-
agonal ice crystals. We find that the corona and glory
phenomena associated with water droplets and halos with
hexagonal ice crystals disappear if the incident light is
highly incoherent.
The relevance of these results to atmospheric radiationis three-fold. First, despite the fact that the solar source is
completely incoherent, which is presumably thermal
emission, the sunlight reaching the surface of the earth
acquires a certain degree of correlation through the
process of propagation. This is a straightforward result of
the van CittertZernike theorem, and a rough estimation
reveals that the sunlight has a spatial coherence length of
about 60mm [7]. Given the size of large atmospheric
particles, the finite coherence length of sunlight will have
observable effects on the pattern of the scattered field.
Second, when using a laser beam instead of natural solar
light in remote sensing, the light beam becomes partially
coherent when passing through atmospheric turbulence.Therefore, it is of practical interest to investigate the effect
Fig. 5. Mueller matrix elements for a sphere in the backward direction (1801). The coherence length s is from 0 to 10. The remaining parameters are the
same asFig. 3.
0 45 90 135 180
0
0.1
0.2
0.3
0.4
0.5
0.6
0.7
0.8
0.9
1
Fig. 6. The spectral degree coherence of the scattered field from a sphere.
is the angle between scattering direction and the z direction. Five
cases, including the coherent case are simulated. The parameters are the
same asFig. 3.
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of spatial coherence in light scattering. Third, even though
there is not a variant of the radiative transfer equation inwhich the scattering matrix derived in this paper can be
inserted, the results obtained here shed light on what
results can be expected in a multiple scattering situation.As it is shown here, all Muller matrix elements become
Fig. 7. Mueller matrix elements for a water droplet of size parameter x80 and refractive indexn 1:33. The coherence length parameter ks has values of
5, 10 and 100.
Fig. 8. Mueller matrix elements for a hexagonal ice crystal with size parameterkL2ka150, whereLis the height andais the semi-width, and refractive
indexn 1:31. The coherence length parameter ks has values of 5, 10 and 100.
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Thus our results provide a potential method to deter-
mine coherence length and for possible applications in
atmospheric remote sensing.
Acknowledgments
George Kattawar acknowledges support by the National
Science Foundation (OCE-1130906). Ping Yang acknowl-
edges support by NASA (NNX11AK37G).
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