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    Characterization of PF flames under different swirl conditions basedon visualization systems

    A. González-Cencerrado ⇑, A. Gil, B. Peña

    Centre of Research for Energy Resources and Consumption (CIRCE), C/Mariano Esquillor Gómez, 15, 50018 Zaragoza, Spain

    h i g h l i g h t s

     Influence of swirl number on different combustion flames has been studied in detail. Flame luminous information is captured by means of a CCD based visualization system.

      Relevant variations concerning dynamical and physical flame features are presented.

      Spatial–temporal characterization of flames highlights the effect of swirl increase.

      A new approach to frequency analysis of semi-industrial PF flames is performed.

    a r t i c l e i n f o

     Article history:

    Received 30 September 2012

    Received in revised form 5 December 2012

    Accepted 23 May 2013

    Available online 11 June 2013

    Keywords:

    SwirlImage processing

    CCD camera

    Pulverized coal

    Gas flame

    a b s t r a c t

    The complex phenomena underlying reacting flows are at present an active research topic for improving

    efficiency and control of industrial combustion processes. The present study assesses the use of a reliable

    and low cost visualization system based on CCD (charged couple device) technology for the identification

    of different flame states as a function of swirl number. The experiments were performed in a 500 kWthpulverized coal (PF) swirl burner. The visualization system was previously used for similar analysis of 

    an atmospheric gas swirl burner of 50 kWth. Both flames were analyzed under low and high swirl condi-

    tions in order to identify possible common features concerning swirl flames. The analysis procedure pro-

    posed in this work extracts different statistical and spectral parameters from the intensity of radiation

    stored by each CCD element. The representation of flame features as two-dimensional distributions

    has led to the identification of typical structures in swirl flows and has allowed us to detect changes

    in flame structure as swirl number increases. Besides, the quantification of aforementioned parameters

    has led to relevant findings concerning frequency analysis and flame stability as a function of swirl. Spe-

    cifically, results show that the characteristic frequency in terms of flame flicker is sensible to changes in

    swirl conditions.

      2013 Elsevier Ltd. All rights reserved.

    1. Introduction

    Pulverized fuel (PF) flames from swirl burners involve many

    influential variables and exhibit large spatial and temporal varia-tions in flow dynamics and heat release. In spite of the vast amount

    of related literature, the complexity of reacting flows under PF

    flames demands a deeper understanding based on reliable experi-

    mental data at industrial scale. Among the potential techniques

    currently under research, flame visualization-based systems pro-

    vide a non-intrusive alternative for the analysis of flame structure.

    In this context, advanced technologies such as Particle Image

    Velocimetry (PIV) or Laser Doppler Anemometry (LDA) have been

    widely used in recent years   [1–4]. These laser-based diagnostic

    methods provide very accurate information from the flame in

    terms of its internal structure, flow oscillations or associated insta-

    bilities. Nevertheless, their applicability is mainly restricted to very

    particular environments: free of soot, with no presence of multi-component fuels or multiple phases and under atmospheric pres-

    sure  [5]. In addition to this, large physical scales and the conse-

    quent reduced optical access to the flame, make very difficult

    their practical implementation on industrial combustion systems.

    There are numerous experimental analyses of gaseous swirl

    flames that usually include reactive conditions and that lead to

    the spatial characterization of flames.  Table 1 includes a summary

    of these experiences indicating remarkable details and measure-

    ments performed in each case. However, literature concerning

    experimental analysis of pulverized fuel flames including reactive

    conditions and leading to spatial characterization is limited to a

    few studies [6,7].

    0016-2361/$ - see front matter     2013 Elsevier Ltd. All rights reserved.http://dx.doi.org/10.1016/j.fuel.2013.05.077

    ⇑ Corresponding author. Tel.: +34 976 762 562; fax: +34 976 762 616.

    E-mail address:  [email protected] (A. González-Cencerrado).

    Fuel 113 (2013) 798–809

    Contents lists available at  SciVerse ScienceDirect

    Fuel

    j o u r n a l h o m e p a g e :  w w w . e l s e v i e r . c o m / l o c a t e / f u e l

    http://dx.doi.org/10.1016/j.fuel.2013.05.077mailto:[email protected]://dx.doi.org/10.1016/j.fuel.2013.05.077http://www.sciencedirect.com/science/journal/00162361http://www.elsevier.com/locate/fuelhttp://www.elsevier.com/locate/fuelhttp://www.sciencedirect.com/science/journal/00162361http://dx.doi.org/10.1016/j.fuel.2013.05.077mailto:[email protected]://dx.doi.org/10.1016/j.fuel.2013.05.077http://crossmark.crossref.org/dialog/?doi=10.1016/j.fuel.2013.05.077&domain=pdf

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    CCD based visualization systems offer a cost-effective alterna-

    tive for monitoring and characterization of combustion flames gi-

    ven its robustness and simplicity of design [8,9]. Different studies

    performed through this techniques have provided valuable infor-

    mation concerning flame temperature and emissivity [10–12], sootconcentration   [13,14]   or quantitative measurements of radical

    emissions  [15]. Vision-based techniques have been also used for

    the analysis and assessment of biomass co-firing at industrial

    scales   [9,16] finding interesting results that suggest different im-

    pacts on flame characteristics.

    The present experimental work deals with the challenge to ob-

    tain a better understanding of strongly radiating turbulent and

    reacting flows from the images acquired with a high speed CCD

    camera. Specifically, the effect of changes in swirl number is inves-

    tigated in two different flames. On the one hand, the visualization

    system is used in a laboratory scale atmospheric gas flame, being

    the results physically interpretable from comparison with PIV

    measures. On the other hand, the procedure is applied to a semi-industrial scale burner of pulverized fuel, involving a participating

    media and a more complicated flow dynamics.

    Both facilities and the visualization system are described in Sec-

    tion  2. A flame visualization system based on a high-speed CCD

    camera was used to capture the image sequences containing the

    spatial–temporal luminous information from the flame. After a

    suitable digital image processing, different flame features are ob-

    tained in terms of statistical and spectral parameters. Results are

    Nomenclature

    CCD charged couple deviceD   nozzle diameter (m) f    characteristic frequency (Hz)HSB high swirl burnerIRZ internal recirculation zone

    LDA laser doppler anemometryLPP lean premixed prevaporizedLSB low swirl burnerL   characteristic length (m)PF pulverized fuelPLIF planar laser induced fluorescencePVC precessing vortex coreQ    volumetric flow rate (m3/s)

    Re   Reynolds number:  Re  ¼  4  _m=plDS-PIV stereo particle image velocimetryS  g ,s   geometric secondary swirl: S  g ,s = 2/3  tan  aSt    Strouhal number:  St  = ( f   L)/V St ⁄ alternative Strouhal number, frequency parameter:

    St  ¼ ð f    D3e Þ=Q V    fluid velocity (m/s)a   vane anglel   dynamic viscosity at ambient temperature (kg/m s)/   air–fuel ratio

     Table 1

    Summary of experimental analysis performed in swirl flames using advanced technologies.

    Ref. Fuel React. Technology Burner Conditions Measurements

    [1]   Propane Yes S-PIV atmosph. LPP Low/high S Velocities, frequencies, flow structures, vorticity

    [2]   — No LDA,acoustic vortex burner Re = 15,000; S  = 1.01 Velocities, flow structures

    [3]   — N o L DA , fl ow v isua lizat ion Front w all (sca le 1/10) D if f. c onfig urat ions I nte ra ct ion swirling jets, flow v isua liza tion,

    velocities

    [4]   N .g . ye s PIV, L DA , p hot og ra phy L ea n non-premix ed swirl-

    stabilized

    S  = 0.82;20 kW Two injection topologies, velocities,

    temperatures

    [38]   Methane Yes S-PIV, PLIF, Rayleigh

    scattering

    Stratified premix.

    turbulent LSB

    27–40 kW;  /  = 0.62 Velocities, temperatures, fuel distribution

    [39]   M ethane Ye s PIV, O H-PL IF ima ging Premix . t urbule nt LS B R e = 77–221;  /  = 0.7 Velocities, OH concentration, flame fronts,

    structures

    [40]   Methane Yes S-PIV, OH-PLIF Gas turbine model

    combustor

    10.3 kW;  /  = 0.75;  S  = 0.55;

    Re = 15,000

    Velocity fields,flame structures

    [41]   N.g. Yes CH-chemiluminiscence,

    photography, acoustic

    Premix. swirler injector   a = 45, diff. operationpressures

    Combust. instabilities,oscillations, CH

    concentrations

    [42]   Gas

    (unspecif.)

    Yes PIV, OH-PLIF, Rayleigh

    thermometry

    LSB 27–40 kW;Re = 20,000–

    30,000; S  = 0.5;  /  = 0.62

    Velocities, vorticity, temperature

    [6]   — No Hot-film sensor,

    visualization

    Coa l burne r S = 0. 344–0. 410 Flow visua liza tion, frac ta l dime nsion,turbulence

    [37]   Pr opane Yes LDA,high speed Pr emix. atmosph. camera,

    acoustic, chemilm.

    S = 0–1.5 Frequency analysis

    [43]   — No LDA, high-speed filming,

    acoustic

    Changeable blade swirler Re = 16,000; S  = 1 Velocities, structures, frequencies

    [44]   Methane Yes LDA,OH-PLIF, Raman

    scatt., chemilm.

    Lean premix. 25–30 kW;  /  = 0.7–0.83 Velocities, OH concentration, temperature,

    instabilities

    [45]   N. g. Ye s O H-PL IF, PIV, Ra ma n spe ct . Le an premix ed D if fe re nt pressures Veloc ity field s, O H c once nt rat ion

    [46]   Methane Yes LDA, OH/CH-PLIF, Raman

    scatt.

    Gas turbine model

    combustor

    7.6–34.9 kW Flow fields

    [47]   Methane Yes LDA, CH-PLIF, Raman scatt. Gas turbine combustor Re = 7500–60,000;

    S  = 0.55–0.9

    Flow field, species and temperature

    measurements, visualization of reaction zones

    [48]   Gas

    (unspecif.)

    Yes Photography, emission

    spect.

    Lean direct injection   a = 30–65 Species distribution,structure

    [49]   Gas

    (unspecif.)

    No PIV, hot-wire anem., high-

    speed photo

    Lean swirl Re = 5700–61,000;  S  = 0.6–

    3.7; confined/unconf.

    Structure, PVC, IRZ dependency with geometric

    and flow features

    [7]   Coal Yes PIV, LES Swirl coal burner S = 0.91 Velocities,species concentration,temperature,

    PIV–LES comparison

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    presented either spatially or as quantitative data depending on the

    analysis procedure.

    Section 3  briefly defines the processing procedure and the cor-

    responding outcomes which are later interpreted as flame param-

    eters. Section 4 presents the results concerning the two flames and

    discussion of their main findings. The conclusions and perspectives

    are finally summarized in Section 5.

    2. Experimental setup

    Two different experimental facilities were used for the study. In

    a first stage, a laboratory premixed gas swirl burner (50 kWth) was

    used. The purpose was to characterize the flame and establish the

    basis for the subsequent analysis of a 500 kWth PF flame, where the

    visualization of the whole flame was not possible. This enables

    swirl flame comparison at very different scales, providing useful

    information to complement the current analysis as a tool for the

    identification of swirled flame features.

     2.1. Test rigs

    The laboratory scale facility comprising the gas burner belongs

    to the Thermal Engineering, Energy and Atmosphere (ITEA) group

    from Carlos III University, Spain. The atmospheric burner was de-

    signed to study swirl flames by means of visual analysis. Accord-

    ingly, its geometry allows good optical access to the whole flame.

    Fig. 1 shows the geometry and dimensions of the burner. The main

    body corresponds to a cylindrical plenum and two coaxial central

    Fig. 1.  Atmospheric gas swirl burner (courtesy of M. Legrand). (a) Real image and (b) scheme of the top and front view of the burner geometry [1]. Dimensions are in mm.

    Fig. 2.  Experimental test facility: 500 kWth   PF swirl burner.

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    pipes ending with a nozzle of 26 mm diameter. Two symmetrical

    opposite pipes with tangential outlets are used to generate the

    swirl motion. The radial distance of these two pipes can be ad-

     justed to control the swirl level. An air-propane flow is premixed

    and then fed into the burner. Further details about burner geome-

    try and design can be found in Refs.  [1,17].

    Pulverized coal combustion experiments were performed in a

    500 kWth   test facility (Fig. 2). It consists of a downward oriented

    swirl burner dedicated to pulverized fuels (mainly biomass andcoal) [18]. The premixed burner has two coaxial injectors for pri-

    mary and secondary air, a refractory quarl to promote flame stabil-

    ity an a cylindrical combustion chamber of 3 m long and 1 m of 

    internal diameter. Different ports along the furnace are available

    for probe installation. Additionally the facility is fully instrumented

    and monitored through and advanced control and data acquisition

    system. Coal is introduced with primary air by the inner duct of the

    burner and is swirled by a volute. With regard to secondary air, a

    movable-vane swirler mechanism provides the rotational motion

    to the air flow. The swirl number is controlled with high precission

    by adjusting the vanes angle (a). The geometric swirl number def-inition is given by this expression S  g ,s = 2/3  tan  a. Secondary air ispreheated up to 250  C with an additional natural gas burner in or-

    der to enhance combustion efficiency. A multifuel feeding systemprovides the on-line regulation of the real mass flow of fuels. Pol-

    lutant emissions are measured at stack using a complete analyzer

    system with gas sampling, sample conditioning, analyzer and sys-

    tem control units. The set of standard analyzers are composed of 

    NDIR (Non-dispersive Infrared) absorption photometers and elec-

    trochemical sensor for O2. Further details can be found on Refs.

    [19,20].

     2.2. Visualization system

    The flame monitoring system, based on a CCD (charged coupled

    device) camera was designed for the visualization of combustion

    flames in both, atmospheric and highly confined enclosures  [21].The harsh environment during tests in the PF facility and the small

    dimensions of the inspection ports determined the final design of 

    the probe. On the one hand, the system relies on a 17 mm remote

    head, located at the end of the probe, which accommodates the ac-

    tive sensor and is fitted to an optical assembly. On the other hand,

    a protective system keeps low work temperatures and good lens

    conditions. It consists of a cylindrical water-cooled jacket made

    of stainless steel with a purgue of air and dimensions: 680 mm

    long and 35 mm outer diameter. This probe is inserted in one of 

    the inspection ports near the burner throat. This arrangement pro-

    vides a suitable flame view area of 315 mm (h)  230 mm (v),

    approximately.

    As regards camera specifications its main characteristics are

    listed in Table 2. It achieves a high-speed frame rate of 120 frames/s (fps) which allows a suitable frequency analysis [22].

    A full characterization stage was reported in a previous work

    (Ref. [20]) but it is briefly presented here. This reduces the distor-

    tion in the acquired flame images caused by thermal fluctuation or

    electronic noise from the system which could lead to misinterpre-

    tations. Following parameters were defined and quantified: non-

    uniform responsivity, instrumental background, noise ratio and

    saturation equivalent exposure [21]. They depend on the CCD sen-

    sor physical structure and the conversion process into an electricalsignal. Several tests in absence of light were performed in order to

    create a master dark frame which was built from the time average

    of gray values for each individual pixel. By subtracting this frame to

    each image, the systematic error is removed. This is the first step of 

    the processing procedure. The global performance parameter for

    non-uniformity was quantified as the standard deviation of the

    dark frame, being around 2.53%, which is an acceptable figure.

    Thermal fluctuation and electrical noise under dark conditions

    were also estimated for every pixel as the standard deviation com-

    posing the time signal (around 1%). Finally, size and distortion of 

    the visualized area were analyzed through a set of tests performed

    on a graph paper uniformly illuminated. The final resulting images

    were scaled using this experimental fitting.

     2.3. Fuel and experimental program

    Tests were first conducted in the 50 kWth   atmospheric swirl

    burner. Several air-propane mixtures were premixed and then

    burned under high (HSB) and low (LSB) swirl conditions. Swirl

    number for the LSB configuration was set around 0.48 while for

    HSB it was near 0.6. It was controlled by changing inner/outer flow

    ratio. Reynolds conditions (Re), referred to the total mass flow rate,

    were similar for both situations (Re = 14,000). CCD camera was lo-

    cated perpendicular to the flame vertical axis to permit a complete

    flame view (see Fig. 4a).

     Table 2

    Camera specifications.

    Parameter

    Active area (mm) 6.4 (h)  4.8 (v)

    Active pixels 659 (h)  494 (v)

    Signal/noise ratio >50 dB (0 dB gain)

    Electronic shutter 1/10,000 s

    Operating temperature 5  C to +45 C

    Dimensions (H  W  L) Head ø17  46 mm (ø  D)CCU 44  29  66 mm

    Spectral range 400–1000 nm

    Max. Spectral response 500 nm

    Focal length 7 mm

     Table 3

    Fuel characterization.

    Coal

    Moisture (as received,%wb) 2.30

    Proximate analysis (%d.b)

    Ash 14.60

    Volatile matter 26.00

    Fixed carbon 57.10

    Ultimate analysis (%d.b)Carbon 69.60

    Hydrogen 4.00

    Nitrogen 2.05

    Sulfur 0.50

    HHV (MJ/kg), (d.b) 27.80

    Mean particle diameter (mm) 0.045

     Table 4

    Summary of main parameters of combustion tests.

    Furnace operating conditions

    Thermal Power input (kWth) 500

    Coal feed rate (kg/h) 68.4

    Excess air (%) 14.6 ± 1.5

    Primary air to fuel ratio 2.3

    Primary air

    Flow rate (kg/h) 157.4 ± 0.08

    Temperature (C) 15

    Geometric swirl number 1.54

    Reynolds number 19,144

    Secondary air

    Flow rate (kg/h) 503.2 ± 12.30

    Temperature (C) 254

    Geome tric swirl numbe r ( nominal) 0 .67

    Reynolds number 25,800

    Mean furnace temperature (C) 980 ± 15

    Swirl numbers (S  g ,s) 0.28; 0.40; 0.67; 0.79; 1.20

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    With regard to experiments performed in the 500 kWth pulver-

    ized fuel swirl burner, a wider range of swirl numbers was ana-

    lyzed, as it is indicated in Table 4. The fuel used in the tests wasa South African coal, with low sulfur content and pulverized to a

    mean particle size of 0.045 mm. Ultimate and proximate analyses

    are shown in Table 3. According to particle size distribution analy-

    sis, 100% of the pulverized coal is under 0.1 mm and 70% under

    0.055 mm.

    Experimental research at laboratory large scale mainly consist

    on combustion tests varying secondary swirl number, while main-

    taining the other relevant parameters nearly constant (Table 4).

    Once steady conditions have been achieved in the combustion

    chamber, after a suitable preheating time, secondary swirl number

    is progressively modified by adjusting the secondary vane angle

    using a vane actuator. Each swirl position is fixed during a suitable

    time period (not less than 15 min) and an average of 3–4 videos are

    then recorded for each swirl condition. Furnace gas temperaturewas around 980 ± 15  C. A slight temperature increase could not

    be avoided due to the slow warming of refractory walls.

    Although most of the videos were recorded at stable conditions,

    some flame images were also registered at transition stages, when

    swirl conditions were changing (while secondary vanes were in

    motion). Transition periods take few minutes until vanes reachthe correct angle. During this interval, the flame is continuously re-

    corded in order to analyze it under variable conditions. Frame rate

    (120 fps), electronic shutter (1/10,000), iris aperture and time

    duration (42 s) were the same for all the videos.

    3. Analysis procedure

    Luminous radiation from the flame reaches the CCD sensor and

    is converted into an electric charge. The charge from each cell is

    transformed into a pixel gray value (ranging from 0 to 255) in

    the corresponding image. According to the camera acquisition

    speed, 120 images per second (fps) are recorded and transmitted

    to the frame grabber installed in the PC, where they are finally

    stored. A collection of thousands of images containing the lumi-nous flame information is the basis for the subsequent analysis.

    It is made over each video starting with the correction of non-uni-

    formity patterns (Section  2.2) followed by the calculation of the

    different flame parameters explained below. The video represents

    a three-dimensional matrix of gray values, where two dimensions

    correspond to space and the third one to time. Fig. 3 outlines the

    two different analyses that can be done as a function of data

    selection.

     Spatial analysis: the time signal of each individual pixel is ana-

    lyzed through statistical and spectral methods. The correspond-

    ing results are represented in form of two dimensional spatial

    distributions which leads to a qualitative characterization of 

    the flame area.

    Fig. 3.   Outline of the processing procedure leading to different flame characterization.

     Table 5

    Flame parameters definition.

    Signal

    characterization

    Statistical/spectral

    parameter

    Mathematical

    expression

    Flame brightness Mean value ( x)    x ¼  1N PN 

    i¼1 xiFluctuation

    amplitude

    Standard deviation (r) r ¼ ffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi ffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi 

    1N 

    PN i¼1   xi    xð Þ

    2q 

    Oscillation

    frequency

    Flicker (F)F  ¼

    PN 1k¼0

      X f kð Þj j f k

    PN 1

    k¼0  X f kð Þj j

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      Temporal analysis: gray values contained in each image are

    averaged. Therefore just one temporal flame luminous signal

    is obtained for each video. From that signal, flame features are

    calculated leading to a quantitative estimation of the flame

    state.

    Statistical and spectral flame parameters linked to geometrical,

    luminous and oscillating properties are calculated from the flame

    videos using specific processing algorithms   [20].   Table 5   shows

    the mathematical expression for each parameter considered in

    the analysis. All the equations are referred to a base set of gray val-

    ues ( x1  . . .  xi  . . .  xN ) which depends on the type of analysis. These

    parameters comprise different statistical moments: mean value

    and standard deviation, which can be interpreted as the flame

    brightness and the amplitude of the flame luminous fluctuations,

    respectively. Both are expressed in gray units (g.v.) that range from

    Fig. 4.  Spatial distribution of flame features under low (LSB) and high (HSB) swirl conditions in a 50 kW th propane swirl burner. (a) Snapshots of real images, (b) Mean value

    (flame brightness, g.v.), (c) Standard deviation (luminous fluctuation amplitude, g.v.) and (d) Flicker (Hz).

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    0 to 255 according to the camera specifications. Flame brightness is

    usually related to the flame size, the volatile content of the fuel and

    the radiation level of chamber walls, when they are present [23]. At

    this point, it is important to take into account the existing differ-

    ences of luminous emission between the gas and the PF flame.

    They are later commented in more detail but the main difference

    is related to the contribution of particles in the PF flame. Therefore,

    the information provided by this parameter cannot be interpreted

    in the same way concerning the two flames.

    Apart from statistical parameters, the Fast Fourier Transform

    (FFT) is used to calculate the Power Spectral Density ( f k) and an

    averaged frequency, called flicker (F ). This parameter corresponds

    to the mean frequency at which the flame fluctuates. Those fluctu-

    ations are caused by the variability of heat release, turbulent mix-

    ing and the resulting eddies existing in a combustion flame   [24].

    Therefore, it can be used as an estimator of different flame condi-

    tion and combustion efficiency [25].

    4. Results and discussion

    In this section main results regarding both flames are presented

    and discussed. It must be noticed that the sources of flame radia-

    tion strongly depends on fuel composition and combustion condi-

    tions. Consequently, these facts must be taken into account for a

    correct interpretation of the flame parameters.

    Specifically, spontaneous emission of electromagnetic radiation

    is derived mainly from solid material (soot, ash, particles), from

    some gas molecules (basically CO2 and H2O), due to the high tem-

    perature reached in flames, and finally, from several excited spe-

    cies coming from specific chemical reactions [26]. In the PF flame

    the contribution of particles represents most of the radiation

    reaching the sensor element, while for the gas flame luminous

    emission is derived from the other sources. Besides, the confine-

    ment of the PF flame influences its structure and behavior   [27]

    apart from the interference of thermal radiation from furnace walls

    and participating media [5].

    Therefore, it is important to bear in mind these obvious differ-

    ences between the two flames which makes that the results cannot

    Fig. 5.  Averaged gray values (g.v) corresponding to the central axis for both flames,

    showing the relative displacement as swirl number is increased.

    Fig. 6.  Comparison of flame front location obtained from different analyses performed in the same burner. (a) PIV measurements (turbulent kinetic energy ( m2/s2)) for LSB

    and HSB conditions, white lines represent the approximate averaged flame front location  [1] and (b) Standard deviation distributions (g.v.) from spatial analysis for LSB andHSB conditions. Countours of high standard deviation values define similar flame fronts.

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    be considered fully comparable. Nevertheless, luminous informa-

    tion from both flames allows a suitable first-step characterization

    in terms of dynamical structure and oscillatory behavior under dif-

    ferent swirl conditions.

    4.1. Results from atmospheric gas flame

    A thorough flame characterization had been performed bymeans of Stereo Particle Image Velocimetry (S-PIV) in a previous

    work   [1]. Low and High Swirl Burner configurations (LSB and

    HSB respectively) under isothermal and reactive conditions were

    covered in the study. Reactive flow results have been compared

    to current analysis in order to improve the interpretation of the

    results.

    Here, LSB and HSB configurations were tested under reactive

    conditions leading to two different flow topologies.   Fig. 4  shows

    the actual image and the spatial distribution of flame parameters

    for both swirl conditions applied to the propane flame. Brightness

    distribution (mean gray value) clearly reveals the great difference

    in flame shape between high and low swirl conditions (Fig. 4b).

    Since the gray level is, in a rough sense, directly related to temper-

    ature [12], concentric distribution of brightness levels representsan approximate map of flame temperatures. Accordingly, the core

    of this structure represents the more intense combustion zone of 

    the flame, with recirculation of active species due to the radial ad-

    verse pressure gradient generated by swirling flow [28]. Therefore

    this area may correspond to the internal recirculation zone (IRZ)

    identified in experimental and numerical studies [29,30].

    Another typical effect of swirl flames that can be appreciated in

    the tests is the attachment of the flame to the burner nozzle when

    swirl number is increased [28,31]. Fig. 5 shows graphically this ef-fect. The analysis is applied to Fig. 4b where mean values distribu-

    tion of both flames (HSB and LSB) is illustrated. A’A and B’B

    sections represent the mean gray values obtained from these

    images versus axial dimension, and they correspond to the central

    axis of the flame. The relative displacement of the flame front be-

    tween both swirl conditions can be easily observed and quantified

    in approximately 7 mm.

    Flow structure produced by swirl burners is characterized by

    the presence of strong toroidal recirculation zones which are

    mainly responsible of flame stabilization  [28,32]. Those zones of 

    reversal flow have been extensively documented and they are usu-

    ally represented by spatial distribution of streamlines which are

    calculated from measured time-mean velocity distribution (see,

    for example Fig.1.2 in Ref.   [27]). These lines set constant stream

    conditions and show two circular flow structures which produce

    the formation of the internal recirculation bubble. Recirculation

    patterns created in these areas affect the hot products and species

    from chemical reactions which are responsible of luminous emis-

    sion. Standard deviation of this luminous fluctuation along the

    flame area is the basis for the current analysis. When it is analyzed,

    the resulting spatial distributions (Fig. 4c) show specific circular

    zones with constant values indicating the presence of particular

    structures similar to those established by theoretical streamlines

    which have been also defined for this particular burner  [17]. These

    results are obtained under different swirl conditions being evident

    even with low swirl number. This fact suggests that standard devi-

    ation values obtained from spatial analysis are related to the flow

    patterns and associated dynamics and highlight the importance of 

    this parameter as a potential tool for the analysis of flamestructure.

    As regards flicker distribution, frequency along the two flames

    is very different. Under HSB conditions, the flame shows lower

    oscillation frequencies than flame under LSB conditions. In both

    cases frequency increases in the radial direction, being highest in

    the flame visible boundary.

    In addition, higher swirl causes an increase of both the width

    and length of the flame reverse flow zone, a well-known effect

    [28]. In the current analysis, the area of higher brightness also in-

    creases in size for higher swirl numbers, as can be shown in Fig. 4b.

    In addition, the location of the two toroidal zones changes with in-

    creased swirl, standing closer to the nozzle. This effect also indi-

    cates the attachment of the flame under HSB conditions.

    Finally, comparison between S-PIV measurements under reac-tive conditions and current results has shown some similarities.

    Legrand et al.  [1]  identified the approximate flame front location

    by computation from seeding density gradients (white lines in

    Fig. 6a). In the current analysis similar flame front boundaries have

    been determined, located by means of standard deviation spatial

    distributions. Black lines in Fig. 6b) represent the contour of high

    standard deviation values which approximately match with the

    flame fronts found by PIV measurements.

    4.2. Pulverized coal flame results

    4.2.1. Pollutant emissions

    CO, SO2 and NO x emissions trends as a function of swirl number

    were analyzed and compared with luminous radiation parameters.Fig. 7 shows averaged values during the corresponding time periodFig. 7.  Averaged values of (a) CO, (b) NOx, and (c)  SO2  emissions as a function of swirl number corresponding to pulverized coal combustion tests.

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    as function of swirl. CO emissions were low, showing good com-

    bustion performance for all swirl conditions. A slight reduction in

    CO concentration with swirl number can be appreciated in

    Fig. 7a), although standard deviation greatly increases at the high-

    est swirl number (1.2), which may be attributed to an increase of 

    flame fluctuation amplitude.

    NOx  emissions trends with swirl strongly reflect differences in

    mixing patterns. Increase and decrease of  NO x with swirl have been

    experimentally reported   [31]. The NOx   reduction at low-

    to-medium swirl flames is attributed to flame stabilization because

    the enhancement of the fuel–air mixing process. Under fuel rich

    conditions in the near burner region fuel-nitrogen is mostly devol-

    atilized and reacts favoring N2   formation over NOx. Our results

    (Fig. 7b) show a NOx   decrease starting with the nominal swirlnumber with a previous increase for lower values indicating an

    improvement in the mixing process  [31]. This initial trend might

    indicate that mixing of secondary air with volatile products takes

    place prior to complete combustion which produces that oxygen

    react with the fuel nitrogen to form NO. This could result in a slight

    increment of NOx before the mixing improvement.

    Finally, SO2  concentration slightly increases with swirl number

    (Fig. 7c). As expected, an inverse dependence of SO2 and CO emis-

    sions with swirl number can be appreciated in Fig. 7a and c, as SO2emissions are directly related to fuel sulfur content and combus-

    tion completion.

    4.2.2. Results from digital analysis

    Results from atmospheric swirl flame measurements and emis-sion trends enables more accurate description of PF flame features

    without ignoring the existing differences of luminous flame emis-

    sion between both. It allows the connection between digital results

    and the dynamical processes present in swirl flames.

    The five different swirl numbers tested have been arranged

    according to high and low swirl conditions. The nominal swirl

    number (0.67) divides both groups (LSB and HSB), and is included

    in the LSB group. Qualitative results of flame features are presented

    below according to this arrangement (Figs. 8 and 9).

    Brightness contours (Fig. 8a) show an increase of flame width

    and luminous level with the swirl rise. As a consequence of swirl

    increase the spreading angle of the flame becomes wider. This ef-

    fect, that can be observed in current spatial results, is already

    known [28] and it has been also experimentally proved under sim-

    ilar conditions   [33]. A brighter inner zone is noticeable for thenominal swirl condition. This might indicate the formation of recir-

    culation flows leading to the internal recirculation zone (IRZ).

    Recirculation zones are only formed beyond a critical swirl number

    >0.6   [28],   which just matchs with the current nominal value

    (0.67). This explains why this area does not appear in the flames

    with lower swirl conditions. On the contrary, brightness distribu-

    tions for HSB conditions (Fig. 9a) highlight the presence of this area

    also showing the flame widening.

    If the area of higher brightness is compared for all the flames

    (LSB and HSB), one more feature concerning swirl flames can be

    appreciated. According to experimental works [33], the volatile re-

    lease and particle heating in the IRZ tends to be greater for inter-

    mediate swirl values. In this case, flame image corresponding to

    nominal swirl conditions (0.67) shows in fact a larger and more

    uniform area of maximum brightness (Fig. 8a). Bearing in mind

    Fig. 8.  Spatial distribution of flame features under relative low swirl conditions (LSB). All figures correspond to the pulverized coal flame operating under nominal conditions.

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    that volatile release increases flame brightness   [16], the current

    observation agrees with published results.

    With regard to standard deviation distributions for LSB condi-

    tions,   Fig. 8b shows how the area of higher values enlarges for

    higher swirl numbers. According to the results obtained for the

    atmospheric gas swirl flame, this feature is linked to flow patterns

    and recirculation zones. Therefore, it can be deduced that increas-

    ing swirl number produces an increase of recirculation patterns

    Fig. 9.   Spatial distribution of flame features under high swirl conditions (HSB). All figures correspond to the pulverized coal flame operating under nominal conditions.

    Fig. 10.   Time evolution of some flame features under different swirl conditions during a coal combustion test. Each value is extracted from the averaged luminous flame

    signal of the corresponding video.

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    also in the pulverized fuel flame. This result is verified also for HSB

    conditions (Fig. 9b). The recirculation zone becomes much more

    intense showing an elongation in the left side. Considering the

    rounded shape of this new structure, it might correspond to the

    swirled secondary air inlet. Intensification of recirculation patterns

    consequently involves the improvement of mixing process. This ef-

    fect agrees with the obtained NOx  trend previously discussed.

    Distribution of flame flicker shows clear differences betweenLSB and HSB conditions. For low swirl numbers (0.28 and 0.40),

    distribution of averaged frequencies is similar, with a wide zone

    of low frequency in the upper central part and a high frequency

    band in the right (Fig. 8c). Nevertheless, for higher swirl numbers

    the lower frequency zone apparently changes moving towards

    the central left side (Fig. 9c). In consequence, higher frequencies

    are moved and reallocated to the right and upper part of the flame.

    The changes in oscillating frequencies reveals how the inner

    dynamical behavior of the flame is altered by changing the swirl

    number of secondary air flow.

    Finally, some interesting conclusions can be deduced from

    quantitative results. The evolution of flame parameters, obtained

    from the averaged luminous signal, is measured during the tests.

    In the course of transition stages, secondary vane angle is progres-

    sively modified according to the procedure detailed in Section 2.3.

    In these periods flame stability is expected to be altered. In order to

    evaluate the usefulness of flame features in detecting those varia-

    tions several videos were recorded during these periods.   Fig. 10

    shows standard deviation and flicker values along the different

    swirl periods during a combustion test. Each value is derived from

    the corresponding video. The evolution of both features clearly

    show opposite trends. Additionally, they are notoriously altered

    in the transition periods which proves its usefulness detecting

    flame variations.

    Apparently an increase in swirl number implies wider fluctua-

    tion of flame luminous radiation and a magnification of low fre-

    quencies over the higher. The improvement in mixing patterns as

    a result of the swirl rise explains the increment of the fluctuation

    amplitude. Otherwise, according to specific publications concern-ing flicker measurements in flames [23], flicker decrease indicates

    that changes in flame geometry prevail over changes of heat re-

    lease rates.

    Another finding derived from temporal analysis is related to the

    frequency variation of the luminous flame signal as function of 

    swirl condition. Frequency analysis concerning both, isothermal

    and reacting swirl flow applications provides a suitable tool for

    detection of PVC dynamics. Through the calculation of a widely

    used dimensionless number, Strouhal number (St), swirling flows

    are analyzed in terms of their precession frequencies. Theoretical

    calculations (usually based on LES) are obtained and contrasted

    to experimental measurements in order to validate the numerical

    simulations. These are commonly performed by acoustic methods

    which provide the characteristic frequency of a certain flow but

    they are usually made under non-reactive conditions since the dif-

    ficulties to measure on real combustion flames.

    Here,a frequency parameter defined in previous publications[27,28,32]   was calculated using flicker as a characteristic fre-

    quency. This value is basically another form of Strouhal number

    and it is directly derived from it. When Strouhal is applied to a bur-

    ner, the velocity of the fluid is derived from the isothermal burner

    flow rate and based on the burner exhaust area. The characteristic

    length is the corresponding burner exhaust diameter (De). There-

    fore, the difference between this parameter and the basis definition

    of Strouhal is the term  p/4. Many authors have used this alterna-tive form of Strouhal number [34–36].It is calculated using the fol-

    lowing expression.

    St  ¼ f    D3e

    Q   ð1Þ

    where   f  is the characteristic frequency (flicker value in this case,Hz),   De   is the exit diameter of the burner (m) and   Q   is the total

    air flow rate (m3/s). Fig. 11 shows the resulting trend by calculating

    its value for the different frequencies obtained under each swirl

    condition, where a parabolic evolution of  St ⁄ versus swirl intensity

    is obtained. A total of 16 experimental data support the curve where

    each point has been defined from different experiments performed

    under similar swirl conditions. Several studies concerning swirling

    flows show similar trends even using different frequency data,

    which are usually obtained by means of acoustic techniques or

    numerical methods [29,37]. This effect has not been studied before

    on coal flames at semi-industrial scales due to the complexity of 

    measurements in these environments. In this sense, our analysis

    represents a promising option to further progress in the under-

    standing of pulverized coal flames.

    5. Conclusions

    An extensive experimental study of different swirl flames has

    been performed by means of a CCD based visualization system.

    The analysis was focused on a pulverized fuel flame of 500 kWthunder several swirl conditions. Additionally, an atmospheric gas

    swirl flame of 50 kWth   was also analyzed performing a similar

    analysis in order to complement the results and obtain additional

    information regarding different swirl flames. In this case, PIV mea-

    surements allowed to prove the usefulness of visualization system

    to identify the flame dynamical differences when swirl changes.

    The spatial characterization of both flames through statistical

    and spectral parameters has led to the identification of typicalstructures of swirl flames such as recirculation areas and flow pat-

    terns. Several differences concerning flame shape or oscillating fre-

    quency between low and high swirl conditions were detected. A

    clear increase of flame width and spreading angle was noticed

    for the coal flame with the swirl rise. Luminous flame intensity

    in the inner area of the flame clearly increases from nominal value

    and higher swirl numbers. This observation may be related to the

    improvement of the mixing patterns as a result of the swirl rise.

    The expected increase in recirculation patterns was also identified

    through the remarkable variation in standard deviation values

    which show a clear increment with the intensification of swirl.

    Finally, several parameters from temporal analysis of the lumi-

    nous flame radiation signal were proved to be potentially useful for

    the identification of changes in the luminous flame rate and there-fore to diagnose the actual state of the flame in terms of stability.Fig. 11.  Frequency parameter (St 

    ) versus swirl number obtained from coalcombustion in a PF swirl burner.

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    A modified Strouhal number has been defined by means of 

    flame flicker, similarly as in the characterization of swirling flows.

    From the analysis, an inverse dependence of swirl number with

    this parameter has been found, which agrees with related litera-

    ture predictions.

    Pollutant emissions obtained in current experimental combus-

    tion tests have shown the expected trends, in accordance with an

    improved mixing process as swirl number is increased. Particu-larly, NOx measurements exhibit close connections with swirl con-

    ditions and, in consequence, with other swirl-related parameters,

    as flicker. Further research is needed to finally establish a more

    accurate trend.

    In summary, in-depth flame characterization under very differ-

    ent swirl conditions allowed obtaining valuable information about

    main variations of flame structure and oscillatory behavior. Up to

    know, spatial details and frequency information could be only ob-

    tained using more advanced and complex technologies and almost

    entirely focused in gas flames. In this sense, the actual system

    means an innovative tool for flame analysis in a wide scale range

    including PF flames under reactive conditions.

     Acknowledgements

    This work has been supported by the project ENE2010-16011

    (Spanish Ministry of Science and Education, R&D Energy Program).

    The authors gratefully acknowledge J. Nogueira and M. Legrand

    (University Carlos III) for their support during the tests with the

    gas burner and for the opportunity of using their facilities. Also

    we whish to thank to C. Bartolomé and I. Ramos, researchers of 

    the Thermal Division of CIRCE, for their help during tests.

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