two-proton radioactivity: an experimentalist’s view
DESCRIPTION
Two-proton radioactivity: an experimentalist’s view. Catalin Borcea CEN Bordeaux-Gradignan and IFIN-HH. Two proton radioactivity – a new decay mode Two-proton emission from light nuclei Decay of 42 Cr and 49 Ni Two-proton radioactivity of 45 Fe - PowerPoint PPT PresentationTRANSCRIPT
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Two-proton radioactivity: an experimentalist’s view
Catalin Borcea CEN Bordeaux-Gradignan and
IFIN-HH
NANUF03, Bucharest September 7-12, 2003
• Two proton radioactivity – a new decay mode• Two-proton emission from light nuclei• Decay of 42Cr and 49Ni • Two-proton radioactivity of 45Fe• Future perspectives and developments
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Stable nuclei
Stable and -unstable nucleiAll observed nuclei:- stable- unstable- particle unstable
Leaving the valley of stability….
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One-proton radioactivity
Physics topics• test of nuclear mass models• nuclear structure beyond stability - single particle ordering and energy - j content of wavefunction - shape of mean-field potential• quantum tunneling through 3D barrier
Model calculationsto determine single-particle level sequence
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Two types of 2p emission: - ground-state emission • long lived: 45Fe, 48Ni, 54Zn • short lived: 6Be, 12O, 16Ne, 19Mg
- emission from excited states • β delayed: 22Al, 31Ar, … • others: 14O, 18Ne, 17Ne
To be measured: • proton energies • proton-proton angle
Two-proton radioactivitySequential emission:
Three-body decay:
2He emission:
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Two-proton radioactivitySequential emission:
Three-body decay:
2He emission:
Measurement of protonsand recoil
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Two types of experiments:
- long-lived nuclei s) implantation and decay- short-lived nuclei ps) : complete kinematics experiments
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Two proton emission
from light nuclei
Mass: A = 6 – 20
Z = 4 – 12 low Coulomb (+ centrifugal) barrier broad states - short half-lives T1/2 = 10-21s – 10-12s decay already in the target
complete-kinematics measurements behind production target
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2p emission from 12O
Total decay energy:
Proton-proton energy:
Proton-proton angle:
R.A. Kryger et al., Phys. Rev. Lett. 74 (1995) 860
Data consistent with 3-body or sequential decay
seq. decay
2He decay
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Experimental Procedure
24Mg fragmentation in SISSI at 95 MeV/uSelection with Alpha spectrometer : 17F, 18Ne, 20MgStripping reactions at entrance of SPEG
GANIL
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Mass of 19Na
19Na 18Ne + p
Reasonable agreement with experiment and predictions
J. Cerny et al.:W. Benenson et al.:
Garvey-Kelson:Pape-Antony:
12.97(7) MeV12.93(1) MeV
12.88(20) MeV13.30(20) MeV
Mass excess: 13.09(5) MeV
MU
ST
MUST
SPEG
Target9Be
20Mg
19Na
18Ne
p
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First mass measurement of 18Na
MU
ST
MUST
SPEG
Target9Be
20Mg
18Na
17Ne
p
18Na 17Ne + p
If assumed to be ground state:- huge Thomas-Ehrman shift 1. peak: 18Na* 17Ne*
2. peak: 18Na 17Ne: 25.04(12)MeV- problems with theoretical calculations
Mass excess: 24.19(5) MeV
Audi-Wapstra: Garvey-Kelson:Pape-Antony:
25.3(4) MeV25.4(2) MeV25.7(2) MeV
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Theoretical calculation for 18Na
Main shell-model components:• 18Na (1-): ([(d5/2)3]3/2+[p1/2]) ([(d5/2)2]2+[s1/2][p1/2])• 18Na (2-): ([(d5/2)3]5/2+[p1/2]) ([(d5/2)2]2+[s1/2][p1/2])• 17Ne (1/2-): ([(d5/2)2]0+[p1/2])• 17Ne (3/2-): ([(d5/2)2]2+[p1/2])
Barrier-penetration predicts all excited states to decay to 17Ne ground state
Shell-model spectroscopic factors:
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2p emission from 17Ne
15O+p
15O+2p
Good agreement with known separation energies and 16F
17.431
16F+p17Ne 15O+2p
17.968
18.25418.398
18.16118.39218.689
16.490
17.778
17Ne* 16F + p 15O + 2p
MUST
MUST
SPEG
Target9Be
18Ne15O
p
p17Ne*
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Proton-proton angle distribution
Three-body center of mass frame: 2p emission from 17Ne*
2HeSequential / 3-body
2He (53%)Sequential (47%)Sum
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Proton-proton angle distribution
Three-body center of mass frame: 2p emission from 17Ne*
• Agreement with MSU data : no angular correlation for Q2p =0.9 MeV states• Indication of angular correlation for higher lying states…..
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New search for 2p emission in 16,17Ne
MU
ST
MUST
VAMOS
Target9Be
17Ne
16,17Ne
Mass
15F+p
14O+2p
14,15O
p
p
SPIRAL24 MeV/u2*104pps
16Ne23.99 MeVΓ = 120 keV
23.89 MeVΓ = 1.2 MeV
19.31 MeV
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Conclusion:
2p emission from 19Mg 19Mg seems to be a good candidate• unexpected effect for 17Ne …. to be checked• determined masses of intermediate nucleus 18Na for • study of one- and two-proton emission from light proton-rich nuclei
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Collaborators:
T. Zerguerras, Y. Blumenfeld, T. Suomijärvi, D. Beaumel, M. Fallot, I. Lhenry-Yvon, J.A. Scarpaci, A. Shrivastava
IPN OrsayB. Blank, M. Chartier, J. Giovinazzo
CEN Bordeaux-GradignanW. Mittig, P. Roussel-Chomaz, H. Savajols
GANIL CaenC. Jouanne, V. Lapoux
DAPNIA SaclayM. Thoennessen
Michigan State University
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Two-proton emission
from medium-mass nuclei
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Two-proton emission from 45Fe ground state
X
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Decay scheme for 45Fe
Possibly very rich decay pattern
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GANIL 1999
• The observation of doubly-magic 48Ni• Study of 42Cr, 49Ni, and 45Fe
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Production of radioactive nuclei at GANIL
• 58Ni @ 75 MeV/A on nickel target• High primary beam intensity: 3-5A
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Production and observation of 48Ni
10 parameters to identify:48Ni: 4 counts49Ni: 106 counts45Fe: 53 counts42Cr: 287 counts
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Spectroscopic studies of 42Cr: a 2p candidate
Charged-particle spectrum:
Decay-time spectrum:
Two-proton ground-state emitter?
• -decay half-life• 1.9 MeV peak too high in energy Most likely -delayed decay
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Spectroscopic studies of 49Ni: a 2p candidate
Charged-particle spectrum: Decay-time spectrum:
• -decay half-life• 3.8 MeV peak too high in energy Most likely -delayed decay
-decay half-life predictions:• Möller et al.: 5.0 ms• Hirsch et al.: (7.3-20.4) ms
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Spectroscopic studies of 45Fe: a 2p candidate
Charged-particle spectrum: Decay-time spectrum:
Too low statistics to decide between 2p emission and decay
-decay half-life predictions:Brown: 15.5 msOrmand: 7 msHirsch et al.: (3 - 7) msTachibana et al.: 12 ms
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Two experiments:• GANIL in July 2000• GSI in July 2001
Two-proton decay of 45Fe
GSI:• low production rate: 6 45Fe implantations in 6 days
• fast data acquisition based on XIA modules
GANIL:• high production rate: 15 45Fe per day
• standard data acquisition (CAMAC – VME)
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Two-proton decay of 45Fe: GANIL data
J. Giovinazzo et al., PRL 89 (2002) 102501
• 58Ni @ 75 MeV/A on nickel target• High primary beam intensity: 3-5A
Detection setup:
Si(Li)
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Two-proton radioactivity of 45Fe: GANIL data
Identification of22 45Fe implants
J. Giovinazzo et al., PRL 89 (2002) 102501
Identification of 45Fe:
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Decay-time spectrum:
Two-proton radioactivity of 45Fe: GANIL data
Decay-energy spectrum: spectrum:
T1/2 = 16.7±7.0 ms
1.14 MeV peak
J. Giovinazzo et al., PRL89 (2002) 102501
Q value in agreement with predictions no pile up for peakhalf-life short enough for 2p emission data in agreement with daughter decay no ’s in coincidence with 1.14 MeV peak
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Two-proton decay of 45Fe: GSI data
The FRS:
M. Pfützner et al., EPJA 14 (2002) 279
Primary beam
650 MeV/u 58Ni
Implantationset-up
Beam current(SEETRAM)
Target 4 g/cm2 Be
S2 degrader3.6 g/cm2 Al
TOF 1, 2, 3(scintillators)
B2B3
E(MUSIC)
IDENTIFICATION IN FLIGHT
B2 p/Z TOF 1,2,3 v
E Z
A/Z
S1 degrader3.2 g/cm2 Al
NaI barrel
Stack of Si detectors7 x 300 m
511 keVIdentified ions
511 keV
B1
B4
Trigger, E300 m Si
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Two-proton decay of 45Fe: GSI data
6 implantation events identified
M. Pfützner et al., EPJA14 (2002) 279
A/Z
0 1 2 3 4 5 60Energy (MeV)
5 correlated decay events:• four 2p decays• one -delayed decay
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Two-proton radioactivity of 45Fe
Q2p = 1.14 MeVT1/2 = 3.8 ms
Clear evidence of 2p radioactivity
No coincident beta or gamma ray withthe 1.14 MeV peak
Peak width: no pile-up
Observed energy in agreement withpredictions
Observation of daughter decays
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Two-proton radioactivity of 45Fe: di-proton model
Experimental half-life: T1/2 = 3.8± ms2.00.8
Di-proton model half-life: 0.02 ms
+ SM spectroscopic factors: 0.12 ms
+ preformation factor ? + resonance energy ?
Lower limit for the half-lifeR-matrix model (Brown-Barker): S-wave p-p interaction : 4-40 ms
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Two-proton radioactivity of 45Fe
L.V. Grigorenko et al.Nice agreement between exp. data and predictions for p wave protonsbut: f-wave protons expected…..
di-proton: - - - -3-body:
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Conclusions
• clear evidence for 2p radioactivity of 45Fe: a new radioactivity
• other candidates: 48Ni, 54Zn• decay mechanism: 2He or 3-body• setup to measure p – p angle and individual energies TPC
Future studies
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First observation of 55Zn and 56Zn
Expected production rate for 54Zn: 10-15 per day
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New setup for 2p experiments on LISE3: TPC
identification
Drift of ionisationelectrons
emitter
protons
X-Y detector
Ele
ctri
c fi
eld
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What information can bring the two-proton radioactivity:• masses of nuclei beyond drip line• pairing in nuclei• sequence of single-particle levels• j content of wavefunctions• deformation• complex tunneling process• …..
Physics case
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CollaboratorsGSI:
M. Pfützner, R. Grzywacz, Z. Janas, J. KurcewiczUniversity of Warsaw
B. Blank, M. Chartier, J. Giovinazzo, A.-S. Lalleman, J.-C. ThomasCEN Bordeaux-Gradignan
E. Badura, H. Geissel, L.V. Grigorenko, M. Hellström, C. Mazzocchi, I. Mukha, G. Münzenberg, C. Plettner, E. Roeckl, R.S. Simon
GSI Darmstadt
M. StanoiuGANIL Caen
C. Bingham, K.P. RycaczewskiOak Ridge National Laboratory
K. SchmidtUniversity Of Edinburgh
GSI:
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Collaborators
GANIL:
J. Giovinazzo, B. Blank, M. Chartier, S. Czajkowski, A. Fleury, M.J. Lopez Jimenez, M.S. Pravikoff, J.-C. Thomas
CEN Bordeaux-Gradignan
G. de France, F. de Oliveira Santos, M. Lewitowicz, V. Maslov, M. StanoiuGANIL Caen
C. BorceaIAP Bucharest
R. Grzywacz, Z. Janas, M. PfütznerUniversity of Warsaw
B.A. BrownNSCL, MSU East Lansing
GANIL: