study of prompt neutron energy spectra in fast neutron induced fission of 238 u

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Study of Prompt Neutron energy spectra in fast neutron induced fission of 238 U ALOK SAXENA Nuclear Physics Division, BARC and Nuclear Data Physics Centre of India

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Study of Prompt Neutron energy spectra in fast neutron induced fission of 238 U. ALOK SAXENA Nuclear Physics Division, BARC and Nuclear Data Physics Centre of India. S. S. Kapoor , R. Ramanna and P. N. Rama Rao , Emission of prompt neutrons in the thermal - PowerPoint PPT Presentation

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Page 1: Study of Prompt Neutron energy spectra in fast neutron induced fission of  238 U

Study of Prompt Neutron energy spectra in fast neutron induced fission of 238U

ALOK SAXENA

Nuclear Physics Division, BARC and Nuclear Data Physics Centre of India

Page 2: Study of Prompt Neutron energy spectra in fast neutron induced fission of  238 U

M.S. Samant, R.P. Anand, R.K. Choudhury, S.S. Kapoor, K. Kumar, D.M. Nadkarni and A. Saxena,

“Determination of nuclear level densities of neutron rich fragment nuclei from measurement of prompt neutron emission spectra,” pp.94-103 (1991) in "Nuclear Data for Neutron Emission in the Fission Process, Proceedings of a Consultants Meeting," INDC(NDS)-251, 1991; IAEA Nuclear Data Section, 252 pages. Compiled by S. Ganesan, Document available at http://www-nds.iaea.or.at/reports-new/indc-reports/indc-nds/indc-nds-0251.pdf

S. S. Kapoor, R. Ramanna and P. N. Rama Rao, Emission of prompt neutrons in the thermalneutron fission of U235, Physical Review, Vol. 131, 283-296 (1963).

Page 3: Study of Prompt Neutron energy spectra in fast neutron induced fission of  238 U

M.S. Samant et al. Phys. Rev. C 51, 3127 – Published 1 June 1995

Page 4: Study of Prompt Neutron energy spectra in fast neutron induced fission of  238 U

α>αBG

α>αBG

α<αBG

α<αBG

β=7x1021 s-1

fo =10-15 10-21 s

ss = 5-30 x10-21 s

ω1 = 1x1021 s-1

tr =8x10-21 s

Pre-saddle delay

Saddle to Scission delay

Total fission delay

A.Saxena et al,Phys.Rev C49,932(1994)

Page 5: Study of Prompt Neutron energy spectra in fast neutron induced fission of  238 U

Measurements at LNL,Legnaro (Italy)

470-630 MeV 80Se + 208Pb

372 MeV 56Fe+232Th288

116

Measurement of fragment mass and kinetic energy and neutron correlations

80Se + 232Th 312124470-630 MeV

R.G.Thomas et al ,Phys.Rev.C75,024604(2007)

EXPERIMENTS PROPOSED BY BARC GROUP

Page 6: Study of Prompt Neutron energy spectra in fast neutron induced fission of  238 U

80Se+208Pb 288116

ExCN (MeV)

0 50 100 150 200 250

tot

0

10

20

30

40

50

80Se+232Th 312124

ExCN (MeV)

0 50 100 150 200 250

tot

0

10

20

30

40

50

ν sf tot =10±2 for Se+Pb

12±1 for Fe+Th

=17±2 for Se+Th

Page 7: Study of Prompt Neutron energy spectra in fast neutron induced fission of  238 U

7Li(p,n0)7Be Reaction as Source of Neutrons

• small kinematic energy spread • reasonable neutron intensity.

7Li + p 7Be + n , Q = -1.64MeV

Used NatLi as the (p,n) threshold of 6Li (7.5%) at 5.9223 MeV is outside the useful lower energy range of the p-7Li reaction.

Page 8: Study of Prompt Neutron energy spectra in fast neutron induced fission of  238 U

8

A schematic diagram of Folded Tandem Ion Accelerator

SpecificationsColumn voltage rating

6MV

Voltage stability

± 2 kV

Heavy ion energy range:

1(n+1) to 5(n+1) MeV

Proton energy range

1 to 5 MeV

Page 9: Study of Prompt Neutron energy spectra in fast neutron induced fission of  238 U

Schematic of Experimental Setup:

Glass Slab

flux: ῀2 x 107neutrons /cm2/s at sample position

5”dia x2” thick

Page 10: Study of Prompt Neutron energy spectra in fast neutron induced fission of  238 U

Fission Ionization Chamber

Page 11: Study of Prompt Neutron energy spectra in fast neutron induced fission of  238 U

Typical Fission Fragment spectrum for 252Cf obtained using small fission detector

FF

Page 12: Study of Prompt Neutron energy spectra in fast neutron induced fission of  238 U

i) Typical view of a NE-213 neutron detector.ii) Front view of a PSD module used for n-g discrimination.

Page 13: Study of Prompt Neutron energy spectra in fast neutron induced fission of  238 U

PSD

Typical Pulse shape discrimination (PSD) spectrum obtained using NE-213 Organic Scintillation Detector for 252Cf Spontaneous fission source

n

gn

g Pulse height Vs PSD spectrum

Page 14: Study of Prompt Neutron energy spectra in fast neutron induced fission of  238 U

TOF

Typical Time of Flight spectrum obtained for 70 cm flight path using NE-213 Detector

n

g

g

n

TOF Vs PSD spectrum

Page 15: Study of Prompt Neutron energy spectra in fast neutron induced fission of  238 U

Fig: Efficiency as a function of neutron kinetic energy.

Incident Neutron Energy0 2 4 6 8 10 12

Effi

cien

cy

0.0

0.1

0.2

0.3

0.4

0.5

Monte-Carlo SimulationPresent Work, (BaF2-Start)

Present Work, (Fission Detector-Start)

Threshold : 140keV

23)(

)exp(2)(

m

m

T

TEEEN

Page 16: Study of Prompt Neutron energy spectra in fast neutron induced fission of  238 U

30 keV threshold

Page 17: Study of Prompt Neutron energy spectra in fast neutron induced fission of  238 U

Neutron Energy (MeV)2 4 6 8 10

N(E

)

10-3

10-2

10-1

100

W. Mannhart evaluationMaxwellian Distribution

Page 18: Study of Prompt Neutron energy spectra in fast neutron induced fission of  238 U

238U(n,f) at En=3.0 MeV

TOF vs PSD

Page 19: Study of Prompt Neutron energy spectra in fast neutron induced fission of  238 U

TOF

Gamma

Neutron

Page 20: Study of Prompt Neutron energy spectra in fast neutron induced fission of  238 U

TOF

Neutron after PSD gate

Page 21: Study of Prompt Neutron energy spectra in fast neutron induced fission of  238 U

238U(n,f) at 2.5 MeV TOF vs PSD

Page 22: Study of Prompt Neutron energy spectra in fast neutron induced fission of  238 U

Neutron after PSD gate

En=2.5 MeV

TOF

Page 23: Study of Prompt Neutron energy spectra in fast neutron induced fission of  238 U

Ein= 2.5MeVN

(E)

10-2

10-1

100

Present ExperimentMaxwellian fit ENDF/B-VII.1

Ein=3.0MeV

Neutron Energy (MeV)

1 2 3 4 5 6 7

N(E

)

10-2

10-1

100

Present ExperimentMaxwellian fitENDF/B-VII.1

Ein=2.0 MeV

N(E

) 10-2

10-1

100

Present workMaxwellian Vladuca and Tudora et al. ENDF/B-VII.1

Page 24: Study of Prompt Neutron energy spectra in fast neutron induced fission of  238 U

Ein= 3.0 MeV

Neutron Energy (MeV)0.1 1 10

Rat

io to

Max

wel

lian

(T=1

.27

MeV

)

0.4

0.6

0.8

1.0

1.2

1.4

ENDF VII.1

Page 25: Study of Prompt Neutron energy spectra in fast neutron induced fission of  238 U

Ein=2.5 MeV

Neutron Energy (MeV)0.1 1 10

Rat

io to

Max

wel

lian

(T=1

.23

MeV

)

0.2

0.4

0.6

0.8

1.0

1.2

1.4

1.6

ENDF VII.1

Page 26: Study of Prompt Neutron energy spectra in fast neutron induced fission of  238 U

Aver

age

Ener

gy (M

eV)

1.7

1.8

1.9

2.0

2.1

2.2

2.3

Literature dataPresent experimentFUP1 Calculations from ref.[21]

1 2 3 4 5 6 7 8

Max

wel

lian

tem

pera

ture

(MeV

)

1.2

1.3

1.4

ENDF/B-IVLiterature dataPresent experiment

Incident Neutron Energy (MeV)

(a)

(b)

Cai Chonghai and Shen Qingbiao, . Nucl. Data Prog., CNIC-00412, No. 3 (1990) 29.

Page 27: Study of Prompt Neutron energy spectra in fast neutron induced fission of  238 U
Page 28: Study of Prompt Neutron energy spectra in fast neutron induced fission of  238 U

Collaborators:

VV DesaiB.K.NayakSV SuryanarayanaArun Agarwal

Further work is in progress to repeat 2.0 MeV measurement and also to improve the statistics for 252Cf data for reducing uncertainties in efficiency data.

Page 29: Study of Prompt Neutron energy spectra in fast neutron induced fission of  238 U

THANK YOU