satellite measurements of volcanic so 2 emissions into the utls simon a. carn 1, kai yang 2,3,...
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Satellite Measurements of Volcanic SO2 Emissions into the UTLS
Simon A. Carn1, Kai Yang2,3, Nickolay A. Krotkov3, and Fred J. Prata4
1. Michigan Technological University, Houghton, MI, USA2. University of Maryland, College Park, MD, USA3. Laboratory for Atmospheres, NASA Goddard Space Flight Center, Greenbelt, MD, USA4. Norwegian Institute for Air Research, Kjeller, Norway
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Tropospheric aerosols(Lifetime ≈ 1-3 weeks)
Passiv
e
SO2 ® H2SO4
Indirect Effects on Clouds
Explos
iv
e
NET COOLIN
G
Stratospheric aerosols(Lifetime ≈ 1-3
years)
Ashfall
Dissolved volatiles
Exsolution
Effectson cirrusclouds
absorption (IR)
IRHeating
emission
emission
IR Cooling
MoreDownwardIR Flux
LessUpwardIR Flux
forward scatter
Enhanced Diffuse Flux
Reduced Direct Flux
Less TotalSolar Flux
Heterogeneous ® Less O3 depletion Solar
Heating
H2SSO2
NET HE
ATING® H2SO4
CO2
H2O
backscatter
absorption(near IR)
Solar Heating
More ReflectedSolar Flux
HCl,BrO, ClO
Effusi
ve
Gas scavenging
?
Effects of volcanic emissions on the climate system
Tropopause(8-17 km)
TROPOSPHERE
STRATOSPHERE
Original slide courtesy of A. Robock
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UV satellite remote sensing of volcanic SO2
1978-2005Total Ozone Mapping Spectrometer (TOMS)
2004-Ozone Monitoring Instrument
(OMI)
2012-Suomi NPP/OMPS
SW PacificApril 23, 2006
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UV satellite volcanic SO2 emissions inventory (1978 – 2013)
• Increase in total explosive volcanic SO2 emissions from 1997-2011
El ChichònPinatubo
[Bluth et al., 1993; Carn et al., 2003]
Nabro
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Increase in tropical stratospheric AOD since 2000
Vernier et al., GRL, 2011Solomon et al., Science, 2011
Increase linked to influence
of tropical volcanic eruptions
Hofmann et al., GRL, 2009
Pinatubo
Ruiz
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UV satellite volcanic SO2 emissions inventory (1978 – 2013)
El Chichon Pinatubo
[Bluth et al., 1993; Carn et al., 2003]
Nabro
TR
OP
ICS
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OMI - SO2, NO2, BrO
TES - SO2
MLS - strat. SO2, HCl
MODIS - SO2, ash, sulfate
AIRS - UTLS SO2, ash
CALIOP (lidar) - cloud altitude, aerosol phase
The A-Train
Aura (2004-) Aqua (2002-)
CALIPSO (2006-)
CPR (radar) – precipitation, hydrometeors
CloudSat (2006-)
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Soufriere HillsRabaul
MLSHCl
MLSSO2
OMISO2
2006
Nyamulagira
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Okmok
Kasatochi
MLSHCl
MLSSO2
OMISO2
2008
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Sarychev Peak
Redoubt
MLSHCl
MLSSO2
OMISO2
2009
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Grimsvötn
Nabro
Nyamulagira
MLSHCl
MLSSO2
OMISO2
2011
Cordon Caulle
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MLSSO2
2012
2013Paluweh Popocatepetl?
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Grimsvötn mammatus (May 2011)
Photos by Jón Ólafur
• Fate of volcanic gases in eruption columns• Gas scavenging on ash and hydrometeors
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Sulfur budget of the Grimsvötn 2011 eruption
OMI - May 22 May 23
May 24
MetOp/IASI – H2SMay 22
L. Clarisse – LATMOS/ULB
Sigmarsson et al., GRL, in review
~0.3 Tg SO2
~29 kt H2S
• H2S/SO2 = ~0.1, similar to in-situ Icelandic gas samples
• ~15 kt S2?• ~120 kt S sequestered on ash• 0.6 Tg SO2 emitted; only 0.3
Tg reached UTLS• 38% S scavenged cf. 20%
[Textor et al., 2003]
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Suomi-NPP/OMPS UV Sensors
NP
Nadir Mapper (NM): swath similar to OMI
Limb instrument:Aerosol and Ozone profiles above tropopause
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Suomi NPP/OMPS NM SO2 data for Paluweh (Indonesia)
Feb 4, 2013Feb 5, 2013
HYSPLIT forward trajectory @ 17 km
HYSPLIT forward trajectory @ 15 km
• Reported (ash) plume altitude = ~14 km
Paluweh
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Suomi NPP/OMPS NM data for Paluweh
CALIPSO Vertical Feature MaskStratospheric aerosol detection
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Aura/OMI data for Paluweh
CALIPSO Vertical Feature MaskStratospheric aerosol detection
• ~0.03 Tg SO2 -> 0.04 Tg H2SO4
• Only 0.01-0.02 Tg/S year required to explain post-2002 strat. AOD increase [Hoffman et al., 2009]
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Direct retrieval of SO2 altitude from UV radiances
• SO2 altitude retrievals for 2008 Kasatochi eruption
[Yang et al., JGR, 2010]
• SO2 altitude directly retrieved from UV radiances
• Validate with CALIPSO, MLS• Reprocessing of entire UV OMI-
OMPS data archive planned (NASA MEaSUREs project)
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Summary
• Long-term record of volcanic SO2 emissions based on UV satellite measurements continues (TOMS, OMI, OMPS)– Increased SO2 flux from explosive volcanism 1997-2011
– Consistent with observed stratospheric AOD trends– Less explosive volcanism in 2012-13– A-Train data (MLS, CALIPSO) provides profile information
• New insights into sulfur gas scavenging in eruption columns– 2011 Grimsvötn (Iceland) eruption: 50% of S scavenged
• Many small tropical eruptions inject SO2 to tropopause level– SO2 sufficient to sustain long-term increase in stratospheric AOD
– Plume altitudes based on ash clouds may underestimate SO2 altitude
• Direct UV SO2 altitude retrievals now available – Reprocessing of all major eruptions planned to develop new altitude-
resolved volcanic SO2 climatology (NASA MEaSUREs)• Acknowledgments: NASA funding (Aura Science Team, Atmospheric Chemistry
Modeling and Analysis program, NPP Science Team, MEaSUREs)
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Time-series of maximum MLS SO2 and HCl
10
40
15
25
68
hP
a
46
hP
a
HCl
SO2
Direct injection
Mon
soon
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OMI SO2 zonal means
Noise Noise Noise Noise
Noise Noise
2011 2008
2009
Nabro
Grimsvötn Okmok
Kasatochi
Sarychev• Nabro was the largest tropical volcanic SO2 emission since the 1991 Pinatubo eruption