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Neutron applications laboratory for ESS-BILBAO Fernando Sordo 1,2 , Miguel Mag´ an 1,2 Santiago Terr´ on 1,2 , Angelo Gighino Novoa 1,2 Jose Manuel Perlado 2 , Javier Bermejo 1 Target and neutron applications group - ESS-BILBAO 1 Instituto de Fusi´on Nuclear - UPM 2 July 7, 2011 Target Group (ESS-BILBAO & IFN ) UCANS-II July 7, 2011 1 / 25

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Neutron applications laboratory for ESS-BILBAO

Fernando Sordo1,2, Miguel Magan1,2

Santiago Terron1,2 , Angelo Gighino Novoa1,2

Jose Manuel Perlado2, Javier Bermejo1

Target and neutron applications group - ESS-BILBAO1

Instituto de Fusion Nuclear - UPM2

July 7, 2011

Target Group (ESS-BILBAO & IFN ) UCANS-II July 7, 2011 1 / 25

Table of contents

1 Introduction

2 Source Term analysis

3 Thermomechanical analysis

4 Gas implantation

5 Applications

6 Comparison between ESS-LAN and ESSB

7 Laboratory geometry estimation

8 Conclusions

Target Group (ESS-BILBAO & IFN ) UCANS-II July 7, 2011 2 / 25

Introduction

Introduction

The ESS-BILBAO Accelerator Center site at the Lejoa UPV/EHU campus, will be provided witha proton accelerator up to 300-400 MeV. In the first construction phase, a beam extraction willbe set at the end of the DTL, which will provide a 50 MeV proton beam with an averageintensity of 2.25 mA and 1.5 ms pulses at a frequency of 20 Hz. These beam characteristicsallow to configure a low intensity neutron source based in the Be (p, n) reaction, which enablesexperimentation with cold neutrons similar to that of LENS. The total beam power will be 112kW, so the configuration of the neutron production target will be based on a rotating disk ofberyllium slabs perpendicularly facing the beam on one side and a cryogenic methane moderatoron the other, with the target-moderator system surrounded by a beryllium reflector. In thispaper, first estimates will be presented for thermomechanical conditions of the target coolingscheme, neutron source intensities, cold neutron pulses, operating dose rates, generated activityand tritium production.

Target Group (ESS-BILBAO & IFN ) UCANS-II July 7, 2011 3 / 25

Source Term analysis

Source term definition

The table shows the comparison between the experimental results and the nuclear models (CEM,Isabel, INCL, and INCL-ABLA). The best fitting model is the Isabel-Dresner, with a relative erroraround 10 % in all the range of relevant energies, which can be considered as adequate. Theresults of the ENDEF-VII cross-section show a sharp drop when going above 55 MeV, which isproduced due to neutron emission data not being available, and thus are completely discarded.

Energy I. Tilquin CEM Isabel INCL INCL-ABLA ENDEF45MeV 0, 056 0, 064 0, 062 0, 066 0, 066 0, 06455MeV 0, 078 0, 084 0, 080 0, 089 0, 088 0, 07765MeV 0, 104 0, 106 0, 103 0, 116 0, 081 0, 059

Source Term analysis (n/proton)

Target Group (ESS-BILBAO & IFN ) UCANS-II July 7, 2011 4 / 25

Source Term analysis

Target Materials

The table shows the total neutron production estimated using Isabel model, for 50 MeV protonshitting different materials. The material that achieves the highest neutron production rates isBeryllium, and thus, it will be the selected material. Lithium produces neutrons with a highenergetic level, and therefore, it could be interesting for some applications.

Material Neutrons/Proton Average Energy (MeV)Carbon 7.54E − 3 8.04Lithium 4.27E − 2 13.15

Beryllium 6.49E − 2 7.76

Target Group (ESS-BILBAO & IFN ) UCANS-II July 7, 2011 5 / 25

Thermomechanical analysis

Themomechanical analysis: Rotating target

From a mechanical point of view, projecting the beam to a single sheet is not possible withoutreaching temperatures and tensions outside the acceptable range in beryllium. In order to reducetemperature and tensions, we chose to distribute the beam between 20 to 40 sheets, arranged ina disk that would turn synchronized with the accelerator pulses.

Target Group (ESS-BILBAO & IFN ) UCANS-II July 7, 2011 6 / 25

Thermomechanical analysis

Themomechanical analysis: Rotating target

The figure shows a proposed schematic for the arrangement of the beryllium sheets (20 elements),with the proton beam normal to the sheets, and parallel to the disk axis.

Target Group (ESS-BILBAO & IFN ) UCANS-II July 7, 2011 7 / 25

Thermomechanical analysis

Themomechanical analysis: Beam angle

In order to avoid high energy neutrons incidence in the thermal neutron experiments, leaning thebeam to the experimental lines will be mandatory. By leaning the beam, the material sectioncan be reduced without altering the thickness seen by the protons and also the footprint of thebeen will be increased. Both effects will allow to reduce stress and temperatures. Figure showstemperature and stress distribution for 20 elements and 20 Hz of beam frequency.

Target Group (ESS-BILBAO & IFN ) UCANS-II July 7, 2011 8 / 25

Thermomechanical analysis

Themomechanical analysis: Beam angle

As shown in the figures, tension and temperature raise reductions are not very sharp. This is dueto three opposed effects: By increasing the slope we can reduce the material thickness, and thebeam drops its energy in a greater ellipse, but the energy deposition per volume unit increases asthe path in the material does.

Temperature and thermal stress

0.0

10.0

20.0

30.0

40.0

50.0

60.0

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80.0

0 1 2 3 4 5

Temperature (o C)

Time (s)

90o

45o

0.0

20.0

40.0

60.0

80.0

100.0

0 1 2 3 4 5

Von Misses Stress (MPa)

Time (s)

90o

45o

Target Group (ESS-BILBAO & IFN ) UCANS-II July 7, 2011 9 / 25

Thermomechanical analysis

Themomechanical analysis: Beam angle

The proton beam hits the sheet at a 45o angle so it produces an elliptical heat deposition profile.Thus, an elliptical temperature and stress distribution will be produced. An stress accumulationin the edges can be noticed so it could be possible to reduce stress if they were rounded.

Temperature and thermal stress at t = 0.25 s

Target Group (ESS-BILBAO & IFN ) UCANS-II July 7, 2011 10 / 25

Thermomechanical analysis

Themomechanical analysis: Cooling channel

In order to conclude target themomechanicalanalysis, a preliminary CFD evaluation ofcooling channel has been performed. A pressuredrop of 5000 Pa will ensure enough velocity toremove heat deposited on beryllium sheep. So,the refrigeration conditions are not very severe.

Figure shows velocity profile on radial direction.Pressure drop could be reduced if edges wererounded.

Target Group (ESS-BILBAO & IFN ) UCANS-II July 7, 2011 11 / 25

Gas implantation

Gas implantation

Only a small fraction of protons from the beam will suffer nuclear interactions, and due to it, alarge amount of free protons will be introduced in the target material. These free protons will getan electron and will become hydrogen. Hydrogen inside a metallic matrix will produce swellingand finally the mechanical failure as in LENS case.

H implantation ( atms/cm2-proton )

-45 -42.5 -40 -37.5 -35

Y (cm)

1

1.1

1.2

1.3

1.4

1.5

1.6

1.7

Z (cm)

0

0.5

1

1.5

2

2.5

3

3.5

4

4.5

H implantation ( atms/cm2-proton )

-45 -42.5 -40 -37.5 -35

Y (cm)

0

0.475

0.95

1.425

1.9

Z (cm)

0.0001

0.001

0.01

0.1

1

10

Target Group (ESS-BILBAO & IFN ) UCANS-II July 7, 2011 12 / 25

Gas implantation

Gas implantation

The LENS beryllium target has an operating time of 156 h for the parameters shown on thetable, so the results were extrapolated, and for lack of a more thorough study, a life of over3000 operating hours can be considered for ESS-BILBAO target. This value is roughly a fullyear operating the facility, which seems entirely reasonable for planning the upkeep and wheelsubstitution.

LENS ESS-B ESS-B 20 elementsAverage Intensity (mA) 0, 62 2, 25

Operation time (h) 156 171 3420Implantation (atms/cm3 − p) 18 4, 5

Evaluation for ESS-BILBAO target life time for 50 MeV protons

Target Group (ESS-BILBAO & IFN ) UCANS-II July 7, 2011 13 / 25

Applications

Applications: High energy and Cold neutrons

Taking into account the source term analysis, a multipurpose experimental facility is proposedwith three experimental lines, two of them for cold neutrons and one for high energy neutrons.

High energy neutron line:The main objective of this line will be measuring of high energy cross sections and test ofinstruments and detectors in this energy range. In order to maximize fast neutrons flux,the high energy line has to be oriented in the beam direction

High energy neutron for aerospace irradiations:Electronic devices for aerospace applications have to be tested on high atmosphereradiation conditions. These conditions can be reproduced at ESS Bilbao in order toperform accelerated irradiations.

Materials irradiationSeveral components of fusion and fission nuclear reactors have to be studied in mediumand low irradiation conditions that could be reproduced on ESS-BILBAO facilities.

Cold neutrons lines:Low energy neutrons lines will be used in close collaboration with the ESS project in orderto test components such as moderators, neutron lines, choppers or instrumentation. TheESS-BILBAO neutrons laboratory could be the test stand for ESS neutronics components.

Target Group (ESS-BILBAO & IFN ) UCANS-II July 7, 2011 14 / 25

Applications

Applications: High energy and Cold neutrons

In order to have a versatile installation, two operational modes have been studied to produceeither fast or thermal-cold neutron flux in the experimental lines. In the high energy mode,reflector material could be part of the shielding in order to minimize dose ratio outside thetarget area.

Fast neutrons mode Cold and thermal neutrons mode

Target Group (ESS-BILBAO & IFN ) UCANS-II July 7, 2011 15 / 25

Applications

Applications: Material Irradiation

The area close to the target inESS-Bilbao could be very interestingfor testing materials in medium and

low irradiations conditions. It will notbe enough for structural materials

high irradiation analysis, but it couldbe representative for several materials(Inertial fusion lens, ITER magnets,

ESS bearings or seals).

Target Group (ESS-BILBAO & IFN ) UCANS-II July 7, 2011 16 / 25

Applications

Applications: Material Irradiation

Neutron flux produced is a mix of high energy neutrons directly from the target, and neutronsmoderated on reflector and shielding. At 8 cm from target surface neutron flux is6.1 · 1012[n/cm2 − s] with and average energy of 5.6 MeV.

106

108

1010

1012

1014

1016

1018

1020

10-810

-710

-610

-510

-410

-310

-210

-110

010

110

2

[n/cm2/MeV-s]

Energy (MeV)

8 cm

17 cm

25 cm

34 cm

Neutron flux in several irradiation positions

106

107

108

109

1010

1011

1012

1013

10-2

10-1

100

101

102

[p/cm2/MeV-s]

Energy (MeV)

8 cm 17 cm 25 cm 34 cm

Photon flux in several irradiation positions

Target Group (ESS-BILBAO & IFN ) UCANS-II July 7, 2011 17 / 25

Applications

Applications: High energy neutron for aerospaceirradiations

Electronic components destined to aerospace applications have to be tested in high energyneutrons environment. CHIPIR instrument in ISIS is focused on testing this type of devices. Thetables shows ISIS-CHIPIR high energy flux (> 10MeV ).

Instrument Mode Flux [n/cm2 − s] Max Energy (MeV)ISIS-Chipir Pencil Beam 4 · 107 800ISIS-Chipir Flood Beam 3 · 105 800

An irradiation area placed at 6 m from ESS-BILBAO target in the TOF line cold produce asimilar neutron flux than ISIS-Chipir, the main difference will be that ESS-BILBAO averageneutron energy will be lower (7-8 MeV compared with 9-10 MeV).

Distance to Target (cm) Flux > 10MeV [n/cm2 − s]300 6,0E+8500 2,1E+8700 1,1E+8

Target Group (ESS-BILBAO & IFN ) UCANS-II July 7, 2011 18 / 25

Applications

Applications: Cold neutrons

The moderator in duty of producingcold neutrons will be a methane “box”at 22k, with a Aluminum cladding, withsome leaning on the beryllium rotatingdisk axis. The aim of such an orien-tation is reducing the high energy neu-tron flux in the experimental lines, sowe must avoid placing the experimentsin the beam projected line.

Target Group (ESS-BILBAO & IFN ) UCANS-II July 7, 2011 19 / 25

Applications

Applications: Cold neutrons

The reflector has a key effect in the shape of the pulse obtained at the moderator (Figures shows5 meV neutrons). Unlike beryllium, lead produces no neutron moderation, and thus tends toreduce brightness and tail, generating a much more “square” pulse.

0

2e+14

4e+14

6e+14

8e+14

1e+15

1.2e+15

1.4e+15

0 300 600 900

[n/cm2-eV-s-sr-MW]

Time (µS)

Beryllium Water Lead

0

5e+13

1e+14

1.5e+14

2e+14

2.5e+14

0 750 1500 2250 3000

[n/cm2-eV-s-sr-MW]

Time (µS)

Beryllium Water Lead

Target Group (ESS-BILBAO & IFN ) UCANS-II July 7, 2011 20 / 25

Comparison between ESS-LAN and ESSB

Comparison with beryllium reflector

ESS-BILBAO peak brightness is a factor of 50 under the peak brightness of ESS-LAN for shortpulse, which is a very good result, considering our neutron generation efficiency is about 500 timeslower. Considering the power difference between both installation (0.1 MW for ESS-BILBAO and5MW for ESS), we can conclude that the short pulse peak of our installation would be about2500 times less than that of ESS. Analyzing a long pulse, we observe a peak factor of 80, so wemay evaluate the difference between both installation in a 4.000 factor.

0

2e+14

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0 200 400 600 800 1000

0

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ESS-BILBAO [n/cm2-eV-s-sr-MW]

ESS [n/cm2-eV-s-sr-MW]

Time (µS)

ESS-B

ESS

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5e+13

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0

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2e+16

ESS-BILBAO [n/cm2-eV-s-sr-MW]

ESS [n/cm2-eV-s-sr-MW]

Time (µS)

ESS-B

ESS

Target Group (ESS-BILBAO & IFN ) UCANS-II July 7, 2011 21 / 25

Comparison between ESS-LAN and ESSB

Comparison with water reflector

The figure shows a compared distribution for a 1 ms pulse duration with a water reflector, wherewe can notice an entirely analogous profile between both sources, just scaled a factor 220. Thisis the scaling factor that shows us that we are using a more efficient moderator-reflector systemthan ESS, but 4 times worse than the Beryllium one. Power difference notwithstanding, we canconclude that it is possible to achieve the same pulse as ESS, just scaled a factor of 10000.

0

5e+13

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0 200 400 600 800 1000

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ESS-BILBAO [n/cm2-eV-s-sr-MW]

ESS [n/cm2-eV-s-sr-MW]

Time (µS)

ESS-B

ESS

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0 750 1500 2250 3000

0.0E+00

4.0E+15

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1.2E+16

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2.0E+16

ESS-BILBAO [n/cm2-eV-s-sr-MW]

ESS [n/cm2-eV-s-sr-MW]

Time (µS)

ESS-B

ESS

Target Group (ESS-BILBAO & IFN ) UCANS-II July 7, 2011 22 / 25

Laboratory geometry estimation

Laboratory layout

With the former results, a first approach of the laboratory configuration can be composed. Thetarget and the reflector system will be installed in a heavily shielded central room. This roomwill have 4, 10cm radius holes. One for the beam entry, and 3 for the experimental lines exits.Experimental areas could be separated by modular concrete panels in order to be able to adaptthe configuration.

Target Group (ESS-BILBAO & IFN ) UCANS-II July 7, 2011 23 / 25

Laboratory geometry estimation

Laboratory layout

ESS BILBAO Neutrons laboratory

Target Group (ESS-BILBAO & IFN ) UCANS-II July 7, 2011 24 / 25

Conclusions

Conclusions

As conclusions for the studies carried out related to ESS-BILBAO neutronic applicationslaboratory, the following highlights can be summarized:

1 A multipurpose facility for high and low energy neutrons is being designed forESS-BILBAO accelerator research center.

2 A solid beryllium rotating target cooled by water can guarantee one operation year in safethermomechanical conditions.

3 High energy neutron line could reproduce atmospheric irradiations conditions for electroniccomponents

4 Irradiation conditions close to the target cold be adequate for medium and low neutronsirradiation for material characterization

5 Cold neutrons produced with a water reflector and methane moderator can reproduce thepulse shape of ESS scaled by a factor 10.000. This neutron brightness could be enough totest ESS components as moderators, instruments, choppers and neutron guides.

Target Group (ESS-BILBAO & IFN ) UCANS-II July 7, 2011 25 / 25