4-2-14 radon presentation - comments on measuring long-term average radon … · 2014-04-01 ·...

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Comments on Measuring Long-Term Average Rd L l Radon Levels Presented To: Presented To: NRC Workshop on Evaluation of Radon and Radon Progeny in Air and Compliance with 10CFR20.1301 and (2) Presented By: Presented By: Douglas B. Chambers, Ph.D. April 2, 2014 1

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Page 1: 4-2-14 Radon Presentation - Comments on Measuring Long-Term Average Radon … · 2014-04-01 · Radon levels change diurnally and by season radon concentrations typically reac h their

Com

men

ts o

n M

easu

ring g

Long

-Ter

m A

vera

ge

Rd

Ll

Rad

on L

evel

sP

rese

nted

To:

Pre

sent

ed T

o:

NR

C W

orks

hop

on E

valu

atio

n of

Rad

on a

nd

Rad

on P

roge

ny in

Air

and

Com

plia

nce

with

10

CFR

20.1

301

and

(2)

Pre

sent

edB

y:P

rese

nted

By:

Dou

glas

B. C

ham

bers

, Ph.

D.

Apr

il 2,

201

4

1

Page 2: 4-2-14 Radon Presentation - Comments on Measuring Long-Term Average Radon … · 2014-04-01 · Radon levels change diurnally and by season radon concentrations typically reac h their

Obj

ectiv

eO

bjec

tive

N

ota

deta

iled

criti

que

ofin

terim

Gui

danc

e,

Not

a d

etai

led

criti

que

of in

terim

Gui

danc

e,

rath

er a sh

ort c

omm

enta

r y o

n na

tura

l lev

els

of

yam

bien

t rad

on, a

nd s

elec

ted

com

men

ts o

n ch

alle

nges

of m

easu

ring

smal

l inc

rem

enta

l (a

bove

bac

kgro

und)

leve

ls o

f Rn-

222

2

Page 3: 4-2-14 Radon Presentation - Comments on Measuring Long-Term Average Radon … · 2014-04-01 · Radon levels change diurnally and by season radon concentrations typically reac h their

Out

door

Rad

onO

utdo

or R

adon

R

adon

rele

ased

from

Ra-

226

in s

oils

is th

e si

ngle

larg

est

sour

ceof

Rn-

222

inth

eat

mos

pher

eso

urce

of

Rn

222

in th

e at

mos

pher

e

Rad

on le

vels

in o

utdo

or a

ir ar

e af

fect

ed b

y th

e re

gion

al

geol

ogy,

met

eoro

logy

, loc

al to

pogr

aphy

…S

dif

di

iN

di

didi

d

Stud

ies

of o

utdo

or a

ir in

Nev

ada

indi

cate

a m

edia

n ou

tdoo

r co

ncen

trat

ion

of 0

.4 p

Ci/L

with

con

cent

ratio

ns o

f up

to 1

.4

pCi/L

at m

easu

red

loca

tions

(Pric

e 19

94)

R

adon

leve

ls c

hang

e di

urna

lly a

nd b

y se

ason

ra

don

conc

entra

tions

typi

cally

reac

h th

eir m

axim

um in

the

sum

mer

to

ear

l y w

inte

r, w

here

as fr

om la

te w

inte

r to

sprin

g, c

once

ntra

tions

y

,p

g,ar

e us

ually

at a

min

imum

as

a re

sult

of m

eteo

rolo

gica

l cha

nges

an

d so

il m

oist

ure

cond

ition

s (N

AS

199

9).

3

Page 4: 4-2-14 Radon Presentation - Comments on Measuring Long-Term Average Radon … · 2014-04-01 · Radon levels change diurnally and by season radon concentrations typically reac h their

Rn-

222

Con

cent

ratio

nD

iurn

al V

aria

tion

SO

UR

CE

: Afte

r Pea

rson

, U.S

. Dep

artm

ent o

f Hea

lth &

Wel

fare

, 196

7,

p,

Page 5: 4-2-14 Radon Presentation - Comments on Measuring Long-Term Average Radon … · 2014-04-01 · Radon levels change diurnally and by season radon concentrations typically reac h their

Rad

on C

once

ntra

tion

in S

oil

Gas

of S

edim

enta

ry R

ocks

y ac

cord

ing

to g

eolo

gica

l ag

e

ac

cord

ing

to ro

ck ty

pe

Jung

et a

l

Page 6: 4-2-14 Radon Presentation - Comments on Measuring Long-Term Average Radon … · 2014-04-01 · Radon levels change diurnally and by season radon concentrations typically reac h their

Out

door

Rad

onco

nt’d

Out

door

Rad

on co

ntd

A

ccor

ding

to N

AS

1999

, mea

sure

men

ts ta

ken

over

the

g,

cont

inen

tal U

S, A

lask

a an

d H

awai

i sho

w th

e hi

ghes

t co

ncen

trat

ions

are

foun

d in

the

Col

orad

o Pl

atea

u w

here

mea

sure

men

tsra

nged

from

05

to0

75pC

i/Lof

whe

re m

easu

rem

ents

rang

ed fr

om 0

.5 to

0.7

5 pC

i/L o

f ai

r (18

.5–3

0 B

q/m

3 )

The

NA

S 19

99 a

lso

repo

rt m

any

area

s w

ith o

utdo

or

rado

n le

vels

rang

ing

from

0.1

2 to

0.3

pC

i/L

6

Page 7: 4-2-14 Radon Presentation - Comments on Measuring Long-Term Average Radon … · 2014-04-01 · Radon levels change diurnally and by season radon concentrations typically reac h their

Type

sof

Rad

onM

onito

ring

(1)

Type

s of

Rad

on M

onito

ring

(1)

Sh

ort T

erm

2

days

up

to 3

mon

ths

U

se re

sults

with

cau

tion

R

adon

con

cent

ratio

ns v

ary

over

long

tim

e pe

riods

. Lo

ng-te

rm d

ata

mos

t rel

evan

t.

Dev

ices

forS

hort

Term

Mon

itorin

gin

clud

e

Dev

ices

for S

hort

Term

Mon

itorin

g in

clud

e–

Act

ivat

ed C

harc

oal A

dsor

ptio

n-E

lect

ret I

on C

ham

ber

–C

harc

oal L

iqui

d S

cint

illat

ion

-C

ontin

uous

Rad

on M

onito

ring

–C

ontin

uous

Wor

king

Lev

el M

onito

r -A

lpha

Tra

ck

7

Page 8: 4-2-14 Radon Presentation - Comments on Measuring Long-Term Average Radon … · 2014-04-01 · Radon levels change diurnally and by season radon concentrations typically reac h their

Type

sof

Rad

onM

onito

ring

(2)

Type

s of

Rad

on M

onito

ring

(2)

Lo

ng T

erm

Mon

itorin

g

3 to

12

mon

ths

in d

urat

ion

R

ecom

men

ded

Dev

ices

for L

ong

Term

Mon

itorin

gA

lh

tk

dt

t–

Alp

ha tr

ack

dete

ctor

–E

lect

ret I

on C

ham

ber

–D

igita

l Det

ecto

r

Lo

ng te

rm m

easu

rem

ent p

rovi

des

bette

r ind

icat

ion

of

annu

al a

vera

ge ra

don

conc

entra

tion

than

sho

rt te

rm

mea

sure

men

t(di

urna

land

seas

onal

effe

cts

alre

ady

mea

sure

men

t (di

urna

l and

sea

sona

l effe

cts

alre

ady

acco

unte

d fo

r)

8

Page 9: 4-2-14 Radon Presentation - Comments on Measuring Long-Term Average Radon … · 2014-04-01 · Radon levels change diurnally and by season radon concentrations typically reac h their

Rec

ent E

xper

ienc

e fr

om In

door

R

dM

ii

iP

HR

adon

Mon

itorin

g in

Por

t Hop

e

SEN

ES re

tain

ed to

com

plet

ep

indo

or ra

don

mon

itorin

g fo

r ap

prox

imat

ely

1350

pro

pert

ies

Cli

tdid

dth

tit

C

lient

dec

ided

that

mon

itors

w

ould

be

alph

a-tr

ack

rado

n m

onito

rssu

pplie

dby

RSS

I(C

R-3

9)m

onito

rs s

uppl

ied

by R

SSI (

CR

39)

Lo

ng-te

rm m

easu

rem

ents

(5-6

mon

ths)

A

n ex

ampl

e to

illu

stra

te c

halle

nges

in m

easu

ring

rado

n tl

tti

at lo

w c

once

ntra

tions

9

Page 10: 4-2-14 Radon Presentation - Comments on Measuring Long-Term Average Radon … · 2014-04-01 · Radon levels change diurnally and by season radon concentrations typically reac h their

Qua

lity

Ass

uran

ce/Q

ualit

y C

ontr

ol

(PtH

)(P

ort H

ope)

D

uplic

ates

(ata

bout

10%

oflo

catio

ns)

D

uplic

ates

(at a

bout

10

% o

f loc

atio

ns)

A

dditi

onal

rado

n m

onito

rs w

ere

depl

oyed

for

QA

/QC

QQ

B

lind

spik

e sa

mpl

es

–30

blin

d sp

ikes

sen

t to

Bow

ser-M

orne

r

Tr

avel

bla

nks

–Tr

avel

bla

nk m

onito

r sen

t with

eac

h sh

ipm

ent

B

lank

s

Bla

nks

–U

nexp

osed

rado

n m

onito

rs, s

ent i

n se

aled

bag

s th

at w

ere

neve

r ope

ned

10

Page 11: 4-2-14 Radon Presentation - Comments on Measuring Long-Term Average Radon … · 2014-04-01 · Radon levels change diurnally and by season radon concentrations typically reac h their

Rad

on E

xpos

ure

in

“Nd”

Bl

k“N

ever

-ope

ned”

Bla

nks

180

120

140

160

Ci-d/L)

Est

imat

ed re

porti

ng li

mit

fb

t0

10

2C

i/L

6080100

on Exposure (pC

of a

bout

0.1

–0.

2 pC

i/L

0204060

Rado

00

1020

3040

50

Sam

ple

Num

ber

11

Page 12: 4-2-14 Radon Presentation - Comments on Measuring Long-Term Average Radon … · 2014-04-01 · Radon levels change diurnally and by season radon concentrations typically reac h their

One

Oth

er C

onsi

dera

tion

-D

ose

is fr

om th

e in

grow

th o

f Rad

on P

roge

ny

1

07

0.8

0.91

ctor

0.4

0.5

0.6

0.7

uilibrium Fac

0.1

0.2

0.3

Equ

00

1020

3040

5060

70

Tim

e (m

inut

es)

Page 13: 4-2-14 Radon Presentation - Comments on Measuring Long-Term Average Radon … · 2014-04-01 · Radon levels change diurnally and by season radon concentrations typically reac h their

Equi

libriu

m F

acto

r (F)

Fi

fDi

as F

unct

ion

of D

ista

nce

Page 14: 4-2-14 Radon Presentation - Comments on Measuring Long-Term Average Radon … · 2014-04-01 · Radon levels change diurnally and by season radon concentrations typically reac h their

NR

CIn

terim

Staf

fGui

danc

eN

RC

Inte

rim S

taff

Gui

danc

e

In

tend

ed fo

r NR

C s

taff

whe

n re

view

ing

uran

ium

g

reco

very

lice

nsee

sur

veys

for r

adon

Su

gges

ts c

an d

emon

stra

te c

ompl

ianc

e by

t

ll

tim

easu

rem

ent o

r cal

cula

tion

0.

1 pC

i/L w

ith d

augh

ters

10

pCi/L

with

outd

augh

ters

10 p

Ci/L

with

out d

augh

ters

“n

et”,

i.e.

, abo

ve b

ackg

roun

d

Cha

lleng

ing

(per

haps

not

pos

sibl

e) to

mea

sure

ann

ual

incr

emen

ts o

f ord

er o

f 0.1

pC

i/L g

iven

nat

ural

var

iatio

n an

d m

easu

rem

ent l

imita

tions

14

Page 15: 4-2-14 Radon Presentation - Comments on Measuring Long-Term Average Radon … · 2014-04-01 · Radon levels change diurnally and by season radon concentrations typically reac h their

Mai

nO

bser

vatio

nsM

ain

Obs

erva

tions

B

ackg

roun

d le

vels

of a

mbi

ent R

n-22

2 ar

e qu

ite

gq

varia

ble

Va

riatio

n in

bac

kgro

und

leve

ls o

f Rn-

222>

0.1

pC

i/L

The

dete

ctio

n le

vel

of tr

ack

etch

det

ecto

rs >

0.1

pC

i/L

Cha

lleng

ing,

per

haps

not

pos

sibl

e, to

mea

sure

suc

h sm

alli

ncre

men

tsw

ithan

ypr

ecis

ion

smal

l inc

rem

ents

with

any

pre

cisi

on

A b

right

-line

app

roac

h do

omed

to fa

ilure

C

onsi

der c

ombi

natio

n of

mod

ellin

g (M

ILD

OS)

with

g

()

“app

ropr

iate

” co

nfirm

atio

n by

mea

sure

men

t (a

ckno

wle

dgin

g lim

itatio

ns a

nd u

se o

f sta

tistic

al te

st)

15